arXiv subjects

Di Xiao

Publications and source records attributed to Di Xiao.

At least 109 records · Page 6Linked to original sources

arXiv2022

Anomalous Second Harmonic Generation from Atomically Thin MnBi2Te4

MnBi2Te4 is a van der Waals topological insulator with intrinsic intralayer ferromagnetic exchange and A-type antiferromagnetic interlayer coupling. Theoretically, it belongs to a class of structurally centrosymmetric crystals whose layered antiferromagnetic order breaks inversion symmetry for even layer numbers, making optical second harmonic generation (SHG) an ideal probe of the coupling between the crystal and magnetic structures. Here, we perform magnetic field and temperature-dependent SHG measurements on MnBi2Te4 flakes ranging from bulk to monolayer thickness. We find that the dominant SHG signal from MnBi2Te4 is unexpectedly unrelated to both magnetic state and layer number. We suggest that surface SHG is the likely source of the observed strong SHG, whose symmetry matches that of the MnBi2Te4-vacuum interface. Our results highlight the importance of considering the surface contribution to inversion symmetry-breaking in van der Waals centrosymmetric magnets.

cond-mat.mtrl-sci↗

arXiv2022

Mixed-dimensional moiré systems of graphitic thin films with a twisted interface

Moiré patterns formed by stacking atomically-thin van der Waals crystals with a relative twist angle can give rise to dramatic new physical properties. The study of moiré materials has so far been limited to structures comprising no more than a few vdW sheets, since a moiré pattern localized to a single two-dimensional interface is generally assumed to be incapable of appreciably modifying the properties of a bulk three-dimensional crystal. Layered semimetals such as graphite offer a unique platform to challenge this paradigm, owing to distinctive properties arising from their nearly-compensated electron and hole bulk doping. Here, we perform transport measurements of dual-gated devices constructed by slightly rotating a monolayer graphene sheet atop a thin bulk graphite crystal. We find that the moiré potential transforms the electronic properties of the entire bulk graphitic thin film. At zero and small magnetic fields, transport is mediated by a combination of gate-tunable moiré and graphite surface states, as well as coexisting semimetallic bulk states that do not respond to gating. At high field, the moiré potential hybridizes with the graphitic bulk states owing to the unique properties of the two lowest Landau bands of graphite. These Landau bands facilitate the formation of a single quasi-two-dimensional hybrid structure in which the moiré and bulk graphite states are inextricably mixed. Our results establish twisted graphene-graphite as the first in a new class of mixed-dimensional moiré materials.

cond-mat.mes-hall↗

arXiv2022

Controlling Andreev bound states with the magnetic vector potential

Tunneling spectroscopy measurements are often used to probe the energy spectrum of Andreev bound states (ABSs) in semiconductor-superconductor hybrids. Recently, this spectroscopy technique has been incorporated into planar Josephson junctions (JJs) formed in two-dimensional electron gases, a potential platform to engineer phase-controlled topological superconductivity. Here, we perform ABS spectroscopy at the two ends of planar JJs and study the effects of the magnetic vector potential on the ABS spectrum. We show that the local superconducting phase difference arising from the vector potential is equal in magnitude and opposite in sign at the two ends, in agreement with a model that assumes localized ABSs near the tunnel barriers. Complemented with microscopic simulations, our experiments demonstrate that the local phase difference can be used to estimate the relative position of localized ABSs separated by a few hundred nanometers.

cond-mat.mes-hall↗

arXiv2022

Dynamical criticality of spin-shear coupling in van der Waals antiferromagnets

The interplay between a multitude of electronic, spin, and lattice degrees of freedom underlies the complex phase diagrams of quantum materials. Layer stacking in van der Waals (vdW) heterostructures is responsible for exotic electronic and magnetic properties, which inspires stacking control of two-dimensional magnetism. Beyond the interplay between stacking order and interlayer magnetism, we discover a spin-shear coupling mechanism in which a subtle shear of the atomic layers can have a profound effect on the intralayer magnetic order in a family of vdW antiferromagnets. Using time-resolved x-ray diffraction and optical linear dichroism measurements, interlayer shear is identified as the primary structural degree of freedom that couples with magnetic order. The recovery times of both shear and magnetic order upon optical excitation diverge at the magnetic ordering temperature with the same critical exponent. The time-dependent Ginzburg-Landau theory shows that this concurrent critical slowing down arises from a linear coupling of the interlayer shear to the magnetic order, which is dictated by the broken mirror symmetry intrinsic to the monoclinic stacking. Our results highlight the importance of interlayer shear in ultrafast control of magnetic order via spin-mechanical coupling.

cond-mat.mtrl-sci↗

arXiv2022

Tunable Exciton-Hybridized Magnon Interactions in a Layered Semiconductor

The interaction between distinct excitations in solids is of both fundamental interest and technological importance. One example of such interactions is coupling between an exciton, a Coulomb bound electron-hole pair, and a magnon, a collective spin excitation. The recent emergence of van der Waals magnetic semiconductors provides a powerful platform for exploring these exciton-magnon interactions and their fundamental properties, such as strong correlation, as well as their photo-spintronic and quantum transduction applications. Here we demonstrate precise control of coherent exciton-magnon interactions in the layered magnetic semiconductor CrSBr. We show that by controlling the direction of applied magnetic fields relative to the crystal axes, and thus the rotational symmetry of the magnetic system, we can tune not only the exciton coupling to the bright magnon, but also to an optically dark mode via magnon hybridization. The exciton-magnon coupling and associated magnon dispersion curves can be further modulated by applying a uniaxial strain. At the critical strain, a dispersionless dark magnon band emerges. Our results demonstrate unprecedented control of the opto-mechanical-magnonic coupling, and a step towards the predictable and controllable implementation of hybrid quantum magnonics.

cond-mat.mes-hall↗

arXiv2022

Hints of a universal width-energy relation for classified fast radio bursts

The total available sample of fast radio bursts (FRBs) has been growing steadily in recent years, facilitating the study of FRBs from a statistical point of view. At the same time, the classification of FRBs is currently an imperative issue. We propose that the brightness temperature of bursts can serve as an ideal criterion for classification. In this work, we gather the available data for all localized FRBs and we find a positive relation between the intrinsic pulse width and burst energy, $T_{\rm i}\propto E_ν^{0.25}$, for three repeating FRBs that is similar to that of our previous work using FRB 20121102A data alone. The critical line $T_{\rm B,cri}$ is found to vary for different FRBs, which may reflect the differences in source properties. This relation can put strong constraints on mainstream radiation mechanisms. It is evident that neither the coherent curvature radiation or synchrotron maser radiation have the capability to reach the high brightness temperature required to reproduce this relation.

astro-ph.HE↗

arXiv2022

Unconventional Charge-density-wave Order in a Dilute d-band Semiconductor

Electron-lattice coupling effects in low dimensional materials give rise to charge density wave (CDW) order and phase transitions. These phenomena are critical ingredients for superconductivity and predominantly occur in metallic model systems such as doped cuprates, transition metal dichalcogenides, and more recently, in Kagome lattice materials. However, CDW in semiconducting systems, specifically at the limit of low carrier concentration region, is uncommon. Here, we combine electrical transport, synchrotron X-ray diffraction and optical spectroscopy to discover CDW order in a quasi-one-dimensional (1D), dilute d-band semiconductor, BaTiS3, which suggests the existence of strong electron-phonon coupling. The CDW state further undergoes an unusual transition featuring a sharp increase in carrier mobility. Our work establishes BaTiS3 as a unique platform to study the CDW physics in the dilute filling limit to explore novel electronic phases.

cond-mat.mtrl-sci↗

arXiv2022

Intercell Moiré Exciton Complexes in Electron Lattices

Excitons, Coulomb-bound electron-hole pairs, play a fundamental role in both optical excitation and correlated phenomena in solids. When an exciton interacts with other quasi-particles, few- and many-body excited states, such as trions, exciton Fermi-polarons, Mahan excitons can appear. Here, we report a new interaction between exciton and charges enabled by unusual quantum confinement in 2D moiré superlattices, which results in novel exciton many-body ground states composed of moiré excitons and correlated electron lattices. Unique to H-stacked (or 60o-twisted) WS2/WSe2 heterobilayer, we found that the interlayer atomic registry and moiré structural reconstruction leads to an interlayer moiré exciton (IME) whose hole in one layer is surrounded by its partner electron's wavefunction spread among three adjacent moiré traps in the other layer. This 3D excitonic structure can enable large in-plane electrical quadrupole moments in addition to the vertical dipole. Upon doping, the electric quadrupole facilitates the binding of IME to the charges in neighboring moiré cells, forming an intercell charged exciton complex. The exciton complex is unveiled by the IME photoluminescence energy jumps when the electron lattices form at both fractional and integer-filled moiré minibands, with replica-like spectral features between successive integer moiré fillings. Our work provides the framework in understanding and engineering emergent exciton many-body states in correlated moiré charge orders.

cond-mat.mes-hall↗

arXiv2022

Gate-tunable proximity effects in graphene on layered magnetic insulators

The extreme versatility of two-dimensional van der Waals (vdW) materials derives from their ability to exhibit new electronic properties when assembled in proximity with dissimilar crystals. For example, although graphene is inherently non-magnetic, recent work has reported a magnetic proximity effect in graphene interfaced with magnetic substrates, potentially enabling a pathway towards achieving a high-temperature quantum anomalous Hall effect. Here, we investigate heterostructures of graphene and chromium trihalide magnetic insulators (CrI$_3$, CrBr$_3$, and CrCl$_3$). Surprisingly, we are unable to detect a magnetic exchange field in the graphene, but instead discover proximity effects featuring unprecedented gate-tunability. The graphene becomes highly hole-doped due to charge transfer from the neighboring magnetic insulator, and further exhibits a variety of atypical transport features. These include highly extended quantum Hall plateaus, abrupt reversals in the Landau level filling sequence, and hysteresis over at least days-long time scales. In the case of CrI$_3$, we are able to completely suppress the charge transfer and all attendant atypical transport effects by gating. The charge transfer can additionally be altered in a first-order phase transition upon switching the magnetic states of the nearest CrI$_3$ layers. Our results provide a roadmap for exploiting the magnetic proximity effect in graphene, and motivate further experiments with other magnetic insulators.

cond-mat.mes-hall↗

arXiv2022

Gate-tunable anomalous Hall effect in a 3D topological insulator/2D magnet van der Waals heterostructure

We demonstrate advantages of samples made by mechanical stacking of exfoliated van der Waals materials for controlling the topological surface state of a 3-dimensional topological insulator (TI) via interaction with an adjacent magnet layer. We assemble bilayers with pristine interfaces using exfoliated flakes of the TI BiSbTeSe2 and the magnet Cr2Ge2Te6, thereby avoiding problems caused by interdiffusion that can affect interfaces made by top-down deposition methods. The samples exhibit an anomalous Hall effect (AHE) with abrupt hysteretic switching. For the first time in samples composed of a TI and a separate ferromagnetic layer, we demonstrate that the amplitude of the AHE can be tuned via gate voltage with a strong peak near the Dirac point. This is the signature expected for the AHE due to Berry curvature associated with an exchange gap induced by interaction between the topological surface state and an out-of-plane-oriented magnet.

cond-mat.mes-hall↗

arXiv2022

Fast Radio Bursts

The era of fast radio bursts (FRBs) was open in 2007, when a very bright radio pulse of unknown origin was discovered occasionally in the archival data of Parkes Telescope. Over the past fifteen years, this mysterious phenomenon have caught substantial attention among the scientific community and become one of the hottest topic in high-energy astrophysics. The total number of events has a dramatic increase to a few hundred recently, benefiting from new dedicated surveys and improved observational techniques. Our understanding of these bursts has been undergoing a revolutionary growth with observational breakthroughs announced consistently. In this chapter, we will give a comprehensive introduction of FRBs, including the latest progress. Starting from the basics, we will go through population study, inherent physical mechanism, and all the way to the application in cosmology. Plenty of open questions exist right now and there is more surprise to come in this active young field.

astro-ph.HE↗

arXiv2022

Light-Induced Ferromagnetism in Moiré Superlattices

Many-body interactions between carriers lie at the heart of correlated physics. The ability to tune such interactions would open the possibility to access and control complex electronic phase diagrams on demand. Recently, moiré superlattices formed by two-dimensional materials have emerged as a promising platform for quantum engineering such phenomena. The power of the moiré system lies in the high tunability of its physical parameters by tweaking layer twist angle, electrical field, moiré carrier filling, and interlayer coupling. Here, we report that optical excitation can drastically tune the spin-spin interactions between moiré trapped carriers, resulting in ferromagnetic order in WS2/WSe2 moiré superlattices over a small range of doping at elevated temperatures. Near the filling factor v = -1/3 (i.e., one hole per three moiré unit cells), as the excitation power at the exciton resonance increases, a well-developed hysteresis loop emerges in the reflective magnetic circular dichroism (RMCD) signal as a function of magnetic field, a hallmark of ferromagnetism. The hysteresis loop persists down to charge neutrality, and its shape evolves as the moiré superlattice is gradually filled, indicating changes of magnetic ground state properties. The observed phenomenon points to a mechanism in which itinerant photo-excited excitons mediate exchange coupling between moiré trapped holes. This exciton-mediated interaction can be of longer range than direct coupling between moiré trapped holes, and thus magnetic order can arise even in the dilute hole regime under optical excitation. This discovery adds a new and dynamic tuning knob to the rich many-body Hamiltonian of moiré quantum matter.

cond-mat.mes-hall↗

arXiv2022

Parity-mixed coupled-cluster formalism for computing parity-violating amplitudes

We formulate a parity-mixed coupled-cluster (PM-CC) approach for high-precision calculations of parity non-conserving amplitudes in mono-valent atoms. Compared to the conventional formalism which uses parity-proper (PP) one-electron orbitals, the PM-CC method is built using parity-mixed (PM) orbitals. The PM orbitals are obtained by solving the Dirac-Hartree-Fock equation with the electron-nucleus electroweak interaction included (PM-DHF). There are several advantages to such a PM-CC formulation: (i) reduced role of correlations, as for the most experimentally-accurate to date ${}^{133}{\rm Cs}\,$ $6S_{1/2}-7S_{1/2}$ transition, the PM-DHF result is only 3% away from the accurate many-body value, while the conventional DHF result is off by 18%; (ii) avoidance of directly summing over intermediate states in expressions for parity non-conserving amplitudes which reduces theoretical uncertainties associated with highly-excited and core-excited intermediate states, and (iii) relatively straightforward upgrade of existing and well-tested large-scale PP-CC codes. We reformulate the CC method in terms of the PM-DHF basis and demonstrate that the cluster amplitudes are complex numbers with opposite parity real and imaginary parts. We then use this fact to map out a strategy through which the new PM-CC scheme may be implemented.

physics.atom-ph↗

arXiv2021

Visualizing Atomically-Layered Magnetism in CrSBr

Two-dimensional (2D) materials can host stable, long-range magnetic phases in the presence of underlying magnetic anisotropy. The ability to realize the full potential of 2D magnets necessitates systematic investigation of the role of individual atomic layers and nanoscale inhomogeneity ($\textit{i.e.}$, strain) on the emergence and stability of both intra- and interlayer magnetic phases. Here, we report multifaceted spatial-dependent magnetism in few-layer CrSBr using magnetic force microscopy (MFM) and Monte Carlo-based magnetic simulations. We perform nanoscale visualization of the magnetic sheet susceptibility from raw MFM data and force-distance curves, revealing a characteristic onset of both intra- and interlayer magnetic correlations as a function of temperature and layer-thickness. We demonstrate that the presence of a single uncompensated layer in odd-layer terraces significantly reduces the stability of the low-temperature antiferromagnetic (AFM) phase and gives rise to multiple coexisting magnetic ground states at temperatures close to the bulk Néel temperature ($\textit{T}$$_N$). Furthermore, the AFM phase can be reliably suppressed using modest fields (~300 Oe) from the MFM probe, behaving as a nanoscale magnetic switch. Our prototypical study of few-layer CrSBr demonstrates the critical role of layer parity on field-tunable 2D magnetism and provides vital design criteria for future nanoscale magnetic devices. Moreover, we provide a roadmap for using MFM for nano-magnetometry of 2D materials, despite the ubiquitous absence of bulk zero-field magnetism in magnetized sheets.

cond-mat.mtrl-sci↗

arXiv2021

New Insights into the Criteria of Fast Radio Burst in the Light of FRB 20121102A

The total event number of fast radio bursts (FRBs) is accumulating rapidly with the improvement of existing radio telescopes and the completion of new facilities. Especially, the Five-hundred-meter Aperture Spherical radio Telescope (FAST) Collaboration has just reported more than one thousand bursts in a short observing period of 47 days \citep{LiD2021}. The interesting bimodal distribution in their work motivates us to revisit the definition of FRBs. In this work, we ascribe the bimodal distribution to two physical kinds of radio bursts, which may have different radiation mechanisms. We propose to use brightness temperature to separate two subtypes. For FRB 20121102A, the critical brightness temperature is $T_{\rm B,cri}\simeq10^{33}\,\rm K$. Bursts with $T_{\rm B}\geq T_{\rm B,cri}$ are denoted as "classical" FRBs, and further we find a tight pulse width-fluence relation ($T\propto\mathcal{F_ν}^{0.306}$) for them. On the contrary, the other bursts are considered as "atypical" bursts that may originate from a different physical process. We suggest that for each FRB event, a similar dividing line should exist but $T_{\rm B,cri}$ is not necessarily the same. Its exact value depends on FRB radiation mechanism and properties of the source.

astro-ph.HE↗

arXiv2021

Spin Waves and Dirac Magnons in a Honeycomb Lattice Zig-zag Antiferromagnet BaNi2(AsO4)2

The topological properties of massive and massless fermionic quasiparticles have been intensively investigated over the past decade in topological materials without magnetism. Recently, the bosonic analogs of such quasiparticles arising from spin waves have been reported in the two-dimensional (2D) honeycomb lattice ferromagnet/antiferromagnet and the 3D antiferromagnet. Here we use time-of-flight inelastic neutron scattering to study spin waves of the S = 1 honeycomb lattice antiferromagnet BaNi2(AsO4)2, which has a zig-zag antiferromagnetic (AF) ground state identical to that of the Kitaev quantum spin liquid candidate alpha-RuCl3. We determine the magnetic exchange interactions in the zig-zag AF ordered phase, and show that spin waves in BaNi2(AsO4)2 have symmetry-protected Dirac points inside the Brillouin zone boundary. These results provide a microscopic understanding of the zig-zag AF order and associated Dirac magnons in honeycomb lattice magnets, and are also important for establishing the magnetic interactions in Kitaev quantum spin liquid candidates.

cond-mat.str-el↗

arXiv2021

Chiral Phonons in Moiré Superlattices

We discover chiral phonons at the lowest-energy bands in moiré superlattices. The moiré chiral phonons we uncover are the collective excitations of the stacking domains. Their origin is uniquely attributed to the stacking configurations whose interlayer binding energy breaks the $C_{2z}$ symmetry on the moiré length scale. Within elastic theory, we use a general symmetry analysis to provide a complete classification of van der Waals heterostructures in respect to hosting moiré chiral phonons and show the calculation for twisted MoS$_2$ as an example. We present a low-energy effective model to qualitatively understand the moiré chiral phonons and show that it captures the essential physics remarkably well. Our result potentially opens up new possibilities in phononic twistronics as the moiré chiral phonons have high tunability, moiré scale wavelengths, excitation energies in only a few meV, and can possibly be mechanically excited.

cond-mat.mes-hall↗

arXiv2021

Axial Higgs Mode Detected by Quantum Pathway Interference in RTe3

The observation of the Higgs boson solidified the standard model of particle physics. However, explanations of anomalies (e.g. dark matter) rely on further symmetry breaking calling for an undiscovered axial Higgs mode. In condensed matter the Higgs was seen in magnetic, superconducting and charge density wave(CDW) systems. Uncovering a low energy mode's vector properties is challenging, requiring going beyond typical spectroscopic or scattering techniques. Here, we discover an axial Higgs mode in the CDW system RTe3 using the interference of quantum pathways. In RTe3 (R=La,Gd), the electronic ordering couples bands of equal or different angular momenta. As such, the Raman scattering tensor associated to the Higgs mode contains both symmetric and antisymmetric components, which can be excited via two distinct, but degenerate pathways. This leads to constructive or destructive interference of these pathways, depending on the choice of the incident and Raman scattered light polarization. The qualitative behavior of the Raman spectra is well-captured by an appropriate tight-binding model including an axial Higgs mode. The elucidation of the antisymmetric component provides direct evidence that the Higgs mode contains an axial vector representation (i.e. a pseudo-angular momentum) and hints the CDW in RTe3 is unconventional. Thus we provide a means for measuring collective modes quantum properties without resorting to extreme experimental conditions.

physics.optics↗