arXiv subjects

Dieter Koelle

Publications and source records attributed to Dieter Koelle.

At least 19 recordsLinked to original sources

arXiv2026

Spatial resolution and point spread function of high-resolution scanning SQUID microscopy probes

Superconducting quantum interference devices (SQUIDs) show exceptional sensitivity to magnetic flux. In scanning SQUID microscopy (SSM), SQUID size and its distance to the sample are minimized in order to map weak magnetic fields with best possible spatial resolution. SQUID-on-lever (SOL) architectures have proven especially effective as SSM probes due to their small sensor size, robustness, and ease of integration with conventional atomic force microscopy hardware. In order to optimize magnetic microscopy carried out with SOL probes and to accurately reconstruct the magnetic fields that they measure, it is essential to know their point spread function (PSF). The size and shape of this PSF are determined by magnetic flux focusing effects, which depend on the characteristic length-scales of the superconductor and the sensor geometry. By simulating the coupling to sources of magnetic flux, this work provides a mathematical description of the SOL PSF, which contains a full description of the probe's magnetic sensitivity and spatial resolution. We then use measurements of a single magnetic skyrmion to measure the magnetic flux response of a real SOL. We demonstrate excellent agreement with flux responses that are obtained from simulations, thereby confirming the calculated PSF and spatial resolution.

cond-mat.supr-con↗

arXiv2026

Tailoring the properties of YBa$_{2}$Cu$_{3}$O$_{7-δ}$ thin films by 30 keV He$^+$ irradiation: An enabling route to superconducting device nanopatterning

Focused helium ion beam (He-FIB) irradiation with 30 keV ions is a key tool for nanoscale patterning and defect engineering in high transition temperature (Tc) cuprate superconducting devices, yet its usable fluence window is constrained by the competing requirements of reliable superconductivity suppression and minimal structural degradation. In this work, we provide a comprehensive dataset on the effects of large-area 30 keV He+ ion exposure on the electric transport and superconducting properties of epitaxial YBa2Cu3O7 (YBCO) thin films. X-ray diffraction shows a fluence-driven loss of crystalline order accompanied by an out-of-plane lattice expansion and an orthorhombic-to-tetragonal transition, culminating at predominant amorphization at the highest fluence of 1 x 10^16 cm^-2. Raman spectra exhibit increasing disorder while lacking signatures of oxygen depletion, indicating that irradiation mainly generates oxygen-related Frenkel defects rather than changing the carrier concentration. Consistently, with increasing fluence, the normal-state resistivity ρ_N(T) at temperature T above Tc increases strongly, while d ρ_N/d T remains nearly unchanged at moderate fluence. The suppression of Tc is accurately described by Abrikosov-Gor'kov pair breaking and reaches complete quenching of superconductivity at 4.5 x 10^15 cm^-2. The anisotropic upper critical fields decrease approximately exponentially with increasing fluence, the vortex activation energy is reduced, and the anisotropy drops, in contrast to oxygen-depleted YBCO. Hall-angle analysis confirms a nearly constant carrier density but a systematic increase in defect scattering and reduced mobility, consistent with a crossover toward the dirty limit at high fluence. These results establish quantitative fluence thresholds and a practical operational window for He-FIB nanopatterning of YBCO quantum circuits.

cond-mat.supr-con↗

arXiv2026

Structural Changes and Transport Properties of $\mathrm{YBa_2Cu_3O_7}$ Locally Modified by a He$^+$ Focused Ion Beam

Irradiation of a material with ions can cause various defects that can lead to structural phase transitions and the modification of the material's properties. Here we study the irradiation of the epitaxyally grown thin films of the high-temperature superconductor $\mathrm{YBa_2Cu_3O_7}$ with $30\,\mathrm{keV}$ He$^{+}$ ions which leads to the expansion of the crystal lattice, decrease of the critical temperature $T_c$ and eventually transition to an insulator. Fabrication of such insulating regions with a focused He-Ion beam with a spot size of $\sim 10\,\mathrm{nm}$ is a powerful technique for fabrication of superconducting nano-devices. Using low-temperature resistivity measurements, diffraction with a nanofocused X-ray beam and atomic force microscopy, we investigated how the structure and the electric transport properties of $\mathrm{YBa_2Cu_3O_7}$ depend on the irradiation dose in a range $10$--$100\,\mathrm{ions/nm^2}$ and on the lateral size of the irradiated area in a range $30$--$5000\,\mathrm{nm}$.

cond-mat.supr-con↗

arXiv2026

Dually tunable YBCO coplanar waveguide resonators based on helium-ion-generated Josephson inductances

Superconducting microwave circuits with and without Josephson inductances are the Swiss Army knife for many experiments and technologies from quantum information science to astrophysical particle detectors. Despite a large variety of existing circuit types, thin film materials and Josephson junction technologies, a flexible and reliable platform for high-magnetic-field and high-temperature applications is yet to be found. In this manuscript, we investigate coplanar waveguide cavities made of the high-temperature cuprate superconductor YBa$_2$Cu$_3$O$_7$ (YBCO), integrated with Josephson inductances and quantum interferometers that are generated by the controlled local irradiation of the YBCO with a focused helium ion beam. We obtain strongly flux-tunable microwave resonators, which not only display periodic interferometer oscillations of resonance frequency and decay rate, but also a superimposed Fraunhofer-like modulation pattern. The latter originates from the magnetic field tuning of the individual Josephson junction critical currents due to the out-of-plane junction barriers. It allows adjusting resonance frequency and flux responsivity independently of each other, potentially enabling tunable microwave circuits with low sensitivity to external magnetic-field noise over a broad range of frequencies. Finally, we investigate the temperature dependence of the cavities, show that they have promising characteristics up to 14$\,$K, and present a model for the junction-induced cavity losses.

quant-ph↗

arXiv2026

Electric-Field Control of Quantum Tunneling Regimes in Focused He-Ion-Beam-Irradiated Oxide Interfaces

Helium focused ion beam irradiation enables the fabrication of tunnel field-effect transistors based on two-dimensional electron systems (2DESs) at an oxide interface.High resolution scanning transmission electron microscopy and strain mapping reveal localized lattice deformation confined to the irradiated regions, which act as nanoscale potential barriers. The barrier profile can be continuously tuned by electrostatic backgating at low temperature without degrading the electronic properties of the 2DES electrodes. Transport measurements demonstrate controlled access to thermionic emission, direct tunneling, and Fowler-Nordheim tunneling within a single device architecture. These results establish He FIB irradiation as a powerful tool for nanoscale functional engineering of complex-oxide interfaces and provide a platform for exploring gate-tunable quantum tunneling phenomena.

cond-mat.mes-hall↗

arXiv2026

Magnetically induced Josephson nano-diodes in field-resilient superconducting microwave circuits

The development of nonlinear and frequency-tunable superconducting microwave circuits for operation in large magnetic fields is of high relevance for hybrid quantum systems such as spin resonance spectrometers, microwave quantum magnonics, dark matter axion detectors or flux-mediated optomechanics. With these exciting perspectives in mind, we investigate niobium-based circuits with integrated nano-constriction quantum interferometers in magnetic in-plane fields of up to several hundred mT. Our experiments reveal an unexpected and pronounced field-induced asymmetry in the bias-flux response of the circuits, which is demonstrated to originate from a field-induced Josephson-diode effect within the nano-constrictions and which enhances the circuit figures of merit in a magnetic field. An intuitive macroscopic Josephson-diode model attributes the effect to inhomogeneous constriction properties and provides us with the diode current-phase relation as a function of the in-plane field. Finally, we demonstrate that in the diode-state the circuit Kerr nonlinearity is bimodal in frequency, not only eliminating alternative explanations for the bias-flux-asymmetries but also being potentially useful for quantum circuit applications. Overall, our report underlines the potential of niobium nano-constriction circuits for high-field hybrid quantum systems, provides a conceptually simple explanation for the diode effect in superconducting nano-structures, and reveals the untapped potential of combining Josephson nano-diodes with microwave quantum circuits.

quant-ph↗

arXiv2026

Imaging short- and long-range magnetic order in a quantum anomalous Hall insulator

The quantum anomalous Hall effect has been observed in several magnetically doped topological insulators, where its robustness and macroscopic magnetization properties have been taken to suggest the presence of long-range ferromagnetic order. However, experiments in such systems have found evidence for both long- and short-range order, leaving the precise nature of the magnetism in these systems unclear. Here, we use scanning superconducting quantum interference device microscopy to study magnetic domains in V-doped (Bi,Sb)$_2$Te$_3$ exhibiting a quantum anomalous Hall effect with precise quantization. By imaging stray magnetic fields as a function of applied field, we map the formation and evolution of domains through magnetic reversal. We reconstruct the magnetization configuration underlying the measured stray field and find that magnetic domains and crystallographic grains are of similar size. Moreover, magnetic reversal is found to occur through domain expansion, typical of ferromagnets, rather than through nucleation at random sites. Our measurements thus reveal a coexistence of both local magnetic interactions within crystallographic grains and long-range ferromagnetic coupling between grains. This behavior in V-doped (Bi,Sb)$_2$Te$_3$ is markedly distinct from that previously reported for Cr-doped (Bi,Sb)$_2$Te$_3$.

cond-mat.mtrl-sci↗

arXiv2025

Tunable and nonlinearity-enhanced dispersive-plus-dissipative coupling in photon-pressure circuits

Photon-pressure circuits are the circuit implementation of the cavity optomechanical Hamiltonian and discussed for qubit readout, low-frequency quantum photonics and dark matter axion detection. Due to the enormous design flexibility of superconducting circuits, photon-pressure systems provide fascinating possibilities to explore unusual parameter regimes of the optomechanical Hamiltonian. Here, we report the realization of a photon-pressure platform, in which a GHz circuit interacts with a MHz circuit via a magnetic-flux-tunable combination of dispersive and dissipative photon-pressure. In addition, both coupling rates are considerably enhanced by nonlinearities of the GHz-mode, which leads to the multi-photon coupling rates scaling stronger with the pump photon number $n_\mathrm{c}$ than the usual $\sqrt{n_\mathrm{c}}$ dependence. We demonstrate that interference of the two interaction paths leads to a Fano-like response in photon-pressure induced transparency, and that the dynamical backaction is considerably modified compared to the dispersive case, including a parametric instability caused by a red-detuned pump tone.

quant-ph↗

arXiv2025

YBa$_2$Cu$_3$O$_7$ nano-constriction Josephson junctions and SQUIDs fabricated by focused helium-ion-beam irradiation

By focused $30\,\mathrm{keV}$ He ion beam irradiation, epitaxially grown YBa$_2$Cu$_3$O$_7$ (YBCO) thin films can be driven from the superconducting to the insulating state with increasing irradiation dose. A properly chosen dose suppresses superconductivity down to $4\,\mathrm{K}$, while crystallinity is still preserved. With this approach we create areas of normal-conducting YBCO that can be used to define resistively shunted constriction-type Josephson junctions (cJJs) on the nanometer scale. We also demonstrate that the fabricated cJJs can be incorporated in direct current superconducting quantum interference devices and can be used as detector junctions in THz antennas.

cond-mat.supr-con↗

arXiv2025

Advanced SQUID-on-lever scanning probe for high-sensitivity magnetic microscopy with sub-100-nm spatial resolution

Superconducting quantum interference devices (SQUIDs) are exceptionally sensitive magnetometers capable of detecting weak magnetic fields. Miniaturizing these devices and integrating them onto scanning probes enables high-resolution imaging at low-temperature. Here, we fabricate nanometer-scale niobium SQUIDs with inner-loop sizes down to 10 nm at the apex of individual planar silicon cantilevers via a combination of wafer-scale optical lithography and focused-ion-beam (FIB) milling. These robust SQUID-on-lever probes overcome many of the limitations of existing devices, achieving spatial resolution better than 100 nm, magnetic flux sensitivity of $0.3~μΦ_0/\sqrt{\rm{Hz}}$, and operation in magnetic fields up to about 0.5 T at 4.2 K. Nanopatterning via Ne- or He-FIB allows for the incorporation of a modulation line for coupling magnetic flux into the SQUID or a third Josephson junction for shifting its phase. Such advanced functionality, combined with high spatial resolution, large magnetic field range, and the ease of use of a cantilever-based scanning probe, extends the applicability of scanning SQUID microscopy to a wide range of magnetic, normal conducting, superconducting, and quantum Hall systems. We demonstrate magnetic imaging of skyrmions at the surface of bulk Cu$_2$OSeO$_3$. Analysis of the point spread function determined from imaging a single skyrmion yields a full-width-half-maximum of 87 nm. Moreover, we image modulated magnetization patterns with a period of 65 nm.

cond-mat.supr-con↗

arXiv2025

A superconducting on-chip microwave cavity for tunable hybrid systems with optically trapped Rydberg atoms

Hybrid quantum systems are highly promising platforms for addressing important challenges of quantum information science and quantum sensing. Their implementation, however, is technologically non-trivial, since each component typically has unique experimental requirements. Here, we work towards a hybrid system consisting of a superconducting on-chip microwave circuit in a dilution refrigerator and optically trapped ultra-cold atoms. Specifically, we focus on the design optimization of a suitable superconducting chip and on the corresponding challenges and limitations. We unfold detailed microwave-cavity engineering strategies for maximized and tunable coupling rates to atomic Rydberg-Rydberg transitions in $\mathrm{^{87}Rb}$ atoms while respecting the boundary conditions due to the presence of a laser beam near the surface of the chip. Finally, we present an experimental implementation of the superconducting microwave chip and discuss the cavity characteristics as a function of temperature and applied dc voltage. Our results illuminate the required consideration aspects for a flexible, tunable superconductor-atom hybrid system, and lay the groundwork for realizing this exciting platform in a dilution refrigerator with vacuum Rabi frequencies approaching the strong-coupling regime.

quant-ph↗

arXiv2024

Non-volatile multi-state electrothermal resistive switching in a strongly correlated insulator thin-film device

Strongly correlated insulators, such as Mott or charge-transfer insulators, exhibit a strong temperature dependence in their resistivity. Consequently, self-heating effects can lead to electrothermal instabilities in planar thin film devices of these materials. When the electrical bias current exceeds a device-specific threshold, the device can switch from a high- to a low-resistance state through the formation of metallic filaments. However, since the current and temperature redistribution effects that create these filaments are sustained by local Joule heating, a reduction of the bias current below a second (lower) threshold leads to the disappearance of filaments, and the device switches back into the high-resistance state. Hence, electrothermal resistive switching is usually volatile. Here, on the contrary, we report on non-volatile resistive switching in a planar $\mathrm{NdNiO}_3$ thin-film device. By combining electrical transport measurements with optical wide-field microscopy, we provide evidence for a metallic filament that persists even after returning the bias current to zero. We attribute this effect to the pronounced hysteresis between the cooling and heating branches in the resistance vs. temperature dependence of the device. At least one hundred intermediate resistance states can be prepared, which are persistent as long as the base temperature is kept constant. Further, the switching process is non-destructive, and thermal cycling can reset the device to its pristine state.

physics.app-ph↗

arXiv2024

YBa$_2$Cu$_3$O$_7$ Josephson diode operating as a high-efficiency ratchet

Using a focused He$^+$ beam for nanopatterning and writing of Josephson barriers we fabricated specially shaped Josephson junctions of in-line geometry in YBa$_2$Cu$_3$O$_7$ thin film microbridges with an asymmetry ratio of critical currents of opposite polarities (non-reciprocity ratio) $\approx 7$ at optimum magnetic field. Those Josephson diodes were subsequently used as ratchets to rectify an applied ac current into a dc voltage. We also demonstrate the operation of such a ratchet in the loaded regime, where it produces a nonzero dc output power and yields a thermodynamic efficiency of up to $75\,\mathrm{\%}$. The ratchet shows record figures of merit: an output dc voltage of up to $212\,\mathrm{μV}$ and an output power of up to $0.2\,\mathrm{nW}$. The device has an essential area $\approx 1\,\mathrm{μm^2}$. For rectification of quasistatic Gaussian noise, the figures of merit are more modest, however the efficiency can be as high as for the deterministic ac drives within some regimes. Since the device is based on YBa$_2$Cu$_3$O$_7$, it can operate at temperatures up to $\sim40\,\mathrm{K}$, where more noise is available for rectification.

cond-mat.supr-con↗

arXiv2024

Vortex matching at 6 T in YBa$_2$Cu$_3$O$_{7-δ}$ thin films by imprinting a 20 nm-periodic pinning array with a focused helium ion beam

Controlled engineering of vortex pinning sites in copper-oxide superconductors is a critical issue in manufacturing devices based on magnetic flux quanta. To address this, we employed a focused He-ion beam (He-FIB) to irradiate thin YBa$_2$Cu$_3$O$_{7-δ}$ films and create ultradense hexagonal arrays of defects with lattice spacings as small as 20 nm. Critical current and magnetoresistance measurements demonstrate efficient pinning by an unprecedentedly high matching field of 6 T visible in a huge temperature range from the critical temperature $T_c$ down to 2 K. These results show that He-FIB irradiation provides excellent opportunities for the development and application of superconducting fluxonic devices based on Abrikosov vortices. In particular, our findings suggest that such devices can operate at temperatures far below $T_c$, where superconductivity is robust.

cond-mat.supr-con↗

arXiv2024

Temporal Evolution of Defects and Related Electric Properties in He-Irradiated YBa$_{2}$Cu$_{3}$O$_{7-δ}$ Thin Films

Thin films of the superconductor YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO) were modified by low-energy light-ion irradiation employing collimated or focused He$^+$ beams, and the long-term stability of irradiation-induced defects was investigated. For films irradiated with collimated beams, the resistance was measured in situ during and after irradiation and analyzed using a phenomenological model. The formation and stability of irradiation-induced defects are highly influenced by temperature. Thermal annealing experiments conducted in an Ar atmosphere at various temperatures demonstrated a decrease in resistivity and allowed us to determine diffusion coefficients and the activation energy $ΔE = (0.31 \pm 0.03)$ eV for diffusive oxygen rearrangement within the YBCO unit cell basal plane. Additionally, thin YBCO films, nanostructured by focused He$^+$-beam irradiation into vortex pinning arrays, displayed significant commensurability effects in magnetic fields. Despite the strong modulation of defect densities in these pinning arrays, oxygen diffusion during room-temperature annealing over almost six years did not compromise the signatures of vortex matching, which remained precisely at their magnetic fields predicted by the pattern geometry. Moreover, the critical current increased substantially within the entire magnetic field range after long-term storage in dry air. These findings underscore the potential of ion irradiation in tailoring the superconducting properties of thin YBCO films.

cond-mat.supr-con↗

arXiv2024

Terahertz emission from mutually synchronized standalone Bi2Sr2CaCu2O8+x intrinsic-Josephson-junction stacks

Suitably patterned single crystals made of the cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (BSCCO), intrinsically forming a stack of Josephson junctions, can generate electromagnetic radiation in the lower terahertz regime. Due to Joule heating the emission power of single stacks seems to be limited to values below 100 $μ$W. To increase the radiation power, mutually synchronized arrays situated on the same BSCCO base crystal have been studied. Mutual electromagnetic interactions via a connecting BSCCO base crystal have been considered essential for synchronization, but the approach still suffers from Joule heating, preventing the synchronization of more than three stacks. In the present paper we show, on the basis of two emitting stacks, that mutual synchronization can also be achieved by stand-alone stacks contacted by gold layers and sharing only a common gold layer. Compared to BSCCO base crystals, the gold layers have a much higher thermal conductivity and their patterning is not very problematic. We analyze our results in detail, showing that the two oscillators exhibit phase correlations over a range of $\pm$0.4 GHz relative to their center frequencies, which we mainly studied between 745 GHz and 765 GHz. However, we also find that strong phase gradients in the beams radiated from both the mutually locked stacks and the unlocked ones play an important role and, presumably, diminish the detected emission power due to destructive interference. We speculate that the effect arises from higher-order cavity modes which are excited in the individual stacks. Our main message is that the mutual interaction provided by a common gold layer may open new possibilities for relaxing the Joule-heating-problem, allowing the synchronization of a higher number of stacks. Our findings may boost attempts to substantially increase the output power levels of the BSCCO terahertz oscillators.

cond-mat.supr-con↗

arXiv2024

Vector-substrate-based Josephson junctions

We present a way to We present a way to fabricate bicrystal Josephson junctions of high-Tc cuprate superconductors that does not require bulk bicrystalline substrates. Based on vector substrate technology, this novel approach makes use of a few tens-of-nanometers-thick bicrystalline membranes transferred onto conventional substrates.We demonstrate 24° YBa2Cu3O7-x Josephson junctions fabricated on sapphire single crystals by utilizing 10-nm-thick bicrystalline membranes of SrTiO3. This technique allows one to manufacture bicrystalline Josephson junctions of high-Tc superconductors on a large variety of bulk substrate materials, providing novel degrees of freedom in designing the junctions and their electronic properties. It furthermore offers the capability to replace the fabrication of bulk bicrystalline substrates with thin-film growth methods

cond-mat.supr-con↗

arXiv2024

Why shot noise does not generally detect pairing in mesoscopic superconducting tunnel junctions

The shot noise in tunneling experiments reflects the Poissonian nature of the tunneling process. The shot noise power is proportional to both the magnitude of the current and the effective charge of the carrier. Shot noise spectroscopy thus enables, in principle, to determine the effective charge q of the charge carriers that tunnel. This can be used to detect electron pairing in superconductors: in the normal state, the noise corresponds to single electron tunneling (q = 1e), while in the paired state, the noise corresponds to q = 2e. Here, we use a newly developed amplifier to reveal that in typical mesoscopic superconducting junctions, the shot noise does not reflect the signatures of pairing and instead stays at a level corresponding to q = 1e. We show that transparency can control the shot noise and this q = 1e is due to the large number of tunneling channels with each having very low transparency. Our results indicate that in typical mesoscopic superconducting junctions one should expect q = 1e noise, and lead to design guidelines for junctions that allow the detection of electron pairing.

cond-mat.supr-con↗