arXiv subjects

Dietmar Weinmann

Publications and source records attributed to Dietmar Weinmann.

At least 19 recordsLinked to original sources

arXiv2024

Going beyond Landauer scattering theory to describe spatially-resolved non-local heating and cooling in quantum thermoelectrics

Spatially-resolved heating and cooling in nanostructures is nowadays measured with various nanoscale thermometry techniques, including scanning thermometry. Yet the most commonly used theory of nanoscale heating and thermoelectricity -- Landauer scattering theory -- is not appropriate to model such measurements. Hence, we analyze a minimal model of spatially-resolved heat transfer between electrons and phonons in simple thermoelectric nanostructures. This combines Landauer scattering formalism with a Boltzmann equation for transport, revealing the non-locality of Joule heating and Peltier cooling induced by a scatterer in a nanowire. The corresponding heating or cooling of the phonons is caused by the voltage drop at the scatterer, but is often maximal at a certain distance from the scatterer. This distance is of the order of the electron-phonon scattering length. Scanning thermal microscopy, such as SQUID-on-tip thermometers, should detect this non-locality as phonon hot spots and cold spots, spatially separated from the scatterer. We provide physical arguments explaining the thermoelectric response of the combined system of wire and scatterer, and in particular, why the resulting heating and cooling is sometimes the opposite to that predicted by the standard Landauer scattering theory.

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arXiv2023

Reconstructing the potential configuration in a high-mobility semiconductor heterostructure with scanning gate microscopy

The weak disorder potential seen by the electrons of a two-dimensional electron gas in high-mobility semiconductor heterostructures leads to fluctuations in the physical properties and can be an issue for nanodevices. In this paper, we show that a scanning gate microscopy (SGM) image contains information about the disorder potential, and that a machine learning approach based on SGM data can be used to determine the disorder. We reconstruct the electric potential of a sample from its experimental SGM data and validate the result through an estimate of its accuracy.

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arXiv2023

Scanning gate microscopy in graphene nanostructures

The conductance of graphene nanoribbons and nanoconstrictions under the effect of a scanning gate microscopy tip is systematically studied. Using a scattering approach for noninvasive probes, the first- and second-order conductance corrections caused by the tip potential disturbance are expressed explicitly in terms of the scattering states of the unperturbed structure. Numerical calculations confirm the perturbative results, showing that the second-order term prevails in the conductance plateaus, exhibiting a universal scaling law for armchair graphene strips. For stronger tips, at specific probe potential widths and strengths beyond the perturbative regime, the conductance corrections reveal the appearance of resonances originated from states trapped below the tip. The zero-transverse-energy mode of an armchair metallic strip is shown to be insensitive to the long-range electrostatic potential of the probe. For nanoconstrictions defined on a strip, scanning gate microscopy allows to get insight into the breakdown of conductance quantization. The first-order correction generically dominates at low tip strength, while for Fermi energies associated with faint conductance plateaus, the second-order correction becomes dominant for relatively small potential tip strengths. In accordance with the spatial dependence of the partial local density of states, the largest tip effect occurs in the central part of the constriction, close to the edges. Nanoribbons and nanoconstrictions with zigzag edges exhibit a similar response as in the case of armchair nanostructures, except when the intervalley coupling induced by the tip potential destroys the chiral edge states.

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arXiv2022

Asymmetric power dissipation in electronic transport through a quantum point contact

We investigate the power dissipated by an electronic current flowing through a quantum point contact in a two-dimensional electron gas. Based on the Landauer-Büttiker approach to quantum transport, we evaluate the power that is dissipated on the two sides of the constriction as a function of the Fermi energy, temperature, and applied voltage. We demonstrate that an asymmetry appears in the dissipation, which is most pronounced when the quantum point contact is tuned to a conductance step where the transmission strongly depends on energy. At low temperatures, the asymmetry is enhanced when the temperature increases. An estimation for the position of the maximum dissipation is provided.

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arXiv2022

Spontaneous orbital magnetization of mesoscopic dipole dimers

Ensembles of gold nanoparticles present a magnetic behavior which is at odds with the weakly diamagnetic response of bulk gold. In particular, an unusual ferromagnetic order has been unveiled by several experiments. Here we investigate if the combined effect of orbital magnetism of conduction electrons and interparticle dipolar interaction can lead to magnetic ordering. Using different model systems of interacting mesoscopic magnetic dipoles, together with a microscopic description of the electron dynamics within the nanoparticles, we find that a spontaneous magnetic moment may arise in dimers of metallic nanoparticles when the latter are characterized by a large orbital paramagnetic susceptibility.

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arXiv2022

Magnetic response of metallic nanoparticles: Geometric and weakly relativistic effects

While the large paramagnetic response measured in certain ensembles of metallic nanoparticles has been assigned to orbital effects of conduction electrons, the spin-orbit coupling has been pointed out as a possible origin of the anomalously large diamagnetic response observed in other cases. Such a relativistic effect, arising from the inhomogeneous electrostatic potential seen by the conduction electrons, might originate from the host ionic lattice, impurities, or the self-consistent confining potential. Here we theoretically investigate the effect of the spin-orbit coupling arising from the confining potential, quantifying its contribution to the zero-field magnetic susceptibility and gauging it against the ones generated by other weakly-relativistic corrections. Two ideal geometries are considered in detail, the sphere and the half-sphere, focusing on the expected increased role of the spin-orbit coupling upon a symmetry reduction, and the application of these results to actual metallic nanoparticles is discussed. The matrix elements of the different weakly-relativistic corrections are obtained and incorporated in a perturbative treatment of the magnetic field, leading to tractable semi-analytical and semiclassical expressions for the case of the sphere, while a numerical treatment becomes necessary for the half-sphere. The correction to the zero-field susceptibility arising from the spin-orbit coupling in a single sphere is quite small, and it is dominated by the weakly-relativistic kinetic energy correction, which in turn remains considerably smaller than the typical values of the nonrelativistic zero-field susceptibility. Moreover, the spin-orbit contribution to the average response for ensembles of nanoparticles with a large size dispersion is shown to vanish. The symmetry reduction in going from the single sphere to the half-sphere does not translate into a significant (...)

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arXiv2021

Deep neural networks for inverse problems in mesoscopic physics: Characterization of the disorder configuration from quantum transport properties

We present a machine learning approach that allows to characterize the disorder potential of a two-dimensional electronic system from its quantum transport properties. Numerically simulated transport data for a large number of disorder configurations is used for the training of artificial neural networks. We show that the trained networks are able to recognize details of the disorder potential of an unknown sample from its transport properties, and that they can even reconstruct the complete potential landscape seen by the electrons.

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arXiv2021

Imaging signatures of the local density of states in an electronic cavity

We use Scanning Gate Microscopy to study electron transport through an open, gate-defined resonator in a Ga(Al)As heterostructure. Raster-scanning the voltage-biased metallic tip above the resonator, we observe distinct conductance modulations as a function of the tip-position and voltage. Quantum mechanical simulations reproduce these conductance modulations and reveal their relation to the partial local density of states in the resonator. Our measurements illustrate the current frontier between possibilities and limitations in imaging the local density of states in buried electron systems using scanning gate microscopy.

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arXiv2021

Signatures of folded branches in the scanning gate microscopy of ballistic electronic cavities

We demonstrate the emergence of classical features in electronic quantum transport for the scanning gate microscopy response in a cavity defined by a quantum point contact and a micron-sized circular reflector. The branches in electronic flow characteristic of a quantum point contact opening on a two-dimensional electron gas with weak disorder are folded by the reflector, yielding a complex spatial pattern. Considering the deflection of classical trajectories by the scanning gate tip allows to establish simple relationships of the scanning pattern, which are in agreement with recent experimental findings.

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arXiv2019

Energy Stability of Branching in the Scanning Gate Response of Two-Dimensional Electron Gases with Smooth Disorder

The branched pattern typically observed through the scanning gate microscopy (SGM) of two dimensional electron gases in the presence of weak, smooth disorder has recently been found to be robust against a very large shift in the Fermi energy of the electron gas. We propose a toy model, where the potential landscape reduces to a single localized feature, that makes it possible to recast the understanding of branch formation through the effect of caustics in an appropriate set of classical trajectories, and it is simple enough to allow for a quantitative analysis of the energy and spatial dependence of the branches. We find the energy stability to be extremely generic, as it rests only upon the assumptions of weak disorder, weak scattering, and the proportionality of the SGM response to the density of classical electron trajectories. Therefore, the robustness against changes of the electron's Fermi energy remains when adopting progressively realistic models of smooth disorder.

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arXiv2018

Orbital magnetism in ensembles of gold nanoparticles

The last two decades have witnessed various experiments reporting very unusual magnetic properties of ensembles of gold nanoparticles surrounded by organic ligands, including ferromagnetic, paramagnetic, or (large) diamagnetic responses. These behaviors are at odds with the small diamagnetic response of macroscopic gold samples. Here we theoretically investigate the possibility that the observed unusual magnetism in capped gold nanoparticles is of orbital origin. Employing semiclassical techniques, we calculate the orbital component to the zero-field susceptibility of individual as well as ensembles of metallic nanoparticles. While the result for the orbital response of individual nanoparticles can exceed by orders of magnitude the bulk Landau susceptibility in absolute value, and can be either diamagnetic or paramagnetic depending on nanoparticle size, we show that the magnetic susceptibility of a noninteracting ensemble of nanoparticles with a smooth size distribution is always paramagnetic at low magnetic fields. In particular, we predict that the zero-field susceptibility follows a Curie-type law for small nanoparticle sizes and/or low temperatures. The calculated field-dependent magnetization of an ensemble of diluted nanoparticles is shown to be in good agreement with existing experiments that yielded a large paramagnetic response. The width of the size distribution of the nanoparticles is identified as a key element for the quantitative determination of the orbital response.

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arXiv2017

Partial local density of states from scanning gate microscopy

Scanning gate microscopy images from measurements made in the vicinity of quantum point contacts were originally interpreted in terms of current flow. Some recent work has analytically connected the local density of states to conductance changes in cases of perfect transmission, and at least qualitatively for a broader range of circumstances. In the present paper, we show analytically that in any time-reversal invariant system there are important deviations that are highly sensitive to imperfect transmission. Nevertheless, the unperturbed partial local density of states can be extracted from a weakly invasive scanning gate microscopy experiment, provided the quantum point contact is tuned anywhere on a conductance plateau. A perturbative treatment in the reflection coefficient shows just how sensitive this correspondence is to the departure from the quantized conductance value and reveals the necessity of local averaging over the tip position. It is also shown that the quality of the extracted partial local density of states decreases with increasing tip radius.

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arXiv2017

Correlation between peak-height modulation and phase-lapses in transport through quantum dots

We show that two intriguing features of mesoscopic transport, namely the modulation of Coulomb blockade peak-heights and the transmission phase-lapses occurring between subsequent peaks, are closely related. Our analytic arguments are corroborated by numerical simulations for chaotic ballistic quantum dots. The correlations between the two properties are experimentally testable. The statistical distribution of the partial-width amplitude, at the heart of the previous relationship, is determined, and its characteristic parameters are estimated from simple models.

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arXiv2017

Spin-relaxation time in the impurity band of wurtzite semiconductors

The spin-relaxation time for electrons in the impurity band of semiconductors with wurtzite crystal structure is determined. The effective Dresselhaus spin-orbit interaction Hamiltonian is taken as the source of the spin relaxation at low temperature and for doping densities corresponding to the metallic side of the metal-insulator transition. The spin-flip hopping matrix elements between impurity states are calculated and used to set up a tight-binding Hamiltonian that incorporates the symmetries of wurtzite semiconductors. The spin-relaxation time is obtained from a semiclassical model of spin diffusion, as well as from a microscopic self-consistent diagrammatic theory of spin and charge diffusion in doped semiconductors. Estimates are provided for particularly important materials. The theoretical spin-relaxation times compare favorably with the corresponding low-temperature measurements in GaN and ZnO. For InN and AlN, we predict that tuning of the spin-orbit coupling constant induced by an external potential leads to a potentially dramatic increase of the spin-relaxation time related to the mechanism under study.

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arXiv2017

Classical origin of conductance oscillations in an integrable cavity

Scanning gate microscopy measurements in a circular ballistic cavity with a tip placed near its center yield a non-monotonic dependence of the conductance on the tip voltage. Detailed numerical quantum calculations reproduce these conductance oscillations, and a classical scheme leads to its physical understanding. The large-amplitude conductance oscillations are shown to be of classical origin, and well described by the effect of a particular class of short trajectories.

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arXiv2016

Nonradiative limitations to plasmon propagation in chains of metallic nanoparticles

We investigate the collective plasmonic modes in a chain of metallic nanoparticles that are coupled by near-field interactions. The size- and momentum-dependent nonradiative Landau damping and radiative decay rates are calculated analytically within an open quantum system approach. These decay rates determine the excitation propagation along the chain. In particular, the behavior of the radiative decay rate as a function of the plasmon wavelength leads to a transition from an exponential decay of the collective excitation for short distances to an algebraic decay for large distances. Importantly, we show that the exponential decay is of a purely nonradiative origin. Our transparent model enables us to provide analytical expressions for the polarization-dependent plasmon excitation profile along the chain and for the associated propagation length. Our theoretical analysis constitutes an important step in the quest for the optimal conditions for plasmonic propagation in nanoparticle chains.

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arXiv2015

Decay of dark and bright plasmonic modes in a metallic nanoparticle dimer

We develop a general quantum theory of the coupled plasmonic modes resulting from the near-field interaction between localized surface plasmons in a heterogeneous metallic nanoparticle dimer. In particular, we provide analytical expressions for the frequencies and decay rates of the bright and dark plasmonic modes. We show that, for sufficiently small nanoparticles, the main decay channel for the dark plasmonic mode, which is weakly coupled to light and, hence, immune to radiation damping, is of nonradiative origin and corresponds to Landau damping, i.e., decay into electron-hole pairs.

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arXiv2014

Parity-dependent localization in $N$ strongly coupled chains

Anderson localization of wave-functions at zero energy in quasi-1D systems of $N$ disordered chains with inter-chain coupling $t$ is examined. Localization becomes weaker than for the 1D disordered chain ($t=0$) when $t$ is smaller than the longitudinal hopping $t'=1$, and localization becomes usually much stronger when $t\gg t'$. This is not so for all $N$. We find "immunity" to strong localization for open (periodic) lateral boundary conditions when $N$ is odd (a multiple of four), with localization that is weaker than for $t=0$ and rather insensitive to $t$ when $t \gg t'$. The peculiar $N$-dependence and a critical scaling with $N$ is explained by a perturbative treatment in $t'/t$, and the correspondence to a weakly disordered effective chain is shown. Our results could be relevant for experimental studies of localization in photonic waveguide arrays.

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