arXiv subjects

Deborah S. Jin

Publications and source records attributed to Deborah S. Jin.

At least 19 recordsLinked to original sources

arXiv2017

Observation of Efimov molecules created from a resonantly interacting Bose gas

We convert a strongly interacting ultracold Bose gas into a mixture of atoms and molecules by sweeping the interactions from resonant to weak. By analyzing the decay dynamics of the molecular gas, we show that in addition to Feshbach dimers it contains Efimov trimers. Typically around 8\% of the total atomic population is bound into trimers, identified by their density-independent lifetime of about 100~$μ$s. The lifetime of the Feshbach dimers shows a density dependence due to inelastic atom-dimer collisions, in agreement with theoretical calculations. We also vary the density of the gas across a factor of 250 and investigate the corresponding atom loss rate at the interaction resonance.

cond-mat.quant-gas↗

arXiv2017

Universal dynamics of a degenerate unitary Bose gas

Understanding the rich behavior that emerges from systems of interacting quantum particles, such as electrons in materials, nucleons in nuclei or neutron stars, the quark-gluon plasma, and superfluid liquid helium, requires investigation of systems that are clean, accessible, and have tunable parameters. Ultracold quantum gases offer tremendous promise for this application largely due to an unprecedented control over interactions. Specifically, $a$, the two-body scattering length that characterizes the interaction strength, can be tuned to any value. This offers prospects for experimental access to regimes where the behavior is not well understood because interactions are strong, atom-atom correlations are important, mean-field theory is inadequate, and equilibrium may not be reached or perhaps does not even exist. Of particular interest is the unitary gas, where $a$ is infinite, and where many aspects of the system are universal in that they depend only on the particle density and quantum statistics. While the unitary Fermi gas has been the subject of intense experimental and theoretical investigation, the degenerate unitary Bose gas has generally been deemed experimentally inaccessible because of three-body loss rates that increase dramatically with increasing $a$. Here, we investigate dynamics of a unitary Bose gas for timescales that are short compared to the loss. We find that the momentum distribution of the unitary Bose gas evolves on timescales fast compared to losses, and that both the timescale for this evolution and the limiting shape of the momentum distribution are consistent with universal scaling with density. This work demonstrates that a unitary Bose gas can be created and probed dynamically, and thus opens the door for further exploration of this novel strongly interacting quantum liquid.

quant-ph↗

arXiv2016

New frontiers with quantum gases of polar molecules

The field of ultracold quantum matter has burgeoned over the last few decades, thanks to the growing capabilities for atomic systems to be probed and manipulated with exquisite control. Researchers can now precisely create and study quantum many-body states that are effectively isolated from the external environment. Much of the work in ultracold matter has focused on systems of alkali or alkaline-earth atoms, mainly due to their ease of cooling. Extending this precise control to molecules has seen rapidly increasing interest and activity, as molecules possess additional degrees of freedom that make them useful for tests of fundamental physics, studying ultracold chemistry and collisions, and engineering qualitatively new types of quantum phases and quantum many-body systems. Here, we review one particularly fruitful research direction: the creation and manipulation of ultracold bialkali molecules. The recent success in creating a quantum gas of polar molecules opens many exciting research opportunities.

cond-mat.quant-gas↗

arXiv2016

Controlling a quantum gas of polar molecules in an optical lattice

The production of molecules from dual species atomic quantum gases has enabled experiments that employ molecules at nanoKelvin temperatures. As a result, every degree of freedom of these molecules is in a well-defined quantum state and exquisitely controlled. These ultracold molecules open a new world of precision quantum chemistry in which quantum statistics, quantum partial waves, and even many-body correlations can play important roles. Moreover, to investigate the strongly correlated physics of many interacting molecular dipoles, we can mitigate lossy chemical reactions by controlling the dimensionality of the system using optical lattices formed by interfering laser fields. In a full three-dimensional optical lattice, chemistry can be turned on or off by tuning the lattice depth, which allows us to configure an array of long-range interacting quantum systems with rich internal structure. Such a system represents an excellent platform for gaining fundamental insights to complex materials based on quantum simulations and also for quantum information processing in the future.

cond-mat.quant-gas↗

arXiv2016

Bose polarons in the strongly interacting regime

When an impurity is immersed in a Bose-Einstein condensate, impurity-boson interactions are expected to dress the impurity into a quasiparticle, the Bose polaron. We superimpose an ultracold atomic gas of $^{87}$Rb with a much lower density gas of fermionic $^{40}$K impurities. Through the use of a Feshbach resonance and RF spectroscopy, we characterize the energy, spectral width and lifetime of the resultant polaron on both the attractive and the repulsive branches in the strongly interacting regime. The width of the polaron in the attractive branch is narrow compared to its binding energy, even as the two-body scattering length formally diverges.

cond-mat.quant-gas↗

arXiv2015

Doublon dynamics and polar molecule production in an optical lattice

Ultracold polar molecules provide an excellent platform to study quantum many-body spin dynamics, which has become accessible in the recently realized low entropy quantum gas of polar molecules in an optical lattice. To obtain a detailed understanding for the molecular formation process in the lattice, we prepare a density distribution where lattice sites are either empty or occupied by a doublon composed of a bosonic atom interacting with a fermionic atom. By letting this disordered, out-of-equilibrium system evolve from a well-defined initial condition, we observe clear effects on pairing that arise from inter-species interactions, a higher partial wave Feshbach resonance, and excited Bloch-band population. When only the lighter fermions are allowed to tunnel in the three-dimensional (3D) lattice, the system dynamics can be well described by theory. However, in a regime where both fermions and bosons can tunnel, we encounter correlated dynamics that is beyond the current capability of numerical simulations. Furthermore, we show that we can probe the microscopic distribution of the atomic gases in the lattice by measuring the inelastic loss of doublons. These techniques realize tools that are generically applicable to heteronuclear diatomic systems in optical lattices and can shed light on molecule production as well as dynamics of a Bose-Fermi mixture.

cond-mat.quant-gas↗

arXiv2015

Creation of a low-entropy quantum gas of polar molecules in an optical lattice

Ultracold polar molecules, with their long-range electric dipolar interactions, offer a unique platform for studying correlated quantum many-body phenomena such as quantum magnetism. However, realizing a highly degenerate quantum gas of molecules with a low entropy per particle has been an outstanding experimental challenge. In this paper, we report the synthesis of a low entropy molecular quantum gas by creating molecules at individual sites of a three-dimensional optical lattice that is initially loaded from a low entropy mixture of K and Rb quantum gases. We make use of the quantum statistics and interactions of the initial atom gases to load into the optical lattice, simultaneously and with good spatial overlap, a Mott insulator of bosonic Rb atoms and a single-band insulator of fermionic K atoms. Then, using magneto-association and optical state transfer, we efficiently produce ground-state molecules in the lattice at those sites that contained one Rb and one K atom. The achieved filling fraction of 25% indicates an entropy as low as $2.2\,k_B$ per molecule. This low-entropy molecular quantum gas opens the door to novel studies of transport and entanglement propagation in a many-body system with long-range dipolar interactions.

cond-mat.quant-gas↗

arXiv2015

Breakdown of Fermi liquid description for strongly interacting fermions

The nature of the normal state of an ultracold Fermi gas in the BCS-BEC crossover regime is an intriguing and controversial topic. While the many-body ground state remains a condensate of paired fermions, the normal state must evolve from a Fermi liquid to a Bose gas of molecules as a function of the interaction strength. How this occurs is still largely unknown. We explore this question with measurements of the distribution of single-particle energies and momenta in a nearly homogeneous gas above $T_c$. The data fit well to a function that includes a narrow, positively dispersing peak that corresponds to quasiparticles and an "incoherent background" that can accommodate broad, asymmetric line shapes. We find that the quasiparticle's spectral weight vanishes abruptly as the strength of interactions is modified, which signals the breakdown of a Fermi liquid description. Such a sharp feature is surprising in a crossover.

cond-mat.quant-gas↗

arXiv2014

Looking for "avalanche-mechanism" loss at an atom-molecule Efimov resonance

The "avalanche mechanism" has been used to relate Efimov trimer states to certain enhanced atom loss features observed in ultracold atom gas experiments. These atom loss features are argued to be a signature of resonant atom-molecule scattering that occurs when an Efimov trimer is degenerate with the atom-molecule scattering threshold. However, observation of these atom loss features has yet to be combined with the direct observation of atom-molecule resonant scattering for any particular atomic species. In addition, recent Monte-Carlo simulations were unable to reproduce a narrow loss feature. We experimentally search for enhanced atom loss features near an established scattering resonance between 40K87Rb Feshbach molecules and 87Rb atoms. Our measurements of both the three-body recombination rate in a gas of 40K and 87Rb atoms and the ratio of the number loss for the two species do not show any broad loss feature and are therefore inconsistent with theoretical predictions that use the avalanche mechanism.

cond-mat.quant-gas↗

arXiv2014

Many-body dynamics of dipolar molecules in an optical lattice

Understanding the many-body dynamics of isolated quantum systems is one of the central challenges in modern physics. To this end, the direct experimental realization of strongly correlated quantum systems allows one to gain insights into the emergence of complex phenomena. Such insights enable the development of theoretical tools that broaden our understanding. Here, we theoretically model and experimentally probe with Ramsey spectroscopy the quantum dynamics of disordered, dipolar-interacting, ultracold molecules in a partially filled optical lattice. We report the capability to control the dipolar interaction strength, and we demonstrate that the many-body dynamics extends well beyond a nearest-neighbor or mean-field picture, and cannot be quantitatively described using previously available theoretical tools. We develop a novel cluster expansion technique and demonstrate that our theoretical method accurately captures the measured dependence of the spin dynamics on molecule number and on the dipolar interaction strength. In the spirit of quantum simulation, this agreement simultaneously benchmarks the new theoretical method and verifies our microscopic understanding of the experiment. Our findings pave the way for numerous applications in quantum information science, metrology, and condensed matter physics.

cond-mat.quant-gas↗

arXiv2013

Suppressing the loss of ultracold molecules via the continuous quantum Zeno effect

We investigate theoretically the suppression of two-body losses when the on-site loss rate is larger than all other energy scales in a lattice. This work quantitatively explains the recently observed suppression of chemical reactions between two rotational states of fermionic KRb molecules confined in one-dimensional tubes with a weak lattice along the tubes [Yan et al., Nature 501, 521-525 (2013)]. New loss rate measurements performed for different lattice parameters but under controlled initial conditions allow us to show that the loss suppression is a consequence of the combined effects of lattice confinement and the continuous quantum Zeno effect. A key finding, relevant for generic strongly reactive systems, is that while a single-band theory can qualitatively describe the data, a quantitative analysis must include multiband effects. Accounting for these effects reduces the inferred molecule filling fraction by a factor of five. A rate equation can describe much of the data, but to properly reproduce the loss dynamics with a fixed filling fraction for all lattice parameters we develop a mean-field model and benchmark it with numerically exact time-dependent density matrix renormalization group calculations.

quant-ph↗

arXiv2013

Differential Scattering and Rethermalization in Ultracold Dipolar Gases

Analytic expressions for the differential cross sections of ultracold atoms and molecules that scatter primarily due to dipolar interactions are derived within the first Born approximation, and are shown to agree with the partial wave expansion. These cross sections are applied to the problem of cross-dimensional rethermalization. Strikingly, the rate of rethermalization can vary by as much as a factor of two, depending on the orientation of polarization of the dipoles. Thus the anisotropic dipole-dipole interaction can have a profound effect even on the behavior of a nondegenerate ultracold gas.

physics.atom-ph↗

arXiv2013

Feshbach molecule formation in a Bose-Fermi mixture

We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of $^{40}$K and $^{87}$Rb atoms, where we can create as many as $7\times 10^4$ $^{40}$K$^{87}$Rb molecules with a conversion efficiency as high as 45%. In the perturbative regime, we find that the conversion efficiency depends linearly on the density overlap of the two gases, with a slope that matches a parameter-free model that uses only the atom masses and the known Feshbach resonance parameters. In the saturated regime, we find that the maximum number of Feshbach molecules depends on the atoms' phase-space density. At higher temperatures, our measurements agree with a phenomenological model that successfully describes the formation of bosonic molecules from either Bose or Fermi gases. However, for quantum degenerate atom gas mixtures, we measure significantly fewer molecules than this model predicts.

cond-mat.quant-gas↗

arXiv2013

Tests of universal three-body physics in an ultracold Bose-Fermi mixture

Recent measurements of Efimov resonances in a number of ultracold atom species have revealed an unexpected universality, in which three-body scattering properties are determined by the van der Waals length of the two-body interaction potential. To investigate whether this universality extends to heteronuclear mixtures, we measure loss rate coefficients in an ultracold trapped gas of $^{40}$K and $^{87}$Rb atoms. We find an Efimov-like resonance in the rate of inelastic collisions between $^{40}$K$^{87}$Rb Feshbach molecules and $^{87}$Rb atoms. However, we do not observe any Efimov-related resonances in the rates of inelastic collisions between three atoms. These observations are compared to previous measurements by the LENS group of Efimov resonances in a $^{41}$K and $^{87}$Rb mixture as well as to recent predictions.

cond-mat.quant-gas↗

arXiv2013

Realizing a lattice spin model with polar molecules

With the recent production of polar molecules in the quantum regime, long-range dipolar interactions are expected to facilitate the understanding of strongly interacting many-body quantum systems and to realize lattice spin models for exploring quantum magnetism. In atomic systems, where interactions require wave function overlap, effective spin interactions on a lattice can be realized via superexchange; however, the coupling is weak and limited to nearest-neighbor interactions. In contrast, dipolar interactions exist in the absence of tunneling and extend beyond nearest neighbors. This allows coherent spin dynamics to persist even at high entropy and low lattice filling. Effects of dipolar interactions in ultracold molecular gases have so far been limited to the modification of chemical reactions. We now report the observation of dipolar interactions of polar molecules pinned in a 3D optical lattice. We realize a lattice spin model with spin encoded in rotational states, prepared and probed by microwaves. This spin-exchange interaction arises from the resonant exchange of rotational angular momentum between two molecules. We observe clear oscillations in the evolution of the spin coherence in addition to an overall decay. The frequency of these oscillations, the strong dependence of the spin coherence time on the lattice filling, and the effect of a multi-pulse sequence designed to reverse dynamics due to two-body exchange interactions all provide evidence of dipolar interactions. We also demonstrate suppression of loss in weak lattices due to a quantum Zeno mechanism. Measurements of these tunneling-induced losses allow us to independently determine the lattice filling factor. These results comprise an initial exploration of the behavior of many-body spin models with direct, long-range spin interactions and lay the groundwork for future studies of many-body dynamics in spin lattices.

physics.atom-ph↗

arXiv2012

Measurement of the Homogeneous Contact of a Unitary Fermi gas

By selectively probing the center of a trapped gas, we measure the local, or homogeneous, contact of a unitary Fermi gas as a function of temperature. Tan's contact, C, is proportional to the derivative of the energy with respect to the interaction strength, and is thus an essential thermodynamic quantity for a gas with short-range correlations. Theoretical predictions for the temperature dependence of C differ substantially, especially near the superfluid transition, Tc, where C is predicted to either sharply decrease, sharply increase, or change very little. For T/T_F>0.4, our measurements of the homogeneous gas contact show a gradual decrease of C with increasing temperature, as predicted by theory. We observe a sharp decrease in C at T/T_F=0.16, which may be due to the superfluid phase transition. While a sharp decrease in C below Tc is predicted by some many-body theories, we find that none of the predictions fully accounts for the data.

cond-mat.quant-gas↗

arXiv2011

Long-lived dipolar molecules and Feshbach molecules in a 3D optical lattice

We have realized long-lived ground-state polar molecules in a 3D optical lattice, with a lifetime of up to 25 s, which is limited only by off-resonant scattering of the trapping light. Starting from a 2D optical lattice, we observe that the lifetime increases dramatically as a small lattice potential is added along the tube-shaped lattice traps. The 3D optical lattice also dramatically increases the lifetime for weakly bound Feshbach molecules. For a pure gas of Feshbach molecules, we observe a lifetime of >20 s in a 3D optical lattice; this represents a 100-fold improvement over previous results. This lifetime is also limited by off-resonant scattering, the rate of which is related to the size of the Feshbach molecule. Individually trapped Feshbach molecules in the 3D lattice can be converted to pairs of K and Rb atoms and back with nearly 100% efficiency.

physics.atom-ph↗

arXiv2005

Fermi Condensates

Ultracold atomic gases have proven to be remarkable model systems for exploring quantum mechanical phenomena. Experimental work on gases of fermionic atoms in particular has seen large recent progress including the attainment of so-called Fermi condensates. In this article we will discuss this recent development and the unique control over interparticle interactions that made it possible.

cond-mat.other↗