arXiv subjects

Dmitri K. Efetov

Publications and source records attributed to Dmitri K. Efetov.

At least 37 records · Page 2Linked to original sources

arXiv2022

Quantum critical behavior in magic-angle twisted bilayer graphene

The flat bands of magic-angle twisted bilayer graphene (MATBG) host strongly-correlated electronic phases such as correlated insulators, superconductors and a strange-metal state. The latter state, believed to be key for understanding the electronic properties of MATBG, is obscured by various phase transitions and thus could not be unequivocally differentiated from a metal undergoing frequent electron-phonon collisions. Here, we report transport measurements in superconducting MATBG in which the correlated insulator states are suppressed by screening. The uninterrupted metallic ground state shows resistivity that is linear in temperature over three decades and spans a broad range of doping including those where a correlation-driven Fermi surface reconstruction occurs. This strange-metal behavior is distinguished by Planckian scattering rates and a linear magnetoresistivity. In contrast, near charge neutrality or a fully-filled flat band, as well as for devices twisted away from the magic angle, we observe the archetypal Fermi liquid behavior. Our measurements demonstrate the existence of a quantum critical phase whose fluctuations dominate the metallic ground state throughout a continuum of doping. Further, we observe a transition to the strange metal upon suppression of the superconducting order, suggesting a relationship between quantum fluctuations and superconductivity in MATBG.

cond-mat.str-el↗

arXiv2022

Materials and devices for fundamental quantum science and quantum technologies

Technologies operating on the basis of quantum mechanical laws and resources such as phase coherence and entanglement are expected to revolutionize our future. Quantum technologies are often divided into four main pillars: computing, simulation, communication, and sensing & metrology. Moreover, a great deal of interest is currently also nucleating around energy-related quantum technologies. In this Perspective, we focus on advanced superconducting materials, van der Waals materials, and moiré quantum matter, summarizing recent exciting developments and highlighting a wealth of potential applications, ranging from high-energy experimental and theoretical physics to quantum materials science and energy storage.

quant-ph↗

arXiv2021

Observation of re-entrant correlated insulators and interaction driven Fermi surface reconstructions at one magnetic flux quantum per moiré unit cell in magic-angle twisted bilayer graphene

The discovery of flat bands with non-trivial band topology in magic angle twisted bi-layer graphene (MATBG) has provided a unique platform to study strongly correlated phe-nomena including superconductivity, correlated insulators, Chern insulators and magnetism. A fundamental feature of the MATBG, so far unexplored, is its high magnetic field Hof-stadter spectrum. Here we report on a detailed magneto-transport study of a MATBG de-vice in external magnetic fields of up to B = 31 T, corresponding to one magnetic flux quan-tum per moiré unit cell Φ0. At Φ0, we observe a re-entrant correlated insulator at a flat band filling factor of ν = +2, and interaction-driven Fermi surface reconstructions at other fillings, which are identified by new sets of Landau levels originating from these. These ex-perimental observations are supplemented by theoretical work that predicts a new set of 8 well-isolated flat bands at Φ0 , of comparable band width but with different topology than in zero field. Overall, our magneto-transport data reveals a qualitatively new Hofstadter spec-trum in MATBG, which arises due to the strong electronic correlations in the re-entrant flat bands.

cond-mat.str-el↗

arXiv2021

Reentrant Correlated Insulators in Twisted Bilayer Graphene at 25T ($2π$ Flux)

Twisted bilayer graphene (TBG) is remarkable for its topological flat bands, which drive strongly-interacting physics at integer fillings, and its simple theoretical description facilitated by the Bistritzer-MacDonald Hamiltonian, a continuum model coupling two Dirac fermions. Due to the large moiré unit cell, TBG offers the unprecedented opportunity to observe reentrant Hofstadter phases in laboratory-strength magnetic fields near $25$T. This Letter is devoted to magic angle TBG at $2π$ flux where the magnetic translation group commutes. We use a newly developed gauge-invariant formalism to determine the exact single-particle band structure and topology. We find that the characteristic TBG flat bands reemerge at $2π$ flux, but, due to the magnetic field breaking $C_{2z} \mathcal{T}$, they split and acquire Chern number $\pm1$. We show that reentrant correlated insulating states appear at $2π$ flux driven by the Coulomb interaction at integer fillings, and we predict the characteristic Landau fans from their excitation spectrum. We conjecture that superconductivity can also be re-entrant at $2π$ flux.

cond-mat.str-el↗

arXiv2021

Magnetic Josephson Junctions and Superconducting Diodes in Magic Angle Twisted Bilayer Graphene

The simultaneous co-existence and gate-tuneability of the superconducting (SC), magnetic and topological orders in magic angle twisted bilayer graphene (MATBG) open up entirely new possibilities for the creation of complex hybrid Josephson junctions (JJ). Here we report on the creation of gate-defined, magnetic Josephson junctions in MATBG, where the weak link is gate-tuned close to the correlated state at a moiré filling factor of ν=-2. A highly unconventional Fraunhofer pattern emerges, which is phase-shifted and asymmetric with respect to the current and magnetic field directions, and shows a pronounced magnetic hysteresis. Interestingly, our theoretical calculations of the JJ with a valley polarized ν=-2 with orbital magnetization as the weak link explain most of these unconventional features without fine tuning the parameters. While these unconventional Josephson effects persist up to the critical temperature Tc ~ 3.5K of the superconducting state, at temperatures below T < 800mK, we observed a pronounced magnetic hysteresis possibly due to further spin-polarization of the ν=-2 state. We demonstrate how the combination of magnetization and its current induced magnetization switching in the MATBG JJ allows us to realize a programmable zero field superconducting diode, which represents a major building block for a new generation of superconducting quantum electronics.

cond-mat.supr-con↗

arXiv2021

Measuring local moiré lattice heterogeneity of twisted bilayer graphene

We introduce a new method to continuously map inhomogeneities of a moiré lattice and apply it to large-area topographic images we measure on open-device twisted bilayer graphene (TBG). We show that the variation in the twist angle of a TBG device, which is frequently conjectured to be the reason for differences between devices with a supposed similar twist angle, is about 0.08° around the average of 2.02° over areas of several hundred nm, comparable to devices encapsulated between hBN slabs. We distinguish between an effective twist angle and local anisotropy and relate the latter to heterostrain. Our results imply that for our devices, twist angle heterogeneity has a roughly equal effect to the electronic structure as local strain. The method introduced here is applicable to results from different imaging techniques, and on different moiré materials.

cond-mat.mes-hall↗

arXiv2020

Competing zero-field Chern insulators in Superconducting Twisted Bilayer Graphene

The discovery of magic angle twisted bilayer graphene (MATBG) has unveiled a rich variety of superconducting, magnetic and topologically nontrivial phases. The existence of all these phases in one material, and their tunability, has opened new pathways for the creation of unusual gate tunable junctions. However, the required conditions for their creation - gate induced transitions between phases in zero magnetic field - have so far not been achieved. Here, we report on the first experimental demonstration of a device that is both a zero-field Chern insulator and a superconductor. The Chern insulator occurs near moire cell filling factor v = +1 in a hBN non-aligned MATBG device and manifests itself via an anomalous Hall effect. The insulator has Chern number C = +-1 and a relatively high Curie temperature of Tc = 4.5 K. Gate tuning away from this state exposes strong superconducting phases with critical temperatures of up to Tc = 3.5 K. In a perpendicular magnetic field above B > 0.5 T we observe a transition of the /C/= +1 Chern insulator from Chern number C = +-1 to C = 3, characterized by a quantized Hall plateau with Ryx = h/3e2. These observations show that interaction-induced symmetry breaking in MATBG leads to zero-field ground states that include almost degenerate and closely competing Chern insulators, and that states with larger Chern numbers couple most strongly to the B-field. By providing the first demonstration of a system that allows gate-induced transitions between magnetic and superconducting phases, our observations mark a major milestone in the creation of a new generation of quantum electronics.

cond-mat.mes-hall↗

arXiv2020

Ultra-fast calorimetric measurements of the electronic heat capacity of graphene

Heat capacity is an invaluable quantity in condensed matter physics, yet it has been so far experimentally inaccessible in two-dimensional (2D) van der Waals (vdW) materials, owing to their ultra-fast thermal relaxation times and the lack of suitable nano-scale thermometers. Here, we demonstrate a novel thermal relaxation calorimetry scheme that allows the first measurements of the electronic heat capacity of graphene Ce. It is enabled by the grouping of a radio-frequency Johnson noise thermometer, which can measure the electronic temperature Te with a measurement sensitivity of δTe ~ 20 mK, and an ultra-fast photo-mixed optical heater, which can simultaneously modulate Te with a frequency of up to Ω=0.2 THz. This combination allows record sensitive and record fast measurements of the electronic heat capacity Ce < 10^(-19) J/K, with an electronic thermal relaxation time τe < 10^(-13), representing orders of magnitude improvements as compared to previous state-of-the-art calorimeters. These features embody a breakthrough in heat capacity metrology of nano-scale and low-dimensional systems, and provide a new avenue for the investigation of their thermodynamic quantities.

cond-mat.mes-hall↗

arXiv2020

Untying the insulating and superconducting orders in magic-angle graphene

The coexistence of superconducting and correlated insulating states in magic-angle twisted bilayer graphene prompts fascinating questions about the relationship of these orders. Independent control of the microscopic mechanisms governing these phases could help uncover their individual roles and shed light on their intricate interplay. Here we report on direct tuning of electronic interactions in this system by changing its separation from a metallic screening layer. We observe quenching of correlated insula-tors in devices with screening layer separations that are smaller than a typical Wannier orbital size of 15nm, and with the twist angles slightly deviating from the magic value 1.10 plus(minus) 0.05 degrees. Upon extinction of the insulating orders, the vacated phase space is taken over by superconducting domes that feature critical temperatures comparable to those in the devices with strong insulators. In addition, we find that insulators at half-filling can reappear in small out-of-plane magnetic fields of 0.4 T, giving rise to quantized Hall states with a Chern number of 2. Our study suggests reexamination of the often-assumed mother-child relation between the insulating and superconducting phases in moire graphene, and illustrates a new approach to directly probe microscopic mechanisms of superconductivity in strongly-correlated systems.

cond-mat.supr-con↗

arXiv2020

Multiple Flat Bands and Topological Hofstadter Butterfly in Twisted Bilayer Graphene Close to the Second Magic Angle

Moiré superlattices in two-dimensional (2D) van der Waals (vdW) heterostructures provide 20 an efficient way to engineer electron band properties. The recent discovery of exotic quantum phases and their interplay in twisted bilayer graphene (tBLG) has built this moiré system one of the most renowned condensed matter platforms (1-10). So far the studies of tBLG has been mostly focused on the lowest two flat moiré bands at the first magic angle θm1 ~ 1.1°, leaving high-order moiré bands and magic angles largely unexplored. Here we report 25 an observation of multiple well-isolated flat moiré bands in tBLG close to the second magic angle θm2 ~ 0.5°, which cannot be explained without considering electron-election interactions. With high magnetic field magneto-transport measurements, we further reveal a qualitatively new, energetically unbound Hofstadter butterfly spectrum in which continuously extended quantized Landau level gaps cross all trivial band-gaps. The 30 connected Hofstadter butterfly strongly evidences the topologically nontrivial textures of the multiple moiré bands. Overall, our work provides a new perspective for understanding the quantum phases in tBLG and the fractal Hofstadter spectra of multiple topological bands.

cond-mat.mes-hall↗

arXiv2020

Graphene-based Josephson junction microwave bolometer

Sensitive microwave detectors are critical instruments in radioastronomy, dark matter axion searches, and superconducting quantum information science. The conventional strategy towards higher-sensitivity bolometry is to nanofabricate an ever-smaller device to augment the thermal response. However, this direction is increasingly more difficult to obtain efficient photon coupling and maintain the material properties in a device with a large surface-to-volume ratio. Here we advance this concept to an ultimately thin bolometric sensor based on monolayer graphene. To utilize its minute electronic specific heat and thermal conductivity, we develop a superconductor-graphene-superconductor (SGS) Josephson junction bolometer embedded in a microwave resonator of resonant frequency 7.9 GHz with over 99\% coupling efficiency. From the dependence of the Josephson switching current on the operating temperature, charge density, input power, and frequency, we demonstrate a noise equivalent power (NEP) of 7 $\times 10^{-19}$ W/Hz$^{1/2}$, corresponding to an energy resolution of one single photon at 32 GHz and reaching the fundamental limit imposed by intrinsic thermal fluctuation at 0.19 K.

cond-mat.mes-hall↗

arXiv2020

Josephson-junction infrared single-photon detector

Josephson junctions (JJs) are ubiquitous superconducting devices, enabling high sensitivity magnetometers and voltage amplifiers, as well as forming the basis of high performance cryogenic computer and superconducting quantum computers. While JJ performance can be degraded by quasiparticles (QPs) formed from broken Cooper pairs, this phenomenon also opens opportunities to sensitively detect electromagnetic radiation. Here we demonstrate single near-infrared photon detection by coupling photons to the localized surface plasmons of a graphene-based JJ. Using the photon-induced switching statistics of the current-biased JJ, we reveal the critical role of QPs generated by the absorbed photon in the detection mechanism. The photon-sensitive JJ will enable a high-speed, low-power optical interconnect for future JJ-based computing architectures.

quant-ph↗

arXiv2020

High-order minibands and interband Landau level reconstruction in graphene moire superlattice

The propagation of Dirac fermions in graphene through a long-period periodic potential would result in a band folding together with the emergence of a series of cloned Dirac points (DPs). In highly aligned graphene/hexagonal boron nitride (G/hBN) heterostructures, the lattice mismatch between the two atomic crystals generates a unique kind of periodic structure known as a moiré superlattice. Of particular interests is the emergent phenomena related to the reconstructed band-structure of graphene, such as the Hofstadter butterfly, topological currents, gate dependent pseudospin mixing, and ballistic miniband conduction. However, most studies so far have been limited to the lower-order minibands, e.g. the 1st and 2nd minibands counted from charge neutrality, and consequently the fundamental nature of the reconstructed higher-order miniband spectra still remains largely unknown. Here we report on probing the higher-order minibands of precisely aligned graphene moiré superlattices by transport spectroscopy. Using dual electrostatic gating, the edges of these high-order minibands, i.e. the 3rd and 4th minibands, can be reached. Interestingly, we have observed interband Landau level (LL) crossinginducing gap closures in a multiband magneto-transport regime, which originates from band overlap between the 2nd and 3rd minibands. As observed high-order minibands and LL reconstruction qualitatively match our simulated results. Our findings highlight the synergistic effect of minibands in transport, thus presenting a new opportunity for graphene electronic devices.

cond-mat.mes-hall↗

arXiv2020

Symmetry broken Chern insulators and magic series of Rashba-like Landau level crossings in magic angle bilayer graphene

Flat-bands in magic angle twisted bilayer graphene (MATBG) have recently emerged as a rich platform to explore strong correlations, superconductivity and mag-netism. However, the phases of MATBG in magnetic field, and what they reveal about the zero-field phase diagram remain relatively unchartered. Here we use magneto-transport and Hall measurements to reveal a rich sequence of wedge-like regions of quantized Hall conductance with Chern numbers C = +(-)1, +(-)2, +(-)3, +(-)4 which nucleate from integer fillings of the moire unit cell v = +(-)3, +(-)2, +(-)1, 0 correspondingly. We interpret these phases as spin and valley polarized Chern insulators, equivalent to quantum Hall ferro-magnets. The exact sequence and correspondence of Chern numbers and filling factors suggest that these states are driven directly by electronic interactions which specifically break time-reversal symmetry in the system. We further study quantum magneto-oscillation in the yet unexplored higher energy dispersive bands with a Rashba-like dis-persion. Analysis of Landau level crossings enables a parameter-free comparison to a newly derived magic series of level crossings in magnetic field and provides constraints on the parameters w0 and w1 of the Bistritzer-MacDonald MATBG Hamiltonian. Over-all, our data provides direct insights into the complex nature of symmetry breaking in MATBG and allows for quantitative tests of the proposed microscopic scenarios for its electronic phases.

cond-mat.str-el↗

arXiv2020

A liquid nitrogen cooled superconducting transition edge sensor with ultra-high responsivity and GHz operation speeds

Photodetectors based on nano-structured superconducting thin films are currently some of the most sensitive quantum sensors and are key enabling technologies in such broad areas as quantum information, quantum computation and radio-astronomy. However, their broader use is held back by the low operation temperatures which require expensive cryostats. Here, we demonstrate a nitrogen cooled superconducting transition edge sensor, which shows orders of magnitude improved performance characteristics of any superconducting detector operated above 77K, with a responsivity of 9.61x10^4 V/W, noise equivalent power of 15.9 fW/Hz-1/2 and operation speeds up to GHz frequencies. It is based on van der Waals heterostructures of the high temperature superconductor Bi2Sr2CaCu2O8, which are shaped into nano-wires with ultra-small form factor. To highlight the versatility of the detector we demonstrate its fabrication and operation on a telecom grade SiN waveguide chip. Our detector significantly relaxes the demands of practical applications of superconducting detectors and displays its huge potential for photonics based quantum applications.

physics.app-ph↗

arXiv2020

Direct evidence for flat bands in twisted bilayer graphene from nano-ARPES

Transport experiments in twisted bilayer graphene revealed multiple superconducting domes separated by correlated insulating states. These properties are generally associated with strongly correlated states in a flat mini-band of the hexagonal moiré superlattice as it was predicted by band structure calculations. Evidence for such a flat band comes from local tunneling spectroscopy and electronic compressibility measurements, reporting two or more sharp peaks in the density of states that may be associated with closely spaced van Hove singularities. Direct momentum resolved measurements proved difficult though. Here, we combine different imaging techniques and angle resolved photoemission with simultaneous real and momentum space resolution (nano-ARPES) to directly map the band dispersion in twisted bilayer graphene devices near charge neutrality. Our experiments reveal large areas with homogeneous twist angle that support a flat band with spectral weight that is highly localized in momentum space. The flat band is separated from the dispersive Dirac bands which show multiple moiré hybridization gaps. These data establish the salient features of the twisted bilayer graphene band structure.

cond-mat.str-el↗

arXiv2019

Critical role of device geometry for the phase diagram of twisted bilayer graphene

The effective interaction between electrons in two-dimensional materials can be modified by their environment, enabling control of electronic correlations and phases. Here, we study the dependence of electronic correlations in twisted bilayer graphene (tBLG) on the separation to the metallic gate(s) in two device configurations. Using an atomistic tight-binding model, we determine the Hubbard parameters of the flat bands as a function of gate separation, taking into account the screening from the metallic gate(s), the dielectric spacer layers and the tBLG itself. We determine the critical gate separation at which the Hubbard parameters become smaller than the critical value required for a transition from a correlated insulator state to a (semi-)metallic phase. We show how this critical gate separation depends on twist angle, doping and the device configuration. These calculations may help rationalise the reported differences between recent measurements of tBLG's phase diagram and suggests that correlated insulator states can be screened out in devices with thin dielectric layers.

cond-mat.str-el↗

arXiv2019

Collective excitations in twisted bilayer graphene close to the magic angle

The electronic properties of twisted bilayer graphene (TBG) can be dramatically different from those of a single graphene layer, in particular when the two layers are rotated relative to each other by a small angle. TBG has recently attracted a great deal of interest, sparked by the discovery of correlated insulating and superconducting states, for twist angle $θ$ close to a so-called 'magic angle' $\approx 1.1°$. In this work, we unveil, via near-field optical microscopy, a collective plasmon mode in charge-neutral TBG near the magic angle, which is dramatically different from the ordinary single-layer graphene intraband plasmon. In selected regions of our samples, we find a gapped collective mode with linear dispersion, akin to the bulk magnetoplasmons of a two-dimensional (2D) electron gas. We interpret these as interband plasmons and associate those with the optical transitions between quasi-localized states originating from the moiré superlattice. Surprisingly, we find a higher plasmon group velocity than expected, which implies an enhanced strength of the corresponding optical transition. This points to a weaker interlayer coupling in the AA regions. These intriguing optical properties offer new insights, complementary to other techniques, on the carrier dynamics in this novel quantum electron system.

cond-mat.str-el↗