arXiv subjects

Demian Levis

Publications and source records attributed to Demian Levis.

At least 37 records · Page 2Linked to original sources

arXiv2022

Dynamics of Motility-Induced clusters: coarsening beyond Ostwald ripening

We study the dynamics of clusters of Active Brownian Disks generated by Motility-Induced Phase Separation, by applying an algorithm that we devised to track cluster trajectories. We identify an aggregation mechanism that goes beyond Ostwald ripening but also yields $z=3$. Active clusters of mass $M$ self-propel with enhanced diffusivity $D\sim$ Pe$^2/\sqrt{M}$. Their fast motion drives aggregation into large fractal structures, which are patchworks of diverse hexatic orders, and coexist with regular, orientationally uniform, smaller ones. To bring out the impact of activity, we perform a comparative study of a passive system that evidences major differences with the active case.

cond-mat.stat-mech↗

arXiv2022

Chiral Active Matter

Chiral active matter comprises particles which can self-propel and self-rotate. Examples range from sperm cells and bacteria near walls to asymmetric colloids and pea-shaped Quincke rollers. In this perspective article we focus on recent developments in chiral active matter. After briefly discussing chiral active motion at a single particle level, we discuss collective phenomena ranging from vortex arrays and patterns made of rotating micro-flocks to states featuring unusual rheological properties.

cond-mat.soft↗

arXiv2022

Dynamics of Topological Defects in the noisy Kuramoto Model in two dimensions

We consider the two-dimensional (2D) noisy Kuramoto model of synchronization with short-range coupling and a Gaussian distribution of intrinsic frequencies, and investigate its ordering dynamics following a quench. We consider both underdamped (inertial) and over-damped dynamics, and show that the long-term properties of this intrinsically out-of-equilibrium system do not depend on the inertia of individual oscillators. The model does not exhibit any phase transition as its correlation length remains finite, scaling as the inverse of the standard deviation of the distribution of intrinsic frequencies. The quench dynamics proceeds via domain growth, with a characteristic length that initially follows the growth law of the 2D XY model, although is not given by the mean separation between defects. Topological defects are generically free, breaking the Berezinskii-Kosterlitz-Thouless scenario of the 2D XY model. Vortices perform a random walk reminiscent of the self-avoiding random walk, advected by the dynamic network of boundaries between synchronised domains; featuring long-time super-diffusion, with the anomalous exponent $α=3/2$.

cond-mat.stat-mech↗

arXiv2022

Microscopic field theory for structure formation in systems of self-propelled particles with generic torques

We derive a dynamical field theory for self-propelled particles subjected to generic torques and forces by explicitly coarse-graining their microscopic dynamics, described by a many-body Fokker-Planck equation. The model includes both intrinsic torques inducing self-rotation, as well as interparticle torques leading to, for instance, the local alignment of particles' orientations. Within this approach, although the functional form of the pairwise interactions does not need to be specified, one can directly map the parameters of the field theory onto the parameters of particle-based models. We perform a linear stability analysis of the homogeneous solution of the field equations and find both long-wavelength and short-wavelength instabilities. The former signals the emergence of a macroscopic structure, which we associate with motility-induced phase separation, while the second one signals the growth of a finite structure with a characteristic size. Intrinsic torques hinder phase separation, pushing the onset of the long-wavelength instability to higher activities. Further, they generate finite-sized structures with a characteristic size proportional to both the self-propulsion velocity and the inverse of the self-rotation frequency. Our results show that a general mechanism might explain why chirality tends to suppress motility-induced phase separation but instead promotes the formation of non-equilibrium patterns.

cond-mat.soft↗

arXiv2022

From Motility-Induced Phase-Separation to Glassiness in Dense Active Matter

Dense active systems are widespread in nature, examples range from bacterial colonies to biological tissues. Dense clusters of active particles can be obtained by increasing the packing fraction of the system or taking advantage of a peculiar phenomenon named motility-induced phase separation (MIPS). In this work, we explore the phase diagram of a two-dimensional model of active glass and show that disordered active materials develop a rich collective behaviour encompassing both MIPS and glassiness. We find that, although the glassy state is almost indistinguishable from that of equilibrium glasses, the mechanisms leading to its fluidization do not have any equilibrium counterpart. Our results can be rationalized in terms of a crossover between a low-activity regime, where glassy dynamics is controlled by an effective temperature, and a high-activity regime, which drives the system towards MIPS.

cond-mat.soft↗

arXiv2022

Impact of dipole-dipole interactions on motility-induced phase separation

We present a hydrodynamic theory for systems of dipolar active Brownian particles which, in the regime of weak dipolar coupling, predicts the onset of motility-induced phase separation (MIPS), consistent with Brownian dynamics (BD) simulations. The hydrodynamic equations are derived by explicitly coarse-graining the microscopic Langevin dynamics, thus allowing for a quantitative comparison of parameters entering the coarse-grained model and particle-resolved simulations. Performing BD simulations at fixed density, we find that dipolar interactions tend to hinder MIPS, as first reported in [Liao et al., Soft Matter, 2020, 16, 2208]. Here we demonstrate that the theoretical approach indeed captures the suppression of MIPS. Moreover, the analysis of the numerically obtained, angle-dependent correlation functions sheds light into the underlying microscopic mechanisms leading to the destabilization of the homogeneous phase.

cond-mat.soft↗

arXiv2022

Epidemic processes on self-propelled particles: continuum and agent-based modelling

Most spreading processes require spatial proximity between agents. The stationary state of spreading dynamics in a population of mobile agents thus depends on the interplay between the time and length scales involved in the epidemic process and their motion in space. We analyze the steady properties resulting from such interplay in a simple model describing epidemic spreading (modeled as a Susceptible-Infected-Susceptible process) on self-propelled particles (performing Run-and-Tumble motion). Focusing our attention on the diffusive long-time regime, we find that the agents' motion changes qualitatively the nature of the epidemic transition characterized by the emergence of a macroscopic fraction of infected agents. Indeed, the transition becomes of the mean-field type for agents diffusing in one, two and three dimensions, while, in the absence of motion, the epidemic outbreak depends on the dimension of the underlying static network determined by the agents' fixed locations. The insights obtained from a continuum description of the system are validated by numerical simulations of an agent-based model. Our work aims at bridging soft active matter physics and theoretical epidemiology, and may be of interest for researchers in both communities.

cond-mat.stat-mech↗

arXiv2021

Phase separation of self-propelled disks with ferromagnetic and nematic alignment

We present a comprehensive study of a model system of repulsive self-propelled disks in two dimensions with ferromagnetic and nematic velocity alignment interactions. We characterize the phase behavior of the system as a function of the alignment and self-propulsion strength, featuring orientational order for strong alignment and Motility-Induced Phase Separation (MIPS) at moderate alignment but high enough self-propulsion. We derive a microscopic theory for these systems yielding a close set of hydrodynamic equations from which we perform a linear stability analysis of the homogenous disordered state. This analysis predicts MIPS in the presence of aligning torques. The nature of the continuum theory allows for an explicit quantitative comparison with particle-based simulations, which consistently shows that ferromagnetic alignment fosters phase separation, while nematic alignment does not alter either the nature or the location of the instability responsible for it. In the ferromagnetic case, such behavior is due to an increase of the imbalance of the number of particle collisions along different orientations, giving rise to the self-trapping of particles along their self-propulsion direction. On the contrary, the anisotropy of the pair correlation function, which encodes this self-trapping effect, is not significantly affected by nematic torques. Our work shows the predictive power of such microscopic theories to describe complex active matter systems with different interaction symmetries and sheds light on the impact of velocity-alignment interactions in Motility-Induced Phase Separation.

cond-mat.soft↗

arXiv2021

Motility-Induced Microphase and Macrophase Separation in a Two-Dimensional Active Brownian Particle System

As a result of nonequilibrium forces, purely repulsive self-propelled particles undergo macrophase separation between a dense and a dilute phase. We present a thorough study of the ordering kinetics of such motility-induced phase separation (MIPS) in active Brownian particles in two dimensions, and we show that it is generically accompanied by microphase separation. The growth of the dense phase follows a law akin to the one of liquid-gas phase separation. However, it is made of a mosaic of hexatic microdomains whose size does not coarsen indefinitely, leaving behind a network of extended topological defects from which microscopic dilute bubbles arise. The characteristic length of these finite-size structures increases with activity, independently of the choice of initial conditions.

cond-mat.stat-mech↗

arXiv2021

Unified analysis of Topological Defects in 2D systems of Active and Passive disks

We provide a comprehensive quantitative analysis of localized and extended topological defects in the steady state of 2D passive and active repulsive Brownian disk systems. We show that, both in and out-of-equilibrium, the passage from the solid to the hexatic is driven by the unbinding of dislocations, in quantitative agreement with the KTHNY singularity. Instead, although disclinations dissociate as soon as the liquid phase appears, extended clusters of defects largely dominate below the solid-hexatic critical line. The latter percolate in the liquid phase very close to the hexatic-liquid transition, both for continuous and discontinuous transitions, in the homogeneous liquid regime. At critical percolation the clusters of defects are fractal with statistical and geometric properties that, within our numerical accuracy, are independent of the activity and compatible with the universality class of uncorrelated critical percolation. We also characterize the spatial organization of different kinds of point-like defects and we show that the disclinations are not free, but rather always very near more complex defect structures. At high activity, the bulk of the dense phase generated by Motility-Induced Phase Separation is characterized by a density of point-like defects, and statistics and morphology of defect clusters, set by the amount of activity and not the packing fraction. Hexatic domains within the dense phase are separated by grain-boundaries along which a finite network of topological defects resides, interrupted by gas bubbles in cavitation. The fractal dimension of this network diminishes for increasing activity. This structure is dynamic in the sense that the defect network allows for an unzipping mechanism that leaves free space for gas bubbles to appear, close, and even be released into the dilute phase.

cond-mat.stat-mech↗

arXiv2021

Clustering of topological defects in two-dimensional melting of active and passive disks

We provide a quantitative analysis of all kinds of topological defects present in 2D passive and active repulsive disk systems. We show that the passage from the solid to the hexatic is driven by the unbinding of dislocations. Instead, although we see dissociation of disclinations as soon as the liquid phase appears, extended clusters of defects largely dominate below the solid-hexatic critical line. The latter percolate at the hexatic-liquid transition in continuous cases or within the coexistence region in discontinuous ones, and their form gets more ramified for increasing activity.

cond-mat.soft↗

arXiv2021

Defects Superdiffusion and Unbinding in a 2D XY Model of Self-Driven Rotors

We consider a non-equilibrium extension of the two-dimensional (2D) XY model, equivalent to the noisy Kuramoto model of synchronization with short-range coupling, where rotors sitting on a square lattice are self-driven by random intrinsic frequencies. We study the static and dynamic properties of topological defects (vortices) and establish how self-spinning affects the Berezenskii-Kosterlitz-Thouless phase transition scenario. The non-equilibrium drive breaks the quasi-long-range ordered phase of the 2D XY model into a mosaic of ordered domains of controllable size and results in self-propelled vortices that generically unbind at any temperature, featuring superdiffusion $\langle r^2(t)\rangle\sim t^{3/2}$ with a Gaussian distribution of displacements. Our work provides a simple framework to investigate topological defects in active matter and sheds new light on the problem of synchronization of locally coupled oscillators.

cond-mat.stat-mech↗

arXiv2020

Fluctuation-Dissipation Relations in the absence of Detailed Balance: formalism and applications to Active Matter

We present a comprehensive study about the relationship between the way Detailed Balance is broken in non-equilibrium systems and the resulting violations of the Fluctuation-Dissipation Theorem. Starting from stochastic dynamics with both odd and even variables under Time-Reversal, we exploit the relation between entropy production and the breakdown of Detailed Balance to establish general constraints on the non-equilibrium steady-states (NESS), which relate the non-equilibrium character of the dynamics with symmetry properties of the NESS distribution. This provides a direct route to derive extended Fluctuation-Dissipation Relations, expressing the linear response function in terms of NESS correlations. Such framework provides a unified way to understand the departure from equilibrium of active systems and its linear response. We then consider two paradigmatic models of interacting self-propelled particles, namely Active Brownian Particles (ABP) and Active Ornstein-Uhlenbeck Particles (AOUP). We analyze the non-equilibrium character of these systems (also within a Markov and a Chapman-Enskog approximation) and derive extended Fluctuation-Dissipation Relations for them, clarifying which features of these active model systems are genuinely non-equilibrium.

cond-mat.stat-mech↗

arXiv2019

Linear response theory and Green-Kubo relations for active matter

We address the question of how interacting active systems in a non-equilibrium steady-state respond to an external perturbation. We establish an extended fluctuation-dissipation theorem for Active Brownian Particles (ABP) which highlights the role played by the local violation of detailed balance due to activity. By making use of a Markovian approximation we derive closed Green-Kubo expressions for the diffusivity and mobility of ABP and quantify the deviations from the Stokes-Einstein relation. We compute the linear response function to an external force using unperturbed simulations of ABP and compare the results with the analytical predictions of the transport coefficients. Our results show the importance of the interplay between activity and interactions in the departure from equilibrium linear response.

cond-mat.stat-mech↗

arXiv2019

Flocking and spreading dynamics in populations of self-propelled agents

Populations of self-propelled mobile agents - animal groups, robot swarms or crowds of people - that exchange information with their surrounding, host fascinating cooperative behaviors. While in many situations of interest the agents motion is driven by the transmission of information (e.g. the presence of an approaching predator) from neighboring peers, previous modeling efforts have focused on situations where agents either sit on static networks, or move independently of the information spreading across the population. Here, we introduce a reference model to tackle this current lack of general framework. We consider mobile agents which align their direction of motion (based on the Kuramoto dynamics) and carry an internal state governed by the Susceptible-Infected-Susceptible (SIS) epidemic process, characterizing the spread of information in the population, and affecting the way agents move in space. We show that the feedback between the agents motion and information spreading is responsible for (i) the enhancement of both flocking and information spreading, (ii) the emergence of complex spatial structures, or swarms, which can be controlled by the velocity of the agents. The SIS dynamics is able to drive a flocking phase transition even in the absence of explicit velocity-alignment, recovering a behavior reminiscent of Vicsek-like systems but featuring macro-phase separation rather than micro-phase separation. We show that the formation of dense swarms at low velocities reduces the epidemic threshold of information spreading with respect to the mean field limit. By bridging together soft active matter physics and agent based modeling of complex systems, we shed light upon a general positive feedback mechanism that crucially affects the collective behavior of mobile agents, providing a reference framework to study realistic situations where this mechanism is at play.

physics.soc-ph↗

arXiv2019

Simultaneous Phase Separation and Pattern Formation in Chiral Active Mixtures

Chiral active particles, or self-propelled circle swimmers, from sperm cells to asymmetric Janus colloids, form a rich set of patterns, which are different from those seen in linear swimmers. Such patterns have mainly been explored for identical circle swimmers, while real-world circle swimmers, typically possess a frequency distribution. Here we show that even the simplest mixture of (velocity-aligning) circle swimmers with two different frequencies, hosts a complex world of superstructures: The most remarkable example comprises a microflock pattern, formed in one species, while the other species phase separates and forms a macrocluster, coexisting with a gas phase. Here, one species microphase-separates and selects a characteristic length scale, whereas the other one macrophase separates and selects a density. A second notable example, here occurring in an isotropic system, are patterns comprising two different characteristic length scales, which are controllable via frequency and swimming speed of the individual particles.

cond-mat.soft↗

arXiv2019

Activity induced synchronization: From Mutual Flocking to Chiral Self-Sorting

Synchronization, the temporal coordination of coupled oscillators, allows fireflies to flash in unison, neurons to fire collectively and human crowds to fall in step on the London Millenium bridge. Here, we interpret active (or self-propelled) chiral microswimmers with a distribution of intrinsic frequencies as motile oscillators and show that they can synchronize over very large distances, even for local coupling in 2D. This opposes to canonical non-active oscillators on static or time-dependent networks, leading to synchronized domains only. A consequence of this activity-induced synchronization is the emergence of a `mutual flocking phase', where particles of opposite chirality cooperate to form superimposed flocks moving at a relative angle to each other, providing a chiral active matter analogue to the celebrated Toner-Tu phase. The underlying mechanism employs a positive feedback loop involving the two-way coupling between oscillators' phase and self-propulsion, and could be exploited as a design principle for synthetic active materials and chiral self-sorting techniques

cond-mat.stat-mech↗

arXiv2018

Full phase diagram of active Brownian disks: from melting to motility-induced phase separation

We establish the complete phase diagram of self-propelled hard disks in two spatial dimensions from the analysis of the equation of state and the statistics of local order parameters. The equilibrium melting scenario is maintained at small activities, with coexistence between active liquid and hexatic order, followed by a proper hexatic phase and a further transition to an active solid. As activity increases, the emergence of hexatic and solid order is shifted towards higher densities. Above a critical activity and for a certain range of packing fractions, the system undergoes MIPS and demixes into low and high density phases; the latter can be either disordered (liquid) or ordered (hexatic or solid) depending on activity.

cond-mat.stat-mech↗