arXiv subjects

Dmitri E. Nikonov

Publications and source records attributed to Dmitri E. Nikonov.

At least 19 recordsLinked to original sources

arXiv2026

A Magnon-Based Electric Field Controlled Magnetoelectric Device for Energy-Efficient Logic-in-Memory

We demonstrate a non-volatile magnetoelectric magnonic memory (MEMM) that enables fully electrical write/read via direct magnon-driven sensing in an insulating antiferromagnet. A fabricated SrIrO3/La-BiFeO3/SrIrO3 trilayer exhibits sub-100 ps switching, a remnant polarization of 20 uC/cm2, and a readout voltage contrast close to 1mV between high and low-resistance states. To connect device physics to circuit behavior, we develop and experimentally validate a compact circuit model that captures spin Hall injection and spin transport. Simulations with optimized material parameters predict output voltages > 100mV, enabling cascading without external amplification. Using this framework, we design MEMM-based memory and logic blocks, including a 1T1R array, two inverter implementations (complementary two-device and single-device), and a three-input majority gate, and evaluate deep-pipelined operation. The model projects switching energies down to 1 aJ per operation and logic propagation delays of 30-60 ps, indicating MEMM as a promising platform for energy-constrained, high throughput computing.

cond-mat.mtrl-sci↗

arXiv2026

Solid-state transcapacitor, a new gain element for logic, memory and interconnects

Today's transistors dictate the voltage and charge scales for both logic and memory. While AI systems are recognized to be limited by memory energy, the dominant share of the energy is expended in the intrachip interconnects whose voltage and charge scales are set by transistors. The energy scaling challenges of transistors can be attributed to simultaneously meeting high current density, high current/impedance modulation, and the inability to lower voltages. Hence, a new logic element that lowers the voltage and charge needs is a priority, not only for lowering logic power but also memory access power. Here, we propose a novel 3-terminal logic element for low energy computing, a solid-state transcapacitor (TCAP). A TCAP is a solid state displacement current modulator realized by a gate which controls the charge-voltage relationship of the channel. Unlike transistors, TCAPs eliminate the dissipative transport current, are not bound by the Boltzmann current modulation limit, and operate with displacement currents limited only by the polarization response and contact resistance. Hence, TCAP circuits may simultaneously overcome the voltage, current density, and current modulation limits of CMOS. We describe a solid state TCAP using a piezoelectric transcapacitor in which a gate-controlled stressor modulates the capacitance of a polar channel via electromechanical coupling. This device achieves inversion and gain, essential for logic, and is functionally equivalent to a 1T-1C memory cell, enabling dense memory. Using voltage scaling, capacitive energy recovery, and high polarization densities of polar materials, the logic based on TCAP offers a pathway to 100 fold lower energy consumption with a delay comparable to ultimately scaled CMOS devices. This approach provides a new potential pathway for low-energy computing beyond the limits of transistors using electro-mechanics and multiferroics.

cond-mat.mes-hall↗

arXiv2024

Voltage-based magnetization switching and reading in magnetoelectric spin-orbit nanodevices

As CMOS technologies face challenges in dimensional and voltage scaling, the demand for novel logic devices has never been greater, with spin-based devices offering scaling potential, at the cost of significantly high switching energies. Alternatively, magnetoelectric materials are predicted to enable low-power magnetization control, a solution with limited device-level results. Here, we demonstrate voltage-based magnetization switching and reading in nanodevices at room temperature, enabled by exchange coupling between multiferroic BiFeO$_3$ and ferromagnetic CoFe, for writing, and spin-to-charge current conversion between CoFe and Pt, for reading. We show that upon the electrical switching of the BiFeO$_3$, the magnetization of the CoFe can be reversed, giving rise to different voltage outputs. Through additional microscopy techniques, magnetization reversal is linked with the polarization state and antiferromagnetic cycloid propagation direction in the BiFeO$_3$. This study constitutes the building block for magnetoelectric spin-orbit logic, opening a new avenue for low-power beyond-CMOS technologies.

cond-mat.mes-hall↗

arXiv2023

Understanding magnetoelectric switching in BiFeO$_3$ thin films

In this work we use a phenomenological theory of ferroelectric switching in BiFeO$_3$ thin films to uncover the mechanism of the two-step process that leads to the reversal of the weak magnetization of these materials. First, we introduce a realistic model of a BiFeO$_3$ film, including the Landau energy of isolated domains as well as the constraints that account for the presence of the substrate and the multidomain configuration found experimentally. We use this model to obtain statistical information about the switching behavior - by running dynamical simulations based on the Landau-Khalatnikov time-evolution equation, including thermal fluctuations - and we thus identify the factors that drive the two-step polarization reversal observed in the experiments. Additionally, we apply our model to test potential strategies for optimizing the switching characteristics.

cond-mat.mtrl-sci↗

arXiv2022

Efficient Optimization with Higher-Order Ising Machines

A prominent approach to solving combinatorial optimization problems on parallel hardware is Ising machines, i.e., hardware implementations of networks of interacting binary spin variables. Most Ising machines leverage second-order interactions although important classes of optimization problems, such as satisfiability problems, map more seamlessly to Ising networks with higher-order interactions. Here, we demonstrate that higher-order Ising machines can solve satisfiability problems more resource-efficiently in terms of the number of spin variables and their connections when compared to traditional second-order Ising machines. Further, our results show on a benchmark dataset of Boolean \textit{k}-satisfiability problems that higher-order Ising machines implemented with coupled oscillators rapidly find solutions that are better than second-order Ising machines, thus, improving the current state-of-the-art for Ising machines.

cs.ET↗

arXiv2022

All-electrical spin-to-charge conversion in sputtered Bi$_x$Se$_{1-x}$

One of the major obstacles to realizing spintronic devices such as MESO logic devices is the small signal magnitude used for magnetization readout, making it important to find materials with high spin-to-charge conversion efficiency. Although intermixing at the junction of two materials is a widely occurring phenomenon, its influence on material characterization and the estimation of spin-to-charge conversion efficiencies is easily neglected or underestimated. Here, we demonstrate all electrical spin-to-charge conversion in Bi$_x$Se$_{1-x}$ nanodevices and show how the conversion efficiency can be overestimated by tens of times depending on the adjacent metal used as a contact. We attribute this to the intermixing-induced compositional change and the properties of a polycrystal that lead to drastic changes in resistivity and spin Hall angle. Strategies to improve the spin-to-charge conversion signal in similar structures for functional devices are discussed.

cond-mat.mes-hall↗

arXiv2022

First-principles Landau-like potential for BiFeO$_3$ and related materials

In this work we introduce the simplest, lowest-order Landau-like potential for BiFeO$_3$ and La-doped BiFeO$_3$ as an expansion around the paraelectric cubic phase in powers of polarization, FeO$_6$ octahedral rotations and strains. We present an analytical approach for computing the model parameters from density functional theory. We illustrate our approach by computing the potentials for BiFeO$_3$ and La$_{0.25}$Bi$_{0.75}$FeO$_3$ and show that, overall, we are able to capture the first-principles results accurately. The computed models allow us to identify and explain the main interactions controlling the relative stability of the competing low-energy phases of these compounds.

cond-mat.mtrl-sci↗

arXiv2022

Integer Factorization with Compositional Distributed Representations

In this paper, we present an approach to integer factorization using distributed representations formed with Vector Symbolic Architectures. The approach formulates integer factorization in a manner such that it can be solved using neural networks and potentially implemented on parallel neuromorphic hardware. We introduce a method for encoding numbers in distributed vector spaces and explain how the resonator network can solve the integer factorization problem. We evaluate the approach on factorization of semiprimes by measuring the factorization accuracy versus the scale of the problem. We also demonstrate how the proposed approach generalizes beyond the factorization of semiprimes; in principle, it can be used for factorization of any composite number. This work demonstrates how a well-known combinatorial search problem may be formulated and solved within the framework of Vector Symbolic Architectures, and it opens the door to solving similarly difficult problems in other domains.

cs.NE↗

arXiv2021

Physics-Based Models for Magneto-Electric Spin-Orbit Logic Circuits

Spintronic devices are a promising beyond-CMOS device option thanks to their energy efficiency and compatibility with CMOS. To accurately capture their multi-physics dynamics, a rigorous treatment of both spin and charge and their inter-conversion is required. Here we present physics-based device models based on 4x4 matrices for the spin-orbit coupling part of the magneto-electric spin-orbit (MESO) device. Also, a more rigorous physics model of ferroelectric and magnetoelectric switching of ferromagnets, based on Landau-Lifshitz-Gilbert (LLG) and Landau-Khalatnikov (LK) equations, is presented. With the combined model implemented in a SPICE circuit simulator environment, simulation results were obtained which show feasibility of MESO implementation and functional operation of buffers, oscillators, and majority gates.

cond-mat.mes-hall↗

arXiv2021

Spin-charge interconversion in KTaO$_3$ two-dimensional electron gases

Oxide interfaces exhibit a broad range of physical effects stemming from broken inversion symmetry. In particular, they can display non-reciprocal phenomena when time reversal symmetry is also broken, e.g., by the application of a magnetic field. Examples include the direct and inverse Edelstein effects (DEE, IEE) that allow the interconversion between spin currents and charge currents. The DEE and IEE have been investigated in interfaces based on the perovskite SrTiO$_3$ (STO), albeit in separate studies focusing on one or the other. The demonstration of these effects remains mostly elusive in other oxide interface systems despite their blossoming in the last decade. Here, we report the observation of both the DEE and IEE in a new interfacial two-dimensional electron gas (2DEG) based on the perovskite oxide KTaO$_3$. We generate 2DEGs by the simple deposition of Al metal onto KTaO$_3$ single crystals, characterize them by angle-resolved photoemission spectroscopy and magnetotransport, and demonstrate the DEE through unidirectional magnetoresistance and the IEE by spin-pumping experiments. We compare the spin-charge interconversion efficiency with that of STO-based interfaces, relate it to the 2DEG electronic structure, and give perspectives for the implementation of KTaO$_3$ 2DEGs into spin-orbitronic devices.

cond-mat.mes-hall↗

arXiv2021

Metal/SrTiO$_3$ two-dimensional electron gases for spin-to-charge conversion

SrTiO$_3$-based two-dimensional electron gases (2DEGs) can be formed through the deposition of epitaxial oxides like LaAlO$_3$ or of reactive metals such as Al. Such 2DEGs possess a finite Rashba spin-orbit coupling that has recently been harnessed to interconvert charge and spin currents through the direct and inverse Edelstein and spin Hall effects. Here we compare the formation and properties of 2DEGs generated in SrTiO$_3$ by the growth of Al, Ta and Y ultrathin films by magnetron sputtering. By combining in situ and ex situ X-ray photoelectron spectroscopy (XPS) we gain insight into the reduction of the SrTiO$_3$ and the appearance of Ti$^{3+}$ states associated with 2DEG formation, its reoxidation by exposure to the air, and the transformation of the metal into its binary oxides. We extract the carrier densities through magnetotransport and compare them with the XPS data. Finally, working with samples covered by an extra layer of NiFe, we perform spin-pumping ferromagnetic resonance experiments and investigate spin-charge conversion as a function of gate voltage. We identify trends in the data across the different sample systems and discuss them as a function of the carrier density and the transparency of the metal oxide tunnel barrier.

cond-mat.mes-hall↗

arXiv2020

Physical Mechanism behind the Hysteresis-free Negative Capacitance Effect in Metal-Ferroelectric-Insulator-Metal Capacitors with Dielectric Leakage and Interfacial Trapped Charges

The negative capacitance (NC) stabilization of a ferroelectric (FE) material can potentially provide an alternative way to further reduce the power consumption in ultra-scaled devices and thus has been of great interest in technology and science in the past decade. In this article, we present a physical picture for a better understanding of the hysteresis-free charge boost effect observed experimentally in metal-ferroelectric-insulator-metal (MFIM) capacitors. By introducing the dielectric (DE) leakage and interfacial trapped charges, our simulations of the hysteresis loops are in a strong agreement with the experimental measurements, suggesting the existence of an interfacial oxide layer at the FE-metal interface in metal-ferroelectric-metal (MFM) capacitors. Based on the pulse switching measurements, we find that the charge enhancement and hysteresis are dominated by the FE domain viscosity and DE leakage, respectively. Our simulation results show that the underlying mechanisms for the observed hysteresis-free charge enhancement in MFIM may be physically different from the alleged NC stabilization and capacitance matching. Moreover, the link between Merz's law and the phenomenological kinetic coefficient is discussed, and the possible cause of the residual charges observed after pulse switching is explained by the trapped charge dynamics at the FE-DE interface. The physical interpretation presented in this work can provide important insights into the NC effect in MFIM capacitors and future studies of low-power logic devices.

physics.app-ph↗

arXiv2020

A micromagnetic study of the switching dynamics of the BiFeO$_3$/CoFe heterojunction

The switching dynamics of a single-domain BiFeO3/CoFe heterojunction is modeled and key parameters such as interface exchange coupling coefficient are extracted from experimental results. The lower limit of the magnetic order response time of CoFe in the BiFeO3/CoFe heterojunction is theoretically quantified to be on to the order of 100 ps. Our results indicate that the switching behavior of CoFe in the BiFeO3/CoFe heterojunction is dominated by the rotation of the Neel vector in BiFeO3 rather than the unidirectional exchange bias at the interface. We also quantify the magnitude of the interface exchange coupling coefficient J_int to be 0.32 pJ/m by comparing our simulation results with the giant magnetoresistance (GMR) curves and the magnetic hysteresis loop in the experiments. To the best of our knowledge, this is the first time that J_int is extracted quantitatively from experiments. Furthermore, we demonstrate that the switching success rate and the thermal stability of the BiFeO3/CoFe heterojunction can be improved by reducing the thickness of CoFe and increasing the length to width aspect ratio of the BiFeO3/CoFe heterojunction. Our theoretical model provides a comprehensive framework to study the magnetoelectric properties and the manipulation of the magnetic order of CoFe in the BiFeO3/CoFe heterojunction.

cond-mat.mtrl-sci↗

arXiv2020

Spin-orbit magnetic state readout in scaled ferromagnetic/heavy metal nanostructures

Efficient detection of the magnetic state at nanoscale dimensions is an important step to utilize spin logic devices for computing. Magnetoresistance effects have been hitherto used in magnetic state detection, but they suffer from energetically unfavorable scaling and do not generate an electromotive force that can be used to drive a circuit element for logic device applications. Here, we experimentally show that a favorable miniaturization law is possible via the use of spin-Hall detection of the in-plane magnetic state of a magnet. This scaling law allows us to obtain a giant signal by spin Hall effect in CoFe/Pt nanostructures and quantify an effective spin-to-charge conversion rate for the CoFe/Pt system. The spin-to-charge conversion can be described as a current source with an internal resistance, i.e., it generates an electromotive force that can be used to drive computing circuits. We predict that the spin-orbit detection of magnetic states can reach high efficiency at reduced dimensions, paving the way for scalable spin-orbit logic devices and memories.

cond-mat.mes-hall↗

arXiv2019

Multi-domain Characterization of Ferroelectric Switching Dynamics with a Physics-based SPICE Circuit Model for Phase Field Simulations

In this paper, the multi-domain nature of ferroelectric (FE) polarization switching dynamics in a metal-ferroelectric-metal (MFM) capacitor is explored through a physics-based phase field approach, where the three-dimensional time-dependent Ginzburg-Landau (TDGL) equation and Poisson's equation are self-consistently solved with the SPICE simulator. Systematically calibrated based on the experimental measurements, the model well captures transient negative capacitance in pulse switching dynamics, with domain interaction and viscosity being the key parameters. It is found that the influence of pulse amplitudes on voltage transient behaviors can be attributed to the fact that the FE free energy profile strongly depends on how the domains are interacted. This finding has an important implication on the charge-boost induced by stabilization of negative capacitance in an FE + dielectric (DE) stack since the so-called capacitance matching needs to be designed at a specific operation voltage or frequency. In addition, we extract the domain viscosity dynamics during polarization switching according to the experimental measurements. For the first time, a physics-based circuit-compatible SPICE model for multi-domain phase field simulations is established to reveal the effect of domain interaction on the FE energy profile and microscopic domain evolution.

physics.app-ph↗

arXiv2019

Benchmarking Physical Performance of Neural Inference Circuits

Numerous neural network circuits and architectures are presently under active research for application to artificial intelligence and machine learning. Their physical performance metrics (area, time, energy) are estimated. Various types of neural networks (artificial, cellular, spiking, and oscillator) are implemented with multiple CMOS and beyond-CMOS (spintronic, ferroelectric, resistive memory) devices. A consistent and transparent methodology is proposed and used to benchmark this comprehensive set of options across several application cases. Promising architecture/device combinations are identified.

cs.ET↗

arXiv2019

Simulation of the Magnetization Dynamics of a Single Domain BiFeO$_3$ Thin Film

The switching dynamics of a single-domain BiFeO$_3$ thin films is investigated through combining the dynamics of polarization and Neel vector. The evolution of the ferroelectric polarization is described by the Landau-Khalatnikov (LK) equation, and the Landau-Lifshitz-Gilbert (LLG) equations for spins in two sublattices to model the time evolution of the antiferromagnetic order (Neel vector) in a G-type antiferromagnet. This work theoretically demonstrates that due to the rotation of the magnetic hard axis following the polarization reversal, the Neel vector can be switched by 180 degrees, while the weak magnetization can remain unchanged. The simulation results are consistent with the ab initio calculation, where the Neel vector rotates during polarization rotation, and also match our calculation of the dynamics of order parameter using Landau-Ginzburg theory. We also find that the switching time of the Neel vector is determined by the speed polarization switching and is predicted to be as short as 30 ps.

cond-mat.mes-hall↗

arXiv2018

Inversion Charge-boost and Transient Steep-slope induced by Free charge-polarization Mismatch in a Ferroelectric-metal-oxide-semiconductor Capacitor

In this letter, the transient behavior of a ferroelectric (FE) metal-oxide-semiconductor (MOS) capacitor is theoretically investigated with a series resistor. It is shown that compared to a conventional high-k dielectric MOS capacitor, a significant inversion charge-boost can be achieved by a FE MOS capacitor due to a steep transient subthreshold swing (SS) driven by the free charge-polarization mismatch. It is also shown that the observation of steep transient SS significantly depends on the viscosity coefficient under Landau's mean field theory, in general representing the average FE time response associated with domain nucleation and propagation. Therefore, this letter not only establishes a theoretical framework that describes the physical origin behind the inversion charge-boost in a FE MOS capacitor, but also shows that the key feature of depolarization effect on a FE MOS capacitor should be the inversion-charge boost, rather than the steep SS (e.g., sub-60mV/dec at room temperature), which cannot be experimentally observed as the measurement time is much longer than the FE response. Finally, we outlines the required material targets for the FE response in field-effect transistors to be applicable for next-generation high-speed and low-power digital switches.

physics.app-ph↗