arXiv subjects

Diane J. Roth

Publications and source records attributed to Diane J. Roth.

8 recordsLinked to original sources

arXiv2025

Strong coupling of collective optical resonances in dielectric metasurfaces

Dielectric metasurfaces can achieve strong light-matter interaction based on several types of collective (nonlocal) resonances, such as surface lattice resonances (SLRs) and quasi bound states in the continuum (quasi-BICs). Spectral selectivity, field enhancement, and high and controllable Q-factors make these resonances appealing for technological applications in lasing, sensing, nonlinear optics, and quantum photon sources. An emerging challenge focuses on tailoring light-matter interaction via mode coupling and hybridization between the fundamental resonances of a metasurface. While strong coupling phenomena have been demonstrated between various resonant modes, the interplay between collective resonances of different natures has not been observed to date. Here, we theoretically, numerically, and experimentally demonstrate the onset of coupling and hybridization between symmetry-protected quasi-BICs and SLRs in a dielectric metasurface. We show the emergence of anticrossing (or Rabi splitting) in the strong coupling regime with suppression of reflection, observed under TE-polarised excitation, and the manifestation of an accidental BIC under TM-polarised illumination as a result of energy exchange between the participating collective resonances in the weak coupling regime. The first effect is accompanied by hybridized near fields of the modes. The observed coupling mechanisms can be controlled by modifying the angle of incidence, polarisation, and surrounding environment. This foundational study on the coupling and hybridization of collective resonances offers insights that can be leveraged for the design of metasurfaces with targeted quasi-aBIC and collective hybridized resonances. It could also open new possibilities to control the near fields associated with such resonances, with promising applications in tunable nanophotonics and light manipulation.

physics.optics↗

arXiv2025

Plasmonic Brownian Ratchets for Directed Transport of Analytes

Controlled long-range transport of micro- and nano-scale objects is a key requirement in lab-on-a-chip and microfluidic applications, enabling the efficient capture, concentration, manipulation, and detection of analytes. Traditional methods such as microfluidic pumps and optical trapping face challenges including high power consumption and limited range of action. This study introduces a plasmonic Brownian ratchet designed for the directed transport of dielectric nanometer-sized particles at low optical powers. Through numerical simulations, the ratchet geometry was optimized to enhance electric fields, optical forces, and trapping potentials. Experimentally, the plasmonic ratchet demonstrated the ability to rectify random thermal motion of 40 nm polysterene spheres over extended distances in a specific direction, achieving velocities up to 2.4 $μ$m/s at excitation powers as low as 0.785 kW/cm^2. This plasmonic ratchet offers a robust and efficient solution for the targeted delivery and concentration of nanoscale analytes on chips, with significant implications for advancing applications in the life sciences.

cond-mat.mes-hall↗

arXiv2024

The 2024 Active Metamaterials Roadmap

Active metamaterials are engineered structures that possess novel properties that can be changed after the point of manufacture. Their novel properties arise predominantly from their physical structure, as opposed to their chemical composition and can be changed through means such as direct energy addition into wave paths, or physically changing/morphing the structure in response to both a user or environmental input. Active metamaterials are currently of wide interest to the physics community and encompass a range of sub-domains in applied physics (e.g. photonic, microwave, acoustic, mechanical, etc.). They possess the potential to provide solutions that are more suitable to specific applications, or which allow novel properties to be produced which cannot be achieved with passive metamaterials, such as time-varying or gain enhancement effects. They have the potential to help solve some of the important current and future problems faced by the advancement of modern society, such as achieving net-zero, sustainability, healthcare and equality goals. Despite their huge potential, the added complexity of their design and operation, compared to passive metamaterials creates challenges to the advancement of the field, particularly beyond theoretical and lab-based experiments. This roadmap brings together experts in all types of active metamaterials and across a wide range of areas of applied physics. The objective is to provide an overview of the current state of the art and the associated current/future challenges, with the hope that the required advances identified create a roadmap for the future advancement and application of this field.

physics.app-ph↗

arXiv2024

Longitudinal field controls vector vortex beams in anisotropic epsilon-near-zero metamaterials

Structured light plays an important role in metrology, optical trapping and manipulation, communications, quantum technologies, nonlinear optics and provides a rich playground for addressing new optical phenomena. Here we demonstrate a novel approach for manipulating vector vortex beams carrying longitudinal field components using metamaterials with extreme anisotropy. Implementing vectorial spectroscopy, we show that the propagation of complex beams with inhomogeneous polarisation is strongly affected by the interplay of the metamaterial anisotropy with the transverse and longitudinal field structure of the beam. This phenomenon is especially pronounced in the epsilon-near-zero regime, exclusively realised for light polarised along the metamaterial optical axis, strongly influencing the interaction of longitudinal fields with the metamaterial. The requirements on the balance between the transverse and longitudinal fields to maintain a polarisation singularity at the beam axis allow control of the beam modal content, filtering diffraction effects and tailoring spatial polarisation distribution. The proposed approach offers important capabilities for wavefront shaping as well as local spatial polarisation engineering. The understanding of the interaction of vector beams with metamaterials opens new opportunities for applications in microscopy, information encoding, biochemical sensing and quantum technologies.

physics.optics↗

arXiv2024

Unidirectional chiral scattering from single enantiomeric plasmonic nanoparticles

Controlling scattering and routing of chiral light at the nanoscale is important for optical information processing and imaging, quantum technologies as well as optical manipulation. Here, we introduce a concept of rotating chiral dipoles in order to achieve unidirectional chiral scattering. Implementing this concept by engineering multipole excitations in plasmonic helicoidal nanoparticles, we experimentally demonstrate enantio-sensitive and highly-directional forward scattering of circularly polarised light. The intensity of this highly-directional scattering is defined by the mutual relation between the handedness of the incident light and the chirality of the structure. The concept of rotating chiral dipoles opens up numerous possibilities for engineering of scattering from chiral nanostructures and optical nano-antennas for the design and application of chiral light-matter interaction.

physics.optics↗

arXiv2023

Dynamic dielectric metasurfaces via control of surface lattice resonances in non-homogeneous environment

Dynamic control of metamaterials and metasurfaces is crucial for many photonic technologies, such as flat lenses, displays, augmented reality devices, and beam steering, to name a few. The dynamic response is typically achieved by controlling the phase and/or amplitude of individual meta-atom resonances using electro-optic, phase-change or nonlinear effects. Here, we propose and demonstrate a new practical strategy for the dynamic control of the resonant interaction of light with dielectric metasurfaces, exploiting the dependence of the interaction between meta-atoms in the array on the inhomogeneity of the surrounding medium. The revealed tuning mechanisms are based on the concept of the surface lattice resonance (SLR), the development of which strongly depends on the difference between permittivities of superstrate and substrate materials. We experimentally demonstrate surface lattice resonances in dielectric (Si) metasurfaces, and reveal two tuning mechanisms corresponding to shifting or damping of the SLR in optofluidic environment. The demonstrated dynamic tuning effect with the observed vivid colour changes may provide a dynamic metasurface approach with high spectral selectivity and enhanced sensitivity for sensors, as well as high-resolution for small pixel size displays.

physics.optics↗

arXiv2020

Machine learning -- based diffractive imaging with subwavelength resolution

Far-field characterization of small objects is severely constrained by the diffraction limit. Existing tools achieving sub-diffraction resolution often utilize point-by-point image reconstruction via scanning or labelling. Here, we present a new imaging technique capable of fast and accurate characterization of two-dimensional structures with at least wavelength/25 resolution, based on a single far-field intensity measurement. Experimentally, we realized this technique resolving the smallest-available to us 180-nm-scale features with 532-nm laser light. A comprehensive analysis of machine learning algorithms was performed to gain insight into the learning process and to understand the flow of subwavelength information through the system. Image parameterization, suitable for diffractive configurations and highly tolerant to random noise was developed. The proposed technique can be applied to new characterization tools with high spatial resolution, fast data acquisition, and artificial intelligence, such as high-speed nanoscale metrology and quality control, and can be further developed to high-resolution spectroscopy

physics.optics↗

arXiv2018

Efficient energy propagation through self-assembled gold nanoparticle chain waveguides

The strong interaction of light with metallic nanoparticles enables field confinement well below the diffraction limit. Plasmonic waveguides consisting of metal nanoparticle chains could be used for the propagation of energy or information on the nanoscale, but high losses have thus far impeded practical applications. Here we demonstrate that efficient waveguiding is possible through gold nanoparticle chains despite the high dissipative losses of gold. A DNA origami directed self-assembly of monocrystalline, spherical nanoparticles allows the interparticle spacing to be decreased to 2 nm or below, which gives rise to lower-energy plasmon resonance modes. Our simulations imply that these lower energy modes allow efficient waveguiding but collapse if interparticle gap sizes are increased. Individual waveguides are characterized with nanometer-resolution by electron energy loss spectroscopy, and directed propagation of energy towards a fluorescent nanodiamond and nanoscale energy conversion is shown by cathodoluminescence imaging spectroscopy on a single-device level. With this approach, micrometer-long propagation lengths might be achieved, enabling applications in information technology, sensing and quantum optics.

physics.optics↗