arXiv subjects

Denis Kochan

Publications and source records attributed to Denis Kochan.

At least 37 records · Page 2Linked to original sources

arXiv2023

Spin-orbit and exchange proximity couplings in graphene/1T-TaS$_2$ heterostructure triggered by a charge density wave

Proximity-induced fine features and spin-textures of the electronic bands in graphene-based van der Waals heterostructures can be explored from the point of tailoring a twist angle. Here we study spin-orbit coupling and exchange coupling engineering of graphene states in the proximity of 1T-TaS$_2$ not triggering the twist, but a charge density wave in 1T-TaS$_2$-a realistic low-temperature phase. Using density functional theory and effective model we found that the emergence of the charge density wave in 1T-TaS$_2$ significantly enhances Rashba spin-orbit splitting in graphene and tilts the spin texture by a significant Rashba angle-in a very similar way as in the conventional twist-angle scenarios. Moreover, the partially filled Ta $d$-band in the charge density wave phase leads to the spontaneous emergence of the in-plane magnetic order that transgresses via proximity from 1T-TaS$_2$ to graphene, hence, simultaneously superimposing along the spin-orbit also the exchange coupling proximity effect. To describe this intricate proximity landscape we have developed an effective model Hamiltonian and provided a minimal set of parameters that excellently reproduces all the spectral features predicted by the first-principles calculations. Conceptually, the charge density wave provides a highly interesting knob to control the fine features of electronic states and to tailor the superimposed proximity effects-a sort of twistronics without twist.

cond-mat.mes-hall↗

arXiv2022

Sign reversal of the AC and DC supercurrent diode effect and 0-$π$-like transitions in ballistic Josephson junctions

The recent discovery of intrinsic supercurrent diode effect, and its prompt observation in a rich variety of systems, has shown that nonreciprocal supercurrents naturally emerge when both space- and time-inversion symmetries are broken. In Josephson junctions, nonreciprocal supercurrent can be conveniently described in terms of spin-split Andreev states. Here, we demonstrate a sign reversal of the supercurrent diode effect, in both its AC and DC manifestations. In particular, the AC diode effect -- i.e., the asymmetry of the Josephson inductance as a function of the supercurrent -- allows us to probe the current-phase relation near equilibrium. Using a minimal theoretical model, we can then link the sign reversal of the AC diode effect to the so-called 0-$π$-like transition, a predicted, but still elusive feature of multi-channel junctions. Our results demonstrate the potential of inductance measurements as sensitive probes of the fundamental properties of unconventional Josephson junctions.

cond-mat.supr-con↗

arXiv2022

Anisotropic vortex squeezing in synthetic Rashba superconductors: a manifestation of Lifshitz invariants

Most of 2D superconductors are of type II, i.e., they are penetrated by quantized vortices when exposed to out-of-plane magnetic fields. In presence of a supercurrent, a Lorentz-like force acts on the vortices, leading to drift and dissipation. The current-induced vortex motion is impeded by pinning at defects, enabling the use of superconductors to generate high magnetic fields without dissipation. Usually, the pinning strength decreases upon any type of pair-breaking. Here we show that in Rashba superconductors the application of an in-plane field leads, instead, to an unexpected enhancement of pinning. When rotating the in-plane component of the field with respect to the current direction, the vortex inductance turns out to be highly anisotropic. We explain this phenomenon as a manifestation of Lifshitz invariant terms in the Ginzburg-Landau free energy, which are enabled by inversion and time-reversal symmetry breaking and lead to an elliptic squeezing of vortex cores. Our experiment provides access to a fundamental property of Rashba superconductors and offers an entirely new approach to vortex manipulation.

cond-mat.supr-con↗

arXiv2022

Spin relaxation, Josephson effect and Yu-Shiba-Rusinov states in superconducting bilayer graphene

Bilayer graphene has two non-equivalent sublattices and, therefore, the same adatom impurity can manifest in spectrally distinct ways-sharp versus broad resonances near the charge neutrality-depending on the sublattice it adsorbs at. Employing Green's function analytical methods and the numerical Kwant package we investigate the spectral and transport interplay between the resonances and superconducting coherence induced in bilayer graphene by proximity to an s-wave superconductor. Analyzing doping and temperature dependencies of quasi-particle spin-relaxation rates, energies of Yu-Shiba-Rusinov states, Andreev spectra and the supercurrent characteristics of Josephson junctions we find unique superconducting signatures discriminating between resonant and off-resonant regimes. Our findings are in certain aspects going beyond the superconducting bilayer graphene and hold for generic s-wave superconductors functionalized by the resonant magnetic impurities.

cond-mat.mes-hall↗

arXiv2022

Counterintuitive gate dependence of weak antilocalization in bilayer graphene/WSe$_2$ heterostructures

Strong gate control of proximity-induced spin-orbit coupling was recently predicted in bilayer graphene/transition metal dichalcogenides (BLG/TMDC) heterostructures, as charge carriers can easily be shifted between the two graphene layers, and only one of them is in close contact to the TMDC. The presence of spin-orbit coupling can be probed by weak antilocalization (WAL) in low field magnetotransport measurements. When the spin-orbit splitting in such a heterostructure increases with the out of plane electric displacement field $\bar D$, one intuitively expects a concomitant increase of WAL visibility. Our experiments show that this is not the case. Instead, we observe a maximum of WAL visibility around $\bar D=0$. This counterintuitive behaviour originates in the intricate dependence of WAL in graphene on symmetric and antisymmetric spin lifetimes, caused by the valley-Zeeman and Rashba terms, respectively. Our observations are confirmed by calculating spin precession and spin lifetimes from an $8\times 8$ model Hamiltonian of BLG/TMDC.

cond-mat.mes-hall↗

arXiv2022

Effect of Rashba and Dresselhaus spin-orbit coupling on supercurrent rectification and magnetochiral anisotropy of ballistic Josephson junctions

Simultaneous breaking of inversion- and time-reversal symmetry in Josephson junction leads to a possible violation of the $I(φ)=-I(-φ)$ equality for the current-phase relation. This is known as anomalous Josephson effect and it produces a phase shift $φ_0$ in sinusoidal current-phase relations. In ballistic Josephson junctions with non-sinusoidal current phase relation the observed phenomenology is much richer, including the supercurrent diode effect and the magnetochiral anisotropy of Josephson inductance. In this work, we present measurements of both effects on arrays of Josephson junctions defined on epitaxial Al/InAs heterostructures. We show that the orientation of the current with respect to the lattice affects the magnetochiral anisotropy, possibly as the result of a finite Dresselhaus component. In addition, we show that the two-fold symmetry of the Josephson inductance reflects in the activation energy for phase slips.

cond-mat.supr-con↗

arXiv2021

Strength of the Hubbard potential and its modification by breathing distortion in $\text{BaBiO}_{3}$

$\text{BaBiO}_{3}$ compound is known as an archetype example of a three-dimensional Holstein model with the realization of the charge density wave state at half-filling and the superconducting state when doped. Although many works are devoted to the study of the electron-phonon interaction in $\text{BaBiO}_{3}$, the influence of the electron-electron Hubbard interaction on the electronic structure in this system is still under quest. In our work, we obtain an analytical expression for the screened Coulomb potential, and along with the basis of \textit{ab initio}-computed maximally localized Wannier orbitals, we quantitatively estimate the magnitude of the effective on-site Hubbard potential scrutinizing the effects of distortion of the crystal lattice. We show that a proper inclusion of the electron-electron interactions into the Holstein model significantly lowers the value of the underlying electron-phonon coupling. Finally, we find that the amplitudes of the repulsive electron-electron potential and its attractive counterpart mediated by the electron-phonon coupling are rather comparable. This may open a way for a realization of the intermediate phase of $\text{BaBiO}_{3}$ in terms of the Holstein-Hubbard model.

cond-mat.mtrl-sci↗

arXiv2021

A Josephson junction supercurrent diode

Transport is called nonreciprocal when not only the sign, but also the absolute value of the current, depends on the polarity of the applied voltage. It requires simultaneously broken inversion and time-reversal symmetries, e.g., by the interplay of spin-orbit coupling and magnetic field. So far, observation of nonreciprocity was always tied to resistivity, and dissipationless nonreciprocal circuit elements were elusive. Here, we engineer fully superconducting nonreciprocal devices based on highly-transparent Josephson junctions fabricated on InAs quantum wells. We demonstrate supercurrent rectification far below the transition temperature. By measuring Josephson inductance, we can link nonreciprocal supercurrent to the asymmetry of the current-phase relation, and directly derive the supercurrent magnetochiral anisotropy coefficient for the first time. A semi-quantitative model well explains the main features of our experimental data. Nonreciprocal Josephson junctions have the potential to become for superconducting circuits what $pn$-junctions are for traditional electronics, opening the way to novel nondissipative circuit elements.

cond-mat.supr-con↗

arXiv2020

Chiral Majorana fermions in graphene from proximity-induced superconductivity

We present a detailed theoretical study of chiral topological superconductor phases in proximity-superconducting graphene systems based on an effective model inspired by DFT simulations. Inducing s-wave superconductivity to quantum anomalous Hall effect systems leads to chiral topological superconductors. For out-of-plane magnetization we find topological superconducting phases with even numbers of chiral Majorana fermions per edge which is correlated to the opening of a nontrivial gap in the bulk system in the $\mathrm{ K}$-points and their connection under particle-hole symmetry. We show that in a quantum anomalous Hall insulator with in-plane magnetization and nontrivial gap opening at $\mathrm{M}$, the corresponding topological superconductor can be tuned to host only single chiral Majorana states at its edge which is promising for proposals exploiting such states for braiding operations.

cond-mat.mes-hall↗

arXiv2020

Impurity resonance effects in graphene $vs$ impurity location, concentration and sublattice occupation

Unique electronic band structure of graphene with its semi-metallic features near the charge neutrality point is sensitive to impurity effects. Using the Lifshitz and Anderson impurity models, we study in detail the disorder induced spectral phenomena in the electronic band structure of graphene, namely, the formation of resonances, quasi-gaps, bound states, impurity sub-bands, and their overall impact on the electronic band restructuring and the associated Mott-like metal-insulator transitions. We perform systematic analytical and numerical study for realistic impurities, both substitutional and adsorbed, focusing on those effects that stem from the impurity adatoms locations (top, bridge, and hollow positions), concentration, host sublattice occupation, perturbation strengths, etc. Possible experimental and practical implications are discussed as well.

cond-mat.mes-hall↗

arXiv2020

Breakdown of the Hebel-Slichter effect in superconducting graphene due to the emergence of Yu-Shiba-Rusinov states at magnetic resonant scatterers

Employing analytical methods and quantum transport simulations we investigate the relaxation of quasiparticle spins in graphene proximitized by an $s$-wave superconductor in the presence of resonant magnetic and spin-orbit active impurities. Off resonance, the relaxation increases with decreasing temperature when electrons scatter off magnetic impurities---the Hebel-Slichter effect---and decreases when impurities have spin-orbit coupling. This distinct temperature~dependence (not present in the normal state) uniquely discriminates between the two scattering mechanisms. However, we show that the Hebel-Slichter picture breaks down at resonances. The emergence of Yu-Shiba-Rusinov bound states within the superconducting gap redistributes the spectral weight away from magnetic resonances. The result is opposite to the Hebel-Slichter expectation: the spin relaxation decreases with decreasing temperature. Our findings hold for generic $s$-wave superconductors with resonant magnetic impurities, but also, as we show, for resonant magnetic Josephson junctions.

cond-mat.mes-hall↗

arXiv2020

Quantum Anomalous Hall Effects in Graphene from Proximity-Induced Uniform and Staggered Spin-Orbit and Exchange Coupling

We investigate an effective model of proximity modified graphene (or symmetrylike materials) with broken time-reversal symmetry. We predict the appearance of quantum anomalous Hall phases by computing bulk band gap and Chern numbers for benchmark combinations of system parameters. Allowing for staggered exchange field enables quantum anomalous Hall effect in flat graphene with Chern number $C=1$. We explicitly show edge states in zigzag and armchair nanoribbons and explore their localization behavior. Remarkably, the combination of staggered intrinsic spin-orbit and uniform exchange coupling gives topologically protected (unlike in time-reversal systems) pseudohelical states, whose spin is opposite in opposite zigzag edges. Rotating the magnetization from out of plane to in plane makes the system trivial, allowing to control topological phase transitions. We also propose, using density functional theory, a material platform---graphene on Ising antiferromagnet MnPSe$_3$---to realize staggered exchange (pseudospin Zeeman) coupling.

cond-mat.mes-hall↗

arXiv2020

Magnetoconductance, Quantum Hall Effect, and Coulomb Blockade in Topological Insulator Nanocones

Magnetotransport through cylindrical topological insulator (TI) nanowires is governed by the interplay between quantum confinement and geometric (Aharonov-Bohm and Berry) phases. Here, we argue that the much broader class of TI nanowires with varying radius -- for which a homogeneous coaxial magnetic field induces a varying Aharonov-Bohm flux that gives rise to a non-trivial mass-like potential along the wire -- is accessible by studying its simplest member, a TI nanocone. Such nanocones allow to observe intriguing mesoscopic transport phenomena: While the conductance in a perpendicular magnetic field is quantized due to higher-order topological hinge states, it shows resonant transmission through Dirac Landau levels in a coaxial magnetic field. Furthermore, it may act as a quantum magnetic bottle, confining surface Dirac electrons and leading to a largely interaction-dominated regime of Coulomb blockade type. We show numerically that the above-mentioned effects occur for experimentally accessible values of system size and magnetic field, suggesting that TI nanocone junctions may serve as building blocks for Dirac electron optics setups.

cond-mat.mes-hall↗

arXiv2019

Spin relaxation in fluorinated single and bilayer graphene

We present a joint experiment-theory study on the role of fluorine adatoms in spin and momentum scattering of charge carriers in dilute fluorinated graphene and bilayer graphene. The experimental spin-flip and momentum scattering rates and their dependence on the density of fluorine and carrier doping are obtained through weak localization and conductivity measurements, respectively, and suggest the role of fluorine as resonant magnetic impurities. For the estimated fluorine concentration of a few 100 ppm, the observed spin lifetimes are in the range of 1-10\,ps. Theoretically, we established tight-binding electronic structures of fluorinated graphene and bilayer graphene by fitting to density functional supercell calculations and performed a comprehensive analysis of the spin-flip and momentum scattering rates within the same devices, aiming to develop a consistent description of both scattering channels. We find that resonant scattering in graphene is very sensitive to the precise position of the resonance level, as well as to the magnitude of the exchange coupling between itinerant carriers and localized spins. The experimental data point to the presence of weak spin-flip scatterers that, at the same time, relax the electron momentum strongly, nearly preserving the electron-hole symmetry. Such scatterers would exhibit resonance energies much closer to the neutrality point than what density functional theory predicts in the dilute limit. The inclusion of a magnetic moment on fluorine adatoms allowed us to qualitatively capture the carrier density dependence of the experimental rates but predicts a greater (weaker) spin (momentum) relaxation rate than the measurements. We discuss possible scenarios that may be responsible for the discrepancies. Our systematic study exposes the complexities involved in accurately capturing the behavior of adatoms on graphene.

cond-mat.mes-hall↗

arXiv2018

Interplay of resonant states and Landau levels in functionalized graphene

Adsorbates can drastically alter physical properties of graphene. Particularly important are adatoms and admolecules that induce resonances at the Dirac point. Such resonances limit electron mobilities and spin relaxation times. We present a systematic tight-binding as well as analytical modeling to investigate the properties of resonant states in the presence of a quantizing magnetic field. Landau levels are strongly influenced by the resonances, especially close to the Dirac point. Here the cyclotron motion of electrons around a defect leads to the formation of circulating local currents which are manifested by the appearance of side peaks around the zero-energy Landau level. Our study is based on realistic parameters for H, F, and Cu adatoms, each exhibiting distinct spectral features in the magnetic field. We also show that by observing a local density of states around an adatom in the presence of Landau levels useful microscopic model parameters can be extracted.

cond-mat.mes-hall↗

arXiv2018

Connection between zero-energy Yu-Shiba-Rusinov states and 0-$π$ transitions in magnetic Josephson junctions

We study the bound state spectrum and 0-$π$ transitions in ballistic quasi-1D superconductor/ferromagnetic insulator/superconductor (S/FI/S) Josephson junctions. In addition to the Andreev bound states, stemming from the phase coherence, the magnetic barrier gives rise to qualitatively different Yu-Shiba-Rusinov (YSR) bound states with genuine spectral features and spin characteristics. We show that zero-energy YSR states are much more robust against scalar tunneling than their Andreev counterparts and also fingerprint a quantum phase transition from the junctions' 0 into the $π$ phase, connected to a measurable reversal of the Josephson current flow; this coincidence persists also in the presence of Rashba spin-orbit coupling.

cond-mat.supr-con↗

arXiv2018

Transport Spectroscopy of Sublattice-Resolved Resonant Scattering in Hydrogen-Doped Bilayer Graphene

We report the experimental observation of sublattice-resolved resonant scattering in bilayer graphene by performing simultaneous cryogenic atomic hydrogen doping and electron transport measurements in ultrahigh vacuum. This allows us to monitor the hydrogen adsorption on the different sublattices of bilayer graphene without atomic-scale microscopy. Specifically, we detect two distinct resonant scattering peaks in the gate-dependent resistance, which evolve as a function of atomic hydrogen dosage. Theoretical calculations show that one of the peaks originates from resonant scattering by hydrogen adatoms on the α-sublattice (dimer site) while the other originates from hydrogen adatoms on the \b{eta}-sublattice (non-dimer site), thereby enabling a method for characterizing the relative sublattice occupancy via transport measurements. Utilizing this new capability, we investigate the adsorption and thermal desorption of hydrogen adatoms via controlled annealing and conclude that hydrogen adsorption on the \b{eta}-sublattice is energetically favored. Through site-selective desorption from the α-sublattice, we realize hydrogen doping with adatoms primarily on a single sublattice, which is highly desired for generating ferromagnetism.

cond-mat.mes-hall↗

arXiv2018

Absence of a giant spin Hall effect in plasma-hydrogenated graphene

The weak spin-orbit interaction in graphene was predicted to be increased, e.g., by hydrogenation. This should result in a sizable spin Hall effect (SHE). We employ two different methods to examine the spin Hall effect in weakly hydrogenated graphene. For hydrogenation we expose graphene to a hydrogen plasma and use Raman spectroscopy to characterize this method. We then investigate the SHE of hydrogenated graphene in the H-bar method and by direct measurements of the inverse SHE. Although a large nonlocal resistance can be observed in the H-bar structure, comparison with the results of the other method indicate that this nonlocal resistance is caused by a non-spin-related origin.

cond-mat.mes-hall↗