arXiv subjects

Derek F. Jackson Kimball

Publications and source records attributed to Derek F. Jackson Kimball.

At least 19 recordsLinked to original sources

arXiv2026

Solid-state nuclear magnetic resonance search for axion-like dark matter with broadband SQUID magnetometry

We report the results of an experimental search for ultralight axion-like dark matter in the mass ranges 19.5--20.5 and 21.5--22 neV. The Cosmic Axion Spin Precession Experiment-electric probes the axion-nuclear electric dipole moment coupling. We perform solid-state nuclear magnetic resonance on $^{207}$Pb spin ensembles which reside in a polarized ferroelectric crystal. The background axion-like dark matter field induces an oscillating torque on the $^{207}$Pb spins via the electric dipole moment coupling $g_{d}$. The experiment is calibrated with pulsed magnetic resonance measurements covering two frequency bands (4.6--5.0 and 5.2--5.3 MHz) that correspond to the axion Compton frequencies associated with the identified axion mass ranges. By sweeping the leading magnetic field applied to the sample, we are able to detect the $^{207}$Pb nuclear magnetic resonance in these frequency ranges using a superconducting quantum interference device, inductively coupled to the sample with a broadband circuit. We establish the upper bounds $|g_{d}| < 4\times 10^{-4}$ GeV$^{-2}$ with 95% confidence in these frequency bands. Our results demonstrate the detection and small-tip angle calibration of low-field $^{207}$Pb nuclear magnetic resonance, allowing for sensitivity to axion-like dark matter in the nanoelectron-volt axion mass range.

hep-ex↗

arXiv2026

Quantum dynamics of a levitated ferromagnetic gyroscope

We develop a quantum model for the rotational dynamics of a freely floating levitated ferromagnetic gyroscope (LFG), emphasizing the interplay between intrinsic spin $\boldsymbol{S}$, mechanical angular momentum $\boldsymbol{L}$, and magnetic torque. The conserved total angular momentum projection along the $z$-directed magnetic field $\boldsymbol{B}$, $J_z=S_z+L_z$, is quantized, leading in the small-libration-amplitude limit to discrete precessional states $|m\rangle$ (eigenstates of $J_z$ with eigenvalues $J_z = m\hbar$) and librational harmonic oscillator states $|n\rangle$ ($n=0,1,2,\ldots$). The discreteness of the energies and dynamical variables is governed by the quantum precession scale $Ω_Q=\hbar/I$, where $I$ is the moment of inertia of the LFG. We find that the phenomenon of LFG precession persists into high-field regimes where the magnitude of the rotational angular momentum associated with precession exceeds the total intrinsic spin. We analyze the complementary quantum limits of localized semiclassical LFG orientation wave packets and exact $J_z$-eigenstates $|m\rangle$, clarifying the relation between classical precession signals and the underlying quantized spin-rotor dynamics. We further show that radio-frequency fields can drive $Δm = \pm 1$ and $Δn = \pm 1$ transitions, enabling ladder spectroscopy, tilt-angle control, and sideband-like coupling between precession and libration. The coupled dynamics also exhibit branch-point magnetic resonances where precession and librational motion become strongly coupled. These results establish a framework for using LFGs not only as ultrasensitive torque and magnetic-field sensors, but also as controllable mesoscopic quantum systems. The techniques developed here may be applied to searches for exotic, beyond-the-standard model spin-dependent interactions, ultralight dark matter, and spin-gravity couplings.

quant-ph↗

arXiv2026

Search for a solar-bound axion halo using the Global Network of Optical Magnetometers for Exotic physics searches

We report on a search for a gravitationally bound solar axion halo using data from the Global Network of Optical Magnetometers for Exotic physics searches (GNOME), a worldwide array of magnetically shielded atomic magnetometers with sensitivity to exotic spin couplings. Motivated by recent theoretical work suggesting that self-interacting ultralight axions can be captured by the Sun's gravitational field and thermalize into the ground state, we develop a signal model for the pseudo-magnetic fields generated by axion-proton gradient couplings in such a halo. The analysis focuses on the fifth GNOME Science Run (69 days, 12 stations), employing a cross-correlation pipeline with time-shifted daily modulation templates to search for the global, direction-dependent, monochromatic signal expected from a solar axion halo. No statistically significant candidate signals are observed. We set 95% confidence-level upper limits on the amplitude of the axion-induced pseudo-magnetic field over the frequency range $\approx 0.05-20$ Hz, translating to constraints on the linear and quadratic axion-proton couplings for halo densities predicted by gravitational capture models and for the maximum overdensities allowed by planetary ephemerides. In the quadratic coupling case, our limits surpass existing astrophysical bounds by over two orders of magnitude across much of the accessible parameter space.

physics.atom-ph↗

arXiv2026

Control of relaxation properties of a macroscopic nuclear spin ensemble

Macroscopic spin ensembles in solids are powerful platforms for quantum sensing and precision metrology. A key challenge is controlling the nuclear spin population relaxation time $T_1$, which can become prohibitively long at cryogenic temperatures due to phonon freeze-out. We demonstrate optical control of the $T_1$ relaxation time of the $^{207}$Pb nuclear spin ensemble in lead-containing ferroelectric crystals PbTiO$_3$ (PT) and (PbMg$_{1/3}$Nb$_{2/3}$O$_3$)$_{2/3}$-(PbTiO$_3$)$_{1/3}$ (PMN-PT). Using X-band electron paramagnetic resonance (EPR) spectroscopy at 10 K, we characterize light-induced paramagnetic centers created by 405 nm laser illumination. In PT, we observe paramagnetic Pb$^{3+}$ centers and their hyperfine interaction with nearby nuclear spins. In PMN-PT, we identify two populations: isotropic Pb$^{3+}$ centers and anisotropic Ti$^{3+}$ centers occupying $d$-orbitals, with spin number densities of $(2.5 \pm 1.0) \times 10^{17}$ cm$^{-3}$ and $(4.1 \pm 1.7) \times 10^{17}$ cm$^{-3}$, respectively. Power-dependent EPR measurements enable extraction of spin relaxation times. We investigate the ionization and recombination dynamics of these transient paramagnetic centers. Using saturation-recovery nuclear magnetic resonance, we demonstrate that laser illumination reduces the $^{207}$Pb nuclear $T_1$ by approximately a factor of two, from $(17 \pm 2)$ s to $(7 \pm 1)$ s at 4.6 MHz, and from $(1550 \pm 40)$ s to $(850 \pm 70)$ s at 40 MHz. We develop a model relating the nuclear relaxation rate to the density of photoinduced paramagnetic centers. This optical control of nuclear spin relaxation provides a pathway toward accelerated thermal polarization and dynamic nuclear polarization in solid-state NMR-based precision measurements, including searches for axion-like dark matter.

cond-mat.other↗

arXiv2026

Floquet engineering of spin-spin interactions in a hybrid atomic system

We demonstrate dynamical control of the effective spin-spin interaction, dominated by Fermi-contact interaction, in a hybrid spin system via parametric modulation. We show that, in an alkali-noble-gas comagnetometer, periodic modulation of the direction of the electron spin polarization with respect to the nuclear polarization leads to a Floquet-induced renormalization of the spin-exchange coupling, governed by a zeroth-order Bessel function. This effect enables continuous tuning and suppression of the effective interaction strength without altering the intrinsic properties of the system. We develop a theoretical model that supports the experimental measurements. The results establish a general mechanism for controlling interaction strengths in hybrid atomic systems and provide new opportunities for precision measurements and quantum memories.

physics.atom-ph↗

arXiv2026

Black hole scalar sirens in the Milky Way

Hypothetical light scalar particles trigger the superradiant instability around spinning black holes (BHs), causing clouds of scalars to grow around the BH. In the presence of sufficiently strong particle self-interactions (characterized by the decay constant $f$), scalars are ejected from BH orbits, resulting in coherent, non-relativistic emissions that continuously carry away the BH's angular momentum. Parameters exist for which cloud growth is much faster, and scalar depletion is much slower, than the age of the Galaxy. This defines a distinct class of astrophysical sources of scalars, which we call BH scalar sirens -- BHs that persistently emit scalars effectively forever. We compute the scalar background from the expected population of $N_\text{BH}\sim 10^{8}$ isolated stellar-mass BHs in the Milky Way, which are sirens for scalars in the mass range $10^{-13}$--$10^{-11}\,$eV and $f\lesssim 10^{14}$--$10^{9}\,$GeV. This provides a detection target independent of early-universe scalar production or cosmological initial conditions. The generated observable signals are up to two orders-of-magnitude larger than those expected from a misaligned cosmic scalar in this mass range. The energy spectrum of emitted scalars is distinctly broader and at higher velocities (up to $\sim 10^{-1}c$) than that of virialized dark matter, and encodes the mass and spin distributions of the BH population. While stellar-mass Milky Way BHs are our primary target, our framework extends to supermassive, intermediate-mass and light BHs. Given the difficulty of directly observing populations of isolated BHs, scalar emissions offer a novel probe of these otherwise invisible objects, highlighting the potential for joint discovery between scalars and BHs, and broadly motivating searches for scalars over many orders-of-magnitude in mass.

hep-ph↗

arXiv2026

Cavity, lumped-circuit, and spin-based detection of axion dark matter: differences and similarities

Axions and axion-like particles are compelling candidates for ultralight bosonic dark matter, forming coherent oscillating fields that can be probed by experiments known as haloscopes. A broad range of haloscope concepts has been developed, including resonant cavity haloscopes, lumped-element circuit detectors, and spin-based experiments, each sensitive to different axion couplings and mass ranges. Rather than attempting an exhaustive survey of all existing approaches, this comparative review provides a unified framework for the major haloscope classes, establishing a common language for the descriptions of signal generation, noise properties, data analysis, and scanning strategies. Key properties of ultralight bosonic dark matter relevant for detection are summarized first, including coherence time, spectral linewidth, and stochasticity under the standard halo model. The discussion then compares cavity, Earth-scale, lumped-element, and spin haloscopes, focusing on expected signal shapes, dominant noise sources, and statistical frameworks for axion searches. Particular emphasis is placed on consistent definitions of signal-to-noise ratio and on how detector bandwidth, axion coherence, and noise characteristics determine optimal scan strategies. By systematically comparing operating principles and performance metrics across these detector families, this framework clarifies shared concepts as well as the essential differences that govern sensitivity in different mass and coupling regimes. The resulting perspective synthesizes current search methodologies and offers guidance for optimizing future haloscope experiments.

hep-ph↗

arXiv2025

Search for Axionlike Dark Matter Using Liquid-State Nuclear Magnetic Resonance

We search for dark matter in the form of axionlike particles (ALPs) in the mass range $5.576741 \,\mathrm{neV/c^2}$ - $5.577733\,\mathrm{neV/c^2}$ by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHz resulted in a sensitivity to the ALP-proton coupling constant of $g_{\mathrm{ap}} \approx 3 \times 10^{-2}\,\mathrm{GeV}^{-1}$. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment's capabilities. CASPEr-Gradient Low-Field will probe the mass range from $4.1\,\mathrm{\peV/c^2}$ to $17\,\mathrm{\neV/c^2}$ with hyperpolarized samples to boost the sensitivity beyond the astronomical limits.

hep-ex↗

arXiv2025

Notes on optimizing a multi-sensor gradient axion-like particle dark matter search

Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for the dark matter. We discuss the scaling of the sensitivity of a galactic ALP dark matter search with the number of sensors, especially in the ultra-light mass regime, where the measurement time is shorter than the coherence time of the ALP field. We compare multiple schemes for daily modulated ALP gradient signals, and show that increasing the number of sensors from 1 to 2 improves the signal-to-noise ratio (SNR) by a factor of 2-3. For more than two sensors, the SNR increases as the square root of the number of sensors. Then, we show that splitting the data into subsets and then averaging its Discrete Fourier Transforms (DFTs) is equivalent to the DFT of the whole dataset in terms of SNR.

hep-ph↗

arXiv2024

Ultralight dark matter detection with levitated ferromagnets

Levitated ferromagnets act as ultraprecise magnetometers, which can exhibit high quality factors due to their excellent isolation from the environment. These instruments can be utilized in searches for ultralight dark matter candidates, such as axionlike dark matter or dark-photon dark matter. In addition to being sensitive to an axion-photon coupling or kinetic mixing, which produce physical magnetic fields, ferromagnets are also sensitive to the effective magnetic field (or "axion wind") produced by an axion-electron coupling. While the dynamics of a levitated ferromagnet in response to a DC magnetic field have been well studied, all of these couplings would produce AC fields. In this work, we study the response of a ferromagnet to an applied AC magnetic field and use these results to project their sensitivity to axion and dark-photon dark matter. We pay special attention to the direction of motion induced by an applied AC field, in particular, whether it precesses around the applied field (similar to an electron spin) or librates in the plane of the field (similar to a compass needle). We show that existing levitated ferromagnet setups can already have comparable sensitivity to an axion-electron coupling as comagnetometer or torsion balance experiments. In addition, future setups can become sensitive probes of axion-electron coupling, dark-photon kinetic mixing, and axion-photon coupling, for ultralight dark matter masses $m_\mathrm{DM}\lesssim\mathrm{feV}$.

hep-ph↗

arXiv2024

Searching for dark matter with a 1000 km baseline interferometer

Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for dark matter. ALP dark matter would manifest as a field oscillating at an (as of yet) unknown frequency. The frequency depends linearly on the ALP mass and plausibly ranges from $10^{-22}$ to $10$ eV/$c^2$. This motivates broadband search approaches. We report on a direct search for ALP dark matter with an interferometer composed of two atomic K-Rb-$^3$He comagnetometers, one situated in Mainz, Germany, and the other in Kraków, Poland. We leverage the anticipated spatio-temporal coherence properties of the ALP field and probe all ALP-gradient-spin interactions covering a mass range of nine orders of magnitude. No significant evidence of an ALP signal is found. We thus place new upper limits on the ALP-neutron, ALP-proton and ALP-electron couplings reaching below $g_{aNN}<10^{-9}$ GeV$^{-1}$, $g_{aPP}<10^{-7}$ GeV$^{-1}$ and $g_{aee}<10^{-6}$ GeV$^{-1}$, respectively. These limits improve upon previous laboratory constraints for neutron and proton couplings by up to three orders of magnitude.

hep-ph↗

arXiv2024

Spin-dependent exotic interactions

Novel interactions beyond the four known fundamental forces in nature (electromagnetic, gravitational, strong and weak interactions), may arise due to "new physics" beyond the standard model, manifesting as a "fifth force". This review is focused on spin-dependent fifth forces mediated by exotic bosons such as spin-0 axions and axionlike particles and spin-1 Z' bosons, dark photons, or paraphotons. Many of these exotic bosons are candidates to explain the nature of dark matter and dark energy, and their interactions may violate fundamental symmetries. Spin-dependent interactions between fermions mediated by the exchange of exotic bosons have been investigated in a variety of experiments, particularly at the low-energy frontier. Experimental methods and tools used to search for exotic spin-dependent interactions, such as atomic comagnetometers, torsion balances, nitrogen-vacancy spin sensors, and precision atomic and molecular spectroscopy, are described. A complete set of interaction potentials, derived based on quantum field theory with minimal assumptions and characterized in terms of reduced coupling constants, are presented. A comprehensive summary of existing experimental and observational constraints on exotic spin-dependent interactions is given, illustrating the current research landscape and promising directions of further research.

hep-ph↗

arXiv2024

Constraints on exotic interactions from scalar spin-spin coupling in tritium deuteride (DT)

A comparison of theoretical and experimental values of the scalar spin-spin interaction ($J$-coupling) in tritium deuteride molecules yield constraints for nucleon-nucleon exotic interactions of the dimensionless coupling strengths $g_Vg_V$, $g_Ag_A$ and $g_pg_p$, corresponding to the exchange of an vector, axial-vector, and pseudoscalar (axionlike) boson. The couplings between proton ($p$) and nucleon ($N$), denoted by $g_V^p g_V^N$, $g_p^p g_p^N$ are constrained to be less than $1.4 \times 10^{-6}$ and $2.7\times 10^{-6}$, respectively, for boson masses around 5 keV. The coupling constant $g_A^p g_A^N$ is constrained to be less than $1.0 \times 10^{-18}$ for boson masses $\leq 100$ eV. It is noteworthy that this study represents the first instance in which constraints on $g_V g_V$ have been established through the analysis of the potential term $V_2 + V_3$ for both tritium deuteride and hydrogen deuteride molecules.

physics.atom-ph↗

arXiv2023

Universal determination of comagnetometer response to spin couplings

We propose and demonstrate a general method to calibrate the frequency-dependent response of self-compensating noble-gas-alkali-metal comagnetometers to arbitrary spin perturbations. This includes magnetic and nonmagnetic perturbations like rotations and exotic spin interactions. The method is based on a fit of the magnetic field response to an analytical model. The frequency-dependent response of the comagnetometer to arbitrary spin perturbations can be inferred using the fit parameters. We demonstrate the effectiveness of this method by comparing the inferred rotation response to an experimental measurement of the rotation response. Our results show that experiments relying on zero-frequency calibration of the comagnetometer response can over- or under-estimate the comagnetometer sensitivity by orders of magnitude over a wide frequency range. Moreover, this discrepancy accumulates over time as operational parameters tend to drift during comagnetometer operation. The demonstrated calibration protocol enables accurate prediction and control of comagnetometer sensitivity to, for example, ultralight bosonic dark-matter fields coupling to electron or nuclear spins as well as accurate monitoring and control of the relevant system parameters.

physics.atom-ph↗

arXiv2023

A Hunt for Magnetic Signatures of Hidden-Photon and Axion Dark Matter in the Wilderness

Earth can act as a transducer to convert ultralight bosonic dark matter (axions and hidden photons) into an oscillating magnetic field with a characteristic pattern across its surface. Here we describe the first results of a dedicated experiment, the Search for Non-Interacting Particles Experimental Hunt (SNIPE Hunt), that aims to detect such dark-matter-induced magnetic-field patterns by performing correlated measurements with a network of magnetometers in relatively quiet magnetic environments (in the wilderness far from human-generated magnetic noise). Our experiment constrains parameter space describing hidden-photon and axion dark matter with Compton frequencies in the 0.5-5.0 Hz range. Limits on the kinetic-mixing parameter for hidden-photon dark matter represent the best experimental bounds to date in this frequency range.

hep-ph↗

arXiv2023

Frequency-scanning considerations in axionlike dark matter spin-precession experiments

Galactic dark matter may consist of axionlike particles (ALPs) that can be described as an "ultralight bosonic field" oscillating at the ALP Compton frequency. The ALP field can be searched for using nuclear magnetic resonance (NMR), where resonant precession of spins of a polarized sample can be sensitively detected. The ALP mass to which the experiment is sensitive is scanned by sweeping the bias magnetic field. The scanning either results in detection of ALP dark matter or rules out ALP dark matter with sufficiently strong couplings to nuclear spins over the range of ALP masses corresponding to the covered span of Larmor frequencies. In this work, scanning strategies are analyzed with the goal of optimizing the parameter-space coverage via a proper choice of experimental parameters (e.g., the effective transverse relaxation time).

physics.atom-ph↗

arXiv2023

Optimization of nuclear polarization in an alkali-noble gas comagnetometer

Self-compensated comagnetometers, employing overlapping samples of spin-polarized alkali and noble gases (for example K-$^3$He) are promising sensors for exotic beyond-the-standard-model fields and high-precision metrology such as rotation sensing. When the comagnetometer operates in the so-called self-compensated regime, the effective field, originating from contact interactions between the alkali valence electrons and the noble-gas nuclei, is compensated with an applied magnetic field. When the comagnetometer begins operation in a given magnetic field, spin-exchange optical pumping establishes equilibrium between the alkali electron-spin polarization and the nuclear-spin polarization. Subsequently, when the magnetic field is tuned to the compensation point, the spin polarization is brought out of the equilibrium conditions. This causes a practical issue for long measurement times. We report on a novel method for closed-loop control of the compensation field. This method allows optimization of the operating parameters, especially magnetic field gradients, in spite of the inherently slow (hours to days) dynamics of the system. With the optimization, higher stable nuclear polarization, longer relaxation times and stronger electron-nuclear coupling are achieved which is useful for nuclear-spin-based quantum memory, spin amplifiers and gyroscopes. The optimized sensor demonstrates a sensitivity comparable to the best previous comagnetometer but with four times lower noble gas density. This paves the way for applications in both fundamental and applied science.

physics.atom-ph↗

arXiv2023

Intensity interferometry for ultralight bosonic dark matter detection

Ultralight bosonic dark matter (UBDM) can be described by a classical wave-like field oscillating near the Compton frequency of the bosons. If a measurement scheme for the direct detection of UBDM interactions is sensitive to a signature quadratic in the field, then there is a near-zero-frequency (dc) component of the signal. Thus, a detector with a given finite bandwidth can be used to search for bosons with Compton frequencies many orders of magnitude larger than its bandwidth. This opens the possibility of a detection scheme analogous to Hanbury Brown and Twiss intensity interferometry. Assuming that the UBDM is virialized in the galactic gravitational potential, the random velocities produce slight deviations from the Compton frequency. These result in stochastic fluctuations of the intensity on a time scale determined by the spread in kinetic energies. In order to mitigate ubiquitous local low-frequency noise, a network of sensors can be used to search for the stochastic intensity fluctuations by measuring cross-correlation between the sensors. This method is inherently broadband, since a large range of Compton frequencies will yield near-zero-frequency components within the sensor bandwidth that can be searched for simultaneously. Measurements with existing sensor networks have sufficient sensitivity to search experimentally unexplored parameter space.

hep-ph↗