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Detlef Lohse

Publications and source records attributed to Detlef Lohse.

At least 163 records · Page 9Linked to original sources

Regime transitions in thermally driven high-Rayleigh number vertical convection

Vertical convection is investigated using direct numerical simulations over a wide range of Rayleigh numbers $10^7\le Ra\le10^{14}$ with fixed Prandtl number $Pr=10$, in a two-dimensional convection cell with unit aspect ratio. It is found that the dependence of the mean vertical centre temperature gradient $S$ on $Ra$ shows three different regimes: In regime I ($Ra \lesssim 5\times10^{10}$), $S$ is almost independent of $Ra$; In the newly identified regime II ($5\times10^{10} \lesssim Ra \lesssim 10^{13}$), $S$ first increases with increasing $Ra$ (regime ${\rm{II}}_a$), reaches its maximum and then decreases again (regime ${\rm{II}}_b$); In regime III ($Ra\gtrsim10^{13}$), $S$ again becomes only weakly dependent on $Ra$, being slightly smaller than in regime I. The transitions between diffeereent regimes are discussd. In the three different regimes, significantly different flow organizations are identified: In regime I and regime ${\rm{II}}_a$, the location of the maximal horizontal velocity is close to the top and bottom walls; However, in regime ${\rm{II}}_b$ and regime III, banded zonal flow structures develop and the maximal horizontal velocity now is in the bulk region. The different flow organizations in the three regimes are also reflected in the scaling exponents in the effective power law scalings $Nu\sim Ra^β$ and $Re\sim Ra^γ$. In regime I, the fitted scaling exponents ($β\approx0.26$ and $γ\approx0.51$) are in excellent agreement with the theoretical predication of $β=1/4$ and $γ=1/2$ for laminar VC (Shishkina, {\it{Phys. Rev. E.}} 2016, 93, 051102). However, in regimes II and III, $β$ increases to a value close to 1/3 and $γ$ decreases to a value close to 4/9. The stronger $Ra$ dependence of $Nu$ is related to the ejection of plumes and larger local heat flux at the walls.

physics.flu-dyn↗

Dissolution of microdroplets in a sparsely miscible liquid confined by leaky walls

When a water droplet is deposited within a sparsely miscible liquid medium such as certain oils, the droplet surprisingly vanishes, even in a confined geometry. Such a phenomenon has crucial consequences for multiphase flows in which confined nano- and/or picoliter droplets are considered. We report here experiments of microdroplet dissolution in microchannels that reveal an enhancement of the shrinkage of confined water microdroplets in oil due to the permeability of the walls - made of polydimethilsiloxane (PDMS) - and a delay when collective effects are present. The system is first modelled assuming that the dissolution of the droplets in its surrounding liquid follows the Epstein-Plesset solution of the diffusion equation. The dissolution of small isolated droplets can indeed be described by this solution of the diffusion equation, while the vanishing of droplets larger than a certain critical value and those closer to other droplets requires numerical simulations which take into account the boundary conditions of the confined system, the neighbouring droplets and interestingly, the evaporative water vapour flux through the PDMS. Our results thus reveal the important role of the water solubility in oil and most remarkably, of the water vapour transport through permeable walls.

physics.flu-dyn↗

Two-layer Thermally Driven Turbulence: Mechanisms for Interface Breakup

It is commonly accepted that the breakup criteria of drops or bubbles in turbulence is governed by surface tension and inertia. However, also {\it{buoyancy}} can play an important role at breakup. In order to better understand this role, here we numerically study Rayleigh-Bénard convection for two immiscible fluid layers, in order to identify the effects of buoyancy on interface breakup. We explore the parameter space spanned by the Weber number $5\leq We \leq 5000$ (the ratio of inertia to surface tension) and the density ratio between the two fluids $0.001 \leq Λ\leq 1$, at fixed Rayleigh number $Ra=10^8$ and Prandtl number $Pr=1$. At low $We$, the interface undulates due to plumes. When $We$ is larger than a critical value, the interface eventually breaks up. Depending on $Λ$, two breakup types are observed: The first type occurs at small $Λ\ll 1$ (e.g. air-water systems) when local filament thicknesses exceed the Hinze length scale. The second, strikingly different, type occurs at large $Λ$ with roughly $0.5 < Λ\le 1$ (e.g. oil-water systems): The layers undergo a periodic overturning caused by buoyancy overwhelming surface tension. For both types the breakup criteria can be derived from force balance arguments and show good agreement with the numerical results.

physics.flu-dyn↗

Growth of respiratory droplets in cold and humid air

The ambient conditions surrounding liquid droplets determine their growth or shrinkage. However, the precise fate of a liquid droplet expelled from a respiratory puff as dictated by its surroundings and the puff itself has not yet been fully quantified. From the view of airborne disease transmission, such as SARS-CoV-2, knowledge of such dependencies are critical. Here we employ direct numerical simulations (DNS) of a turbulent respiratory vapour puff and account for the mass and temperature exchange with respiratory droplets and aerosols. In particular, we investigate how droplets respond to different ambient temperatures and relative humidity (RH) by tracking their Lagrangian statistics. We reveal and quantify that in cold and humid environments, as there the respiratory puff is supersaturated, expelled droplets can first experience significant growth, and only later followed by shrinkage, in contrast to the monotonic shrinkage of droplets as expected from the classical view by William F. Wells (1934). Indeed, cold and humid environments diminish the ability of air to hold water vapour, thus causing the respiratory vapour puff to super-saturate. Consequently, the super-saturated vapour field drives the growth of droplets that are caught and transported within the humid puff. To analytically predict the likelihood for droplet growth, we propose a model for the axial RH based on the assumption of a quasi-stationary jet. Our model correctly predicts super-saturated RH conditions and is in good quantitative agreement with our DNS. Our results culminate in a temperature-RH map that can be employed as an indicator for droplet growth or shrinkage.

physics.flu-dyn↗

Scaling in internally heated convection: a unifying theory

We offer a unifying theory for turbulent purely internally heated convection, generalizing the unifying theories of Grossmann and Lohse (2000, 2001) for Rayleigh--Bénard turbulence and of Shishkina, Grossmann and Lohse (2016) for turbulent horizontal convection, which are both based on the splitting of the kinetic and thermal dissipation rates in respective boundary and bulk contributions. We obtain the mean temperature of the system and the Reynolds number (which are the response parameters) as function of the control parameters, namely the internal thermal driving strength (called, when nondimensionalized, the Rayleigh--Roberts number) and the Prandtl number. The results of the theory are consistent with our direct numerical simulations.

physics.flu-dyn↗

Characterizing the turbulent drag properties of rough surfaces with a Taylor--Couette setup

Wall-roughness induces extra drag in wall-bounded turbulent flows. Mapping any given roughness geometry to its fluid dynamic behaviour has been hampered by the lack of accurate and direct measurements of skin-friction drag. Here the Taylor-Couette (TC) system provides an opportunity as it is a closed system and allows to directly and reliably measure the skin-friction. However, the wall-curvature potentially complicates the connection between the wall friction and the wall roughness characteristics. Here we investigate the effects of a hydrodynamically fully rough surface on highly turbulent, inner cylinder rotating, TC flow. We find that the effects of a hydrodynamically fully rough surface on TC turbulence, where the roughness height k is three orders of magnitude smaller than the Obukhov curvature length Lc (which characterizes the effects of curvature on the turbulent flow, see Berghout et al. arXiv: 2003.03294, 2020), are similar to those effects of a fully rough surface on a flat plate turbulent boundary layer (BL). Hence, the value of the equivalent sand grain height ks, that characterizes the drag properties of a rough surface, is similar to those found for comparable sandpaper surfaces in a flat plate BL. Next, we obtain the dependence of the torque (skin-friction drag) on the Reynolds number for given wall roughness, characterized by ks, and find agreement with the experimental results within 5 percent. Our findings demonstrate that global torque measurements in the TC facility are well suited to reliably deduce wall drag properties for any rough surface.

physics.flu-dyn↗

Pattern formation during the impact of a partially-frozen binary droplet on a cold surface

Impact of a droplet on an undercooled surface is a complex phenomenon as it simultaneously instigates several physical processes that cover a broad spectrum of transport phenomena and phase-transition. Here, we report and explain an unexpected but highly relevant phenomenon of fingered growth of the solid-phase. It emerges during the impact of a binary droplet that freezes from the outside prior to the impact on the undercooled surface. We establish that the presence of pre-solidified material at the advancing contact line fundamentally changes the resulting dynamics, namely by modifying the local flow mobility that leads to an instability analogous to viscous fingering. Moreover, we delineate the interplay between the interfacial deformations of the impacting droplet and patterned growth of the solid-phase as disconnected patterns emerge at faster impacts.

physics.flu-dyn↗

Electrochemically Induced pH Change: Time-Resolved Confocal Fluorescence Microscopy Measurements and Comparison with Numerical Model

Confocal fluorescence microscopy is a proven technique, which can image near-electrode pH changes. For a complete understanding of electrode processes, time-resolved measurements are required, which have not yet been provided. Here we present the first measurements of time-resolved pH profiles with confocal fluorescence microscopy. The experimental results compare favorably with a one-dimensional reaction-diffusion model; this holds up to the point where the measurements reveal three-dimensionality in the pH distribution. Specific factors affecting the pH measurement such as attenuation of light and the role of dye migration are also discussed in detail. The method is further applied to reveal the buffer effects observed in sulfate-containing electrolytes. The work presented here is paving the way toward the use of confocal fluorescence microscopy in the measurement of 3D time-resolved pH changes in numerous electrochemical settings, for example in the vicinity of bubbles.

physics.app-ph↗

Effect of axially varying sandpaper roughness on bubbly drag reduction in Taylor-Couette turbulence

We experimentally investigate the influence of alternating rough and smooth walls on bubbly drag reduction (DR). We apply rough sandpaper bands of width $s$ between $48.4\,mm$ and $148.5\,mm$, and roughness height $k = 695\,μm$, around the smooth inner cylinder (IC) of the Twente Turbulent Taylor-Couette facility. Between sandpaper bands, the IC is left uncovered over similar width $s$, resulting in alternating rough and smooth bands, a constant pattern in axial direction. We measure the DR in water that originates from introducing air bubbles to the fluid at (shear) Reynolds numbers $\textit{Re}_s$ ranging from $0.5 \times 10^6$ to $1.8 \times 10^6$. Results are compared to bubbly DR measurements with a completely smooth IC and an IC that is completely covered with sandpaper of the same roughness $k$. The outer cylinder is left smooth for all variations. Results are also compared to bubbly DR measurements where a smooth outer cylinder is rotating in opposite direction to the smooth IC. This counter rotation induces secondary flow structures that are very similar to those observed when the IC is composed of alternating rough and smooth bands. For the measurements with roughness, the bubbly DR is found to initially increase more strongly with $\textit{Re}_s$, before levelling off to reach a value that no longer depends on $\textit{Re}_s$. This is attributed to a more even axial distribution of the air bubbles, resulting from the increased turbulence intensity of the flow compared to flow over a completely smooth wall at the same $\textit{Re}_s$. The air bubbles are seen to accumulate at the rough wall sections in the flow. Here, locally, the drag is largest and so the drag reducing effect of the bubbles is felt strongest. Therefore, a larger maximum value of bubbly DR is found for the alternating rough and smooth walls compared to the completely rough wall.

physics.flu-dyn↗

Evaporation-Induced Crystallization of Surfactants in Sessile Multicomponent Droplets

Surfactants have been widely studied and used in controlling droplet evaporation. In this work, we observe and study the crystallization of sodium dodecyl sulfate (SDS) within an evaporating glycerol-water mixture droplet. The crystallization is induced by the preferential evaporation of water, which decreases the solubility of SDS in the mixture. As a consequence, the crystals shield the droplet surface and cease the evaporation. The universality of the evaporation characteristics for a range of droplet sizes is revealed by applying a diffusion model, extended by Raoult's law. To describe the nucleation and growth of the crystals, we employ the 2-dimensional crystallization model of Weinberg [J. Non-Cryst. Solids 1991, 134, 116]. The results of this model compare favorably to our experimental results. Our findings may inspire the community to reconsider the role of high concentration of surfactants in a multicomponent evaporation system.

physics.flu-dyn↗

Drop Impact on Hot Plates: Contact times, Lift-off and the Lamella Rupture

When a liquid drop impacts on a heated substrate, it can remain deposited, or violently boil in contact, or lift off with or without ever touching the surface. The latter is known as the Leidenfrost effect. The duration and area of the liquid--substrate contact is highly relevant for the heat transfer, as well as other effects such as corrosion. However, most experimental studies rely on side view imaging to determine contact times, and those are often mixed with the time until the drop lifts off from the substrate. Here, we develop and validate a reliable method of contact time determination using high-speed X-ray and Total Internal Reflection measurements. We exemplarily compare contact and lift-off times on flat silicon and sapphire substrates. We show that drops can rebound even without formation of a complete vapor layer, with a wide range of lift-off times. On sapphire, we find a local minimum of lift-off times much shorter than by capillary rebound in the comparatively low-temperature regime of transition boiling / thermal atomization. We elucidate the underlying mechanism related to spontaneous rupture of the lamella and receding of the contact area.

physics.flu-dyn↗

Speeding up biphasic reactions with surface nanodroplets

Biphasic chemical reactions compartmentalized in small droplets offer advantages, such as streamlined procedures for chemical analysis, enhanced chemical reaction efficiency and high specificity of conversion. In this work, we experimentally and theoretically investigate the rate for biphasic chemical reactions between acidic nanodroplets on a substrate surface and basic reactants in a surrounding bulk flow. The reaction rate is measured by droplet shrinkage as the product is removed from the droplets by the flow. In our experiments, we determine the dependence of the reaction rate on the flow rate and the solution concentration. The theoretical analysis predicts that the life time $τ$ of the droplets scales with Peclet number $Pe$ and the reactant concentration in the bulk flow $c_{re,bulk}$ as $τ\propto Pe^{-3/2}c_{re,bulk}^{-1}$, in good agreement with our experimental results. Furthermore, we found that the product from the reaction on an upstream surface can postpone the droplet reaction on a downstream surface, possibly due to the adsorption of interface-active products on the droplets in the downstream. The time of the delay decreases with increasing $Pe$ of the flow and also with increasing reactant concentration in the flow, following the scaling same as that of the reaction rate with these two parameters. Our findings provide insight for the ultimate aim to enhance droplet reactions under flow conditions.

cond-mat.soft↗

The effect of Prandtl number on turbulent sheared thermal convection

In turbulent wall sheared thermal convection, there are three different flow regimes, depending on the relative relevance of thermal forcing and wall shear. In this paper we report the results of direct numerical simulations of such sheared Rayleigh-Bénard convection, at fixed Rayleigh number $Ra=10^6$, varying the wall Reynolds number in the range $0 \leq Re_w \leq 4000$ and Prandtl number $0.22 \leq Pr \leq 4.6$, extending our prior work by Blass et al. (2020), where $Pr$ was kept constant at unity and the thermal forcing ($Ra$) varied. We cover a wide span of bulk Richardson numbers $0.014 \leq Ri \leq 100$ and show that the Prandtl number strongly influences the morphology and dynamics of the flow structures. In particular, at fixed $Ra$ and $Re_w$, a high Prandtl number causes stronger momentum transport from the walls and therefore yields a greater impact of the wall shear on the flow structures, resulting in an increased effect of $Re_w$ on the Nusselt number. Furthermore, we analyse the thermal and kinetic boundary layer thicknesses and relate their behaviour to the resulting flow regimes. For the largest shear rates and $Pr$ numbers, we observe the emergence of a Prandtl-von Karman log-layer, signalling the onset of turbulent dynamics in the boundary layer. Finally, our results allow to extend the Grossmann-Lohse theory for heat transport in Rayleigh-Bénard convection to the sheared case, universally describing $Nu(Ra,Pr,Re_w)$.

physics.flu-dyn↗

Bubbly drag reduction using a hydrophobic inner cylinder in Taylor-Couette turbulence

In this study we experimentally investigate bubbly drag reduction in a highly turbulent flow of water with dispersed air at $5.0 \times 10^{5} \leq \text{Re} \leq 1.7 \times 10^{6}$ over a non-wetting surface containing micro-scale roughness. To do so, the Taylor-Couette geometry is used, allowing for both accurate global drag and local flow measurements. The inner cylinder - coated with a rough, hydrophobic material - is rotating, whereas the smooth outer cylinder is kept stationary. The crucial control parameter is the air volume fraction $α$ present in the working fluid. For small volume fractions ($α< {4}\,\%$), we observe that the surface roughness from the coating increases the drag. For large volume fractions of air ($α\geq 4\,\%$), the drag decreases compared to the case with both the inner and outer cylinders uncoated, i.e. smooth and hydrophilic, using the same volume fraction of air. This suggests that two competing mechanisms are at place: on the one hand the roughness invokes an extension of the log-layer - resulting in an increase in drag - and on the other hand there is a drag-reducing mechanism of the hydrophobic surface interacting with the bubbly liquid. The balance between these two effects determines whether there is overall drag reduction or drag enhancement. For further increased bubble concentration $α= {6}\,\%$ we find a saturation of the drag reduction effect. Our study gives guidelines for industrial applications of bubbly drag reduction in hydrophobic wall-bounded turbulent flows.

physics.flu-dyn↗

Double maxima of angular momentum transport in $η=0.91$ TC turbulence

We use experiments and direct numerical simulations to probe the phase-space of low-curvature Taylor--Couette (TC) flow in the vicinity of the ultimate regime. The cylinder radius ratio is fixed at $η=r_i/r_o=0.91$. Non-dimensional shear drivings (Taylor numbers $\text{Ta}$) in the range $10^7\leq\text{Ta}\leq10^{11}$ are explored for both co- and counter-rotating configurations. In the $\text{Ta}$ range $10^8\leq\text{Ta}\leq10^{10}$, we observe two local maxima of the angular momentum transport as a function of the cylinder rotation ratio, which can be described as either as "co-" and "counter-rotating" due to their location or as "broad" and "narrow" due to their shape. We confirm that the broad peak is accompanied by the strengthening of the large-scale structures, and that the narrow peak appears once the driving (Ta) is strong enough. As first evidenced in numerical simulations by Brauckmann \emph{et al.}~(2016), the broad peak is produced by centrifugal instabilities and that the narrow peak is a consequence of shear instabilities. We describe how the peaks change with $\text{Ta}$ as the flow becomes more turbulent. Close to the transition to the ultimate regime when the boundary layers (BLs) become turbulent, the usual structure of counter-rotating Taylor vortex pairs breaks down and stable unpaired rolls appear locally. We attribute this state to changes in the underlying roll characteristics during the transition to the ultimate regime. Further changes in the flow structure around $\text{Ta}\approx10^{10}$ cause the broad peak to disappear completely and the narrow peak to move. This second transition is caused when the regions inside the BLs which are locally smooth regions disappear and the whole boundary layer becomes active.

physics.flu-dyn↗

Flow organization in laterally unconfined Rayleigh-Bénard turbulence

We investigate the large-scale circulation (LSC) of turbulent Rayleigh-Bénard convection in a large box of aspect ratio $Γ=32$ for Rayleigh numbers up to $Ra=10^9$ and at a fixed Prandtl number $Pr=1$. A conditional averaging technique allows us to extract statistics of the LSC even though the number and the orientation of the structures vary throughout the domain. We find that various properties of the LSC obtained here, such as the wall-shear stress distribution, the boundary layer thicknesses and the wind Reynolds number, do not differ significantly from results in confined domains ($Γ\approx 1$). This is remarkable given that the size of the structures (as measured by the width of a single convection roll) more than doubles at the highest $Ra$ as the confinement is removed. An extrapolation towards the critical shear Reynolds number of $Re_s^{\textrm{crit}} \approx 420$, at which the boundary layer (BL) typically becomes turbulent, predicts that the transition to the ultimate regime is expected at $Ra_{\textrm{crit}} \approx \mathcal{O}(10^{15})$ in unconfined geometries. This result is in line with the Göttingen experimental observations. Furthermore, we confirm that the local heat transport close to the wall is highest in the plume impacting region, where the thermal BL is thinnest, and lowest in the plume emitting region, where the thermal BL is thickest. This trend, however, weakens with increasing $Ra$.

physics.flu-dyn↗

Competing Marangoni and Rayleigh convection in evaporating binary droplets

For a small sessile or pendant droplet it is generally assumed that gravity does not play any role once the Bond number is small. This is even assumed for evaporating binary sessile or pendant droplets, in which convective flows can be driven due to selective evaporation of one component and the resulting concentration and thus surface tension differences at the air-liquid interface. However, recent studies have shown that in such droplets gravity indeed can play a role and that natural convection can be the dominant driving mechanism for the flow inside evaporating binary droplets (Edwards et al., Phys. Rev. Lett. 121, 184501 (2018); Li et al., Phys. Rev. Lett. 122, 114501 (2019)). In this study, we derive and validate a quasi-stationary model for the flow inside evaporating binary sessile and pendant droplets, which successfully allows to predict the prevalence and the intriguing interaction of Rayleigh and/or Marangoni convection on the basis of a phase diagram for the flow field expressed in terms of the Rayleigh and Marangoni numbers.

physics.flu-dyn↗

Rayleigh-Taylor instability by segregation in an evaporating multi-component microdroplet

The evaporation of multi-component droplets is relevant to various applications but challenging to study due to the complex physicochemical dynamics. Recently, Li (2018) reported evaporation-triggered segregation in 1,2-hexanediol-water binary droplets. In this present work, we added 0.5 wt% silicone oil into the 1,2-hexanediol-water binary solution. This minute silicone oil concentration dramatically modifies the evaporation process as it triggers an early extraction of the 1,2-hexanediol from the mixture. Surprisingly, we observe that the segregation of 1,2-hexanediol forms plumes, rising up from the rim of the sessile droplet towards the apex during the droplet evaporation. By orientating the droplet upside down, i.e., by studying a pendant droplet, the absence of the plumes indicates that the flow structure is induced by buoyancy, which drives a Rayleigh-Taylor instability (i.e., driven by density differences & gravitational acceleration). From micro-PIV measurement, we further prove that the segregation of the non-volatile component (1,2-hexanediol) hinders the evaporation near the contact line, which leads to a suppression of the Marangoni flow in this region. Hence, on long time scales, gravitational effects play the dominant role in the flow structure, rather than Marangoni flows. We compare the measurement of the evaporation rate with the diffusion model of Popov (2005), coupled with Raoult's law and the activity coefficient. This comparison indeed confirms that the silicone-oil-triggered segregation of the non-volatile 1,2-hexanediol significantly delays the evaporation. With an extended diffusion model, in which the influence of the segregation has been implemented, the evaporation can be well described.

physics.flu-dyn↗