arXiv subjects

Diyar Talbayev

Publications and source records attributed to Diyar Talbayev.

15 recordsLinked to original sources

arXiv2026

Synthesizing superoscillations with just two frequencies

Superoscillations, band-limited signals that locally oscillate faster than their highest Fourier component, have recently enabled superspectroscopy and super-sensing. Previous experiments [Phys. Rev. Lett. 131, 153803 (2023), https://doi.org/10.1103/PhysRevLett.131.153803 and APL Photonics 10, 086107 (2025), https://doi.org/10.1063/5.0271556] relied on combining four quasi-sinusoidal harmonics to generate temporal superoscillations. Here, we show that just two harmonics are sufficient to produce superoscillations of comparable quality, as quantified by the local frequency. By reanalyzing prior experimental data with two harmonics (0.5 and 0.6 THz) and performing new experiments with 0.9 and 1 THz harmonics, we demonstrate a twofold enhancement in local frequency relative to the highest frequency component -- matching the enhancement previously achieved with four harmonics. We provide a simple analytical explanation for the bichromatic superoscillations based on near-complete destructive interference, and identify an optimal frequency separation of approximately 10% that balances the superoscillatory frequency enhancement against signal amplitude. This simplification substantially lowers the experimental barrier to implementing superoscillation-based technology.

physics.optics↗

arXiv2025

Bose-Einstein condensate sub-wavelength confinement via superoscillations

Optical lattices are essential tools in ultra-cold atomic physics. Here we demonstrate theoretically that sub-wavelength confinement can be achieved in these lattices through superoscillations. This generic wave phenomenon occurs when a local region of the wave oscillates faster than any of the frequencies in its global Fourier decomposition. To illustrate how sub-wavelength confinement can be achieved via superoscillations, we consider a one-dimensional tri-chromatic optical potential confining a spinless Bose-Einstein Condensate of $^{87}$Rb atoms. By numerical optimization of the relative phases and amplitudes of the optical trap's frequency components, it is possible to generate superoscillatory spatial regions. Such regions contain multiple density peaks at sub-wavelength spacing. This work establishes superoscillations as a viable route to sub-wavelength BEC confinement in blue-detuned optical lattices.

cond-mat.quant-gas↗

arXiv2024

Tuning the terahertz response of liquids by creating polar many-body excitations

A surprising result from the theory of quantum control is the degree to which the properties of a physical system can be manipulated. Both atomic and many-body solid state models admit the possibility of creating a 'driven imposter', in which the optical response of one material mimics that of a dynamically distinct system. Here we apply these techniques to polarons in polar liquids. Such quasiparticles describe solvated electrons interacting with many-body degrees of freedom of their environment. The polaron frequency, which depends on the electron concentration in the liquid, is controlled with a pump field, rendering the polaron frequency of three different liquids identical. The experiments demonstrate the feasibility of 'polar impostorons', a so far purely theoretical phenomenon.

quant-ph↗

arXiv2023

Super-sensing: 100-Fold enhancement in THz time-domain spectroscopy contrast via superoscillating waveform shaping

Superoscillations are a phenomenon where a band-limited wave may locally oscillate faster than its highest Fourier component. They are a product of destructive interference between the wave's constituent harmonics. In this article, we demonstrate that superoscillations enable a new functionality in linear optical sensing -- the 100-fold enhancement in the optical contrast of the terahertz wave passing through two similar samples. To achieve this enhancement, we optimize the optical contrast in the time domain in a short observation window by varying the relative phases between the fundamental harmonics that make up the input terahertz wave. We find that the contrast is maximized when the wave intensity is minimized locally within the observation window, which naturally leads to the emergence of the superoscillations. We observe the 100-fold contrast enhancement both in our numerical simulations with Gaussian time-domain harmonics and in our experimental realization with narrow-band quasi-sinusoidal terahertz harmonics. Our results will have profound influence on terahertz sensing and imaging applications in medicine, pharmaceuticals, stand-off hazard detection, and nondestructive evaluation.

physics.optics↗

arXiv2023

Superoscillations Made Super Simple

In ordinary circumstances the highest frequency present in a wave is the highest frequency in its Fourier decomposition. It is however possible for there to be a spatial or temporal region of the wave which locally oscillates at a still greater frequency, in a phenomenon known as superoscillation. Superoscillations find application in wide range of disciplines, but at present their generation is based upon constructive approaches which are difficult to implement. Here we address this, exploiting the fact that superoscillations are a product of destructive interference to produce a prescription for generating superoscillations from the superposition of arbitrary waveforms. As a first test of the technique, we use it to combine four THz laser fields generated by periodically poled Lithium Niobate. From this, we are able to predict and observe for the first time THz optical superoscillations in the temporal domain. The ability to generate superoscillations in this manner has potential application in a wide range of fields. It may for example contribute to the experimental realization of the complex pulses required by quantum control, and the generation of attosecond pulses without resorting to nonlinear processes.

physics.optics↗

arXiv2018

Measurement of quadratic Terahertz optical nonlinearities using second harmonic lock-in detection

We present a method to measure quadratic Terahertz optical nonlinearities in Terahertz time-domain spectroscopy. We use a rotating linear polarizer (a polarizing chopper) to modulate the amplitude of the incident THz pulse train. We use a phase-sensitive lock-in detection at the fundamental and the second harmonic of the modulation frequency to separate the materials' responses that are linear and quadratic in Terahertz electric field. We demonstrate this method by measuring the quadratic Terahertz Kerr effect in the presence of the much stronger linear electro-optic effect in the (110) GaP crystal. We propose that the method can be used to detect Terahertz second harmonic generation in noncentrosymmetric media in time-domain spectroscopy, with broad potential applications in nonlinear Terahertz photonics and related technology.

physics.app-ph↗

arXiv2018

High-temperature terahertz optical diode effect without magnetic order in polar FeZnMo$_3$O$_8$

We present a terahertz spectroscopic study of polar ferrimagnet FeZnMo$_3$O$_8$. Our main finding is a giant high-temperature optical diode effect, or nonreciprocal directional dichroism, where the transmitted light intensity in one direction is over 100 times lower than intensity transmitted in the opposite direction. The effect takes place in the paramagnetic phase with no long-range magnetic order in the crystal, which contrasts sharply with all existing reports of the terahertz optical diode effect in other magnetoelectric materials, where the long-range magnetic ordering is a necessary prerequisite. In \fzmo, the effect occurs resonantly with a strong magnetic dipole active transition centered at 1.27 THz and assigned as electron spin resonance between the eigenstates of the single-ion anisotropy Hamiltonian. We propose that the optical diode effect in paramagnetic FeZnMo$_3$O$_8$ is driven by signle-ion terms in magnetoelectric free energy.

cond-mat.str-el↗

arXiv2017

Giant THz surface plasmon polariton induced by high-index dielectric metasurface

We use computational approaches to explore the role of a high-refractive-index dielectric TiO2 grating with deep subwavelength thickness on InSb as a tunable coupler for THz surface plasmons. We find a series of resonances as the grating couples a normally-incident THz wave to standing surface plasmon waves on both thin and thick InSb layers. In a marked contrast with previously-explored metallic gratings, we observe the emergence of a much stronger additional resonance. The mechanism of this giant plasmonic resonance is well interpreted by the dispersion of surface plasmon excited in the air\TiO2\InSb trilayer system. We demonstrate that both the frequency and the intensity of the giant resonance can be tuned by varying dielectric grating parameters, providing more flexible tunability than metallic gratings. The phase and amplitude of the normally-incident THz wave are spatially modulated by the dielectric grating to optimize the surface plasmon excitation. The giant surface plasmon resonance gives rise to strong enhancement of the electric field above the grating structure, which can be useful in sensing and spectroscopy applications.

physics.app-ph↗

arXiv2017

Terahertz frequency magnetoelectric effect in Ni doped CaBaCo$_4$O$_7$

We present a study of terahertz frequency magnetoelectric effect in ferrimagnetic pyroelectric CaBaCo$_4$O$_7$ and its Ni-doped variants. The terahertz absorption spectrum of these materials consists of spin excitations and low-frequency infrared-active phonons. We studied the magnetic-field-induced changes in the terahertz refractive index and absorption in magnetic fields up to 17 T. We find that the magnetic field modulates the strength of infrared-active optical phonons near 1.2 and 1.6 THz. We use the Lorentz model of the dielectric function to analyze the measured magnetic-field dependence of the refractive index and absorption. We propose that most of the magnetoelectric effect is contributed by the optical phonons near 1.6 THz and higher-frequency resonances. Our experimental results can be used to construct and validate more detailed theoretical descriptions of magnetoelectricity in CaBaCo$_{4-x}$Ni$_x$O$_7$.

cond-mat.str-el↗

arXiv2016

Beyond the effective mass approximation: predictive theory of the nonlinear optical response of conduction electrons

We present an experimental and computational study of the nonlinear optical response of conduction electrons to intense terahertz (THz) electric field. Our observations (saturable absorption and an amplitude-dependent group refractive index) can be understood on the qualitative level as the breakdown of the effective mass approximation. However, a predictive theoretical description of the nonlinearity has been missing. We propose a model based on the semiclassical electron dynamics, a realistic band structure, and the free electron Drude parameters to accurately calculate the experimental observables in InSb. Our results open a path to predictive modeling of the conduction-electron optical nonlinearity in semiconductors, metamaterials, as well as high-field effects in THz plasmonics.

cond-mat.mes-hall↗

arXiv2016

Thin InSb layers with metallic gratings: a novel platform for spectrally-selective THz plasmonic sensing

We present a computational study of terahertz optical properties of a grating-coupled plasmonic structure based on micrometer-thin InSb layers. We find two strong absorption resonances that we interpret as standing surface plasmon modes and investigate their dispersion relations, dependence on InSb thickness, and the spatial distribution of the electric field. The observed surface plasmon modes are well described by a simple theory of the air/InSb/air trilayer. The plasmonic response of the grating/InSb structure is highly sensitive to the dielectric environment and the presence of an analyte (e.g., lactose) at the InSb interface, which is promising for terahertz plasmonic sensor applications. We determine the sensor sensitivity to be 7200 nm per refractive index unit (or 0.06 THz per refractive index unit). The lower surface plasmon mode also exhibits a splitting when tuned in resonance with the vibrational mode of lactose at 1.37 THz. We propose that such interaction between surface plasmon and vibrational modes can be used as the basis for a new sensing modality that allows the detection of terahertz vibrational fingerprints of an analyte.

cond-mat.mes-hall↗

arXiv2016

The role of spin fluctuations in the conductivity of CrO$_2$

We present a time-resolved terahertz spectroscopic study of the half-metallic ferromagnet CrO$_2$. The ultrafast conductivity dynamics excited by an optical pump displays a very short (several picoseconds) and a very long (several hundred picoseconds) characteristic time scales. We attribute the former to the electron-phonon relaxation and the latter to the spin-lattice relaxation. We use this distinction to quantify the relative contribution of the scattering by spin fluctuations to the resistivity of CrO$_2$: we find that they contribute less than one half of all scattering events below room temperature. This contribution rises to $\sim70$ % as the temperature approaches $T_C$=390 K. The small effect of spin fluctuations on the resistivity is unexpected in the light of the proposed double-exchange nature of the electronic and magnetic properties of CrO$_2$.

cond-mat.str-el↗

arXiv2015

Novel Layered Iridate Ba7Ir3O13+δ Thin Films with Colossal Permittivity

Ba7Ir3O13+δ in thin film form is discovered. These films are characterized by colossal permittivity (CP) ~104 at room temperature, attributable to the colossal internal barrier layer capacitance effect at atomically thin domain boundaries. These findings suggest a new route to seeking novel CP materials through designing atomically thin domain boundaries.

cond-mat.mtrl-sci↗

arXiv2014

Spin-dependent polaron formation dynamics in Eu$_{0.75}$Y$_{0.25}$MnO$_3$ probed by femtosecond pump-probe spectroscopy

We present a femtosecond optical pump-probe study of the multiferroic manganite Eu$_{0.75}$Y$_{0.25}$MnO$_3$. The optical response of the material at pump energies of 1.55 and 3.1 eV is dominated by the $d$-$d$ and $p$-$d$ transitions of the Mn$^{3+}$ ions. The relaxation of photoexcited electrons includes the relaxation of the Jahn-Teller distortion and polaron trapping at Mn$^{2+}$ and Mn$^{4+}$ sites. Ultrafast switching of superexchange interactions due to modulated $e_g$ orbital occupancy creates a localized spin excitation, which then decays on a time scale of tens of picoseconds at low temperatures. The localized spin state decay appears as a tremendous increase in the amplitude of the photoinduced reflectance, due to the strong coupling of optical transitions to the spin-spin correlations in the crystalline $a$-$b$ plane.

cond-mat.str-el↗

arXiv2006

Large Nonlinear Kerr Angle in non-Centrosymmetric Fe/AlGaAs (001)Heterostructure

A large nonlinear magneto-optical effect is observed in a non-centrosymmetric Fe/AlGaAs (001) heterostructure. This effect is a direct consequence of interference between second-harmonic optical waves of magnetic and crystallographic origin, generated at ferromagnetic Fe interface and bulk AlGaAs, respectively. The longitudinal nonlinear Kerr rotation is measured to be 1.6 degrees along the [1-10] hard axis, about two orders of magnitude stronger than the linear equivalent. The rotational second-harmonic signal shows large magnetic contrast along all the in-plane directions, demonstrating a high sensitivity to the magnetization of an anisotropic interface in the longitudinal geometry.

cond-mat.mtrl-sci↗