arXiv subjects

Detlef Lohse

Publications and source records attributed to Detlef Lohse.

At least 91 records · Page 5Linked to original sources

arXiv2023

Buoyancy-driven attraction of active droplets

Active oil droplets in a liquid are believed to repel due to the Marangoni effect, while buoyancy effects caused by the density difference between the droplets, diffusing product, and ambient fluid are usually overlooked. Recent experiments have observed active droplet clustering phenomena due to buoyancy-driven convection (Kruger et al. Eur. Phys. J. E, vol. 39, 2016, pp.1-9). In this study, we numerically analyze the buoyancy effect in addition to Marangoni flow, characterized by Peclet number $Pe$. The buoyancy effects originate from (i) the density difference between the droplet and the ambient liquid, which is characterized by Galileo number $Ga$, and (ii) the density difference between the diffusing product (i.e. filled micelles) and the ambient liquid, characterized by a solutal Rayleigh number $Ra$. We analyze how the attracting and repulsing behavior depends on the control parameters $Pe$, $Ga$, and $Ra$. We find that while Marangoni flow causes repulsion, the buoyancy effect leads to attraction, and even collisions can take place at high Ra. We also observe a delayed collision as $Ga$ increases. Moreover, we derive that the attracting velocity, characterized by a Reynolds number $Re_d$, is proportional to $Ra^{1/4}/(l/R)$, where $l/R$ is the normalized distance by radius between neighboring droplets. Finally, we obtain repulsive velocity, characterized by $Re_{rep}$, as proportional to $PeRa^{-0.38}$. The balance of attractive and repulsive effects results in $Pe \sim Ra^{0.63}$, which agrees with the transition curve between regimes with and without collision.

physics.flu-dyn↗

arXiv2023

Resonance behavior of a compliant piezo-driven inkjet channel with an entrained microbubble

Microbubbles entrained in a piezo-driven drop-on-demand (DOD) printhead disturb the acoustics of the microfluidic ink channel and thereby the jetting behavior. Here, the resonance behavior of an ink channel as a function of the microbubble size and the number of bubbles is studied through theoretical modeling and experiments. The system is modeled as a set of two coupled harmonic oscillators: one corresponding to the compliant ink channel and one to the microbubble. The predicted and measured eigenfrequencies are in excellent agreement. It was found that the resonance frequency is independent of the bubble size as long as the compliance of the bubble dominates over that of the piezo actuator. An accurate description of the eigenfrequency of the coupled system requires the inclusion of the increased inertance of the entrained microbubble due to confinement. We show that the inertance of a confined bubble can be accurately obtained by using a simple potential flow approach. The model is further validated by the excellent agreement between the modeled and measured microbubble resonance curves. The present work therefore provides physical insight in the coupled dynamics of a compliant ink channel with an entrained microbubble.

physics.flu-dyn↗

arXiv2023

Interplay between advective, diffusive, and active barriers in Rayleigh-Bénard flow

Our understanding of the material organization of complex fluid flows has recently benefited from mathematical developments in the theory of objective coherent structures. These methods have provided a wealth of approaches that identify transport barriers in three-dimensional (3D) turbulent flows. Specifically, theoretical advances have been incorporated into numerical algorithms that extract the most influential advective, diffusive and active barriers to transport from data sets in a frame-indifferent fashion. To date, however, there has been very limited investigation into these objectively-defined transport barriers in 3D unsteady flows with complicated spatiotemporal dynamics. Similarly, no systematic comparison of advective, diffusive and active barriers has been carried out in a 3D flow with both thermal and shear-driven features. In our study, we utilize simulations of turbulent rotating Rayleigh-Bénard convection to uncover the interplay between advective transport barriers (Lagrangian coherent structures), material barriers to diffusive heat transport and objective Eulerian barriers to momentum transport. For a range of (inverse) Rossby numbers, we visualize each type of barrier and quantify their role as barriers to momentum and heat transport under changes in the relative influence of mechanical and thermal forces.

physics.flu-dyn↗

arXiv2023

Ice melting in salty water: layering and non-monotonic dependence on the mean salinity

The presence of salt in ocean water strongly affects the melt rate and the shape evolution of ice, both of utmost relevance in geophysical and ocean flow and thus for the climate. To get a better quantitative understanding of the physical mechanics at play in ice melting in salty water, we numerically investigate the lateral melting of an ice block in stably stratified saline water, using a realistic, nonlinear equation of state (EOS). The developing ice shape from our numerical results shows good agreement with the experiments and theory from Huppert & Turner (J. Fluid Mech. 100, 367 (1980)). Furthermore, we find that the melt rate of ice depends non-monotonically on the mean ambient salinity: It first decreases for increasing salt concentration until a local minimum is attained, and then increases again. This non-monotonic behavior of the ice melt rate is due to the competition among salinity-driven buoyancy, temperature-driven buoyancy, and salinity-induced stratification. We develop a theoretical model based on the energy balance which gives a prediction of the salt concentration for which the melt rate is minimal, and is consistent with our data. Our findings give insight into the interplay between phase transitions and double-diffusive convective flows.

physics.flu-dyn↗

arXiv2023

Reconciling airborne disease transmission concerns with energy saving requirements: the potential of UV-C pathogen deactivation and air distribution optimization

The COVID-19 pandemic caused a paradigm shift in our way of using heating, ventilation, and air-conditioning (HVAC) systems in buildings. In the early stages of the pandemic, it was indeed advised to reduce the reuse and thus the recirculation of indoor air to minimize the risk of contamination through inhalation of virus-laden aerosol particles emitted by humans when coughing, sneezing, speaking or breathing. However, such recommendations are not compatible with energy saving requirements stemming from climate change and energy price increase concerns, especially in winter and summer when the fraction of outdoor air supplied to the building needs to be significantly heated or cooled down. In this experimental study, we aim at providing low-cost and low-energy solutions to modify the ventilation strategies currently used in many buildings to reduce the risk of respiratory disease transmission. We find that ultraviolet germicidal irradiation (UVGI) modules added to the HVAC system are very efficient at inactivating pathogens present in aerosols, leading to good indoor air quality even with significant indoor air recirculation. Moreover, we show that an optimal placement of the air exhaust vents relative to air supply vents can improve the ventilation efficiency, with significant consequences in terms of energy savings.

physics.soc-ph↗

arXiv2023

The emergence of bubble-induced scaling in thermal spectra in turbulence

We report on the modification of the spectrum of a passive scalar inside a turbulent flow by the injection of large bubbles. While the spectral modification through bubbles is well known and well analyzed for the velocity fluctuations, little is known on how bubbles change the fluctuations of an approximately passive scalar, in our case temperature. Here we uncover the thermal spectral scaling behavior of a turbulent multiphase thermal mixing layer. The development of a $-3$ spectral scaling is triggered. By injecting large bubbles ($\text{Re}_{\text{bub}} = \mathcal{O}(10^2)$) with gas volume fractions $α$ up to 5\%. For these bubbly flows, the $-5/3$ scaling is still observed at intermediate frequencies for low $α$ but becomes less pronounced when $α$ further increases and it is followed by a steeper $-3$ slope for larger frequencies. This $-3$ scaling range extends with increasing gas volume fraction. The $-3$ scaling exponent coincides with the typical energy spectral scaling for the velocity fluctuations in high Reynolds number bubbly flows. We identify the frequency scale of the transition from the $-5/3$ scaling to the $-3$ scaling and show how it depends on the gas volume fraction.

physics.flu-dyn↗

arXiv2023

Elastocapillary Worthington jets

The retraction of an impacting droplet on a non-wetting substrate is often associated with the formation of a Worthington jet, which is fed by the retracting liquid. A non-Newtonian rheology of the liquid is known to affect the retraction of the impacting droplet. Here we present a novel phenomenon related to the impact of viscoelastic droplets on non-wettable substrates. We reveal that the viscoelasticity of the liquid results in an \emph{elastocapillary} regime in the stretching Worthington jet, distinguished by a pinned contact line and a slender jet that does not detach from the droplet. We identify the impact conditions, in the Weber number -- Deborah number phase space, for observing these \emph{elastocapillary} Worthington jets. Such jets exhibit an effectively nearly linear (in time) variation of the strain rate. Upon further extension, the jet exhibits beads-on-a-string structures, characteristic of the \emph{elastocapillary} thinning of slender viscoelastic liquid filaments. The \emph{elastocapillary} Worthington jet is not only relevant for a droplet impact on a solid substrate scenario, but can also be expected in other configurations where a Worthington jet is observed for viscoelastic liquids, such as drop impact on a liquid pool and bubble bursting at an interface.

physics.flu-dyn↗

arXiv2023

Double-diffusive transport in multicomponent vertical convection

Motivated by the ablation of vertical ice faces in salt water, we use three-dimensional direct numerical simulations to investigate the heat and salt fluxes in two-scalar vertical convection. For parameters relevant to ice-ocean interfaces in the convection-dominated regime, we observe that the salinity field drives the convection and that heat is essentially transported as a passive scalar. By varying the diffusivity ratio of heat and salt (i.e., the Lewis number $Le$), we identify how the different molecular diffusivities affect the scalar fluxes through the system. Away from the walls, we find that the heat transport is determined by a turbulent Prandtl number of $Pr_t\approx 1$ and that double-diffusive effects are practically negligible. However, the difference in molecular diffusivities plays an important role close to the boundaries. In the (unrealistic) case where salt diffused faster than heat, the ratio of salt-to-heat fluxes would scale as $Le^{1/3}$, consistent with classical nested scalar boundary layers. However, in the realistic case of faster heat diffusion (relative to salt), we observe a transition towards a $Le^{1/2}$ scaling of the ratio of the fluxes. This coincides with the thermal boundary layer width growing beyond the thickness of the viscous boundary layer. We find that this transition is not determined by a critical Lewis number, but rather by a critical Prandtl number $Pr\approx 10$, slightly below that for cold seawater where $Pr=14$. We compare our results to similar studies of sheared and double-diffusive flow under ice shelves, and discuss the implications for fluxes in large-scale ice-ocean models. By coupling our results to ice-ocean interface thermodynamics, we describe how the flux ratio impacts the interfacial salinity, and hence the strength of solutal convection and the ablation rate.

physics.flu-dyn↗

arXiv2022

Interfacial aggregation of self-propelled Janus colloids in sessile droplets

Living microorganisms in confined systems typically experience an affinity to populate boundaries. The reason for such affinity to interfaces can be a combination of their directed motion and hydrodynamic interactions at distances larger than their own size. Here we will show that self-propelled Janus particles (polystyrene particles partially coated with platinum) immersed in droplets of water and hydrogen peroxide tend to accumulate in the vicinity of the liquid/gas interface. Interestingly, the interfacial accumulation occurs despite the presence of an evaporation-driven flow caused by a solutal Marangoni flow, which typically tends to redistribute the particles within the droplet's bulk. By performing additional experiments with passive colloids (flow tracers) and comparing with numerical simulations for both particle active motion and the fluid flow, we disentangle the dominating mechanisms behind the observed interfacial particle accumulation. These results allow us to make an analogy between active Janus particles and some biological microswimmers concerning how they interact with their environment.

physics.flu-dyn↗

arXiv2022

When does an impacting drop stop bouncing?

Non-wetting substrates allow impacting liquid drops to spread, recoil, and takeoff, provided they are not too heavy (Biance et al. 2006) or too viscous (Jha et al. 2020). In this article, using direct numerical simulations with the volume of fluid method, we investigate how viscous stresses and gravity conspire against capillarity to inhibit drop rebound. Close to the bouncing to non-bouncing transition, we evidence that the initial spreading stage can be decoupled from the later retraction and takeoff, allowing to understand the rebound as a process converting the surface energy of the spread liquid into kinetic energy. Drawing an analogy with coalescence induced jumping, we propose a criterion for the transition from the bouncing to the non-bouncing regime, namely by the condition $Oh_c + Bo_c \sim 1$, where $Oh_c$ and $Bo_c$ are the Ohnesorge number and Bond number at the transition, respectively. This criterion is in excellent agreement with the numerical results. We also elucidate the mechanisms of bouncing inhibition in the heavy and viscous drops limiting regimes by calculating the energy budgets and relating them to the drop's shape and internal flow.

physics.flu-dyn↗

arXiv2022

Drop impact on viscous liquid films

When a liquid drop falls on a solid substrate, the air layer in between them delays the occurrence of liquid--solid contact. For impacts on smooth substrates, the air film can even prevent wetting, allowing the drop to bounce off with dynamics identical to that observed for impacts on superamphiphobic materials. In this article, we investigate similar bouncing phenomena, occurring on viscous liquid films, that mimic atomically smooth substrates, with the goal to probe their effective repellency. We elucidate the mechanisms associated to the bouncing to non-bouncing (floating) transition using experiments, simulations, and a minimal model that predicts the main characteristics of drop impact, the contact time, and the coefficient of restitution. In the case of highly viscous or very thin films, the impact dynamics is not affected by the presence of the viscous film. Within this substrate--independent limit, bouncing is suppressed once the drop viscosity exceeds a critical value as on superamphiphobic substrates. For thicker or less viscous films, both the drop and film properties influence the rebound dynamics and conspire to inhibit bouncing above a critical film thickness. This substrate--dependent regime also admits a limit, for low viscosity drops, in which the film properties alone determine the limits of repellency.

physics.flu-dyn↗

arXiv2022

Sodium chloride inhibits effective bubbly drag reduction in turbulent bubbly Taylor-Couette flows

Using the Taylor--Couette geometry we experimentally investigate the effect of salt on drag reduction caused by bubbles present in the flow. We combine torque measurements with optical high-speed imaging to relate the bubble size to the drag experienced by the flow. Previous findings have shown that a small percentage of air (4%) can lead to dramatic drag reduction (40%). In contrast to previous laboratory experiments, which mainly used fresh water, we will vary the salinity from fresh water to the average salinity of ocean water. We find that the drag reduction is increasingly more inhibited for increasing salt concentration; going from 40% for fresh water to just 15% for sea water. Salts present in the working fluid inhibit coalescence events, resulting in smaller bubbles in the flow and with that, decreasing the drag reduction. Above a critical salinity, increasing the salinity has no further effect on the bubble sizes in the flow and thus the drag experienced by the flow. Our new findings demonstrate the importance of NaCl on the bubbly drag reduction mechanism, and will further challenge the naval architects to implement promising air lubrication systems on marine vessels.

physics.flu-dyn↗

arXiv2022

Towards realistic simulations of human cough: effect of droplet emission duration and spread angle

Human respiratory events, such as coughing and sneezing, play an important role in the host-to-host airborne transmission of diseases. Thus, there has been a substantial effort in understanding these processes: various analytical or numerical models have been developed to describe them, but their validity has not been fully assessed due to the difficulty of a direct comparison with real human exhalations. In this study, we report a unique comparison between datasets that have both detailed measurements of a real human cough using spirometer and particle tracking velocimetry, and direct numerical simulation at similar conditions. By examining the experimental data, we find that the injection velocity at the mouth is not uni-directional. Instead, the droplets are injected into various directions, with their trajectories forming a cone shape in space. Furthermore, we find that the period of droplet emissions is much shorter than that of the cough: experimental results indicate that the droplets with an initial diameter $\gtrsim 10μ$m are emitted within the first 0.05 s, whereas the cough duration is closer to 1 s. These two features (the spread in the direction of injection velocity and the short duration of droplet emission) are incorporated into our direct numerical simulation, leading to an improved agreement with the experimental measurements. Thus, to have accurate representations of human expulsions in respiratory models, it is imperative to include parametrisation of these two features.

physics.flu-dyn↗

arXiv2022

Evaporation of a sessile colloidal water-glycerol droplet: Marangoni ring formation

The transport and aggregation of particles in suspensions is an important process in many physicochemical and industrial processes. In this work, we study the transport of particles in an evaporating binary droplet. Surprisingly, the accumulation of particles occurs not only at the contact line (due to the coffee-stain effect) or at the solid substrate (due to sedimentation), but also at a particular radial position near the liquid-air interface, forming a "ring", which we term as the Marangoni ring. The formation of this ring is primarily attributed to the solutal Marangoni flow triggered by the evaporation dynamics of the water-glycerol droplet. Experiments and simulations show fair agreement in the volume evolution and the general structure of the solutal Marangoni flow, that is, the Marangoni vortex. Experiments show that the location of the Marangoni ring is strongly correlated with the Marangoni vortex. However, finite element numerical simulations fail to describe the particle distribution seen in the experiments. Interestingly, the particles not only accumulate to form the Marangoni ring but also assemble as colloidal crystals close to the liquid-air interface, yielding iridescence. The formation of the colloidal crystals in the experiments is strong evidence that non-hydrodynamic interactions, which are not represented in the simulations, also play a significant role in our system.

physics.flu-dyn↗

arXiv2022

Entrapment of Interfacial Nanobubbles on Nano Structured Surfaces

Spherical-cap-shaped interfacial nanobubbles (NBs) forming on hydrophobic surfaces in aqueous solutions have extensively been studied both from a fundamental point of view and due to their relevance for various practical applications. In this study, the nucleation mechanism of spontaneously generated NBs at solid-liquid interfaces of immersed nanostructured hydrophobic surfaces is studied. Depending on the size and density of the surface nanostructures, NBs with different size and density were reproducibly and deterministically obtained. A two-step process can explain the NB nucleation, based on the crevice model, i.e., entrapped air pockets in surface cavities which grow by diffusion. The results show direct evidence for the spontaneous formation of NBs on a surface at its immersion. Next, the influence of size and shape of the nanostructures on the nucleated NBs are revealed. In particular, on non-circular nanopits we obtain NBs with a non-circular footprint, demonstrating the strong pinning forces at the three-phase contact line.

physics.flu-dyn↗

arXiv2022

Physiochemical hydrodynamics of the phase segregation in an evaporating binary microdroplet

Phase segregation triggered by selective evaporation can emerge in multicomponent systems, leading to complex physiochemical hydrodynamics. Recently, Li et al. (Phys. Rev. Lett., vol. 120, 2018, 224501) and Kim & Stone (J. Fluid Mech., vol. 850, 2018, pp. 769-783) reported a segregative behavior (i.e., demixing) in an evaporating binary droplet. In this work, by means of experiments and theoretical analysis, we investigate the flow dynamics after the occurrence of the phase segregation. As example, we take the 1,2-hexanediol-water binary droplet system. First, we experimentally reveal the overall physiochemical hydrodynamics of the evaporation process, including the segregative behavior and the resulting flow structure close to the substrate. By quantifying the evolution of the radial flow, we identify three successive life stages of the evaporation process. At Stage I, a radially outward flow is observed. It is driven by the Marangoni effect. At the transition to Stage II, the radial flow partially reverses, starting from the contact line. This flow breaks the axial symmetry and remarkably is driven by the segregation itself. Finally at Stage III, the flow decays as the evaporation gradually ceases. At this stage the segregation has grown to the entire droplet, and the flow is again controlled by the Marangoni effect. The resulting Marangoni flow homogenizes the distribution of the entrapped volatile water over the whole droplet.

physics.flu-dyn↗

arXiv2022

High humidity enhances the evaporation of non-aqueous volatile sprays

We experimentally investigate the evaporation of very volatile liquid droplets (Novec 7000 Engineered Fluid) in a turbulent spray. Droplets with diameters of the order of a few micrometers are produced by a spray nozzle and then injected into a purpose-built enclosed dodecahedral chamber, where the ambient temperature and relative humidity in the chamber are carefully controlled. We observe water condensation on the rapidly evaporating droplet, both for the spray and for a single acoustically levitated millimetric Novec 7000 droplet. We further examine the effect of humidity, and reveal that a more humid environment leads to faster evaporation of the volatile liquid, as well as more water condensation. This is explained by the much larger latent heat of water. We extend an analytical model based on Fick's law to quantitatively account for the data.

physics.flu-dyn↗

arXiv2022

Vorticity-induced flow-focusing leads to bubble entrainment in an inkjet printhead: synchrotron X-ray and volume-of-fluid visualizations

The oscillatory flows present in an inkjet printhead can lead to strong deformations of the air-liquid interface at the nozzle exit. Such deformations may lead to an inward directed air jet with bubble pinch-off and the subsequent entrainment of an air bubble, which is highly detrimental to the stability of inkjet printing. Understanding the mechanisms of bubble entrainment is therefore crucial in improving print stability. In the present work, we use ultrafast X-ray phase-contrast imaging and direct numerical simulations based on the Volume-of-Fluid method to study the mechanisms underlying the bubble entrainment in a piezo-acoustic printhead. We first demonstrate good agreement between experiments and numerics. We then show the different classes of bubble pinch-off obtained in experiments, and that those were also captured numerically. The numerical results are then used to show that the baroclinic torque, which is generated at the gas-liquid interface due to the misalignment of density and pressure gradients, results in a flow-focusing effect that drives the formation of the air jet from which a bubble can pinch-off.

physics.flu-dyn↗