Searcharxiv⌕ Search

arXiv subjects

Debanjan Chowdhury

Publications and source records attributed to Debanjan Chowdhury.

At least 55 records · Page 3Linked to original sources

Collective density fluctuations of strange metals with critical Fermi surfaces

Recent spectroscopic measurements in a number of strongly correlated metals that exhibit non-Fermi liquid like properties have observed evidence of anomalous frequency and momentum-dependent charge-density fluctuations. Specifically, in the strange metallic regime of the cuprate superconductors, there is a featureless particle-hole continuum exhibiting unusual power-laws, and experiments suggest that the plasmon mode decays into this continuum in a manner that is distinct from the expectations of conventional Fermi liquid theory. Inspired by these new experimental developments, we address the nature of low-energy collective modes and the particle-hole continua for different "solvable" lattice models of non-Fermi liquids that host a critical Fermi surface -- a sharp electronic Fermi surface without any low-energy electronic quasiparticles. We scrutinize theoretically the possible existence of a long-lived zero-sound mode, which is renormalized to the plasma frequency in the presence of long-ranged coulomb interactions, and its decay into the continuum over a wide range of frequencies and momenta. Quite remarkably, some of the models analyzed here can account for certain aspects of the universal experimental observations, that clearly lie beyond the purview of standard Fermi liquid theory.

cond-mat.str-el↗

Diamagnetic response and phase stiffness for interacting isolated narrow bands

A platform that serves as an ideal playground for realizing ``high'' temperature superconductors are materials where the electrons' kinetic energy is completely quenched, and interactions provide the only energy scale in the problem for $T_c$. However, when the non-interacting bandwidth for a set of isolated bands is small compared to the scale of the interactions, the problem is inherently non-perturbative and requires going beyond the traditional mean-field theory of superconductivity. In two spatial dimensions, $T_c$ is controlled by the superconducting phase stiffness. Here we present a general theoretical framework for computing the electromagnetic response for generic model Hamiltonians, which controls the maximum possible superconducting phase stiffness and thereby $T_c$, without resorting to any mean-field approximation. Importantly, our explicit computations demonstrate that the contribution to the phase stiffness arises from (i) ``integrating out'' the remote bands that couple to the microscopic current operator, and (ii) the density-density interactions projected onto the isolated narrow bands. Our framework can be used to obtain an upper bound on the phase stiffness, and relatedly the superconducting transition temperature, for a range of physically inspired models involving both topological and non-topological narrow bands with arbitrary density-density interactions. We discuss a number of salient aspects of this formalism by applying it to a specific model of interacting flat bands and compare it against the known $T_c$ from independent numerically exact computations.

cond-mat.str-el↗

Continuous Mott transition in moiré semiconductors: role of long-wavelength inhomogeneities

Recent experiments in moiré transition metal dichalcogenide materials have reported the observation of a continuous bandwidth-tuned transition from a metal to a paramagnetic Mott insulator at a fixed filling of one electron per moiré unit cell. The electrical transport measurements reveal a number of puzzling features that are seemingly at odds with the theoretical expectations of an interaction induced, but disorder-free, bandwidth-tuned metal-insulator transition. In this work, we include the effects of long-wavelength inhomogeneities, building on the results for a continuous metal-insulator transition at fixed filling in the clean limit. We examine the effects of meso-scale inhomogeneities near the critical point on transport using the framework of random resistor networks, highlighting the salient differences from a simple percolation-based picture. We place our results in the context of recent and ongoing experiments.

cond-mat.str-el↗

Intermediate-scale theory for electrons coupled to frustrated local-moments

A classic route for destroying long-lived electronic quasiparticles in a weakly interacting Fermi liquid is to couple them to other low-energy degrees of freedom that effectively act as a bath. We consider here the problem of electrons scattering off the spin fluctuations of a geometrically frustrated antiferromagnet, whose non-linear Landau-Lifshitz dynamics, which remains non-trivial at all temperatures, we model in detail. At intermediate temperatures and in the absence of any magnetic ordering, the fluctuating local-moments lead to a non-trivial angular anisotropy of the scattering-rate along the Fermi surface, which disappears with increasing temperature, elucidating the role of "hot-spots". Over a remarkably broad window of intermediate and high temperatures, the electronic properties can be described by employing a local approximation for the dynamical spin-response. This we contrast with the more familiar setup of electrons scattering off classical phonons, whose high-temperature limit differs fundamentally on account of their unbounded Hilbert space. We place our results in the context of layered magnetic delafossite compounds.

cond-mat.str-el↗

Investigation of Planckian behavior in a high-conductivity oxide: PdCrO$_2$

The layered delafossite metal PdCrO$_2$ is a natural heterostructure of highly conductive Pd layers Kondo coupled to localized spins in the adjacent Mott insulating CrO$_2$ layers. At high temperatures $T$ it has a $T$-linear resistivity which is not seen in the isostructural but non-magnetic PdCoO$_2$. The strength of the Kondo coupling is known, as-grown crystals are extremely high purity and the Fermi surface is both very simple and experimentally known. It is therefore an ideal material platform in which to investigate 'Planckian metal' physics. We do this by means of controlled introduction of point disorder, measurement of the thermal conductivity and Lorenz ratio and studying the sources of its high temperature entropy. The $T$-linear resistivity is seen to be due mainly to elastic scattering and to arise from a sum of several scattering mechanisms. Remarkably, this sum leads to a scattering rate within 10$\%$ of the Planckian value of $k_BT/$$\hbar$.

cond-mat.str-el↗

Fractionalization and topology in amorphous electronic solids

Band-topology is traditionally analyzed in terms of gauge-invariant observables associated with crystalline Bloch wavefunctions. Recent work has demonstrated that many of the free fermion topological characteristics survive even in an amorphous setting. In this work, we extend these studies to incorporate the effect of strong repulsive interactions on the fate of topology and other correlation induced phenomena. Using a parton-based approach, we obtain the interacting phase diagram for an electronic two-orbital model with tunable topology in a two dimensional amorphous network. In addition to the (non-)topological phases that are adiabatically connected to the free fermion limit, we find a number of strongly interacting amorphous analogs of crystalline Mott insulating phases with non-trivial chiral neutral edge modes, and a fractionalized Anderson insulating phase. The amorphous networks thus provide a new playground for studying a plethora of exotic states of matter, and their glassy dynamics, due to the combined effects of non-trivial topology, disorder, and strong interactions.

cond-mat.str-el↗

Sachdev-Ye-Kitaev Models and Beyond: A Window into Non-Fermi Liquids

We present a review of the Sachdev-Ye-Kitaev (SYK) model of compressible quantum many-body systems without quasiparticle excitations, and its connections to various theoretical studies of non-Fermi liquids in condensed matter physics. The review is placed in the context of numerous experimental observations on correlated electron materials. Strong correlations in metals are often associated with their proximity to a Mott transition to an insulator created by the local Coulomb repulsion between the electrons. We explore the phase diagrams of a number of models of such local electronic correlation, employing a dynamical mean field theory in the presence of random spin exchange interactions. Numerical analyses and analytical solutions, using renormalization group methods and expansions in large spin degeneracy, lead to critical regions which display SYK physics. The models studied include the single-band Hubbard model, the $t$-$J$ model and the two-band Kondo-Heisenberg model in the presence of random spin exchange interactions. We also examine non-Fermi liquids obtained by considering each SYK model with random four-fermion interactions to be a multi-orbital atom, with the SYK-atoms arranged in an infinite lattice. We connect to theories of sharp Fermi surfaces without any low-energy quasiparticles in the absence of spatial disorder, obtained by coupling a Fermi liquid to a gapless boson; a systematic large $N$ theory of such a critical Fermi surface, with SYK characteristics, is obtained by averaging over an ensemble of theories with random boson-fermion couplings. Finally, we present an overview of the links between the SYK model and quantum gravity and end with an outlook on open questions.

cond-mat.str-el↗

Theory of a continuous bandwidth-tuned Wigner-Mott transition

We develop a theory for a continuous bandwidth-tuned transition at fixed \textit{fractional} electron filling from a metal with a generic Fermi surface to a `Wigner-Mott' insulator that spontaneously breaks crystalline space-group symmetries. Across the quantum critical point, (i) the entire electronic Fermi surface disappears abruptly upon approaching from the metallic side, and (ii) the insulating charge gap and various order parameters associated with the spontaneously broken space-group symmetries vanish continuously upon approaching from the insulating side. Additionally, the insulating side hosts a Fermi surface of neutral spinons. We present a framework for describing such continuous metal-insulator transitions (MITs) and analyze the example of a bandwidth-tuned transition at a filling, $ν=1/6$, for spinful electrons on the triangular lattice. By extending the theory to a certain large-$N$ limit, we provide a concrete example of such a continuous MIT and discuss numerous experimental signatures near the critical point. We place our results in the context of recent experiments in moiré transition metal dichalcogenide materials.

cond-mat.str-el↗

Universal scaling for disordered viscoelastic matter near the onset of rigidity

The onset of rigidity in interacting liquids, as they undergo a transition to a disordered solid, is associated with a rearrangement of the low-frequency vibrational spectrum. In this letter, we derive scaling forms for the singular dynamical response of disordered viscoelastic networks near both jamming and rigidity percolation. Using effective-medium theory, we extract critical exponents, invariant scaling combinations and analytical formulas for universal scaling functions near these transitions. Our scaling forms describe the behavior in space and time near the various onsets of rigidity, for rigid and floppy phases and the crossover region, including diverging length and time scales at the transitions.

cond-mat.soft↗

Universal scaling for disordered viscoelastic matter II: Collapses, global behavior and spatio-temporal properties

Disordered viscoelastic materials are ubiquitous and exhibit fascinating invariant scaling properties. In a companion article, we have presented comprehensive new results for the critical behavior of the dynamic susceptibility of disordered elastic systems near the onset of rigidity. Here we provide additional details of the derivation of the singular scaling forms of the longitudinal response near both jamming and rigidity percolation. We then discuss global aspects associated with these forms, and make scaling collapse plots for both undamped and overdamped dynamics in both the rigid and floppy phases. We also derive critical exponents, invariant scaling combinations and analytical formulas for universal scaling functions of several quantities such as transverse and density responses, elastic moduli, viscosities, and correlation functions. Finally, we discuss tentative experimental protocols to measure these behaviors in colloidal suspensions.

cond-mat.soft↗

Interpreting Angle Dependent Magnetoresistance in Layered Materials: Application to Cuprates

The evolution of the low temperature electronic structure of the cuprate metals from the overdoped to the underdoped side has recently been addressed through Angle-Dependant Magneto-Resistance (ADMR) experiments in La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$. The results show a striking difference between hole dopings $p = 0.24$ and $p = 0.21$ which lie on either side of a putative quantum critical point at intermediate $p$. Motivated by this, we here study the theory of ADMR in correlated layered materials, paying special attention to the role of angle dependent quasiparticle weights $Z_{\mathbf{k}}$. Such a $Z_{\mathbf{k}}$ is expected to characterize a number of popular models of the cuprate materials, particularly when underdoped. Further, in the limit of weak interlayer hopping the quasiparticle weight will affect the $c$-axis transport measured in ADMR experiments. We show that proper inclusion of the quasiparticle weight does not support an interpretation of the data in terms of a $(π, π)$ spin density wave ordered state, in agreement with the lack of direct evidence for such order. We show that a simple model of Fermi surface reconfiguring across a van Hove point captures many of the striking differences seen between $p = 0.21$ and $p = 0.24$. We comment on why such a model may be appropriate for interpreting the ADMR data, despite having a large Fermi surface at $p = 0.21$, seemingly in contradiction with other evidence for a small Fermi surafce at that doping level.

cond-mat.str-el↗

Heuristic bounds on superconductivity and how to exceed them

What limits the value of the superconducting transition temperature ($T_c$) is a question of great fundamental and practical importance. Various heuristic upper bounds on $T_c$ have been proposed, expressed as fractions of the Fermi temperature, $T_F$, the zero-temperature superfluid stiffness, $ρ_s(0)$, or a characteristic Debye frequency, $ω_0$. We show that while these bounds are physically motivated and are certainly useful in many relevant situations, none of them serve as a fundamental bound on $T_c$. To demonstrate this, we provide explicit models where $T_c/T_F$ (with an appropriately defined $T_F$), $T_c/ρ_s(0)$, and $T_c/ω_0$ are unbounded.

cond-mat.supr-con↗

Does filling-dependent band renormalization aid pairing in twisted bilayer graphene?

Magic-angle twisted bilayer graphene exhibits a panoply of many-body phenomena that are intimately tied to the appearance of narrow and well-isolated electronic bands. The microscopic ingredients that are responsible for the complex experimental phenomenology include electron-electron (phonon) interactions and non-trivial Bloch wavefunctions associated with the narrow bands. Inspired by recent experiments, we focus on two independent quantities that are considerably modified by Coulomb interaction driven band renormalization, namely the density of states and the minimal spatial extent associated with the Wannier functions. First, we show that a filling-dependent enhancement of the density of states, caused by band flattening, in combination with phonon-mediated attraction due to electron-phonon umklapp processes, increases the tendency towards superconducting pairing in a range of angles around magic-angle. Second, we demonstrate that the minimal spatial extent associated with the Wannier functions, which contributes towards increasing the superconducting phase stiffness, also develops a non-trivial enhancement due to the interaction induced renormalization of the Bloch wavefunctions. While our modeling of superconductivity assumes a weak electron-phonon coupling and does not consider many of the likely relevant correlation effects, it explains simply the experimentally observed robustness of superconductivity in the wide range of angles that occurs in the relevant range of fillings.

cond-mat.str-el↗

Pairing in magic-angle twisted bilayer graphene: role of phonon and plasmon umklapp

Identifying the microscopic mechanism for superconductivity in magic-angle twisted bilayer graphene (MATBG) is an outstanding open problem. While MATBG exhibits a rich phase-diagram, driven partly by the strong interactions relative to the electronic bandwidth, its single-particle properties are unique and likely play an important role in some of the phenomenological complexity. Some of the salient features include an electronic bandwidth smaller than the characteristic phonon bandwidth and a non-trivial structure of the underlying Bloch wavefunctions. We perform a theoretical study of the cooperative effects due to phonons and plasmons on pairing in order to disentangle the distinct role played by these modes on superconductivity. We consider a variant of MATBG with an enlarged number of fermion flavors, $N \gg 1$, where the study of pairing instabilities reduces to the conventional (weak-coupling) Eliashberg framework. In particular, we show that certain umklapp processes involving mini-optical phonon modes, which arise physically as a result of the folding of the original acoustic branch of graphene due to the moiré superlattice structure, contribute significantly towards enhancing pairing. We also investigate the role played by the dynamics of the screened Coulomb interaction on pairing, which leads to an enhancement in a narrow window of fillings, and study the effect of external screening due to a metallic gate on superconductivity. At strong coupling the dynamical pairing interaction leaves a spectral mark in the single particle tunneling density of states. We thus predict such features will appear at specific frequencies of the umklapp phonons corresponding to the sound velocity of graphene times an integer multiple of the Brillouin zone size.

cond-mat.supr-con↗

Bad metallic transport in geometrically frustrated models

We study the transport properties for a family of geometrically frustrated models on the triangular lattice with an interaction scale far exceeding the single-particle bandwidth. Starting from the interaction-only limit, which can be solved exactly, we analyze the transport and thermodynamic behavior as a function of filling and temperature at the leading non-trivial order in the single-particle hopping. Over a broad range of intermediate temperatures, we find evidence of a dc resistivity scaling linearly with temperature and with typical values far exceeding the quantum of resistance, $h/e^2$. At a sequence of commensurate fillings, the bad-metallic regime eventually crosses over into interaction induced insulating phases in the limit of low temperatures. We discuss the relevance of our results to experiments in cold-atom and moiré heterostructure based platforms.

cond-mat.str-el↗

Continuous Mott transition in semiconductor moiré superlattices

The evolution of a Landau Fermi liquid into a nonmagnetic Mott insulator with increasing electronic interactions is one of the most puzzling quantum phase transitions in physics. The vicinity of the transition is believed to host exotic states of matter such as quantum spin liquids, exciton condensates and unconventional superconductivity. Semiconductor moiré materials realize a highly controllable Hubbard model simulator on a triangular lattice, providing a unique opportunity to drive a metal-insulator transition (MIT) via continuous tuning of the electronic interactions. Here, by electrically tuning the effective interaction strength in MoTe2/WSe2 moiré superlattices, we observe a continuous MIT at a fixed filling of one electron per unit cell. The existence of quantum criticality is supported by the scaling behavior of the resistance, a continuously vanishing charge-gap as the critical point is approached from the insulating side, and a diverging quasiparticle effective mass from the metallic side. We also observe a smooth evolution of the low-temperature magnetic susceptibility across the MIT and find no evidence of long-range magnetic order down to ~ 5% of the Curie-Weiss temperature. The results signal an abundance of low-energy spinful excitations on the insulating side that is further corroborated by the presence of the Pomeranchuk effect on the metallic side. Our results are consistent with the universal critical theory of a continuous MIT from a Landau Fermi liquid to a nonmagnetic Mott insulator in two dimensions.

cond-mat.str-el↗

Direct observation of distinct minibands in moiré superlattices

Moiré superlattices comprised of stacked two-dimensional materials present a versatile platform for engineering and investigating new emergent quantum states of matter. At present, the vast majority of investigated systems have long moiré wavelengths, but investigating these effects at shorter, incommensurate wavelengths, and at higher energy scales, remains a challenge. Here, we employ angle-resolved photoemission spectroscopy (ARPES) with sub-micron spatial resolution to investigate a series of different moiré superlattices which span a wide range of wavelengths, from a short moiré wavelength of 0.5 nm for a graphene/WSe2 (g/WSe2) heterostructure, to a much longer wavelength of 8 nm for a WS2/WSe2 heterostructure. We observe the formation of minibands with distinct dispersions formed by the moiré potential in both systems. Finally, we discover that the WS2/WSe2 heterostructure can imprint a surprisingly large moiré potential on a third, separate layer of graphene (g/WS2/WSe2), suggesting a new avenue for engineering moiré superlattices in two-dimensional materials.

cond-mat.mtrl-sci↗

Deconfined Metal-Insulator Transitions in Quantum Hall Bilayers

We propose that quantum Hall bilayers in the presence of a periodic potential at the scale of the magnetic length can host examples of a Deconfined Metal-Insulator Transition (DMIT), where a Fermi liquid (FL) metal with a generic electronic Fermi surface evolves into a gapped insulator (or, an insulator with Goldstone modes) through a continuous quantum phase transition. The transition can be accessed by tuning a single parameter, and its universal critical properties can be understood using a controlled framework. At the transition, the two layers are effectively decoupled, where each layer undergoes a continuous transition from a FL to a generalized composite Fermi liquid (gCFL). The thermodynamic and transport properties of the gCFL are similar to the usual CFL, while its spectral properties are qualitatively different. The FL-gCFL quantum critical point hosts a sharply defined Fermi surface without long-lived electronic quasiparticles. Immediately across the transition, the two layers of gCFL are unstable to forming an insulating phase. We discuss the topological properties of the insulator and various observable signatures associated with the DMIT.

cond-mat.str-el↗