arXiv subjects

Dmitry S. Smirnov

Publications and source records attributed to Dmitry S. Smirnov.

8 recordsLinked to original sources

arXiv2026

Proximity effects of chiral magnetization on transition metal dichalcogenides monolayers

We consider the proximity effects of a commensurate chiral $120^{\circ}$ Néel magnetic structure on the transport and optical properties of a transition metal dichalcogenide monolayer (TMD ML). The enlarged magnetic unit cell leads to the folding of the Brillouin zone and enables efficient intervalley spin-flip scattering. Starting from a six band tight binding model, we develop an effective $k\cdot p$ model, which describes the coupling between charge carriers in the TMD ML and the chiral magnetization. We predict the anomalous antiferromagnetic Hall effect (AHE) for conduction electrons and describe it accounting for the interplay between anomalous velocity, side jump, and skew scattering contributions. The proximity of the chiral magnetization also leads to the mixing and splitting of the exciton resonances in the two valleys which are related by the time reversal symmetry despite zero net magnetization. Finally, we demonstrate the possibility to measure the distribution of in-plane orientation of the chiral magnetization through Faraday rotation and the ellipticity of incident linearly polarized light.

cond-mat.mes-hall↗

arXiv2026

Valley-controlled chiral magnetism in transition metal dichalcogenide monolayers

We put forward the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction in transition metal dichalcogenide monolayers as a tool to create and control a chiral magnetic texture. We show that in the spin-valley locking regime, the RKKY interaction acts as a Dzyaloshinskii-Moriya coupling with an effective spin rotation period exactly equal to the tripled lattice constant. Using mean field theory and classical Monte Carlo simulations, we demonstrate that this interaction qualitatively reshapes the phase diagram of atomically thin antiferromagnets. It destroys the chirality-related phase transition by selecting a single chirality value even when the RKKY interaction is small. At the same time, it shifts the Berezinskii-Kosterlitz-Thouless transition associated with spins orientation to higher temperatures. We argue that the valley degree of freedom of electrons mediating the RKKY interaction provides a powerful control knob for exploring non-universal phase transitions and quantum spin liquid states in two-dimensional van der Waals heterostructures.

cond-mat.mes-hall↗

arXiv2026

Hyperfine versus exchange interaction in the spin dynamics of spatially indirect excitons in CsPbI$_{3}$ perovskite nanocrystals

We study the dynamics of recombination, optical orientation, and optical alignment of excitons in ensembles of CsPbI$_{3}$ nanocrystals (NCs), synthesized in a glass matrix. In large NCs with size exceeding 16 nm, the low-energy photoluminescence is contributed by the emission of indirect in real space excitons formed by spatially separated electrons and holes, which are localized at the NC/glass interface. The recombination dynamics of an ensemble of such excitons extends from tens of nanoseconds to microseconds and exhibits a power-law dependence. Their optical alignment and optical orientation reveal a peculiar spin dynamics caused by excitons influenced by the exchange interaction, varying by orders of magnitude. We develop a theory of the polarized photoluminescence of triplet excitons, taking into account the interplay between the electron-hole exchange interaction, their Zeeman effect, and their hyperfine interaction with the nuclei. This model reveals that for the excitons with the smallest exchange splitting we reach the regime, where the exciton fine structure becomes dominated by the hyperfine interaction with the random nuclear spin fluctuations in the NCs.

cond-mat.mes-hall↗

arXiv2024

Hidden anisotropy controls spin-photon entanglement in a charged quantum dot

Photon entanglement is indispensable for optical quantum technologies. Measurement-based optical quantum computing and all-optical quantum networks rely on multiphoton cluster states consisting of indistinguishable entangled photons. A promising method for creating such cluster states on demand is spin-photon entanglement using the spin of a resident charge carrier in a quantum dot, precessing in a weak external magnetic field. In this work, we show theoretically and experimentally that spin-photon entanglement is strongly affected by the hidden anisotropy of quantum dots, which can arise from mechanical stress, shape anisotropy and even specific crystal structure. In the measurements of time-resolved photoluminescence and cross-polarized second-order photon correlation function in a magnetic field, the anisotropy manifests itself in the spin dynamics and, as a consequence, in the spin-photon concurrence. The measured time-filtered spin-photon Bell state fidelity depends strongly on the excitation polarization and reaches an extremely high value of 94% at maximum. We specify the magnetic field and excitation polarization directions that maximize spin-photon entanglement and thereby enhance the fidelity of multiphoton entangled states.

cond-mat.mes-hall↗

arXiv2024

Birefringent spin-photon interface generates polarization entanglement

A spin-photon interface based on the luminescence of a singly charged quantum dot in a micropillar cavity allows for the creation of photonic entangled states. Current devices suffer from cavity birefringence, which limits the generation of spin-photon entanglement. In this paper, we theoretically study the light absorption and emission by the interface with an anisotropic cavity and derive the maximal excitation and spin-photon entanglement conditions. We show that the concurrence of the spin-photon state equal to one and complete quantum dot population inversion can be reached for a micropillar cavity with any degree of birefringence by tuning the quantum dot resonance strictly between the cavity modes. This sweet spot is also valid for generating a multiphoton cluster state, as we demonstrate by calculating the three-tangle and fidelity with the maximally entangled state.

quant-ph↗

arXiv2019

Spin inertia and polarization recovery in quantum dots: Role of pumping strength and resonant spin amplification

Spin inertia measurements are a novel experimental tool to study long-time spin relaxation processes in semiconductor nanostructures. We develop a theory of the spin inertia effect for resident electrons and holes localized in quantum dots. We consider the spin orientation by short optical pulses with arbitrary pulse area and detuning from the trion resonance. The interaction with an external longitudinal magnetic field and the hyperfine interaction with the nuclear spin bath is considered in both the ground and excited (trion) states of the quantum dots. We analyze how the spin inertia signal depends on the magnetic field (polarization recovery) and on the modulation frequency of the helicity of the pump pulses as well as on their power and detuning. In particular, we elaborate how approaching the saturation limit of the spin polarization influences the measurements. The quantitative description of spin inertia measurements will enable the determination of the parameters of spin dynamics such as the spin relaxation times in the ground and excited states and the parameters of the hyperfine interaction. Finally, we predict the emergence of resonant spin amplification due to the transverse components of the nuclear spin fluctuations, which manifests itself as oscillations of the spin polarization as a function of the longitudinal magnetic field.

cond-mat.mes-hall↗

arXiv2018

Hole-capture competition between a single quantum dot and an ionized acceptor

We study the competition of hole capture between an In(Ga)As quantum dot and a directly adjacent ionized impurity in view of spin-photon interfaces. The Kerr rotation noise spectroscopy at 4.2 K shows that the hole-capture probability of the In(Ga)As quantum dot is about one order of magnitude higher compared to the hole-capture probability of the ionized impurity and suggests that a simultaneous occupation of quantum dot and impurity by a hole is efficiently suppressed due to Coulomb interaction. A theoretical model of interconnected spin and charge noise allows the quantitative specification of all relevant time scales.

cond-mat.mes-hall↗

arXiv2014

Spin noise in a quantum dot ensemble: from a quantum mechanical to a semi-classical description

Spin noise spectroscopy is a promising technique for revealing the microscopic nature of spin dephasing processes in quantum dots. We compare the spin-noise in an ensemble of singly charged quantum dots calculated by two complementary approaches. The Chebyshev polynomial expansion technique (CET) accounts for the full quantum mechanical fluctuation of the nuclear spin bath and a semi-classical approach (SCA) is based on the averaging the electron spin dynamics over all different static Overhauser field configurations. We observe a remarkable agreement between both methods in the high-frequency part of the spectra, while the low-frequency part is determined by the long time fluctuations of the Overhauser field. We find small differences in the spectra depending on the distribution of hyperfine couplings. The spin-noise spectra in strong enough magnetic fields where the nuclear dynamics is quenched calculated by two complimentary approaches are in perfect agreement.

cond-mat.mes-hall↗