arXiv subjects

Di Zheng

Publications and source records attributed to Di Zheng.

7 recordsLinked to original sources

arXiv2025

Extreme polaritonic interactions in a room-temperature deterministic sub-nanocavity quantum electrodynamic platform

Pushing nanoscale optical confinement to its ultimate limits defines the regime of nano-cavity quantum electrodynamics (nano-cQED), where light--matter interactions approach the fundamental quantum limits of individual atoms, e.g., picocavities. However, realizing such extreme confinement in a stable and controllable manner remains a key challenge. Here, we introduce a van der Waals material-based nano-cQED platform by coupling monolayer MoS2 excitons to plasmonic sub-nanocavities formed via assembly of ultrasmall gold clusters (3-5 nm) in the nanogap of a nanoparticle-on-mirror nanocavity. These clusters emulate the field-confining role of atomic protrusions of the picocavities through a resonance-insensitive lightning-rod effect, achieving deep-subwavelength mode volumes. In this nano-cQED testbed, we observe pronounced multi-branch Rabi splittings and ultrastrong lower-branch polaritonic photoluminescence with up to 10^4-fold enhancement. This deterministic architecture provides a controllable pathway to access picocavity-like behavior and opens new opportunities for single-molecule spectroscopy and the exploration of nano-cQED.

physics.optics↗

arXiv2025

Novel multifunctional plasmonic fiber probe: Enabling plasmonic heating and SERS sensing for biomedical applications

Optical fiber-based platforms are increasingly explored as compact, minimally invasive tools for integrated photonic functionalities in biomedical applications. Among these, the combination of plasmonic heating and optical sensing on a single fiber tip offers compelling opportunities for localized photothermal actuation and in situ molecular detection. In this work, we present a multifunctional plasmonic fiber probe (PFP) that enables spectral multiplexing of thermo-plasmonic heating and surface-enhanced Raman spectroscopy (SERS). This dual capability is achieved by integrating gold nanoislands (AuNIs) onto the flat facet of a multimode optical fiber using a solid-state dewetting process - a straightforward and scalable fabrication method that avoids the complexity of lithographic techniques. We characterize how the morphology of the AuNIs modulates optical extinction, photothermal response, and electromagnetic field enhancement across the visible and near-infrared spectrum. Specifically, we demonstrate efficient, wavelength-dependent heating under visible light and strong SERS signal enhancement under near-infrared excitation, both supported by electromagnetic and thermal simulations. The ability to decouple photothermal stimulation and Raman sensing in a single, fiber-integrated device addresses a current gap in lab-on-fiber technologies, where multifunctional operation is often constrained to a single wavelength.

physics.med-ph↗

arXiv2025

Direct Nucleation of Hierarchical Nanostructures on Plasmonic Fiber Optics Enables Enhanced SERS Performance

We present an innovative fabrication method to achieve bottom-up in situ surface-overstructured Au nanoislands (NIs) with tunable grades of surface coverage, elongation, and branching, directly on micro-optical fibers for sensing applications. These all-in-gold hierarchical nanostructures consist of NIs coated with surface protrusions of various morphologies. They are created in solution using a selective seeded growth approach, whereby additional gold growth is achieved over Au NIs formerly developed on the fiber facet by a solid-state dewetting approach. The morphology of nanosized surface-NI overstructuring can be adjusted from multi-dot-decorated Au NIs to multi-arm-decorated Au NIs. This engineering of optical fibers allows for improved remote surface-enhanced Raman spectroscopy (SERS) molecular detection. By combining solid-state dewetting and wet-chemical approaches, we achieve stable in-contact deposition of surface-overstructured NIs with the optical fiber solid substrate, alongside precise control over branching morphology and anisotropy extent. The fiber optic probes engineered by surface-overstructured NIs exhibit outstanding sensing performance in an instant and through-fiber detection scheme, achieving a remarkable detection limit at 10-7 M for the R6G aqueous solution. These engineered probes demonstrate an improved detection limit by one order of magnitude and enhanced peak prominence compared to devices solely decorated with pristine NIs.

physics.optics↗

arXiv2024

Tunable Nanoislands Decorated Tapered Optical Fibers Reveal Concurrent Contributions in Through-Fiber SERS Detection

Creating plasmonic nanoparticles on a tapered optical fiber tip enables a remote SERS sensing probe, ideal for challenging sampling scenarios like biological tissue, specific cells, on-site environmental monitoring, and deep brain structures. However, nanoparticle patterns fabricated from current bottom-up methods are mostly random, making geometry control difficult. Uneven statistical distribution, clustering, and multilayer deposition introduce uncertainty in correlating device performance with morphology. Here, we employ a tunable solid-state dewetting method to create densely packed monolayer Au nanoislands (NIs) with varied geometric parameters, directly contacting the silica TF surface. These patterns exhibit analyzable nanoparticle sizes, densities, and uniform distribution across the entire taper surface, enabling a systematic investigation of particle size, density, and analyte effects on the SERS performance of the through-fiber detection system. The study is focused on the SERS response of a widely employed benchmark Rhodamine 6G molecule and Serotonin, a neurotransmitter with high relevance for the neuroscience field. The numerical simulations and limit of detection (LOD) experiments on R6G show that the increase of the total near-field enhancement volume promotes the SERS sensitivity of the probe. However, for serotonin we observed a different behavior linked to its interaction with the nanoparticle's surface. The obtained LOD is as low as 10-7 M, a value not achieved so far in a through-fiber detection scheme. Therefore, we believe our work offers a strategy to design nanoparticle-based remote SERS sensing probes and provide new clues to discover and understand the intricate plasmonic-driven chemical reactions.

physics.optics↗

arXiv2023

Robust Adaptive Control of STATCOMs to Mitigate Inverter-Based-Resource (IBR)-Induced Oscillations

The interaction among inverter-based resources (IBRs) and power network may cause small-signal stability issues, especially in low short-circuit-level grids. Besides, integrating static synchronous compensators (STATCOMs) in a multi-IBR system for voltage support can deteriorate small-signal stability. However, it is still challenging to fully understand the impact mechanism of STATCOMs on IBR-induced oscillation issues and to design optimal STATCOMs' control for dampening these oscillation issues in a multi-IBR system due to complex system dynamics and varying operating conditions. To tackle these challenges, this paper proposes a novel method to reveal how STATCOMs influence IBR-induced oscillation issues in a multi-IBR system from the viewpoint of grid strength, which can consider varying operating conditions. Based on this proposed method, critical operating conditions are identified, wherein the system tends to be most unstable. Moreover, we demonstrate that robust small-signal stability issues of the multi-IBR system with STATCOMs can be simplified as that of multiple subsystems under critical operating conditions, which avoids exhaustive studies on many operating conditions with detailed system models. On this basis, an adaptive control-parameter design method is proposed for STATCOMs to ensure system robust stability under varying operating conditions. The proposed methods are validated by a modified IEEE39-node test system.

eess.SY↗

arXiv2020

Mechanical dissipation below 1$μ$Hz with a cryogenic diamagnetic-levitated micro-oscillator

Ultralow dissipation plays an important role in sensing applications and exploring macroscopic quantum phenomena using micro-and nano-mechanical systems. We report a diamagnetic-levitated micro-mechanical oscillator operating at a low temperature of 3K with measured dissipation as low as 0.59 $μ$Hz and a quality factor as high as $2 \times 10^7$. To the best of our knowledge the achieved dissipation is the lowest in micro- and nano-mechanical systems to date, orders of magnitude improvement over the reported state-of-the-art systems based on different principles. The cryogenic diamagnetic-levitated oscillator described here is applicable to a wide range of mass, making it a good candidate for measuring both force and acceleration with ultra-high sensitivity. By virtue of the naturally existing strong magnetic gradient, this system has great potential in quantum spin mechanics study.

quant-ph↗

arXiv2019

Room temperature test of the Continuous Spontaneous Localization model using a levitated micro-oscillator

The Continuous Spontaneous Localization (CSL) model predicts a tiny break of energy conservation via a weak stochastic force acting on physical systems, which triggers the collapse of the wave function. Mechanical oscillators are a natural way to test such a force; in particular levitated micro-mechanical oscillator has been recently proposed to be an ideal system. We report a proof-of-principle experiment with a micro-oscillator generated by a micro-sphere diamagnetically levitated in a magneto-gravitational trap under high vacuum. Due to the ultra-low mechanical dissipation, the oscillator provides a new upper bound on the CSL collapse rate, which gives an improvement of two orders of magnitude over the previous bounds in the same frequency range, and partially reaches the enhanced collapse rate suggested by Adler. Although being performed at room temperature, our experiment has already exhibits advantages over those operating at low temperatures previously reported. Our results experimentally show the potential of magneto-gravitational levitated mechanical oscillator as a promising method for testing collapse model. Further improvements in cryogenic experiments are discussed.

quant-ph↗