arXiv subjects

Dipranjan Chatterjee

Publications and source records attributed to Dipranjan Chatterjee.

4 recordsLinked to original sources

arXiv2026

Gapped 1/9 Magnetization Plateau in the Anisotropic Kagome Antiferromagnet Y-kapellasite

Fractional magnetization plateaus provide a sensitive probe of many-body spin states in frustrated quantum magnets, yet their microscopic origin in kagome antiferromagnets remains unresolved. This is particularly true of the mysterious $1/9$ plateau, which is predicted by theory but infrequently observed in experiment. Here, we investigate this problem in the $S = 1/2$ anisotropic kagome antiferromagnet Y-kapellasite, Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$, using pulsed-field magnetization measurements on single crystals and high-field $^{35}$Cl NMR. We identify a hierarchy of field-induced fractional features, including $1/3$ and $1/9$ plateaus, as well as a weaker low-field feature. Analysis of the NMR spectra and the magnetic susceptibility across the $1/9$ plateau demonstrate that it is accompanied by an ordered local spin configuration, a strong suppression of low-energy spin fluctuations and activated behavior, consistent with a gapped fractional state. These features differ from those in the only other material YCu$_3$(OH)$_6$Br$_2$[Br$_{1-y}$(OH)$_y$] in which this plateau is observed, implying a surprising robustness of the $1/9$ state to the details of the underlying magnetism.

cond-mat.str-el↗

arXiv2025

Vector spin polarization evolution determined in an entangled muon-fluorine system under pulsed excitation

A spin-polarized muon implanted into a fluoride forms a coupled F--$\mu$--F complex in which the muon spin and neighbouring fluorine nuclear spins become entangled. Here we apply radio-frequency (RF) excitation to this coupled system and use the three-dimensional distribution of emitted positrons to reconstruct the time-dependent evolution of the muon spin polarization. This three-dimensional readout, using single spin detection, is not possible in a single NMR experiment and demonstrates significant advantages that are achieved by using RF muon techniques. We demonstrate the application of this vector-readout method to the experimental observation of a muon spin echo signal that is controlled by the dipolar coupling to fluorine, as well as to a double resonance experiment, in which we use pulses tuned to separate frequencies to address both the muon and fluorine spins. This targeted approach, in which selective RF pulses can control the muon spin and other spins to which it is coupled, provides a novel route for probing systems of entangled spins.

cond-mat.str-el↗

arXiv2025

Emergence of a Fluctuating Ground State in Y-kapellasite under Pressure

Y-kapellasite (Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$), which hosts an original anisotropic kagome sublattice, is a promising candidate for studying elusive and complex correlated physics. It exhibits a theoretically predicted in-plane $(1/3, 1/3)$ magnetic order [1] but its magnetic interaction values place it close to a phase boundary to a spin liquid state [2]. Our $\mu$SR measurements under hydrostatic pressure demonstrate the complete suppression of static magnetism in favor of a fully dynamical ground state at $2.3$~GPa. Complementary high-pressure x-ray and optical phonon measurements reveal a gradual reduction of the kagome anisotropy, enhancing magnetic frustration without structural transitions. Our results establish Y-kapellasite as a rare clean kagome model in which long-range order is suppressed by pressure-tuned frustration, the first fingerprint for the realization of a quantum spin liquid without strong disorder.

cond-mat.str-el↗

arXiv2025

Spin dynamics in the Dirac $U(1)$ spin liquid YbZn$_2$GaO$_5$

YbZn$_2$GaO$_5$ is a promising candidate for realizing a quantum spin liquid (QSL) state, particularly owing to its lack of significant site disorder. Pulsed-field magnetometry at 0.5 K shows magnetization saturating near 15 T, with a corrected saturation moment of 2.1(1) $\mu_\mathrm{B}$ after subtracting the van Vleck contribution. Our zero-field $\mu$SR measurements down to milliKelvin temperatures provide evidence for a dynamic ground state and the absence of magnetic order. To probe fluctuations in the local magnetic field at the muon site, we performed longitudinal field $\mu$SR experiments. These results provide evidence for spin dynamics with a field dependence that is consistent with a U1A01 Dirac QSL as a plausible description of the ground state.

cond-mat.str-el↗