arXiv subjects

Davide Grassani

Publications and source records attributed to Davide Grassani.

17 recordsLinked to original sources

arXiv2026

Enhancing broadband second harmonic generation in a thin film lithium niobate racetrack resonator with tunable-coupling

Second harmonic generation in thin film periodically poled lithium niobate (PPLN) is constrained by an efficiency-bandwidth trade-off and fabrication-sensitive scaling. We demonstrate a racetrack resonator incorporating a short PPLN section and a tunable Mach-Zehnder interferometer coupler that enables in situ control of the coupling condition, compensating fabrication tolerances and stabilizing operation near critical coupling. The telecom pump is resonantly enhanced, while the near-infrared second harmonic is generated in single pass, eliminating dual-resonance requirements. The device achieves a 35 times efficiency enhancement over a non-resonant structure while maintaining a 7 nm bandwidth. This architecture provides a robust platform for broadband integrated frequency doubling.

physics.optics↗

arXiv2026

Test of a 34 GHz EOM laser frequency comb at ESPRESSO

Laser frequency combs (LFCs) are a promising technology for wavelength calibration of astronomical high-resolution spectrographs requiring utmost accuracy and stability, since they directly translate the fundamental SI time standard from the radio frequency regime to optical frequencies. However, they have so far seen limited use in practice, due to their complexity, incomplete wavelength coverage, but also the challenges in the data analysis they imply. Here, we present a detailed test of a 34 GHz electro-optic modulation comb with the ESPRESSO spectrograph. Using thin-film lithum-niobate waveguides for broadening and harmonic generation, the setup provides partial coverage of the IR, visible, and near-UV spectral ranges. We focus on assessing the quality of the delivered spectra and their capability to facilitate accurate and stable wavelength calibration. We present a detailed analysis of the spectrally-diffuse background, the line width, and characterize the line-spread function over a broader width than possible with the ESPRESSO facility LFC. Comparing both combs, we find strong local discrepancies in the wavelength calibration accuracy up to 15m/s , which correlate with the echellogram structure. These do not originate from the lasers, but from misalignments in the ESPRESSO calibration unit, highlighting the strong need to make instrument fiber feeds more robust to light-injection effects. Nevertheless, we demonstrate excellent stability of the wavelength calibration, with a scatter of only 17cm/s . This, however, can only be achieved when accurately modeling the non-Gaussian line-spread function, showcasing the need for advanced data analysis techniques when dealing with LFC spectra.

astro-ph.IM↗

arXiv2025

High-purity frequency-degenerate photon pair generation via cascaded SFG/SPDC in thin film lithium niobate

Frequency-degenerate photon pairs generated using nonlinear photonic integrated devices are a crucial resource for scalable quantum information processing and metrology. However, their realization is hindered by unwanted parametric processes occurring within the same phase matching band, which degrade the signal-to-noise ratio and reduce the purity of the associated quantum states. Here, we propose a dual-pump scheme to produce frequency-degenerate photon pairs, based on cascaded sum-frequency generation and spontaneous parametric down-conversion occurring within a single waveguide, while strongly suppressing parasitic photon pair generation from single-pump processes. This approach significantly simplifies the design compared to microresonator-based methods and enables both pumping and collection of photon pairs entirely in the telecom band. We experimentally validate the concept in a layer-poled thin film lithium niobate waveguide, achieving frequency-degenerate photon pair generation with a brightness of \SI{1.0(3)e5}{\hertz \per \nm \per \square \milli \watt } and a 40 dB suppression of unwanted single-pump processes.

quant-ph↗

arXiv2024

Ultrabroadband tunable difference frequency generation in standardized thin-film lithium niobate platform

Thin-film lithium niobate (TFLN) on insulator is a promising platform for nonlinear photonic integrated circuits (PICs) due to its strong light confinement, high second-order nonlinearity, and flexible quasi-phase matching for three-wave mixing processes via periodic poling. Among the three-wave mixing processes of interest, difference frequency generation (DFG) can produce long wave infrared (IR) light from readily available near IR inputs. While broadband DFG is well studied for mid-IR frequencies, achieving broadband idler generation within the telecom window (near C-band) and the short-wave infrared (near 2 micron) is more challenging due to stringent dispersion profile requirements, especially when using standardized TFLN thicknesses. In this paper, we investigate various standard waveguide designs to pinpoint favorable conditions for broadband DFG operation covering several telecom bands. Our simulations identify viable designs with a possible 3-dB conversion efficiency bandwidth (CE-BW) of 300 nm and our measurements show idler generation from 1418 nm to 1740 nm, limited by our available sources, experimentally confirming our design approach. Furthermore, temperature tuning allows further shift of the idler towards the mid-IR, up to 1819 nm. We also achieve a stretched wavelength range of idler generation by leveraging the longitudinal variation of the waveguide in addition to poling. Finally, our numerical simulations show the possibility of extending the CE-BW up to 780 nm while focusing on waveguide cross-sections that are available for fabrication within a foundry. Our work provides a methodology that bridges the deviations between fabricated and designed cross-sections, paving a way for standardized broadband DFG building blocks.

physics.optics↗

arXiv2024

Ultraviolet astronomical spectrograph calibration with laser frequency combs from nanophotonic lithium niobate waveguides

Astronomical precision spectroscopy underpins searches for life beyond Earth, direct observation of the expanding Universe and constraining the potential variability of physical constants across cosmological scales. Laser frequency combs can provide the critically required accurate and precise calibration to the astronomical spectrographs. For cosmological studies, extending the calibration with such astrocombs to the ultraviolet spectral range is highly desirable, however, strong material dispersion and large spectral separation from the established infrared laser oscillators have made this exceedingly challenging. Here, we demonstrate for the first time astronomical spectrograph calibrations with an astrocomb in the ultraviolet spectral range below 400 nm. This is accomplished via chip-integrated highly nonlinear photonics in periodically-poled, nano-fabricated lithium niobate waveguides in conjunction with a robust infrared electro-optic comb generator, as well as a chip-integrated microresonator comb. These results demonstrate a viable route towards astronomical precision spectroscopy in the ultraviolet and may contribute to unlocking the full potential of next generation ground- and future space-based astronomical instruments.

physics.optics↗

arXiv2020

A nonreciprocal optical resonator with broken time-invariance for arbitrarily high time-bandwidth performance

Most present-day resonant systems, throughout physics and engineering, are characterized by a strict time-reversal symmetry between the rates of energy coupled in and out of the system, which leads to a trade-off between how long a wave can be stored in the system and the system bandwidth. Any attempt to reduce the losses of the resonant system, and hence store a (mechanical, acoustic, electronic, optical, atomic, or of any other nature) wave for more time, will inevitably also reduce the bandwidth of the system. Until recently, this time-bandwidth limit has been considered fundamental, arising from basic Fourier reciprocity. A recent theory suggested that it might in fact be overcome by breaking Lorentz reciprocity in the resonant system, reinvigorated a debate about whether (or not) this was indeed the case. Here, we report an experimental realization of a cavity where, inducing nonreciprocity by breaking the time invariance, we do overcome the fundamental time-bandwidth limit of ordinary resonant systems by a factor of 30, in full agreement with accompanying numerical simulations. We show that, although in practice experimental constraints limit our scheme, the time bandwidth product can be arbitrarily large, simply dictated by the finesse of the cavity. Our experimental realization uses a simple macroscopic, time-variant, fiber-optic cavity, where we break Lorentz reciprocity by non-adiabatically opening the cavity, injecting a pulse of large bandwidth, and then closing the cavity, storing the pulse which can be released on-demand at a later time. Our results open the path for designing resonant systems, ubiquitous in physics and engineering, that can simultaneously be broadband (i.e., ultrafast) and possessing long storage times, thereby unleashing fundamentally new functionalities in wave physics and wave-matter interactions.

physics.optics↗

arXiv2018

Highly efficient 4 micron light generation through fs-fiber laser driven supercontinuum in Si$_3$N$_4$ waveguides

Directly accessing the middle infrared, the molecular functional group spectral region, via supercontinuum generation processes based on turn-key fiber lasers offers the undeniable advantage of simplicity and robustness. Recently, the assessment of the coherence of the mid-IR dispersive wave in silicon nitride waveguides, pumped at telecom wavelength, established an important first step towards mid-IR frequency comb generation based on such compact systems. Yet, the spectral reach and efficiency still fall short for practical implementation. Here, we experimentally demonstrate for the first time to our knowledge, that fs-fiber laser driven systems based on large-cross section silicon nitride waveguides can reach, with powers sufficient to drive dual-comb spectroscopy, the important greenhouse gases spectral region near 4 micron, typically accessed through different frequency generation or more complex approaches. We show, from a 2 micron femtosecond fiber laser, up to 30% power conversion and milliwatt-level output powers, proving that such sources are suitable candidate for compact, chip-integrated spectroscopic and sensing applications.

physics.optics↗

arXiv2017

Mid-infrared frequency comb generation with silicon nitride nano-photonic waveguides

Mid-infrared optical frequency combs are of significant interest for molecular spectroscopy due to the large absorption of molecular vibrational modes on one hand, and the ability to implement superior comb-based spectroscopic modalities with increased speed, sensitivity and precision on the other hand. Substantial advances in mid-infrared frequency comb generation have been made in recent years based on nonlinear frequency conversion, microresonator Kerr frequency combs, quantum cascade lasers and mode locking regimes. Here we demonstrate a simple, yet effective method for the direct generation of mid-infrared optical frequency combs in the region from ${2.5-4~μ{\rm m}}$, i.e. ${2500-4000~{\rm cm}^{-1}}$ covering a large fraction of the functional group region, directly from a conventional and compact erbium-fiber-based femtosecond laser in the telecommunication band (i.e. ${1.55~μ{\rm m}}$). The wavelength conversion is based on dispersive wave generation within the supercontinuum process in large-cross-section and dispersion-engineered silicon nitride (${\rm Si_3N_4}$) waveguides. The long-wavelength dispersive wave, with its position lithographically determined, performs as a mid-infrared frequency comb, whose coherence is demonstrated via optical heterodyne measurements. Such a simple and versatile approach to mid-infrared frequency comb generation is suitable for spectroscopic applications in the first mid-infrared atmospheric window. Moreover, the compactness and simplicity of the approach have the potential to realize compact dual-comb spectrometers. The generated combs have a fine teeth-spacing, making them also suitable for gas phase analysis.

physics.optics↗

arXiv2017

Large second harmonic generation enhancement in SiN waveguides by all-optically induced quasi phase matching

Integrated waveguides exhibiting efficient second-order nonlinearities are crucial to obtain compact and low power optical signal processing devices. Silicon nitride (SiN) has shown second harmonic generation (SHG) capabilities in resonant structures and single-pass devices leveraging intermodal phase matching, which is defined by waveguide design. Lithium niobate allows compensating for the phase mismatch using periodically poled waveguides, however the latter are not reconfigurable and remain difficult to integrate with SiN or silicon (Si) circuits. Here we show the all-optical enhancement of SHG in SiN waveguides by more than 30 dB. We demonstrate that a Watt-level laser causes a periodic modification of the waveguide second-order susceptibility. The resulting second order nonlinear grating has a periodicity allowing for quasi phase matching (QPM) between the pump and SH mode. Moreover, changing the pump wavelength or polarization updates the period, relaxing phase matching constraints imposed by the waveguide geometry. We show that the grating is long term inscribed in the waveguides, and we estimate a second order nonlinearity of the order of 0.3 pm/V, while a maximum conversion efficiency (CE) of 1.8x10-6 W-1 cm-2 is reached.

physics.optics↗

arXiv2016

Mid-infrared continuous wave parametric amplification in tapered chalcogenide microstructured fibers

As photon mixing is not inherently limited to any specific spectral region, parametric processes represent a compelling solution for all-optical signal processing in spectral windows not easily accessible by other technologies. Particularly, the continuous-wave pumping scheme is essential for any application requiring modulated signals or precise spectroscopic characterization. Highly nonlinear fibers enabled record performances for wavelength conversion and amplification in the telecommunication band, however no waveguiding platforms have yet solved the trade-off between high-nonlinearity, low propagation losses and dispersion in the mid-infrared. Here, we show mid-infrared continuous-wave parametric amplification in a GeAsSe fiber. Leveraging state-of-the-art fabrication techniques, a novel tapered photonic crystal fiber geometry enabling 4.5 dB signal amplification and 2 dB idler conversion efficiency is experimentally demonstrated using only 125 mW of pump in the 2 micron wavelength range. This result is not only the first ever continuous-wave parametric amplification measured at 2 micron, in any waveguide, but also establishes GeAsSe PCF tapers as the most promising all-fibered, high efficiency continuous-wave parametric converter for advanced applications in the mid-infrared.

physics.optics↗

arXiv2016

Energy correlations of photon pairs generated by a silicon microring resonator probed by Stimulated Four Wave Mixing

Compact silicon integrated devices, such as micro-ring resonators, have recently been demonstrated as efficient sources of quantum correlated photon pairs. The mass production of integrated devices demands the implementation of fast and reliable techniques to monitor the device performances. In the case of time-energy correlations, this is particularly challenging, as it requires high spectral resolution that is not currently achievable in coincidence measurements. Here we reconstruct the joint spectral density of photons pairs generated by spontaneous four-wave mixing in a silicon ring resonator by studying the corresponding stimulated process, namely stimulated four wave mixing. We show that this approach, featuring high spectral resolution and short measurement times, allows one to discriminate between nearly-uncorrelated and highly-correlated photon pairs.

quant-ph↗

arXiv2014

An integrated source of spectrally filtered correlated photons for large scale quantum photonic systems

We demonstrate the generation of quantum-correlated photon-pairs combined with the spectral filtering of the pump field by more than 95dB using Bragg reflectors and electrically tunable ring resonators. Moreover, we perform demultiplexing and routing of signal and idler photons after transferring them via a fiber to a second identical chip. Non-classical two-photon temporal correlations with a coincidence-to-accidental ratio of 50 are measured without further off-chip filtering. Our system, fabricated with high yield and reproducibility in a CMOS process, paves the way toward truly large-scale quantum photonic circuits by allowing sources and detectors of single photons to be integrated on the same chip.

quant-ph↗

arXiv2014

A micrometer-scale integrated silicon source of time-energy entangled photons

Entanglement is a fundamental resource in quantum information processing. Several studies have explored the integration of sources of entangled states on a silicon chip but the sources demonstrated so far require millimeter lengths and pump powers of the order of hundreds of mWs to produce an appreciable photon flux, hindering their scalability and dense integration. Microring resonators have been shown to be efficient sources of photon pairs, but entangled state emission has never been demonstrated. Here we report the first demonstration of a microring resonator capable of emitting time-energy entangled photons. We use a Franson experiment to show a violation of Bell's inequality by as much as 11 standard deviations. The source is integrated on a silicon chip, operates at sub-mW pump power, emits in the telecom band with a pair generation rate exceeding 10$^7$ Hz per $nm$, and outputs into a photonic waveguide. These are all essential features of an entangled states emitter for a quantum photonic networks.

quant-ph↗

arXiv2013

Active stabilization of a Michelson interferometer at an arbitrary phase with sub-nm resolution

We report on the active stabilization of a Michelson interferometer at an arbitrary phase angle with a precision better than one degree at $λ= 632.8$ nm, which corresponds to an optical path difference between the two arms of less than 1 nm. The stabilization method is ditherless and the error signal is computed from the spatial shift of the interference pattern of a reference laser, measured in real-time with a CCD array detector. We discuss the usefulness of this method for nanopositioning, optical interferometry and quantum optical experiments.

physics.optics↗

arXiv2013

Stimulated and spontaneous four-wave mixing in silicon-on-insulator coupled photonic wire nano-cavities

We report on four-wave mixing in coupled photonic crystal nano-cavities on a silicon-on-insulator platform. Three photonic wire cavities are side-coupled to obtain three modes equally separated in energy. The structure is designed to be self-filtering, and we show that the pump is rejected by almost two orders of magnitudes. We study both the stimulated and the spontaneous four-wave mixing processes: owing to the small modal volume, we find that signal and idler photons are generated with a hundred-fold increase in efficiency as compared to silicon micro-ring resonators.

cond-mat.mes-hall↗

arXiv2012

Ultra-low power generation of twin photons in a compact silicon ring resonator

We demonstrate efficient generation of correlated photon pairs by spontaneous four wave mixing in a 5 μm radius silicon ring resonator in the telecom band around 1550 nm. By optically pumping our device with a 200 μW continuous wave laser, we obtain a pair generation rate of 0.2 MHz and demonstrate photon time correlations with a coincidence-to-accidental ratio as high as 250. The results are in good agreement with theoretical predictions and show the potential of silicon micro-ring resonators as room temperature sources for integrated quantum optics applications.

physics.optics↗

arXiv2012

From Classical Four-Wave Mixing to Parametric Fluorescence in Silicon micro-ring resonators

Four-wave mixing can be stimulated or occur spontaneously. The first process is intrinsically much stronger, and well understood through classical nonlinear optics. The latter, also known as parametric fluorescence, can be explained only in the framework of a quantum theory of light. We experimentally demonstrate that, in a micro-ring resonator, there exists a simple relation between the efficiencies of these two processes, which is independent of the nonlinearity and size of the ring. In particular we show that the average power generated by parametric fluorescence can be immediately estimated from a classical FWM experiment. These results suggest that classical nonlinear characterization of a photonic integrated structure can provide accurate information on its nonlinear quantum properties.

quant-ph↗