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Deniz Aybas

Publications and source records attributed to Deniz Aybas.

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Solid-state nuclear magnetic resonance search for axion-like dark matter with broadband SQUID magnetometry

We report the results of an experimental search for ultralight axion-like dark matter in the mass ranges 19.5--20.5 and 21.5--22 neV. The Cosmic Axion Spin Precession Experiment-electric probes the axion-nuclear electric dipole moment coupling. We perform solid-state nuclear magnetic resonance on $^{207}$Pb spin ensembles which reside in a polarized ferroelectric crystal. The background axion-like dark matter field induces an oscillating torque on the $^{207}$Pb spins via the electric dipole moment coupling $g_{d}$. The experiment is calibrated with pulsed magnetic resonance measurements covering two frequency bands (4.6--5.0 and 5.2--5.3 MHz) that correspond to the axion Compton frequencies associated with the identified axion mass ranges. By sweeping the leading magnetic field applied to the sample, we are able to detect the $^{207}$Pb nuclear magnetic resonance in these frequency ranges using a superconducting quantum interference device, inductively coupled to the sample with a broadband circuit. We establish the upper bounds $|g_{d}| < 4\times 10^{-4}$ GeV$^{-2}$ with 95% confidence in these frequency bands. Our results demonstrate the detection and small-tip angle calibration of low-field $^{207}$Pb nuclear magnetic resonance, allowing for sensitivity to axion-like dark matter in the nanoelectron-volt axion mass range.

hep-ex

Control of relaxation properties of a macroscopic nuclear spin ensemble

Macroscopic spin ensembles in solids are powerful platforms for quantum sensing and precision metrology. A key challenge is controlling the nuclear spin population relaxation time $T_1$, which can become prohibitively long at cryogenic temperatures due to phonon freeze-out. We demonstrate optical control of the $T_1$ relaxation time of the $^{207}$Pb nuclear spin ensemble in lead-containing ferroelectric crystals PbTiO$_3$ (PT) and (PbMg$_{1/3}$Nb$_{2/3}$O$_3$)$_{2/3}$-(PbTiO$_3$)$_{1/3}$ (PMN-PT). Using X-band electron paramagnetic resonance (EPR) spectroscopy at 10 K, we characterize light-induced paramagnetic centers created by 405 nm laser illumination. In PT, we observe paramagnetic Pb$^{3+}$ centers and their hyperfine interaction with nearby nuclear spins. In PMN-PT, we identify two populations: isotropic Pb$^{3+}$ centers and anisotropic Ti$^{3+}$ centers occupying $d$-orbitals, with spin number densities of $(2.5 \pm 1.0) \times 10^{17}$ cm$^{-3}$ and $(4.1 \pm 1.7) \times 10^{17}$ cm$^{-3}$, respectively. Power-dependent EPR measurements enable extraction of spin relaxation times. We investigate the ionization and recombination dynamics of these transient paramagnetic centers. Using saturation-recovery nuclear magnetic resonance, we demonstrate that laser illumination reduces the $^{207}$Pb nuclear $T_1$ by approximately a factor of two, from $(17 \pm 2)$ s to $(7 \pm 1)$ s at 4.6 MHz, and from $(1550 \pm 40)$ s to $(850 \pm 70)$ s at 40 MHz. We develop a model relating the nuclear relaxation rate to the density of photoinduced paramagnetic centers. This optical control of nuclear spin relaxation provides a pathway toward accelerated thermal polarization and dynamic nuclear polarization in solid-state NMR-based precision measurements, including searches for axion-like dark matter.

cond-mat.other

The COSMIC WISPers White Paper: The physics case for Weakly Interacting Slim Particles

Axions and other very weakly interacting slim particles (WISPs), with masses below 1 GeV, arise naturally in many extensions of the Standard Model of particle physics. In particular, they could offer a new framework to explain the nature of dark matter and may help address a range of puzzling observations in astrophysics and particle physics. This review provides an overview of ongoing WISP searches and outlines the prospects for the next decade, spanning their theoretical motivation, indirect signatures in astrophysical observations, and dedicated laboratory experiments. It is based on the work carried on by the EU-funded COST Action ``Cosmic WISPers in the Dark Universe: Theory, astrophysics, and experiments'' (CA21106, https://www.cost.eu/actions/CA21106). This network plays a key role in coordinating and supporting WISP searches across Europe, while also contributing to the development of a roadmap aimed at securing European leadership in this research area. It is emphasized that Europe is currently pursuing a rich, diverse, and cost-effective experimental program, with the potential to deliver one or more transformative discoveries.

hep-ph

Cavity, lumped-circuit, and spin-based detection of axion dark matter: differences and similarities

Axions and axion-like particles are compelling candidates for ultralight bosonic dark matter, forming coherent oscillating fields that can be probed by experiments known as haloscopes. A broad range of haloscope concepts has been developed, including resonant cavity haloscopes, lumped-element circuit detectors, and spin-based experiments, each sensitive to different axion couplings and mass ranges. Rather than attempting an exhaustive survey of all existing approaches, this comparative review provides a unified framework for the major haloscope classes, establishing a common language for the descriptions of signal generation, noise properties, data analysis, and scanning strategies. Key properties of ultralight bosonic dark matter relevant for detection are summarized first, including coherence time, spectral linewidth, and stochasticity under the standard halo model. The discussion then compares cavity, Earth-scale, lumped-element, and spin haloscopes, focusing on expected signal shapes, dominant noise sources, and statistical frameworks for axion searches. Particular emphasis is placed on consistent definitions of signal-to-noise ratio and on how detector bandwidth, axion coherence, and noise characteristics determine optimal scan strategies. By systematically comparing operating principles and performance metrics across these detector families, this framework clarifies shared concepts as well as the essential differences that govern sensitivity in different mass and coupling regimes. The resulting perspective synthesizes current search methodologies and offers guidance for optimizing future haloscope experiments.

hep-ph

Exploring the Dark Universe: A European Strategy for Axions and other WISPs Discovery

Axions and other very weakly interacting slim (with $m <$ 1 GeV) particles (WISPs) are a common feature of several extensions of the Standard Model of Particle Physics. The search of WISPs was already recommended in the last update of the European strategy on particle physics (ESPP). After that, the physics case for WISPs has gained additional momentum. Indeed, WISPs may provide a new paradigm to explain the nature of dark matter and puzzling astrophysical and particle physics observations. This document briefly summarizes current searches for WISPs and the perspectives in this research field for the next decade, ranging from their theoretical underpinning, over their indirect observational consequences in astrophysics, to their search in laboratory experiments. It is stressed that in Europe a rich, diverse, and low-cost experimental program is already underway with the potential for one or more game-changing discoveries. In this context, it is also reported the role of the EU funded COST Action ''Cosmic WISPers in the Dark Universe: Theory, astrophysics, and experiments'' (CA21106, https://www.cost.eu/actions/CA21106) in coordinating and supporting WISPs searches in Europe, shaping a roadmap to track the strategy to guarantee a European leadership in this field of research. This document has been submitted in March 2025 as an input to the update process of the ESPP.

hep-ph

Spectral signatures of axionlike dark matter

We derive spectral line shapes of the expected signal for a haloscope experiment searching for axionlike dark matter. The knowledge of these line shapes is needed to optimize an experimental design and data analysis procedure. We extend the previously known results for the axion-photon and axion-gluon couplings to the case of gradient (axion-fermion) coupling. A unique feature of the gradient interaction is its dependence not only on magnitudes but also on directions of velocities of galactic halo particles, which leads to the directional sensitivity of the corresponding haloscope. We also discuss the daily and annual modulations of the gradient signal caused by the Earth's rotational and orbital motions. In the case of detection, these periodic modulations will be an important confirmation that the signal is sourced by axionlike particles in the halo of our Galaxy.

hep-ph

Search for axion-like dark matter using solid-state nuclear magnetic resonance

We report the results of an experimental search for ultralight axion-like dark matter in the mass range 162 neV to 166 neV. The detection scheme of our Cosmic Axion Spin Precession Experiment (CASPEr) is based on a precision measurement of $^{207}$Pb solid-state nuclear magnetic resonance in a polarized ferroelectric crystal. Axion-like dark matter can exert an oscillating torque on $^{207}$Pb nuclear spins via the electric-dipole moment coupling $g_d$, or via the gradient coupling $g_{\text{aNN}}$. We calibrated the detector and characterized the excitation spectrum and relaxation parameters of the nuclear spin ensemble with pulsed magnetic resonance measurements in a 4.4 T magnetic field. We swept the magnetic field near this value and searched for axion-like dark matter with Compton frequency within a 1 MHz band centered at 39.65 MHz. Our measurements place the upper bounds $|g_d|<9.5\times10^{-4}\,\text{GeV}^{-2}$ and $|g_{\text{aNN}}|<2.8\times10^{-1}\,\text{GeV}^{-1}$ (95% confidence level) in this frequency range. The constraint on $g_d$ corresponds to an upper bound of $1.0\times 10^{-21}\,\text{e}\cdot\text{cm}$ on the amplitude of oscillations of the neutron electric dipole moment, and $4.3\times 10^{-6}$ on the amplitude of oscillations of CP-violating $θ$ parameter of quantum chromodynamics. Our results demonstrate the feasibility of using solid-state nuclear magnetic resonance to search for axion-like dark matter in the nano-electronvolt mass range.

hep-ex

Quantum sensitivity limits of nuclear magnetic resonance experiments searching for new fundamental physics

Nuclear magnetic resonance is a promising experimental approach to search for ultra-light axion-like dark matter. Searches such as the cosmic axion spin-precession experiments (CASPEr) are ultimately limited by quantum-mechanical noise sources, in particular, spin-projection noise. We discuss how such fundamental limits can potentially be reached. We consider a circuit model of a magnetic resonance experiment and quantify three noise sources: spin-projection noise, thermal noise, and amplifier noise. Calculation of the total noise spectrum takes into account the modification of the circuit impedance by the presence of nuclear spins, as well as the circuit back-action on the spin ensemble. Suppression of the circuit back-action is especially important in order for the spin-projection noise limits of searches for axion-like dark matter to reach the quantum chromodynamic axion sensitivity.

quant-ph

Search for axion-like dark matter with ferromagnets

Existence of dark matter indicates the presence of unknown fundamental laws of nature. Ultralight axion-like particles are well-motivated dark matter candidates, emerging naturally from theories of physics at ultrahigh energies. We report the results of a direct search for the electromagnetic interaction of axion-like dark matter in the mass range that spans three decades from 12 peV to 12 neV. The detection scheme is based on a modification of Maxwell's equations in the presence of axion-like dark matter, which mixes with a static magnetic field to produce an oscillating magnetic field. The experiment makes use of toroidal magnets with iron-nickel alloy ferromagnetic powder cores, which enhance the static magnetic field by a factor of 24. Using SQUIDs, we achieve a magnetic sensitivity of 150 $\text{aT}/\sqrt{\text{Hz}}$, at the level of the most sensitive magnetic field measurements demonstrated with any broadband sensor. We recorded 41 hours of data and improved the best limits on the magnitude of the axion-like dark matter electromagnetic coupling constant over part of our mass range, at 20 peV reaching $4.0 \times 10^{-11} \text{GeV}^{-1}$ (95\% confidence level). Our measurements are starting to explore the coupling strengths and masses of axion-like particles where mixing with photons could explain the anomalous transparency of the universe to TeV gamma-rays.

hep-ex

Sensitivity enhancement for a light axion dark matter search with magnetic material

The sensitivity of experimental searches for axion dark matter coupled to photons is typically proportional to the strength of the applied static magnetic field. We demonstrate how a permeable material can be used to enhance the magnitude of this static magnetic field, and therefore improve the sensitivity of such searches in the low frequency lumped-circuit limit. Using gadolinium iron garnet toroids at temperature 4.2 K results in a factor of 4 enhancement compared to an air-core toroidal design. The enhancement is limited by magnetic saturation. Correlation of signals from three such toroids allows efficient rejection of systematics due to electromagnetic interference. The sensitivity of a centimeter-scale axion dark matter search based on this approach is on the order of $g_{aγγ}\approx10^{-9}$ GeV$^{-1}$ after 8 hours of data collection for axion masses near $10^{-10}$ eV. This approach may substantially extend the sensitivity reach of large-volume lumped element axion dark matter searches.

physics.ins-det

The Cosmic Axion Spin Precession Experiment (CASPEr): a dark-matter search with nuclear magnetic resonance

The Cosmic Axion Spin Precession Experiment (CASPEr) is a nuclear magnetic resonance experiment (NMR) seeking to detect axion and axion-like particles which could make up the dark matter present in the universe. We review the predicted couplings of axions and axion-like particles with baryonic matter that enable their detection via NMR. We then describe two measurement schemes being implemented in CASPEr. The first method, presented in the original CASPEr proposal, consists of a resonant search via continuous-wave NMR spectroscopy. This method offers the highest sensitivity for frequencies ranging from a few Hz to hundreds of MHz, corresponding to masses $ m_{\rm a} \sim 10^{-14}$--$10^{-6}$ eV. Sub-Hz frequencies are typically difficult to probe with NMR due to the diminishing sensitivity of magnetometers in this region. To circumvent this limitation, we suggest new detection and data processing modalities. We describe a non-resonant frequency-modulation detection scheme, enabling searches from mHz to Hz frequencies ($m_{\rm a} \sim 10^{-17}$--$10^{-14} $ eV), extending the detection bandwidth by three decades.

physics.ins-det

Application of Spin-Exchange Relaxation-Free Magnetometry to the Cosmic Axion Spin Precession Experiment

The Cosmic Axion Spin Precession Experiment (CASPEr) seeks to measure oscillating torques on nuclear spins caused by axion or axion-like-particle (ALP) dark matter via nuclear magnetic resonance (NMR) techniques. A sample spin-polarized along a leading magnetic field experiences a resonance when the Larmor frequency matches the axion/ALP Compton frequency, generating precessing transverse nuclear magnetization. Here we demonstrate a Spin-Exchange Relaxation-Free (SERF) magnetometer with sensitivity $\approx 1~{\rm fT/\sqrt{Hz}}$ and an effective sensing volume of 0.1 $\rm{cm^3}$ that may be useful for NMR detection in CASPEr. A potential drawback of SERF-magnetometer-based NMR detection is the SERF's limited dynamic range. Use of a magnetic flux transformer to suppress the leading magnetic field is considered as a potential method to expand the SERF's dynamic range in order to probe higher axion/ALP Compton frequencies.

physics.atom-ph