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Davit Petrosyan

Publications and source records attributed to Davit Petrosyan.

10 recordsLinked to original sources

Model of the magnon Kerr effect in a highly anisotropic ferromagnet

The magnon Kerr effect is a nonlinear phenomenon that occurs universally in any ferromagnet with finite magnetic anisotropy. It manifests itself as a magnon population-dependent change in the magnon dispersion relation. Here, we derive the Hamiltonian for the magnon Kerr effect for a thin film with uniaxial anisotropy. We consider the external field, parallel, perpendicular, and at an intermediate angle to the anisotropy axis, and determine the Kerr coefficient in each case. We show how the nonlinearity scales for different magnetic materials as a function of magnon frequency and magnetic sample volume. Moreover, we derive the equations of motion for a hybrid cavity-magnon system with such thin-film magnon Kerr nonlinearity, to obtain populations of photons and magnons, and scattering matrix terms for the microwave transmission of the cavity, relevant for experimental observations.

cond-mat.mes-hall

Disambiguating electrical detection of magnetization dynamics in magnetic insulators

Electrical detection of magnetization dynamics in magnetic insulators underpins both fundamental studies of magnon transport and the development of low-loss magnonic devices. In heavy-metal/magnetic-insulator heterostructures, spin pumping and spin-torque ferromagnetic resonance (ST-FMR) are widely used for this purpose and are often treated separately in different measurement geometries. In practice, the competition between these two effects gives rise to electrical voltage signals of opposite signs, which can lead to ambiguous interpretations of the underlying physics. Here, we show how to disambiguate their respective contributions and provide a framework for interpreting experiments involving microwave excitation of magnetic insulators and detection of magnetization dynamics via spin-charge conversion in heavy metals. We systematically investigate spin pumping and ST-FMR in nonlocal and local devices using Pt-capped thin films of thulium and bismuth-yttrium iron garnets. We show how spin-wave character, magnetic dissipation, magnetic field orientation and device geometry govern the sign and magnitude of the resulting signals. In several cases, the voltage generated by microwave excitation changes sign between an out-of-plane or in-plane magnetic configuration. We disentangle a contribution due to spin pumping, induced by exponentially decaying propagating spin waves, and a weakly distance-dependent contribution from ST-FMR, remotely induced by inductive coupling. We show that both the spin wave excitation profile across the film thickness and magnetic damping largely determine which of the two contributions dominates. Hence, the sign of the electrical signal cannot be uniquely assigned to the chirality of the magnon modes.

cond-mat.mes-hall

Coherent Microwave Driving of Domain Wall Depinning in a Ferrimagnetic Garnet

Coherent control of domain wall dynamics offers a route to fast manipulation of magnetic textures beyond thermally activated motion. We demonstrate resonant excitation of linear and nonlinear dynamics of a pinned domain wall in a ferrimagnetic garnet thin film driven by a microwave field. Using scanning nitrogen-vacancy magnetometry and nonlocal spin-pumping measurements, we identify a low-frequency mode inside the magnon gap, originating from the localized oscillatory motion of a domain wall across a pinning line defined by a Pt stripline. Upon increasing the microwave drive into the nonlinear regime, this mode enables domain wall depinning at reduced external magnetic fields. Micromagnetic simulations reveal a progression from localized oscillations to partial relocation between pinning sites and, ultimately, complete escape from the pinning region with increasing driving power. These results establish resonant excitation of domain walls at engineered pinning sites as a mechanism for manipulating magnetic textures via localized nonlinear dynamics.

cond-mat.mes-hall

Loop-gap resonators achieving strong magnon-photon coupling in magnetic insulator thin films

Magnon-photon hybrid systems consisting of a three-dimensional electromagnetic resonator and a bulk magnetic insulator constitute the standard experimental platform in cavity magnonics. Here, we demonstrate a modular loop-gap resonator design optimized to couple with thin films of magnetic insulators. We achieve the strong-coupling regime using this loop-gap resonator coupled to a 75~nm-thick epitaxial film of yttrium iron garnet at room temperature. We further show how to perform field-differential spectroscopy of the hybrid magnon-photon system, which eliminates the unwanted signal from other loop-gap modes uncoupled to the magnetic film. In addition to the uniform ferromagnetic resonance mode, the loop-gap resonator enables an hybridization with the standing spin-wave modes forming across the thickness of the film. Our approach unlocks the use of epitaxial films and multilayers of magnetic insulators to tune the magnon band structure in cavity magnonics experiments.

cond-mat.mes-hall

Magnon Kerr effect in a magnetic thin film strongly coupled to a microwave resonator

Cavity magnonics investigates hybrid systems where magnons interact coherently with photons, providing a platform to harness light-matter interaction in magnetic materials. Progress in this field hinges on achieving stronger and tunable nonlinear effects, which are essential for controlling magnon dynamics and frequency conversion. Here, we demonstrate the magnon Kerr effect in an anisotropic magnonic system comprising a 200~nm-thick yttrium iron garnet film strongly coupled to a three-dimensional microwave resonator. The strong shape anisotropy significantly enhances the magnon Kerr effect compared to a sphere of equivalent volume, while the cavity enables sensitive probing of magnetization dynamics. We demonstrate continuous tunability of the magnitude and sign of the Kerr shift by controlling the static orientation of the magnetization. Input-output modeling of the magnon-photon interaction provides a consistent description of our system and Kerr coefficients matching the experimental results. Our findings demonstrate a scalable approach to enhancing Kerr anharmonicity in hybrid magnon-photon systems while preserving strong coupling.

cond-mat.mes-hall

Ultrathin bismuth-yttrium iron garnet films with tunable magnetic anisotropy

We report on the epitaxial growth of nm-thick films of bismuth-substituted yttrium iron garnet (BiYIG) by high-temperature off-axis radio-frequency magnetron sputtering. We demonstrate accurate control of the magnetic properties by tuning of the sputtering parameters and epitaxial strain on various (111)-oriented garnet substrates. BiYIG films with up to -0.80\% lattice mismatch with the substrate remain fully strained up to 60~nm-thick, maintaining a high crystalline quality. Transmission electron microscopy and energy-dispersive X-ray spectroscopy confirm coherent epitaxial growth, the absence of defects, and limited interdiffusion at the BiYIG/substrate interface. Varying the tensile or compressive strain between -0.80\% and +0.56\% in BiYIG allows for accurate compensation of the total magnetic anisotropy through magneto-elastic coupling. The effective magnetic anisotropy of sputtered BiYIG films can be further tuned via the off-axis deposition angle and the oxygen flow during growth, which determine the cation stoichiometry. Under optimized growth conditions, a ferromagnetic resonance (FMR) linewidth of 1~mT at 10~GHz is reliably obtained even for thicknesses as low as 10~nm. We also report small FMR linewidths in ultrathin (2-5~nm) BiYIG films grown on diamagnetic substrate yttrium scandium gallium garnet. These findings highlight the promise of low-damping, strain-engineered nm-thick BiYIG films for implementing advanced functionalities in spin-orbitronic and magnonic devices. Specifically, the magnetic-anisotropy compensation and low damping enable large cone-angle magnetization dynamics immune to magnon-magnon nonlinear scattering.

cond-mat.mtrl-sci

Low-temperature-compatible iron garnet films grown by liquid phase epitaxy

Single-crystalline yttrium iron garnet (YIG) thin films (< 100 nm) form the backbone of magnonics, owing to the record-low losses affecting their magnetization dynamics. However, thin epitaxial YIG has mostly been investigated under ambient temperatures, limited by the paramagnetic losses occurring at low temperatures due to the gadolinium gallium garnet (GGG) substrates required for epitaxial growth. Driven by a growing interest in magnonic devices that can operate in cryogenic conditions and address quantum information applications, there is a strong need for iron garnet epitaxial films grown on diamagnetic substrates that can maintain low losses at low temperatures. In this work, we use liquid phase epitaxy (LPE) to grow ultrathin films of strained YIG on a commercial diamagnetic substrate, yttrium scandium gallium garnet (YSGG). We investigate their magnetization dynamics in the 3-300 K temperature range, and compare them to equivalent films grown on paramagnetic GGG. We demonstrate for LPE YIG on YSGG substrates a ferromagnetic resonance linewidth below 1 mT at 3 K, together with a very weak temperature and frequency dependence of the losses. The growth of YIG/YSGG by LPE provides a straightforward approach to producing iron garnet thin films for use in low-temperature investigations.

cond-mat.mtrl-sci

Lattice-tunable substituted iron garnets for low-temperature magnonics

The synthesis of nm-thick epitaxial films of iron garnets by physical vapor deposition has opened up exciting opportunities for the on-chip generation and processing of microwave signals encoded in magnons. However, iron garnet thin films suffer from demanding lattice-matching and stoichiometry requirements. Here a new approach to their synthesis is developed, enabling a precise and continuous tuning of iron garnet compositions based on the co-sputtering of binary oxides. By substituting a controlled proportion of iron with additional yttrium, Y$_{3}$(Y$_{x}$Fe$_{5-x}$)O$_{12}$ films of high crystalline quality are obtained, combining a widely tunable lattice parameter and excellent magnetization dynamics. This enables iron garnet thin films suited for cryogenic applications, which have long remained impractical due to microwave losses caused by paramagnetic garnet substrates. Low-temperature ferromagnetic resonance confirms the elimination of substrate paramagnetic losses for Y$_{3}$(Y$_{x}$Fe$_{5-x}$)O$_{12}$ films lattice-matched to Y$_{3}$Sc$_{2}$Ga$_{3}$O$_{12}$ (YSGG), a diamagnetic substrate. The Y$_{3}$(Y$_{x}$Fe$_{5-x}$)O$_{12}$ system can be matched to other substrates such as (Gd,Y)$_{3}$Sc$_{2}$Ga$_{3}$O$_{12}$. Bi-substituted films of (Bi$_{0.8}$Y$_{2.2}$)Fe$_{5}$O$_{12}$ also have ideal lattice matching to YSGG, demonstrating the versatility of this approach. This opens unprecedented options for cation substitutions in iron garnet films, offering a promising avenue to new properties and quantum magnonic devices operating in low-temperature environments.

cond-mat.mtrl-sci

Orbital Pumping in Ferrimagnetic Insulators

We report the detection of pure orbital currents generated by both coherent and thermal magnons in the magnetic insulator Bi-doped yttrium iron garnet (BiYIG). The pumping of orbital and spin currents is jointly investigated in nano-devices made of naturally oxidized Cu, pure Cu, Pt, and Cr. The absence of charge conduction in BiYIG and the negligible spin-to-charge conversion of oxidized Cu allows us to disambiguate the orbital current contribution. Comparative measurements on YIG and BiYIG show that the origin of the orbital pumping in BiYIG/oxidized Cu is the dynamics of the orbital magnetization in the magnetic insulator. In Cr, the pumping signal is dominated by the negative spin Hall effect rather than the positive orbital Hall effect, indicating that orbital currents represent a minority of the total angular momentum current pumped from the magnetic insulator. Our results also evidence that improving the interfacial transparency significantly enhances pumping efficiencies not only for spin, but also for orbital currents.

cond-mat.mes-hall

Quantum Spin Hall Effect in Magnetic Graphene

A promising approach to attain long-distance coherent spin propagation is accessing topological spin-polarized edge states in graphene. Achieving this without external magnetic fields necessitates engineering graphene band structure, obtainable through proximity effects in van der Waals heterostructures. In particular, proximity-induced staggered potentials and spin-orbit coupling are expected to form a topological bulk gap in graphene with gapless helical edge states that are robust against disorder. In this work, we detect the spin-polarized helical edge transport in graphene at zero external magnetic field, allowed by the proximity of an interlayer antiferromagnet, CrPS$_4$. We show the coexistence of the quantum spin Hall (QSH) states and magnetism in graphene, where the induced spin-orbit and exchange couplings also give rise to a large anomalous Hall (AH) effect. The detection of the QSH states at zero external magnetic field, together with the AH signal that persists up to room temperature, opens the route for practical applications of magnetic graphene in quantum spintronic circuitries.

cond-mat.mes-hall