arXiv subjects

Diederik S. Wiersma

Publications and source records attributed to Diederik S. Wiersma.

At least 19 recordsLinked to original sources

arXiv2024

Experimental determination of effective light transport properties in fully anisotropic media

Structurally anisotropic materials are ubiquitous in several application fields, yet their accurate optical characterization remains challenging due to the lack of general models linking their scattering coefficients to the macroscopic transport observables, and the need to combine multiple measurements to retrieve their direction-dependent values. Here, we present an improved method for the experimental determination of light transport tensor coefficients from the diffusive rates measured along all three directions, based on transient transmittance measurements and a generalized Monte Carlo model. We apply our method to the characterization of light transport properties in two common anisotropic materials - polytetrafluoroethylene (PTFE) tape and paper - highlighting the magnitude of systematic deviations that are typically incurred when neglecting anisotropy.

physics.optics↗

arXiv2024

Diffusion of light in structurally anisotropic media with uniaxial symmetry

Anisotropic light transport is extremely common among scattering materials, yet a comprehensive picture of how macroscopic diffusion is determined by microscopic tensor scattering coefficients is not fully established yet. In this work, we present a theoretical and experimental study of diffusion in structurally anisotropic media with uniaxially symmetric scattering coefficients. Exact analytical relations are derived in the case of index-matched turbid media, unveiling the general relation between microscopic scattering coefficients and the resulting macroscopic diffusion tensor along different directions. Excellent agreement is found against anisotropic Monte Carlo simulations up to high degrees of anisotropy, in contrast with previously proposed approaches. The obtained solutions are used to analyze experimental measurements of anisotropic light transport in polystyrene foam samples under different degrees of uniaxial compression, providing a practical example of their applicability.

physics.optics↗

arXiv2023

Breakdown of self-similarity in light transport

Transport processes underpin a multitude of phenomena, ranging from the propagation of atoms on lattices, to the mobility patterns of microorganisms and earthquakes, to name a few. The dynamics of these processes is very rich and key to understanding the complex nature of the underlying physics, but the way in which we classify them is often too simplistic to fully reflect this complexity. Here, we report on the experimental observation of a breakdown of self-similar propagation for light inside a scattering medium - a transport regime exhibiting different scaling rates for each spatial moment of the associated probability distribution. Notably, we show that this phenomenon arises for light waves even in the simple case of isotropic and homogeneous disorder, and can be controlled by tuning the turbidity of the system. These results support the idea that the traditional dichotomy between normal and anomalous diffusion is reductive and that a richer framework should be constructed based on the concept of self-similarity as this class of transport regimes may be far more common that it is currently believed. In addition, this insight can help understand scenarios where transport is dominated by rare propagation events, as in non-linear and active media, or more generally in other fields of research.

physics.optics↗

arXiv2023

Physical Realization of a Hyper Unclonable Function

Disordered photonic structures are promising materials for the realization of physical unclonable functions (PUF), physical objects that can overcome the limitations of conventional digital security methods and that enable cryptographic protocols immune against attacks by future quantum computers. One PUF limitation, so far, has been that their physical configuration is either fixed or can only be permanently modified, and hence allowing only one token per device. We show that it is possible to overcome this limitation by creating a reconfigurable structure made by light-transformable polymers, in which the physical structure of the unclonable function itself can be reversibly reconfigured. We term this novel concept Hyper PUF or HPUF in that it allows a large number of physical unclonable functions to co-exist simultaneously within one and the same device. The physical transformation of the structure is done all-optically in a reversible and spatially controlled fashion. Our novel technology provides a massive enhancement in security generating more complex keys containing a larger amount of information. At the same time, it allows for new applications, for example serving multiple clients on a single encryption device and the practical implementation of quantum secure authentication of data.

cond-mat.mes-hall↗

arXiv2020

Spatial coherence of light inside three dimensional media

Speckle is maybe the most fundamental interference effect of light in disordered media, giving rise to fascinating physical phenomena and enabling applications in imaging, spectroscopy or cryptography, to name a few. While speckle formed outside a sample is easily measured and analysed, true bulk speckle, as formed inside random media, is difficult to investigate directly due to the obvious issue of physical access. Furthermore, its proper theoretical description poses enormous challenges. Here we report on the first direct measurements of intensity correlations of light inside a disordered medium, using embedded DNA strings decorated with emitters separated by a controlled nanometric distance. Our method provides in situ access to fundamental properties of bulk speckles as their size and polarization degrees of freedom, both of which are found to deviate significantly from theoretical predictions. The deviations are explained, by comparison with rigorous numerical calculations, in terms of correlations among polarization components and non-universal near-field contributions at the nanoscale.

physics.optics↗

arXiv2020

Optimized White Reflectance in Photonic Network Structures

Three-dimensional disordered networks are receiving increasing attention as versatile architectures for highly scattering materials. However, due to their complex morphology, little is still known about the interplay between their structural and optical properties. Here, we describe a simple algorithm that allows to generate photonic network structures inspired by that of the Cyphochilus beetle, famous for the bright white reflectance of its thin cuticular scales. The model allows to vary the degree of structural anisotropy and filling fraction of the network independently, revealing the key contribution of these two parameters to the overall scattering efficiency. Rigorous numerical simulations show that the obtained structures can exceed the broadband reflectance of the beetle while using less material, providing new insights for the design of advanced scattering materials.

physics.optics↗

arXiv2020

Generalized bioinspired approach to a daytime radiative cooling "skin"

Energy-saving cooling materials with strong operability are desirable towards sustainable thermal management. Inspired by the cooperative thermo-optical effect in fur of polar bear, we develop a flexible and reusable cooling skin via laminating a polydimethylsiloxane film with a highly-scattering polyethylene aerogel. Owing to its high porosity of 97.9% and tailored pore size of 3.8 +- 1.4 micrometers, superior solar reflectance of 0.96 and high transparency to irradiated thermal energy of 0.8 can be achieved at a thickness of 2.7 mm. Combined with low thermal conductivity of 0.032 W/m/K of the aerogel, the cooling skin exerts midday sub-ambient temperature drops of 5-6 degrees in a metropolitan environment, with an estimated limit of 14 degrees under ideal service conditions. We envision that this generalized bilayer approach will construct a bridge from night-time to daytime radiative cooling and pave the way for economical, scalable, flexible and reusable cooling materials.

physics.app-ph↗

arXiv2020

Diagnostics and characterization of photonic circuits by wide-field spatio-temporal imaging

The growing diffusion of integrated photonic technologies requires fast and non-invasive quality control techniques for mass-production. We present a general diagnostic technique for sub-ps imaging of photonic circuits combining wide-field optical microscopy and optical gating. The simultaneous access to multiple parameters of a photonic structure enables an unprecedented characterization of its functional design as opposed to typical single-domain techniques such as frequency or time domain reflectometry and near-field microscopy. The non-contact and non-perturbative nature of the technique makes it relevant for both planar and three-dimensional circuits, as well as for silicon, polymeric or hybrid platforms. We apply our technique to different photonic chip components fabricated by Direct Laser Writing, revealing the spatial and temporal hallmarks of fabrication imperfections causing losses or deviations from the intended device behavior. At the same time, the technique allows in situ probing of key properties of photonic devices as the local propagation constants of guided modes or the quality factor of resonant elements. Our method is relevant for both the scientific and the industrial communities as it lends itself to be scaled up to in-line quality control thanks to its non-scanning nature.

physics.optics↗

arXiv2019

Biomimetic Polymer Film with Brilliant Brightness Using a One-Step Water Vapor-Induced Phase Separation Method

The scales of the white Cyphochilus beetles are endowed with unusual whiteness arising from the exceptional scattering efficiency of their disordered ultrastructure optimized through millions of years of evolution. Here, a simple, one-step method based on water vapor-induced phase separation (VIPS) is developed to prepare ultra-thin polystyrene (PS) films with similar microstructure and comparable optical performance. A typical biomimetic 3.5 um PS film exhibits a diffuse reflectance of 61% at 500 nm, which translates into a transport mean free path below 1 um. A complete optical characterization through Monte Carlo simulations reveals how such scattering performance arises from the scattering coefficient and scattering anisotropy, whose interplay provides insight into the morphological properties of the material. The potential of bright-white coatings as smart sensors or wearable devices is highlighted using a treated ultra-thin film as a real-time sensor for human exhalation.

physics.app-ph↗

arXiv2019

Multichannel remote polarization control enabled by nanostructured Liquid Crystalline Networks

In this article we demonstrate that a grating fabricated through nanoscale volumetric crosslinking of a liquid crystalline polymer enables remote polarization control over the diffracted channels. This functionality is a consequence of the responsivity of liquid crystal networks upon light stimuli. Tuning the photonic response of the device is obtained thanks to both a refractive index and a shape change of the grating elements induced by a molecular rearrangement under irradiation. In particular, the material anisotropy allows for nontrivial polarization state management over multiple beams. Absence of any liquid component and a time response down to 0.2 milliseconds make our device appealing in the fields of polarimetry and optical communications.

physics.optics↗

arXiv2018

Structured Optical Materials Controlled by Light

Materials of which the optical response is determined by their structure are of much interest both for their fundamental properties and applications. Examples range from simple gratings to photonic crystals. Obtaining control over the optical properties is of crucial importance in this context, and it is often attempted by electro-optical effect or by using magnetic fields. In this paper, we introduce the use of light to switch and tune the optical response of a structured material, exploiting a physical deformation induced by light itself. In this new strategy, light drives an elastic reshaping, which leads to different spectral properties and hence to a change in the optical response. This is made possible by the use of liquid crystalline networks structured by Direct Laser Writing. As a proof of concept, a grating structure with sub-millisecond time-response is demonstrated for optical beam steering exploiting an optically induced reversible shape-change. Experimental observations are combined with finite-element modeling to understand the actuation process dynamics and to obtain information on how to tune the time and the power response of this technology. This optical beam steerer serves as an example for achieving full optical control of light in broad range of structured optical materials.

physics.optics↗

arXiv2017

CELES: CUDA-accelerated simulation of electromagnetic scattering by large ensembles of spheres

CELES is a freely available MATLAB toolbox to simulate light scattering by many spherical particles. Aiming at high computational performance, CELES leverages block-diagonal preconditioning, a lookup-table approach to evaluate costly functions and massively parallel execution on NVIDIA graphics processing units using the CUDA computing platform. The combination of these techniques allows to efficiently address large electrodynamic problems ($>10^4$ scatterers) on inexpensive consumer hardware. In this paper, we validate near- and far-field distributions against the well-established multi-sphere $T$-matrix (MSTM) code and discuss the convergence behavior for ensembles of different sizes, including an exemplary system comprising $10^5$ particles.

physics.comp-ph↗

arXiv2016

Spatio-temporal visualization of light transport in complex photonic structures

Spatio-temporal imaging of light propagation is very important in photonics because it provides the most direct tool available to study the interaction between light and its host environment. Sub-ps time resolution is needed to investigate the fine and complex structural features that characterize disordered and heterogeneous structures, which are responsible for a rich array of transport physics that have not yet been fully explored. A newly developed wide-field imaging system enables us to present a spatio-temporal study on light transport in various disordered media, revealing properties that could not be properly assessed using standard techniques. By extending our investigation to an almost transparent membrane, a configuration that has been difficult to characterize until now, we unveil the peculiar physics exhibited by such thin scattering systems with transport features that go beyond mainstream diffusion modeling, despite the occurrence of multiple scattering.

physics.optics↗

arXiv2015

Path length enhancement in disordered media for increased absorption

We theoretically and numerically investigate the capability of disordered media to enhance the optical path length in dielectric slabs and augment their light absorption efficiency due to scattering. We first perform a series of Monte Carlo simulations of random walks to determine the path length distribution in weakly to strongly (single to multiple) scattering, non-absorbing dielectric slabs under normally incident light and derive analytical expressions for the path length enhancement in these two limits. Quite interestingly, while multiple scattering is expected to produce long optical paths, we find that media containing a vanishingly small amount of scatterers can still provide high path length enhancements due to the very long trajectories sustained by total internal reflection at the slab interfaces. The path length distributions are then used to calculate the light absorption efficiency of media with varying absorption coefficients. We find that maximum absorption enhancement is obtained at an optimal scattering strength, in-between the single-scattering and the diffusive (strong multiple-scattering) regimes. This study can guide experimentalists towards more efficient and potentially low-cost solutions in photovoltaic technologies.

physics.optics↗

arXiv2014

Localization in one-dimensional chains with Lévy-type disorder

We study Anderson localization of the classical lattice waves in a chain with mass impurities distributed randomly through a power-law relation $s^{-(1+α)}$ with $ s $ as the distance between two successive impurities and $α>0$. This model of disorder is long-range correlated and is inspired by the peculiar structure of the complex optical systems known as Lévy glasses. Using theoretical arguments and numerics, we show that in the regime in which the average distance between impurities is finite with infinite variance, the small-frequency behaviour of the localization length is $ ξ_α(ω) \sim ω^{-α} $. The physical interpretation of this result is that, for small frequencies and long wavelengths, the waves feel an effective disorder whose fluctuations are scale-dependent. Numerical simulations show that an initially localized wavepacket attains, at large times, a characteristic inverse power-law front with an $ α$-dependent exponent which can be estimated analytically.

cond-mat.stat-mech↗

arXiv2014

Walk dimension for light in complex disordered media

Transport in complex systems is characterized by a fractal dimension -- the walk dimension -- that indicates the diffusive or anomalous nature of the underlying random walk process. Here we report on the experimental retrieval of this key quantity, using light waves propagating in disordered media. The approach is based on measurements of the time-resolved transmission, in particular on how the lifetime scales with sample size. We show that this allows one to retrieve the walk dimension and apply the concept to samples with varying degree of fractal heterogeneity. In addition, the method provides the first experimental demonstration of anomalous light dynamics in a random medium.

physics.optics↗

arXiv2014

Light transport and localization in two-dimensional correlated disorder

Structural correlations in disordered media are known to affect significantly the propagation of waves. In this article, we theoretically investigate the transport and localization of light in 2D photonic structures with short-range correlated disorder. The problem is tackled semi-analytically using the Baus-Colot model for the structure factor of correlated media and a modified independent scattering approximation. We find that short-range correlations make it possible to easily tune the transport mean free path by more than a factor of 2 and the related localization length over several orders of magnitude. This trend is confirmed by numerical finite-difference time-domain calculations. This study therefore shows that disorder engineering can offer fine control over light transport and localization in planar geometries, which may open new opportunities in both fundamental and applied photonics research.

physics.optics↗

arXiv2013

Transport in quenched disorder: light diffusion in strongly heterogeneous turbid media

We present a theoretical and experimental study of light transport in disordered media with strongly heterogeneous distribution of scatterers formed via non-scattering regions. Step correlations induced by quenched disorder are found to prevent diffusivity from diverging with increasing heterogeneity scale, contrary to expectations from annealed models. Spectral diffusivity is measured for a porous ceramic where nanopores act as scatterers and macropores render their distribution heterogeneous. Results agree well with Monte Carlo simulations and a proposed analytical model.

cond-mat.dis-nn↗