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Deric Session

Publications and source records attributed to Deric Session.

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Probing Quantum Anomalous Hall States in Twisted Bilayer WSe2 via Attractive Polaron Spectroscopy

Moir\'e superlattices in semiconductors exhibit a rich variety of interaction-induced topological states, including quantum anomalous Hall (QAH) effects. A recent study hinted that twisted WSe2 homobilayer (tWSe2) could host a QAH state but lacked direct evidence of ferromagnetism, a key hallmark of this phase. Here, we report the first direct evidence of QAH states in tWSe2 with spontaneous ferromagnetism. Specifically, we employ polarization-resolved attractive polaron spectroscopy on a dual-gated, 2 degree tWSe2 and observe direct signatures of spontaneous time-reversal symmetry breaking at hole filling \nu = 1. Together with a Chern number measurement via Streda formula analysis, we identify this magnetized state as a topological state, characterized by C = 1. Furthermore, we demonstrate that these topological and magnetic properties are tunable via a finite displacement field, between a QAH ferromagnetic state and an antiferromagnetic state. Our findings position tWSe2 as a highly versatile, stable, and optically addressable platform for investigating topological order and strong correlations in two-dimensional landscapes.

cond-mat.str-el

Giant enhancement of exciton diffusion near an electronic Mott insulator

Bose-Fermi mixtures naturally appear in various physical systems. In semiconductor heterostructures, such mixtures can be realized, with bosons as excitons and fermions as dopant charges. However, the complexity of these hybrid systems challenges the comprehension of the mechanisms that determine physical properties such as mobility. In this study, we investigate interlayer exciton diffusion in an H-stacked WSe$_2$/WS$_2$ heterobilayer. Our measurements are performed in the ultra-low exciton density regime at low temperatures to examine how the presence of charges affects exciton mobility. Remarkably, for charge doping near the Mott insulator phase, we observe a giant enhancement of exciton diffusion of three orders of magnitude compared to charge neutrality. We attribute this observation to mobile valence holes, which experience a suppressed moir\'e potential due to the electronic charge order in the conduction band, and recombine with any conduction electron in a non-monogamous manner. This new mechanism emerges for sufficiently large fillings in the vicinity of correlated generalized Wigner crystal and Mott insulating states. Our results demonstrate the potential to characterize correlated electron states through exciton diffusion and provide insights into the rich interplay of bosons and fermions in semiconductor heterostructures.

cond-mat.str-el

Optical pumping of electronic quantum Hall states with vortex light

A fundamental requirement for quantum technologies is the ability to coherently control the interaction between electrons and photons. However, in many scenarios involving the interaction between light and matter, the exchange of linear or angular momentum between electrons and photons is not feasible, a condition known as the dipole-approximation limit. An example of a case beyond this limit that has remained experimentally elusive is when the interplay between chiral electrons and vortex light is considered, where the orbital angular momentum of light can be transferred to electrons. Here, we present a novel mechanism for such an orbital angular momentum transfer from optical vortex beams to electronic quantum Hall states. Specifically, we identify a robust contribution to the radial photocurrent, in an annular graphene sample within the quantum Hall regime, that depends on the vorticity of light. This phenomenon can be interpreted as an optical pumping scheme, where the angular momentum of photons is transferred to electrons, generating a radial current, and the current direction is determined by the vorticity of the light. Our findings offer fundamental insights into the optical probing and manipulation of quantum coherence, with wide-ranging implications for advancing quantum coherent optoelectronics.

cond-mat.mes-hall

Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moir\'e $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer

Understanding the Hubbard model is crucial for investigating various quantum many-body states and its fermionic and bosonic versions have been largely realized separately. Recently, transition metal dichalcogenides heterobilayers have emerged as a promising platform for simulating the rich physics of the Hubbard model. In this work, we explore the interplay between fermionic and bosonic populations, using a $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer device that hosts this hybrid particle density. We independently tune the fermionic and bosonic populations by electronic doping and optical injection of electron-hole pairs, respectively. This enables us to form strongly interacting excitons that are manifested in a large energy gap in the photoluminescence spectrum. The incompressibility of excitons is further corroborated by measuring exciton diffusion, which remains constant upon increasing pumping intensity, as opposed to the expected behavior of a weakly interacting gas of bosons, suggesting the formation of a bosonic Mott insulator. We explain our observations using a two-band model including phase space filling. Our system provides a controllable approach to the exploration of quantum many-body effects in the generalized Bose-Fermi-Hubbard model.

cond-mat.mes-hall