arXiv subjects

Dihao Sun

Publications and source records attributed to Dihao Sun.

11 recordsLinked to original sources

arXiv2026

Signatures of quantum chaos in phonon-polariton billiards

We use scanning near-field optical microscopy to image hyperbolic phonon polaritons in hexagonal boron nitride (hBN) billiards with integrable and chaotic geometries. In Sinai billiards, we observe irregular mode patterns consistent with quantum scarring, together with an unexpected sensitivity to weak probe perturbations. These random-wave features coexist with non-chaotic one-dimensional boundary modes arising from nontrivial polariton reflection at the billiard edge. As the billiard boundary becomes increasingly complex, the Fourier transforms of the measured signals evolve toward ring-like structures consistent with Berry's random-wave conjecture. We develop a numerical framework based on the Helmholtz equation with generalized boundary conditions that encode angle-dependent reflection phase shifts. The calculated level statistics exhibit a crossover from Poisson-like behavior in integrable billiards to Wigner-Dyson-like behavior in chaotic geometries, with small deviations from the canonical form arising from nonlinear boundary conditions that require self-consistent bulk-boundary analysis. Theoretical analysis based on dissipative Green's functions qualitatively reproduces the near-field data. These results establish mesoscopic van der Waals billiards as a rich platform for studying generalized chaotic dynamics of hybrid light-matter polaritons.

cond-mat.mes-hall↗

arXiv2025

Electrically driven plasmon-polaritonic bistability in Dirac electron tunneling transistors

Bistability-two distinct stable states under identical parameter-is not only a fundamental physical concept but also of importance in practical applications. While plasmon-polaritonic bistability representing history-dependent stable states within plasmonic systems has been theoretically predicted, it has yet to be demonstrated experimentally due to challenges in realizing suitable nonlinearity at feasible electric-field strengths. Here, we report the experimental observation of electrically driven plasmon-polaritonic bistability in graphene/hexagonal-boron-nitride/graphene tunneling transistors, achieved through momentum-conserving resonant tunneling of Dirac electrons. Using a small twist angle between graphene layers, we engineered devices exhibiting both electronic and plasmon-polaritonic bistability. This bistable plasmonic behavior can be precisely tuned through load resistance and electrostatic gating. Our findings open new pathways for exploring nonlinear optical and electronic phenomena in van der Waals heterostructures and mark a significant advance in nanoplasmonics, with potential applications in optical memory, sensing, and optoelectronic switching.

cond-mat.mes-hall↗

arXiv2025

Ultrafast Charge-Doping via Photo-Thermionic Injection in van der Waals Devices

Van der Waals (vdW) heterostructures of two-dimensional (2D) materials have become a rich playground for the exploration of correlated quantum phases, and recent studies have begun to probe their non-equilibrium dynamics under femtosecond laser excitation. In a time-resolved experiment, optical excitation of the multilayer structure can lead not only to rich dynamic responses from the target layers, such as moir\'e interfaces, but also to additional device functionality from the layer degree of freedom. Here, we investigate optical excitation in a prototypical moir\'e device of dual-gated twisted WSe2 bilayers, with few-layer graphite gates and hexagonal boron nitride (hBN) spacers. We establish an ultrafast photodoping mechanism in the moir\'e bilayer from photo-thermionic emission of the graphite gates. Using transient reflectance experiments, we reveal photo-induced hole injection evidenced by: (i) a shift of gate voltages at which optical signatures of correlated insulators are observed, (ii) a persistent optical signature indicative of charge diffusion at microsecond timescales and local charge buildup from pulse-to-pulse accumulation, and (iii) photoinduced absorption due likely to transient formation of correlated insulators. We further demonstrate that the injected holes can be selectively controlled by tuning the excitation energy, fluence, and gate bias.

cond-mat.str-el↗

arXiv2025

Photoinduced Metal-to-Insulator Transitions in 2D Moir\'e Devices

Photoexcitation has been utilized to control quantum matter and to uncover metastable phases far from equilibrium. Among demonstrations to date, the most common is the photo-induced transition from correlated insulators to metallic states; however, the reverse process without initial orders has not been observed. Here, we show ultrafast metal-to-insulator transition in gate-doped WS2/WSe2 and WSe2/WSe2 moir\'e devices using photo-thermionic hole injection from graphite gates. The resulting correlated insulators are metastable, with lifetimes exceeding microseconds. These findings establish an effective mechanism for the ultrafast control of correlated electronic phases in van der Waals heterostructures.

cond-mat.str-el↗

arXiv2025

Dynamic Interfacial Quantum Dipoles in Charge Transfer Heterostructures

Hysteretic gate responses of two-dimensional material heterostructures serve as sensitive probes of the underlying electronic states and hold significant promise for the development of novel nanoelectronic devices. Here we identify a new mechanism of hysteretic behavior in graphene/$h$BN/$\alpha$-$\mathrm{RuCl_3}$ charge transfer field effect devices. The hysteresis loop exhibits a sharp onset under low temperatures and evolves symmetrically relative to the charge transfer equilibrium. Unlike conventional flash memory devices, the charge transfer heterostructure features a transparent tunneling barrier and its hysteretic gate response is induced by the dynamic tuning of interfacial dipoles originating from quantum exchange interactions. The system acts effectively as a ferroelectric and gives rise to remarkable tunability of the hysteretic gate response under external electrical bias. Our work unveils a novel mechanism for engineering hysteretic behaviors via dynamic interfacial quantum dipoles.

cond-mat.mes-hall↗

arXiv2025

Flat band excitons in a three-dimensional supertwisted spiral transition metal dichalcogenide

A new frontier in van der Waals twistronics is the development of three-dimensional (3D) supertwisted materials, where each successive atomic layer rotates by the same angle. While two-dimensional (2D) moire systems have been extensively studied, the unique phenomena arising from 3D twistronics remain largely unexplored. In this work, we report the discovery of flat-band excitons in 3D supertwisted WS2, revealed by systematic photoluminescence (PL) experiments and electronic structure calculations. These excitons retain key features of 2D moire transition metal dichalcogenides (TMDs)-such as layer confinement, moire-driven localization, and strong Coulomb interactions-while also offering advantages in scalability and enhanced optical responses in three dimensions. Beyond the PL signatures reminiscent of 2D A excitons, we observe novel direct and indirect exciton emission uniquely tied to the supertwist geometry. Using generalized Bloch band theory and local density of states calculations that incorporate screw rotational symmetry, we uncovered the coexistence of 2D and 3D flatband gaps. These flat-band excitons serve as sensitive probes of the electronic properties of 3D supertwisted semiconductors and open new pathways for applications in quantum optoelectronics.

physics.app-ph↗

arXiv2025

Cavity-altered superconductivity

Is it feasible to alter the ground state properties of a material by engineering its electromagnetic environment? Inspired by theoretical predictions, experimental realizations of such cavity-controlled properties without optical excitation are beginning to emerge. Here, we devised and implemented a novel platform to realize cavity-altered materials. Single crystals of hyperbolic van der Waals (vdW) compounds provide a resonant electromagnetic environment with enhanced density of photonic states and prominent mode confinement. We interfaced hexagonal boron nitride (hBN) with the molecular superconductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br ($\kappa$-ET). The frequencies of infrared (IR) hyperbolic modes of hBN match the IR-active carbon-carbon stretching molecular resonance of ($\kappa$-ET) implicated in superconductivity. Nano-optical data supported by first-principles molecular Langevin dynamics simulations confirm the presence of resonant coupling between the hBN hyperbolic cavity modes and the carbon-carbon stretching mode in ($\kappa$-ET). Meissner effect measurements via magnetic force microscopy demonstrate a strong suppression of superfluid density near the hBN/($\kappa$-ET) interface. Non-resonant control heterostructures, including RuCl$_3$/($\kappa$-ET) and hBN/$\text{Bi}_2\text{Sr}_2\text{CaCu}_2\text{O}_{8+x}$, do not display the superfluid suppression. These observations suggest that hBN/($\kappa$-ET) realizes a cavity-altered superconducting ground state. Our work highlights the potential of dark cavities devoid of external photons for engineering electronic ground state properties of complex quantum materials.

cond-mat.supr-con↗

arXiv2024

Low-Energy Electronic Structure in the Unconventional Charge-Ordered State of ScV$_6$Sn$_6$

Kagome vanadates {\it A}V$_3$Sb$_5$ display unusual low-temperature electronic properties including charge density waves (CDW), whose microscopic origin remains unsettled. Recently, CDW order has been discovered in a new material ScV$_6$Sn$_6$, providing an opportunity to explore whether the onset of CDW leads to unusual electronic properties. Here, we study this question using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy (STM). The ARPES measurements show minimal changes to the electronic structure after the onset of CDW. However, STM quasiparticle interference (QPI) measurements show strong dispersing features related to the CDW ordering vectors. A plausible explanation is the presence of a strong momentum-dependent scattering potential peaked at the CDW wavevector, associated with the existence of competing CDW instabilities. Our STM results further indicate that the bands most affected by the CDW are near vHS, analogous to the case of {\it A}V$_3$Sb$_5$ despite very different CDW wavevectors.

cond-mat.str-el↗

arXiv2023

Evidence for a Superfluid-to-solid Transition of Bilayer Excitons

One of the most spectacular properties associated with Bose-Einstein condensation (BEC) is superfluidity in which the system exhibits zero viscosity and flows without dissipation. The superfluid phase has been observed in wide ranging Bosonic systems spanning naturally occurring quantum fluids, such as liquid helium, to engineered platforms such as bilayer excitons and cold atom systems. Theoretical works have proposed that interactions could drive the BEC ground state into another exotic phase that simultaneously exhibits properties of both a crystalline solid and a superfluid - termed a supersolid. Identifying a material system, however, that hosts the predicted BEC solid phase, driven purely by interactions and without imposing an external lattice potential, has remained elusive. Here we report observation of a superfluid to insulator transition in the layer-imbalanced regime of bilayer magneto-excitons. Mapping the transport behavior of the bilayer condensate as a function of density and temperature, suggests that the insulating phase is an ordered state of dilute excitons, stabilized by dipole interactions. The insulator melts into a recovered superfluid upon increasing the temperature, which could indicate that the low temperature solid is also a quantum coherent phase.

cond-mat.mes-hall↗

arXiv2022

Electron spin resonance and collective excitations in magic-angle twisted bilayer graphene

In a strongly correlated system, collective excitations contain key information regarding the electronic order of the underlying ground state. An abundance of collective modes in the spin and valley isospin channels of magic-angle graphene moir\'e bands has been alluded to by a series of recent experiments. However, direct observation of collective excitations has remained elusive due to the lack of a spin probe. In this work, we use a resistively-detected electron spin resonance technique to look for low-energy collective excitations in magic-angle twisted bilayer graphene. We report direct observation of collective modes in the form of microwave-induced resonance near half filling of the moir\'e flatbands. The frequency-magnetic field dependence of these resonance modes sheds light onto the nature of intervalley spin coupling, allowing us to extract parameters such as intervalley exchange interaction and spin stiffness. Two independent observations testify that the generation and detection of the microwave resonance relies on the strong correlation within the flat moir\'e energy band. First, the onset of robust resonance response coincides with the spontaneous flavor polarization at half moir\'e filling, and remains absent in the density range where the underlying Fermi surface is isospin unpolarized. Second, we performed the same resonance measurement on graphene monolayer and bilayer samples, including twisted bilayer with a large twist angle, where flatband physics is absent. We observe no indication of resonance response in these samples across a large range of carrier density, microwave frequency and power. A natural explanation is that the resonance response near the magic angle originates from "Dirac revivals" and the resulting isospin order.

cond-mat.mes-hall↗

arXiv2017

Quench Dynamics of Josephson Current in a Topological Josephson Junction

The $4\pi$ Josephson Effect is a distinguishing feature of a topological Josephson junction. However, stringent conditions make it hard to observe in experiments. Here we numerically study the transient transport properties in a topological Josephson junction. We show that the $4\pi$ Josephson current can be sustained for a significant time (around several $\mu s$ with suitable conditions). Furthermore, we compare the behaviors of Josephson current in different conditions, identifying three main regimes: First, when both the superconducting wires of the Josephson junction lie in the topologically nontrivial region, the $4\pi$ Josephson current can appear with a suddenly applied DC voltage. Second, when one superconducting wire lies in the trivial region and the other one lies in the non-trivial region, the Josephson current is $2\pi$ periodic but unstable with the evolving of time. Third, when both wires lie in the trivial region, a stable $2\pi$ Josephson current is observed. These results can facilitate fine-tuning of the experiment parameters in order to finally observe the $4\pi$ Josephson current in a topological Josephson junction.

cond-mat.mes-hall↗