arXiv subjects

Dmitry Budker

Publications and source records attributed to Dmitry Budker.

At least 55 records · Page 3Linked to original sources

arXiv2025

Hyperpolarized Molecular Nuclear Spins Achieve Magnetic Amplification

The use of nuclear spins as physical sensing systems is disadvantaged by their low signal responsivity, particularly when compared to sensing techniques based on electron spins. This primarily results from the small nuclear gyromagnetic ratio and the difficulties in achieving high spin polarization. Here we develop a new approach to investigating the response of hyperpolarized molecular nuclear spins to magnetic fields and demonstrate orders-of-magnitude enhanced magnetic responsivity over state-of-the-art proton and Overhauser magnetometers. Using hyperpolarized molecules with proton spins, we report the realization of magnetic amplification in linear and nonlinear types. We further extend this amplification to hyperpolarized scalar-coupled multi-spin molecules and observe substantial magnetic amplification exceeding 10%. Moreover, we observe an anomalous amplification with dispersive frequency dependence that originates from magnetic interference effects. Our work highlights the potential of hyperpolarized molecular nuclear spins for use in a new class of quantum sensors, with promising applications in both applied and fundamental physics, including highly accurate absolute magnetometry and the exploration of axion-nucleon exotic interactions.

quant-ph↗

arXiv2025

Nuclear spin relaxation in zero- to ultralow-field magnetic resonance spectroscopy

Nuclear-magnetic-resonance experiments can interrogate a broad spectrum of molecular-tumbling regimes and can accurately measure interatomic distances in solution with sub-nanometer resolution. In the zero- to ultralow-field (ZULF) regime, population and coherence decay reveal nontrivial behavior due to strong coupling between nuclear spins. We note, in particular, the surprising effects that different resonances show different relaxation rates, depending on (i) the (pre)polarizing magnet field and the shuttling trajectory to the detection region at nano- and microtesla fields, (ii) the strength of the measurement field, (iii) the detection method (single-channel or quadrature), and even (iv) the nutation angle induced by the excitation pulse. We describe herein experimental data of relaxation rates measured for a 13C-labeled formic acid sample, with an atomic-magnetometer-based ZULF setup, and develop a theoretical framework to explain the detected effects and extract molecular properties. The observed effects could be used for spectral assignment, for the establishment of specific motional regimes, for image contrast, and for the characterization of relaxation processes at nano- to microtesla magnetic fields.

physics.chem-ph↗

arXiv2025

Low-field all-optical detection of superconductivity using NV nanodiamonds

Nitrogen-vacancy centers in nanodiamond offer a microwave-free, noninvasive platform for probing superconductors via near zero-field cross-relaxation magnetometry. We demonstrate this by depositing nanodiamonds on YBCO thin films to measure critical parameters: transition temperature and penetration field. This method leverages nanodiamond fluorescence modulation as a result of magnetic field variation with 1mT amplitude to observe the Meissner effect and field scans to measure the penetration field. The approach is minimally invasive and can be applied to superconducting samples with rough surfaces, facilitating the study of flux vortices and critical phenomena in complex geometries.

cond-mat.supr-con↗

arXiv2025

Study of the elusive $5s-4f$ level crossing in highly charged osmium with optical transitions suitable for physics beyond the Standard Model searches

Optical transitions of highly charged ions can be very sensitive to hypothetical beyond-the-Standard-Model phenomena. Those near the $5s-4f$ level crossing, where the $5s$ and $4f$ are degenerate are especially promising. We present predictions from atomic theory and measurements of Os$^{15,16,17+}$ at an electron beam ion trap for identification of several transitions suitable for searches for a hypothetical fifth force and possible violations of local Lorentz invariance. The electric quadrupole (E2) transitions of Os$^{16+}$ that were found are especially suitable for frequency metrology due to their small linewidth of 44 $μ$Hz. Our calculations show the need for including enough inner-shell excitations to predict transition rates between configurations, which can otherwise be overestimated. Ultimately, the predicted interconfiguration transitions were too weak to be detected.

physics.atom-ph↗

arXiv2025

Search for Axionlike Dark Matter Using Liquid-State Nuclear Magnetic Resonance

We search for dark matter in the form of axionlike particles (ALPs) in the mass range $5.576741 \,\mathrm{neV/c^2}$ - $5.577733\,\mathrm{neV/c^2}$ by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHz resulted in a sensitivity to the ALP-proton coupling constant of $g_{\mathrm{ap}} \approx 3 \times 10^{-2}\,\mathrm{GeV}^{-1}$. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment's capabilities. CASPEr-Gradient Low-Field will probe the mass range from $4.1\,\mathrm{\peV/c^2}$ to $17\,\mathrm{\neV/c^2}$ with hyperpolarized samples to boost the sensitivity beyond the astronomical limits.

hep-ex↗

arXiv2025

Trapping of electrons and $^{40}\textrm{Ca}^+$ ions in a dual-frequency Paul trap

We demonstrate the operation of a dual-frequency Paul trap and characterize its performance by storing either electrons or calcium ions while applying two quadrupole fields simultaneously which oscillate at $Ω_\textrm{fast} = 2π\times 1.6$ GHz and $Ω_\textrm{slow} = 2π\times 2$ MHz. The particles are loaded and stored in the trap under various conditions followed by detection employing an electron multiplier tube. We find that tens of electrons or ions can be trapped for up to ten milliseconds and a small fraction remains trapped even after hundreds of milliseconds. During dual-frequency operation we find that while the number of trapped electrons rapidly decreases with increase of the $Ω_\textrm{slow}$ field amplitude, the number of trapped ions shows no dependence on the $Ω_\textrm{fast}$ field amplitude as supported by our extensive numerical simulations. We aim to use a similar trap for synthesising antihydrogen from antiprotons and positrons. Accordingly, we discuss open challenges such as the co-trapping of oppositely charged species and particle trap duration.

physics.atom-ph↗

arXiv2025

Quantum Imaging of Ferromagnetic van der Waals Magnetic Domain Structures at Ambient Conditions

Recently discovered 2D van der Waals magnetic materials, and specifically Iron-Germanium-Telluride ($\rm Fe_{5}GeTe_{2}$), have attracted significant attention both from a fundamental perspective and for potential applications. Key open questions concern their domain structure and magnetic phase transition temperature as a function of sample thickness and external field, as well as implications for integration into devices such as magnetic memories and logic. Here we address key questions using a nitrogen-vacancy center based quantum magnetic microscope, enabling direct imaging of the magnetization of $\rm Fe_{5}GeTe_{2}$ at sub-micron spatial resolution as a function of temperature, magnetic field, and thickness. We employ spatially resolved measures, including magnetization variance and cross-correlation, and find a significant spread in transition temperature yet with no clear dependence on thickness down to 15 nm. We also identify previously unknown stripe features in the optical as well as magnetic images, which we attribute to modulations of the constituting elements during crystal synthesis and subsequent oxidation. Our results suggest that the magnetic anisotropy in this material does not play a crucial role in their magnetic properties, leading to a magnetic phase transition of $\rm Fe_{5}GeTe_{2}$ which is largely thickness-independent down to 15 nm. Our findings could be significant in designing future spintronic devices, magnetic memories and logic with 2D van der Waals magnetic materials.

cond-mat.mtrl-sci↗

arXiv2025

Laser fluence-dependent production of molecular thorium ions in different charge states for trapped-ion experiments

Thorium ions and molecules, recognized for their distinctive nuclear and atomic attributes, are central to numerous trapped-ion experiments globally. Our study introduces an effective, compact source of thorium ions produced via laser ablation of microgram-scale, salt-based samples. We thoroughly analyze the variety of ion species and charge states generated at varying laser fluences. Utilizing 10$μ$g of thorium fluoride crystals and laser fluences between $1.00 - 7.00$ J$\cdot$cm$^{-2}$ we produce thorium molecular ions $^{232}$ThF$_x$$^{n+}$ (with $x= 0 - 3$ and charge states up to $n = 3+$), including ThF$^{2+}$ and ThF$^{3+}$. These species are particularly relevant for spectroscopy; ThF$^{3+}$ is valuable for its stable closed-shell configuration, while ThF$^{2+}$, which is isoelectronic to RaF, offers a unique probe for studying nuclear structure and fundamental symmetries due to its simple electronic structure with a single unpaired electron. Density functional theory calculations of the distribution of positive charge in the produced molecular cations and the simplicity of this setup indicate that this method is easily transferable to other actinide systems.

physics.atom-ph↗

arXiv2025

Quantum Magnetic J-Oscillators

We introduce quantum J-oscillators that exploit intrinsic nuclear spin-spin (scalar J) couplings in molecules to produce phase-coherent oscillations. Operated in zero magnetic field and driven by a digital feedback, they operate from sub-hertz to a few tens of hertz frequencies. In a proof-of-principle experiment on [15N]-acetonitrile, the oscillator produced a 337 uHz linewidth over 3000 s, more than two orders narrower than in conventional zero-field NMR. This may facilitate precision measurements of J-coupling constants and allows distinguishing mixtures of molecules whose zero-field NMR spectra would otherwise be hard to separate. In addition, the combination of strongly coupled spin systems and programmable feedback turns the J-oscillator into a compact tabletop (and, eventually, chip-scale) platform for exploring nonlinear spin dynamics, including chaos, dynamical phase transitions, and perhaps time-crystal behavior. By uniting high-resolution spectroscopy and controllable quantum dynamics in a single, magnet-free setup, J-oscillators open new opportunities for applications where ultraprecise frequency references or molecular fingerprints are required.

quant-ph↗

arXiv2025

Solving tricky quantum optics problems with assistance from (artificial) intelligence

The capabilities of modern artificial intelligence (AI) as a ``scientific collaborator'' are explored by engaging it with three nuanced problems in quantum optics: state populations in optical pumping, resonant transitions between decaying states (the Burshtein effect), and degenerate mirrorless lasing. Through iterative dialogue, the authors observe that AI models--when prompted and corrected--can reason through complex scenarios, refine their answers, and provide expert-level guidance, closely resembling the interaction with an adept colleague. The findings highlight that AI democratizes access to sophisticated modeling and analysis, shifting the focus in scientific practice from technical mastery to the generation and testing of ideas, and reducing the time for completing research tasks from days to minutes.

quant-ph↗

arXiv2025

Improved constraints on exotic interactions between electron and proton in hydrogen

Atomic spectroscopy can be used to search for new bosons that carry exotic forces between elementary fermions. A comparison of a recent precise measurement [Bullis \textit{et al.}, Phys. Rev. Lett. \textbf{130}, 203001 (2023)] of the hyperfine splitting of the 2S$_{1/2}$ electronic levels of hydrogen and up-to-date bound-state quantum electrodynamics theory yields improved constraints on electron-proton exotic interactions of the dimensionless coupling strengths $g_Ag_A$, $g_pg_p$, and $g_Vg_V$ corresponding to the exchange of a axial-vector, pseudoscalar (axionlike) or vector boson, respectively.

physics.atom-ph↗

arXiv2025

Search for a parity-violating long-range spin-dependent interaction

High-sensitivity quantum sensors are a promising tool for experimental searches for beyond-Standard-Model interactions. Here, we demonstrate an atomic comagnetometer operating under a resonantly-coupled hybrid spin-resonance (HSR) regime to probe P-odd, T-even interactions. The HSR regime enables robust nuclear-electron spin coupling, enhancing measurement bandwidth and stability without compromising the high sensitivity of spin-exchange relaxation-free magnetometers. To minimize vibration noise from velocity-modulated sources, we implement a multistage vibration isolation system, achieving a vibration noise reduction exceeding 700-fold. We establish new constraints on vector-boson-mediated parity-violating interactions, improving experimental sensitivity by three orders of magnitude compared to previous limits. The new constraints complement existing astrophysical and laboratory studies of potential extensions to the Standard Model.

quant-ph↗

arXiv2025

Levitated Sensor for Magnetometry in Ambient Environment

Levitated particle systems have gained significant attention as a rapidly advancing platform for precision sensing, offering low-loss, highly isolated environments by eliminating mechanical contact and associated noise. Current room-temperature levitation techniques are primarily sensitive to acceleration, with magnetic sensing often relying on the Meissner effect, which is impractical under ambient conditions. Here, we demonstrate a diamagnetically stabilized magnetically levitated magnet magnetometer (LeMaMa), where the motion of the magnet is detected optically. Leveraging strong spin-lattice coupling in the ferromagnet to suppress spin-projection noise and minimizing dissipation through levitation, we achieve a sensitivity of 32 fT $/Hz^{1/2}$. This sensitivity is adequate for a wide range of applications in biology, chemistry, and fundamental physics, matching the performance of leading technologies like SQUIDs and atomic magnetometers, while offering the distinct advantage of operating at room temperature and under Earth's magnetic field.

physics.ins-det↗

arXiv2025

Status of the Proton EDM Experiment (pEDM)

The Proton EDM Experiment (pEDM) is the first direct search for the proton electric dipole moment (EDM) with the aim of being the first experiment to probe the Standard Model (SM) prediction of any particle EDM. Phase-I of pEDM will achieve $10^{-29} e\cdot$cm, improving current indirect limits by four orders of magnitude. This will establish a new standard of precision in nucleon EDM searches and offer a unique sensitivity to better understand the Strong CP problem. The experiment is ideally positioned to explore physics beyond the Standard Model (BSM), with sensitivity to axionic dark matter via the signal of an oscillating proton EDM and across a wide mass range of BSM models from $\mathcal{O}(1\text{GeV})$ to $\mathcal{O}(10^3\text{TeV})$. Utilizing the frozen-spin technique in a highly symmetric storage ring that leverages existing infrastructure at Brookhaven National Laboratory (BNL), pEDM builds upon the technological foundation and experimental expertise of the highly successful Muon $g$$-$$2$ Experiments. With significant R\&D and prototyping already underway, pEDM is preparing a conceptual design report (CDR) to offer a cost-effective, high-impact path to discovering new sources of CP violation and advancing our understanding of fundamental physics. It will play a vital role in complementing the physics goals of the next-generation collider while simultaneously contributing to sustaining particle physics research and training early-career researchers during gaps between major collider operations.

hep-ex↗

arXiv2025

Notes on optimizing a multi-sensor gradient axion-like particle dark matter search

Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for the dark matter. We discuss the scaling of the sensitivity of a galactic ALP dark matter search with the number of sensors, especially in the ultra-light mass regime, where the measurement time is shorter than the coherence time of the ALP field. We compare multiple schemes for daily modulated ALP gradient signals, and show that increasing the number of sensors from 1 to 2 improves the signal-to-noise ratio (SNR) by a factor of 2-3. For more than two sensors, the SNR increases as the square root of the number of sensors. Then, we show that splitting the data into subsets and then averaging its Discrete Fourier Transforms (DFTs) is equivalent to the DFT of the whole dataset in terms of SNR.

hep-ph↗

arXiv2025

Dark Matter Search with a Resonantly-Coupled Hybrid Spin System

Recent advances in tabletop quantum sensor technology have enabled searches for nongravitational interactions of dark matter (DM). Traditional axion DM experiments rely on sharp resonance, resulting in extensive scanning time to cover a wide mass range. In this work, we present a broadband approach in an alkali-${}^{21}$Ne spin system. We identify two distinct hybrid spin-coupled regimes: a self-compensation (SC) regime at low frequencies and a hybrid spin resonance (HSR) regime at higher frequencies. By utilizing these two distinct regimes, we significantly enhance the bandwidth of ${}^{21}$Ne nuclear spin compared to conventional nuclear magnetic resonance, while maintaining competitive sensitivity. We present a comprehensive broadband search for axion-like dark matter, covering 5 orders of magnitude of Compton frequencies range within $[10^{-2}, \, 10^3]$ Hz. We set new constraints on the axion dark matter interactions with neutrons and protons, accounting for the effects of DM stochasticity. For the axion-neutron coupling, our results reach a low value of $|g_{ann}|\le 3\times 10^{-10}$ in the frequency range $[2\times 10^{-2}, \, 4]$ Hz surpassing astrophysical limits and providing the strongest laboratory constraints in the $[10, \, 100]$ Hz range. For the axion-proton coupling, we offer the best terrestrial constraints for the frequency ranges $[2\times 10^{-2}, \, 5]$Hz and $[16, \, 7\times 10^{2}]$ Hz.

hep-ph↗

arXiv2025

Constraints on new vector boson mediated electron-nucleus interactions from spectroscopy of polar diatomic molecules

A measurement of parity violation in the hyperfine structure of $^{138}$Ba$^{19}$F [E. Altuntaş et al. Phys. Rev. Lett. 120, 142501 (2018)] is reinterpreted with electronic structure calculations in terms of beyond Standard Model vector boson mediated electron-nucleus interactions. Our results set constraints on previously unexplored, new boson mediated axial vector-vector nucleus-electron interactions. Similar bounds are obtained by analyzing the atomic parity violation experiment with $^{133}$Cs. Moreover, we show that future experiments with cold heavy diatomic molecules like $^{225}$RaF can improve the present sensitivity to axial vector-vector nucleus-electron and nucleon-nucleus interactions by up to five orders of magnitudes.

hep-ph↗

arXiv2025

Searching for Exotic Interactions between Antimatter

We show that atomic antimatter spectroscopy can be used to search for new bosons that carry spin-dependent exotic forces between antifermions. A comparison of a recent precise measurement of the hyperfine splitting of the $1$S and $2$S electronic levels of antihydrogen and bound-state quantum electrodynamics theory yields the first tests of positron-antiproton exotic interactions, constraining the dimensionless coupling strengths $g_pg_p$, $g_Vg_V$ and $g_Ag_A$, corresponding to the exchange of a pseudoscalar (axionlike), vector, or axial-vector boson, respectively. We also discuss new tests of CPT invariance with exotic spin-dependent and spin-independent interactions involving antimatter.

physics.atom-ph↗