arXiv subjects

Dirk Backes

Publications and source records attributed to Dirk Backes.

18 recordsLinked to original sources

arXiv2026

X-ray magnetic circular dichroism evidence of intrinsic $d$-wave altermagnetism in rutile-structure NiF$_2$

We present the x-ray magnetic circular dichroism (XMCD) at the Ni $L_{2,3}$-edge as an evidence of the $d$-wave altermagnetism in rutile-structure NiF$_2$. Sizable XMCD signal is observed in excellent agreement with theoretical simulations. Owing to a considerable net magnetization due to spin canting, the XMCD spectrum consists of an altermagnetic signal as well as a non-negligible ferromagnetic contribution. We verify experimentally that the XMCD spectrum can be written as a sum of contributions from altermagnetism and weak ferromagnetism. Two experimental methods to isolate the ferromagnetic contribution are shown to yield essentially the same result. These are dependence of XMCD on applied magnetic fields below the N\'eel temperature and the XMCD measured in applied field above the N\'eel temperature. Our results demonstrate the utility of XMCD as a probe for altermagnetic materials with the coexisting weak ferromagnetism induced by the relativistic spin-orbit coupling.

cond-mat.str-el↗

arXiv2025

Magnon-magnon coupling efficiency of $\eta$=0.5 in weakly pinned synthetic antiferromagnets

Synthetic antiferromagnets (SAFs) consist of two ferromagnetic layers that are antiferromagnetically coupled. These systems support complex dynamical magnetic excitations, where interlayer coupling gives rise to both in-phase (acoustic) and anti-phase (optical) magnonic modes. Typically, simultaneous excitation of both modes requires breaking the symmetry between the ferromagnetic layers -- commonly achieved through slight misalignment of the experimental setup or by modifying the intrinsic magnetic properties. In our approach, we utilize a pinned synthetic antiferromagnet (pSAF), where one of the ferromagnetic layers is exchange-coupled to an antiferromagnet. We demonstrate that by tuning the thickness of the antiferromagnet and slightly enhancing the magnetic anisotropy of the pinned layer, both acoustic and optical modes can be efficiently excited -- without the need for experimental misalignment or changes to the intrinsic material properties. Under specific conditions, the magnon dispersion relations exhibit anti-crossing behavior, resulting in the emergence of a magnonic bandgap -- a clear signature of strong magnon-magnon coupling. The coupling efficiency $\eta$, defined as the ratio between the bandgap and the characteristic frequency, reaches $\eta = 0.5$, approaching the ultra-strong coupling regime ($\eta = 1$). The combination of strong mode hybridization, a sizable magnonic bandgap, and high ferromagnetic resonance (FMR) coherence over large areas -- all achieved at room temperature without cryogenic cooling -- underscores the potential of these systems for quantum magnonic applications, including quantum computing.

cond-mat.mes-hall↗

arXiv2025

Low energy excitations in A-site ordered SmBaMn2O6

The electron in a solid can be considered a bound state of the three independent, fundamental degrees of freedom creating quasi-particles: spinons, carrying the electron spin; plasmons carrying the collective charge mode and orbitons carrying its orbital degree of freedom. These fundamental degrees of freedom could form ordering states in which dynamics or collective motions could occurr and manifest as low-energy excitations. The exotic properties that appear in the materials exhibiting these electronic orderings are associated with these low-energy excitations. Although the orbital order (OO) and its coupling to the spin system creates very interesting phenomena, the microscopic origin of OO has been much less explored than other electronic properties as it is very difficult to directly access experimental information from OO. Due to the recent improvement in energy resolution and flux, soft x-ray resonant inelastic scattering (RIXS) allows for a re-examination of orbital excitations in manganites. Here, we present a study of low energy excitations in half doped A-site ordered SmBaMn_{2}O_{6} through a combination of RIXS and soft x-ray resonant elastic scattering (REXS) measurements. The obtained experimental data confirm the OO at \mathbf{q} = (0.25, 0.25, 0) and find various low energy excitations below 200 meV. while several excitations can be assigned to be of magnetic and phononic origin, a group of excitations between 80 and 200 meV show a temperature dependence distinctively following that of the OO making them possible candidates for orbital excitations.

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arXiv2022

Identifiying the domain wall spin structure in current-induced switching of antiferromagnetic NiO/Pt

The understanding of antiferromagnetic domain walls, which are the interface between domains with different N\'eel order orientations, is a crucial aspect to enable the use of antiferromagnetic materials as active elements in future spintronic devices. In this work, we demonstrate that in antiferromagnetic NiO/Pt bilayers circular domain structures can be generated by switching driven by electrical current pulses. The generated domains are T-domains, separated from each other by a domain wall whose spins are pointing toward the average direction of the two T-domains rather than the common axis of the two planes. Interestingly, this direction is the same for the whole circular domain indicating the absence of strong Lifshitz invariants. The domain wall can be micromagnetically modeled by strain distributions in the NiO thin film induced by the MgO substrate, deviating from the bulk anisotropy. From our measurements we determine the domain wall width to have a full width at half maximum of $\Delta = 98 \pm 10$ nm, demonstrating strong confinement.

cond-mat.mtrl-sci↗

arXiv2022

Wafer-scale epitaxial growth of the thickness-controllable van der Waals ferromagnet CrTe2 for reliable magnetic memory applications

To harness the intriguing properties of two-dimensional van der Waals (vdW) ferromagnets (FMs) for versatile applications, the key challenge lies in the reliable material synthesis for scalable device production. Here, we demonstrate the epitaxial growth of single-crystalline 1T-CrTe2 thin films on 2-inch sapphire substrates. Benefiting from the uniform surface energy of the dangling bond-free Al2O3(0001) surface, the layer-by-layer vdW growth mode is observed right from the initial growth stage, which warrants precise control of the sample thickness and atomically smooth surface morphology across the entire wafer. Moreover, the presence of the Coulomb interaction at the CrTe2/Al2O3 interface serves as an effective tuning parameter to tailor the anomalous Hall response, and the structural optimization of the CrTe2-based spin-orbit torque device leads to a substantial switching power reduction by 54%. Our results may lay out a general framework for the design of energy-efficient spintronics based on configurable vdW FMs.

cond-mat.mtrl-sci↗

arXiv2022

Reconfigurable Reservoir Computing in a Magnetic Metamaterial

In-materia reservoir computing (RC) leverages the intrinsic physical responses of functional materials to perform complex computational tasks. Magnetic metamaterials are exciting candidates for RC due to their huge state space, nonlinear emergent dynamics, and non-volatile memory. However, to be suitable for a broad range of tasks, the material system is required to exhibit a broad range of properties, and isolating these behaviours experimentally can often prove difficult. By using an electrically accessible device consisting of an array of interconnected magnetic nanorings -- a system shown to exhibit complex emergent dynamics -- here we show how reconfiguring the reservoir architecture allows exploitation of different aspects the system's dynamical behaviours. This is evidenced through state-of-the-art performance in diverse benchmark tasks with very different computational requirements, highlighting the additional computational configurability that can be obtained by altering the input/output architecture around the material system.

cond-mat.mes-hall↗

arXiv2022

Ultrafast X-ray imaging of the light-induced phase transition in VO2

Using light to control transient phases in quantum materials is an emerging route to engineer new properties and functionality, with both thermal and non-thermal phases observed out of equilibrium. Transient phases are expected to be heterogeneous, either through photo-generated domain growth or by generating topological defects, and this impacts the dynamics of the system. However, this nanoscale heterogeneity has not been directly observed. Here we use time- and spectrally resolved coherent X-ray imaging to track the prototypical light induced insulator-to-metal phase transition in vanadium dioxide on the nanoscale with femtosecond time resolution. We show that the early-time dynamics are independent of the initial spatial heterogeneity and observe a 200 fs switch to the metallic phase. A heterogeneous response emerges only after hundreds of picoseconds. Through spectroscopic imaging, we reveal that the transient metallic phase is a highly orthorhombically strained rutile metallic phase, an interpretation that is in contrast to those based on spatially averaged probes. Our results demonstrate the critical importance of spatially and spectrally resolved measurements for understanding and interpreting the transient phases of quantum materials.

cond-mat.str-el↗

arXiv2020

An insulating doped antiferromagnet with low magnetic symmetry as a room temperature spin conduit

We report room temperature long-distance spin transport of magnons in antiferromagnetic thin film hematite doped with Zn. The additional dopants significantly alter the magnetic anisotropies, resulting in a complex equilibrium spin structure that is capable of efficiently transporting spin angular momentum at room temperature without the need for a well-defined, pure easy-axis or easy-plane anisotropy. We find intrinsic magnon spin-diffusion lengths of up to 1.5 {\mu}m, and magnetic domain governed decay lengths of 175 nm for the low frequency magnons, through electrical transport measurements demonstrating that the introduction of non-magnetic dopants does not strongly reduce the transport length scale showing that the magnetic damping of hematite is not significantly increased. We observe a complex field dependence of the non-local signal independent of the magnetic state visible in the local magnetoresistance and direct magnetic imaging of the antiferromagnetic domain structure. We explain our results in terms of a varying and applied-field-dependent ellipticity of the magnon modes reaching the detector electrode allowing us to tune the spin transport.

cond-mat.mes-hall↗

arXiv2020

Electrical detection of the spin reorientation transition in antiferromagnetic TmFeO$_3$ thin films by spin Hall magnetoresistance

TmFeO$_3$ (TFO) is a canted antiferromagnet that undergoes a spin reorientation transition (SRT) with temperature between 82 K and 94 K in single crystals. In this temperature region, the N\'eel vector continuously rotates from the crystallographic $c$-axis (below 82 K) to the $a$-axis (above 94 K). The SRT allows for a temperature control of distinct antiferromagnetic states without the need for a magnetic field, making it apt for applications working at THz frequencies. For device applications, thin films of TFO are required as well as an electrical technique for reading out the magnetic state. Here we demonstrate that orthorhombic TFO thin films can be grown by pulsed laser deposition and the detection of the SRT in TFO thin films can be accessed by making use of the all electrical spin Hall magnetoresistance (SMR), in good agreement for the temperature range where the SRT occurs. Our results demonstrate that one can electrically detect the SRT in insulators.

cond-mat.mtrl-sci↗

arXiv2020

Identification of N\'eel vector orientation in antiferromagnetic domains switched by currents in NiO/Pt thin films

Understanding the electrical manipulation of antiferromagnetic order is a crucial aspect to enable the design of antiferromagnetic devices working at THz frequency. Focusing on collinear insulating antiferromagnetic NiO/Pt thin films as a materials platform, we identify the crystallographic orientation of the domains that can be switched by currents and quantify the N\'eel vector direction changes. We demonstrate electrical switching between different T-domains by current pulses, finding that the N\'eel vector orientation in these domains is along $[\pm5\ \pm5\ 19]$, different compared to the bulk $<11\bar{2}>$ directions. The final state of the N\'eel vector $\textbf{n}$ switching after current pulses $\textbf{j}$ along the $[1\ \pm1\ 0]$ directions is $\textbf{n}\parallel \textbf{j}$. By comparing the observed N\'eel vector orientation and the strain in the thin films, assuming that this variation arises solely from magnetoelastic effects, we quantify the order of magnitude of the magnetoelastic coupling coefficient as $b_{0}+2b_{1}=3*10^7 J\ m^{-3}$ . This information is key for the understanding of current-induced switching in antiferromagnets and for the design and use of such devices as active elements in spintronic devices.

cond-mat.mtrl-sci↗

arXiv2018

Thickness dependence of electron-electron interactions in topological p-n junctions

Electron-electron interactions in topological p-n junctions consisting of vertically stacked topological insulators are investigated. n-type Bi2Te3 and p-type Sb2Te3 of varying relative thicknesses are deposited using molecular beam epitaxy and their electronic properties measured using low-temperature transport. The screening factor is observed to decrease with increasing sample thickness, a finding which is corroborated by semi-classical Boltzmann theory. The number of two-dimensional states determined from electron-electron interactions is larger compared to the number obtained from weak-antilocalization, in line with earlier experiments using single layers.

cond-mat.mes-hall↗

arXiv2016

Effect of temperature on spin-transfer torque induced magnetic solitons

Spin-transfer torques in a nanocontact to an extended magnetic film can create spin waves that condense to form dissipative droplet solitons. Here we report an experimental study of the temperature dependence of the current and applied field thresholds for droplet soliton formation, as well as the nanocontact's electrical characteristics associated with droplet dynamics. Nucleation of droplet solitons requires higher current densities at higher temperatures, in contrast to typical spin-transfer torque induced switching between static magnetic states. Magnetoresistance and electrical noise measurements show that soliton instabilities become more pronounced with increasing temperature. These results are of fundamental interest in understanding the influence of thermal noise on droplet solitons, and in controlling their dynamics.

cond-mat.mes-hall↗

arXiv2016

Topological states and phase transitions in Sb$_2$Te$_3$-GeTe multilayers

Topological insulators (TIs) are bulk insulators with exotic 'topologically protected' surface conducting modes. It has recently been pointed out that when stacked together, interactions between surface modes can induce diverse phases including the TI, Dirac semimetal, and Weyl semimetal. However, currently a full experimental understanding of the conditions under which topological modes interact is lacking. Here, working with multilayers of the TI Sb$_2$Te$_3$ and the band insulator GeTe, we provide experimental evidence of a multiple topological modes in a single Sb$_2$Te$_3$-GeTe-Sb$_2$Te$_3$ structure. Furthermore, we show that reducing the thickness of the GeTe layer induces a phase transition from a Dirac-like phase to a gapped phase. By comparing different multilayer structures we demonstrate that this transition occurs due to the hybridisation of states associated with different TI films. Our results demonstrate that the Sb$_2$Te$_3$-GeTe system offers strong potential towards manipulating topological states as well as towards controlledly inducing various topological phases.

cond-mat.mes-hall↗

arXiv2015

'Metal'-like transport in high-resistance, high aspect ratio two-dimensional electron gases

We investigate the striking absence of strong localisation observed in mesoscopic two-dimensional electron gases (2DEGs) (Baenninger et al 2008 Phys. Rev. Lett. 100 1016805, Backes et al 2015 Phys. Rev. B 92 235427) even when their resistivity $\rho >> h/e^2$. In particular, we try to understand whether this phenomenon originates in quantum many-body effects, or simply percolative transport through a network of electron puddles. To test the latter scenario, we measure the low temperature (low-$T$) transport properties of long and narrow 2DEG devices in which percolation effects should be heavily suppressed in favour of Coulomb blockade. Strikingly we find no indication of Coulomb blockade and that the high-$\rho$, low-$T$ transport is exactly similar to that previously reported in mesoscopic 2DEGs with different geometries. Remarkably, we are able to induce a `metal'-insulator transition (MIT) by applying a perpendicular magnetic field $B$. We present a picture within which these observations fit into the more conventional framework of the 2D MIT.

cond-mat.mes-hall↗

arXiv2015

Observation of droplet soliton drift resonances in a spin-transfer-torque nanocontact to a ferromagnetic thin film

Magnetic droplet solitons are non-linear dynamical modes that can be excited in a thin film with perpendicular magnetic anisotropy with a spin-transfer-torque. Although droplet solitons have been proved to be stable with a hysteretic response to applied currents and magnetic fields at low temperature, measurements at room temperature indicate less stability and reduced hysteresis width. Here, we report evidence of droplet soliton drift instabilities, leading to drift resonances, at room temperature that explains their lower stability. Micromagnetic simulations show that the drift instability is produced by an effective field asymmetry in the nanocontact region that can have different origins.

cond-mat.mes-hall↗

arXiv2015

Observation of geometry dependent conductivity in two-dimensional electron systems

We report electrical conductivity $\sigma$ measurements on a range of two-dimensional electron gases (2DEGs) of varying linear extent. Intriguingly, at low temperatures ($T$) and low carrier density ($n_{\mathrm{s}}$) we find the behavior to be consistent with $\sigma \sim L^{\alpha}$, where $L$ is the length of the 2DEG along the direction of transport. Importantly, such scale-dependent behavior is precisely in accordance with the scaling hypothesis of localization~[Abrahams~\textit{et al.}, Phys. Rev. Lett. \textbf{42}, 673 (1979)] which dictates that in systems where the electronic wave function $\xi$ is localized, $\sigma$ is not a material-specific parameter, but depends on the system dimensions. From our data we are able to construct the "$\beta$-function" $\equiv (h/e^2) d \ln \sigma / d \ln L$ and show this to be strongly consistent with theoretically predicted limiting values. These results suggest, remarkably, that the electrons in the studied 2DEGs preserve phase coherence over lengths $\sim~10~\mu$m. This suggests the utility of the 2DEGs studied towards applications in quantum information as well as towards fundamental investigations into many-body localized phases.

cond-mat.mes-hall↗

arXiv2015

Determining energy relaxation length scales in two-dimensional electron gases

We present measurements of the energy relaxation length scale $\ell$ in two-dimensional electron gases (2DEGs). A temperature gradient is established in the 2DEG by means of a heating current, and then the elevated electron temperature $T_e$ is estimated by measuring the resultant thermovoltage signal across a pair of deferentially biased bar-gates. We adapt a model by Rojek and K\"{o}nig [Phys. Rev. B \textbf{90}, 115403 (2014)] to analyse the thermovoltage signal and as a result extract $\ell$, $T_e$, and the power-law exponent $\alpha_i$ for inelastic scattering events in the 2DEG. We show that in high-mobility 2DEGs, $\ell$ can attain macroscopic values of several hundred microns, but decreases rapidly as the carrier density $n$ is decreased. Our work demonstrates a versatile low-temperature thermometry scheme, and the results provide important insights into heat transport mechanisms in low-dimensional systems and nanostructures. These insights will be vital for practical design considerations of future nanoelectronic circuits.

cond-mat.mes-hall↗

arXiv2014

Stable Magnetic Droplet Solitons in Spin Transfer Nanocontacts

Magnetic thin films with perpendicular magnetic anisotropy (PMA) have localized excitations that correspond to reversed dynamically precessing magnetic moments, known as magnetic droplet solitons. Fundamentally, these excitations are associated with an attractive interaction between elementary spin-excitations (i.e., magnons) and were predicted to occur in PMA materials in the absence of damping [1,2]. While damping, present in all magnetic materials, suppresses these excitations, it is now possible to compensate damping by spin transfer torques through electrical current flow in nanometer scale contacts to ferromagnetic thin films [3,4]. A theory predicts the appearance of magnetic droplet solitons at a threshold current in nanocontacts [5] and, recently, experimental signatures of droplet nucleation have been reported [6]. However, thus far, they have been observed to be nearly reversible excitations, with only partially reversed magnetization and to be subject to instabilities that cause them to drift away from the nanocontacts (i.e., drift instabilities) [6]. Here we show that magnetic droplet solitons can be stabilized in a spin transfer nanocontact. Further, they exhibit a strong hysteretic response to fields and currents and a nearly fully reversed magnetization in the contact. These observations, in addition to their fundamental interest, open up new applications for magnetic droplet solitons as multi-state high frequency current and field tunable oscillators.

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