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Davide Valentinis

Publications and source records attributed to Davide Valentinis.

12 recordsLinked to original sources

The flow of local quantum fluids: Conservation laws and vertex corrections from many-body linear-response theory with local self-energy

In non-diffusive conduction regimes of strongly correlated quantum electron systems, electromagnetic perturbations simultaneously probe the electronic dynamics in time and space: the exchanged energy $\hbar \omega$ excites retarded, i.e., frequency-dependent, many-body interactions, while the probing spatial modulation renders the response spatially nonlocal, i.e., dependent on the external wave vector $\vec{q}$. This work determines the exact nonlocal electrodynamic response of such dynamical quantum fluids under the assumptions of local, frequency-dependent interactions and charge/mass conservation. The latter is ensured by Bethe-Salpeter equations for renormalized interaction vertices, entering the Kubo formalism for two-particle correlation functions (e.g., for density, currents, momentum, stress). Within such framework, it is shown that vertex corrections generally vanish at $q=0$ for single-particle dispersions with inversion symmetry and for bare interaction vertices that are odd with respect to specific point group transformations in momentum space, including inversion for vector vertices, and mirror reflections or two- or higher-fold rotations for tensor vertices. In addition, for quadratic dispersion vertex corrections identically vanish from the current-current correlation function, at any momentum $\vec{q}$ and frequency $\omega$. The robustness of these criteria against further symmetry breaking, multiband effects, and additionally imposing momentum conservation, is discussed, with application to the Hall viscosity of Landau levels. Explicit expressions for generic nonlocal correlation functions are derived for Fermi liquids (with well-defined quasiparticle peaks) and non-Fermi liquids (devoid of quasiparticles), for arbitrary local self-energies.

cond-mat.str-el

Superlinear Hall angle and carrier mobility from non-Boltzmann magnetotransport in the spatially disordered Yukawa-Sachdev-Ye-Kitaev model on a square lattice

Exact numerical results for the dc magnetoconductivity tensor of the two-dimensional spatially disordered Yukawa-Sachdev-Ye-Kitaev (2D-YSYK) model on a square lattice, at first order in applied perpendicular magnetic field, are obtained from the self-consistent disorder-averaged solution of the 2D-YSYK saddle-point equations. This system describes fermions endowed with a Fermi surface and coupled to a bosonic scalar field through spatially random Yukawa interactions. The resulting local and energy-dependent fermionic self-energies are employed in the Kubo formalism to calculate the longitudinal and Hall conductivities, the Hall coefficient, the carrier mobility, and the cotangent of the Hall angle, at fixed fermion density. From the interplay between YSYK interactions and square-lattice embedding, and the non-Boltzmann frequency-dependent self energies, we find nontrivial evolution of the magnetotransport coefficients as a function of temperature and YSYK interaction strength, notably a superlinear evolution of the Hall-angle cotangent and the inverse carrier mobility with temperature, concomitant with linear-in-temperature resistivity, in an extended crossover regime above the low-temperature Marginal Fermi Liquid (MFL) ground state. Our model and results provide a controlled theoretical framework to interpret magnetotransport experiments, at linear order in applied magnetic field, in strange-metal phases found in strongly correlated solid-state electron systems.

cond-mat.str-el

Strange metal and superconductor in the two-dimensional Yukawa-Sachdev-Ye-Kitaev model

The two-dimensional Yukawa-Sachdev-Ye-Kitaev (2d-YSYK) model provides a universal theory of quantum phase transitions in metals in the presence of quenched random spatial fluctuations in the local position of the quantum critical point. It has a Fermi surface coupled to a scalar field by spatially random Yukawa interactions. We present full numerical solutions of a self-consistent disorder averaged analysis of the 2d-YSYK model in both the normal and superconducting states, obtaining electronic spectral functions, frequency-dependent conductivity, and superfluid stiffness. Our results reproduce key aspects of observations in the cuprates as analyzed by Michon et al. (arXiv:2205.04030). We also find a regime of increasing zero temperature superfluid stiffness with decreasing superconducting critical temperature, as is observed in bulk cuprates.

cond-mat.str-el

On non-local electrical transport in anisotropic metals

We discuss various aspects of non-local electrical transport in anisotropic metals. For a metal with circular Fermi surface, the scattering rates entering the local conductivity and viscosity tensors are well-defined, corresponding to eigenfrequencies of the linearized collision operator. For anisotropic metals, we provide generalized formulas for these scattering rates and use a variational approximation to show how they relate to microscopic transition probabilities. We develop a simple model of a collision operator for a metal of arbitrary Fermi surface with finite number of quasi-conserved quantities, and derive expressions for the wavevector-dependent conductivity $\sigma(q)$ and the spatially-varying conductivity $\sigma(x)$ for a long, narrow channel. We apply this to the case of different rates for momentum-conserving and momentum-relaxing scattering, deriving closed-form expressions for $\sigma(q)$ and $\sigma(x)$ -- beyond generalizing from circular to arbitrary Fermi surface geometry, this represents an improvement over existing methods which solve the relevant differential equation numerically rather than in closed form. For the specific case of a diamond Fermi surface, we show that, if transport signatures were interpreted via a model for a circular Fermi surface, the diagnosis of the underlying transport regime would differ based on experimental orientation and based on whether $\sigma(q)$ or $\sigma(x)$ was considered. Finally, we discuss the bulk conductivity. While the common lore is that ``momentum''-conserving scattering does not affect bulk resistivity, we show that \textit{crystal momentum}-conserving scattering -- such as normal electron-electron scattering -- can affect the bulk resistivity for an anisotropic Fermi surface. We derive a simple formula for this contribution.

cond-mat.mes-hall

Cyclotron resonance and quantum oscillations of critical Fermi surfaces

Kohn's theorem places strong constraints on the cyclotron response of Fermi liquids. Recent observations of a doping dependence in the cyclotron mass of La$_{2-x}$Sr$_x$CuO$_4$ (Legros et al., Phys. Rev. B 106, 195110 (2022)) are therefore surprising because the cyclotron mass can only be renormalized by large momentum umklapp interactions which are not expected to vary significantly with doping. We show that a version of Kohn's theorem continues to apply to disorder-free non-Fermi liquids with a critical boson near zero momentum. However, marginal Fermi liquids arising from a spatially random Yukawa coupling between the electrons and bosons do give rise to significant corrections to the cyclotron mass which we compute. This is the same theory which yields linear-in-temperature resistivity and other properties of strange metals at zero fields (Patel et al., Science 381, 790 (2023)).

cond-mat.str-el

Correlation between phase stiffness and condensation energy across the non-Fermi to Fermi-liquid crossover in the Yukawa-Sachdev-Ye-Kitaev model on a lattice

We construct and analyze a lattice generalization of the Yukawa-Sachdev-Ye-Kitaev model, where spinful fermions experience on-site, random, all-to-all interactions with an Einstein bosonic mode, and random intersite coherent hopping. We obtain the exact self-consistent numerical solution of the model at mean-field level, and analytical approximations, for all values of fermion-boson coupling and hopping, under the spin-singlet ansatz and at particle-hole symmetry, both in the normal and superconducting states, thus tracing the entire phase diagram. In the normal state, the competition between hopping and coupling leads to crossovers between Fermi-liquid and non-Fermi liquid states, as reflected by the fermionic and bosonic spectral functions and the normal-state entropy. We calculate the finite phase stiffness of the superconducting state through the equilibrium electromagnetic response. Furthermore, we study the critical temperature $T_c$, as well as the spectral functions, the quasiparticle weight, the gap, and the condensation energy in the superconducting state. At weak coupling, we retrieve a disordered generalization of Bardeen-Cooper-Schrieffer theory. At strong coupling, asymptotically $T_c$ saturates but the stiffness decreases, which suggests strong superconducting fluctuations. $T_c$ is maximum in the single-dot limit, while the stiffness peaks exactly at the crossover between non-Fermi liquid and Fermi-liquid phases. We discover that the quasiparticle weight, the stiffness, and the condensation energy, are all correlated as a function of coupling, reminiscent of the correlations observed in high-temperature cuprate superconductors.

cond-mat.supr-con

BCS to incoherent superconductivity crossovers in the Yukawa-SYK model on a lattice

We provide a quantitative and controlled analysis of the phase diagram of the the Yukawa-SYK model on a lattice, in the normal and superconducting states. We analyze the entire crossover from BCS/weak-coupling to Eliashberg/strong coupling superconductivity, as a function of fermion-boson interaction strength and hopping parameter. Cooper pairs of sharp Fermi-liquid quasiparticles at weak coupling evolve into pairing of fully incoherent fermions in the non-Fermi liquid regime. The crossovers leave observable traces in the critical temperature, the zero-temperature and zero-energy gap, the entropy, and the phase stiffness.

cond-mat.supr-con

Kinetic theory of the non-local electrodynamic response in anisotropic metals: skin effect in 2D systems

The electrodynamic response of ultra-pure materials at low temperatures becomes spatially non-local. This non-locality gives rise to phenomena such as hydrodynamic flow in transport and the anomalous skin effect in optics. In systems characterized by an anisotropic electronic dispersion, the non-local dynamics becomes dependent on the relative orientation of the sample with respect to the applied field, in ways that go beyond the usual, homogeneous response. Such orientational dependence should manifest itself not only in transport experiments, as recently observed, but also in optical spectroscopy. In this paper we develop a kinetic theory for the distribution function and the transverse conductivity of two- and three-dimensional Fermi systems with anisotropic electronic dispersion. By expanding the collision integral into the eigenbasis of a collision operator, we include momentum-relaxing scattering as well as momentum-conserving collisions. We examine the isotropic 2D case as a reference, as well as anisotropic hexagonal and square Fermi-surface shapes. We apply our theory to the quantitative calculation of the skin depth and the surface impedance, in all regimes of skin effect. We find qualitative differences between the frequency dependence of the impedance in isotropic and anisotropic systems. Such differences are shown to persist even for more complex 2D Fermi surfaces, including the ''supercircle'' geometry and an experimental parametrization for PdCoO$_2$, which deviate from an ideal polygonal shape. We study the orientational dependence of skin effect due to Fermi-surface anisotropy, thus providing guidance for the experimental study of non-local optical effects.

cond-mat.str-el

Non-local electrodynamics in ultra-pure PdCoO$_{2}$

The motion of electrons in the vast majority of conductors is diffusive, obeying Ohm's law. However, the recent discovery and growth of high-purity materials with extremely long electronic mean free paths has sparked interest in non-ohmic alternatives, including viscous and ballistic flow. Although non-ohmic transport regimes have been discovered across a range of materials, including two-dimensional electron gases, graphene, topological semimetals, and the delafossite metals, determining their nature has proved to be challenging. Here, we report on a new approach to the problem, employing broadband microwave spectroscopy of the delafossite metal PdCoO$_{2}$ in three distinct sample geometries that would be identical for diffusive transport. The observed differences, which go as far as differing power laws, take advantage of the hexagonal symmetry of PdCoO$_{2}$. This permits a particularly elegant symmetry-based diagnostic for non-local electrodynamics, with the result favouring ballistic over strictly hydrodynamic flow. Furthermore, it uncovers a new effect for ballistic electron flow, owing to the highly facetted shape of the hexagonal Fermi surface. We combine our extensive dataset with an analysis of the Boltzmann equation to characterize the non-local regime in PdCoO$_{2}$. More broadly, our results highlight the potential of broadband microwave spectroscopy to play a central role in investigating exotic transport regimes in the new generation of ultra-high conductivity materials.

cond-mat.mes-hall

Quantum discontinuity fixed point and renormalization group flow of the SYK model

We determine the global renormalization group (RG) flow of the Sachdev-Ye-Kitaev (SYK) model. This flow allows for an understanding of the surprising role of critical slowing down at a quantum first-order transition in strongly-correlated electronic systems. From a simple truncation of the infinite hierarchy of the exact functional RG flow equations we identify several fixed points: Apart from a stable fixed point, associated with the celebrated non-Fermi liquid state of the model, we find another stable fixed point related to an integer-valence state. These stable fixed points are separated by a discontinuity fixed point with one relevant direction, describing a quantum first-order transition. Most notably, the fermionic spectrum continues to be quantum critical even at the discontinuity fixed point. This rules out a description of this quantum first-order transition in terms of a local effective Ising variable that is established for classical transitions. It reveals that quantum phase coexistence can be a genuine critical state of matter.

cond-mat.str-el

Modulation of superconductivity by quantum confinement in doped strontium titanate

Quantum confinement in a thin-film geometry offers viable routes for tuning the critical properties of superconductors through modification of both density of states and pairing interaction. Low-density systems like doped strontium titanate are especially susceptible to these confinement-induced effects. In this paper, we show that the superconducting critical temperature $T_c$ is enhanced through quantum confinement in SrTiO$_3$/SrTi$_{1-x}$Nb$_x$O$_3$/SrTiO$_3$ heterostructures at $x=1\%$ concentration, by measuring resistivity transitions and the Hall carrier density for different thicknesses of the doped layer. We observe a nonmonotonic raise of $T_c$ with decreasing layer thickness at constant carrier density as estimated from the Hall effect. We analyze the results by solving a two-band model with a pairing interaction reproducing the density-dependent $T_c$ of doped SrTiO$_3$ in the bulk, that we confine to a potential well established self-consistently by the charged Nb dopants. The evolution of the theoretical $T_c$ with thickness agrees well with experiments. We point out the possible role of density inhomogeneities and suggest novel methods for engineering superconductivity in epitaxial thin films.

cond-mat.supr-con

Electromagnetic properties of viscous charged fluids

We provide a general theoretical framework to describe the electromagnetic properties of viscous charged fluids, consisting for example of electrons in certain solids or plasmas. We confirm that finite viscosity leads to multiple modes of evanescent electromagnetic waves at a given frequency, one of which is characterized by a negative index of refraction, as previously discussed in a simplified model by one of the authors. In particular we explain how optical spectroscopy can be used to probe the viscosity. We concentrate on the impact of this on the coefficients of refraction and reflection at the sample-vacuum interface. Analytical expressions are obtained relating the viscosity parameter to the reflection and transmission coefficients of light. We demonstrate that finite viscosity has the effect to decrease the reflectivity of a metallic surface, while the electromagnetic field penetrates more deeply. While on a phenomenological level there are similarities to the anomalous skin effect, the model presented here requires no particular assumptions regarding the corpuscular nature of the charge liquid. A striking consequence of the branching phenomenon into two degenerate modes is the occurrence in a half-infinite sample of oscillations of the electromagnetic field intensity as a function of distance from the interface.

cond-mat.str-el