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Dmitry V. Chichinadze

Publications and source records attributed to Dmitry V. Chichinadze.

At least 19 recordsLinked to original sources

Weak localization and antilocalization corrections to nonlinear transport: a semiclassical Boltzmann treatment

The nonlinear transport regime is manifested in the nonlinear current-voltage characteristic of the system. An example of such a nonlinear regime is a setup in which current is injected into the sample and the measured voltage drop is quadratic in the injected current. Such a quadratic nonlinear regime requires inversion symmetry to be broken. This is the same symmetry condition as one needs to observe weak antilocalization, which can be prominent in two-dimensional systems. Here, we study the effects of weak (anti)localization on second-order nonlinear transport in two-dimensional systems using the semiclassical Boltzmann approach. We solve for quasiparticle distribution function up to the second order in the applied external electric field and calculate linear and nonlinear conductivity tensors for a toy model. We find that localization effects could lead to a sign change of the nonlinear conductivity tensor -- a phenomenon observed in transition metal dichalcogenide and in single-layer graphene devices.

cond-mat.mes-hall↗

Metamagnetism in UTe2: the roles of itinerancy and localization

The metamagnetic transition in UTe$_2$ plays a key role in stabilizing two enigmatic field-induced superconducting phases. One of these phases (SC2) is truncated by the transition, lying directly below it, while the other (SC3) sits predominantly above it and appears to be stabilized because of it. While numerous pulsed field studies have examined this transition, comparatively few steady field experiments have investigated it. Here we report a suite of measurements of metamgnetism in UTe$_2$, at ambient pressure by torque magnetometry and extraction magnetometry techniques, and of the magnetoconductance under pressure. Our steady field measurements resolve a complex sub-structure within the transition, with separate features that possess different temperature evolutions, pointing to distinct contributions from itinerant and localized moments. The itinerant contribution might relate to a possible spin-density wave state. We theoretically model the evolution of Kondo and RKKY interactions and propose that the SC2 state is stabilized under pressure due to the collapse of magnetic anisotropy, leading to an enhancement of longitudinal spin fluctuations along the hard $b$ axis, which are pair-forming in the $p$-wave channel.

cond-mat.str-el↗

Giant nonlinear conductivity in 2D electron gas from substrate-induced dipolar scattering

Despite a surge of interest in the nonlinear transport in 2D materials, a fundamental puzzle remains: existing theoretical frameworks are unable to quantitatively account for the giant nonlinear conductivities ($\gtrsim 1 \frac{μ\text{m}}{Ω\text{V}}$) recently reported in 2D van der Waals heterostructures. Here, we introduce a mechanism based on electron scattering from a substrate-induced dipole array linked to short-range impurities. We show that the strict kinematic constraints, inherent to 2D scattering, lead to a singular enhancement of the nonlinear response, fundamentally dictating a natural scale of $1 \frac{μ\text{m}}{Ω\text{V}}$.

cond-mat.str-el↗

Electrically-controllable superconducting memory effect in UTe2

If a computer could be assembled from superconducting components, the energy efficiency would far surpass that of conventional electronics. Historic research efforts towards this goal yielded pivotal breakthroughs in the development and discovery of scanning tunnelling microscopy and high temperature superconductivity. Although recent strides have been taken in advancing superconducting diode and switching technologies, harnessing read/writeable memory functionality in superconducting platforms has remained challenging. Here we show that bulk single crystal specimens of the triplet superconductor candidate uranium ditelluride (UTe$_2$) possess such properties. Upon applying a magnetic field to access an intermediate regime straddling two distinct superconducting phases, we find that direct current pulses can push the material in and out of a metastable state possessing an enhanced critical current $J_c$. This switching is controllable by the strength and duration of the stimuli, with the system `remembering' whether it is in the high or low $J_c$ state for extended periods. We interpret this to be due to competition between two distinct vortex species, which can be perturbatively pushed into a non-equilibrium high-disorder configuration with stronger pinning forces and thus higher $J_c$. Rather than requiring proximate magnetic or semiconducting interfaces, this memory functionality appears to be an intrinsic property of UTe$_2$ rooted in the superconducting order itself. Our findings underscore the rich complexity of quantum vortex matter, and demonstrate the viability of engineering a new class of superconducting memory elements with ultralow-power switching.

cond-mat.supr-con↗

Upper critical in-plane magnetic field in quasi-2D layered superconductors

The study of the interplay of applied external magnetic field and superconductivity has been invigorated by recent works on Bernal bilayer and rhombohedral multilayer graphene. These studies, with and without proximitized spin-orbit coupling, have opened up a new frontier in the exploration of unconventional superconductors as they offer a unique platform to investigate superconductivity with high degree of in-plane magnetic field resilience and even magnetic field-induced superconductivity. Here, we present a framework for analyzing the upper critical in-plane magnetic field data in multilayer superconductors. Our framework relies on an analytically tractable superconducting pairing model that captures the normal state phenomenology of these systems and applies it to calculate the relationship between the upper critical field $H_{c2}$ and the corresponding critical temperature $T_{c}$. We study the $H_{c2}-T_{c}$ critical curve as a function of experimental parameters (Ising and Rashba spin-orbit coupling) and depairing mechanisms (Zeeman and orbital coupling) for both spin-singlet and spin-triplet pairing. By applying our framework to analyze four recent Bernal bilayer graphene-WSe$_2$ experiments [1-4], we identify an apparent discrepancy between fitted and measured spin-orbit parameters, which we propose can be explained by an enhancement of the Landé g factor in the Bernal bilayer graphene experiments.

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Re-entrant unconventional superconductivity induced by rare-earth substitution in Nd1-xEuxNiO2 thin films

High temperature superconductivity is typically associated with strong coupling and a large superconducting gap, yet these characteristics have not been demonstrated in the nickelates. Here, we provide experimental evidence that Eu substitution in the spacer layer of Nd1-xEuxNiO2 (NENO) thin films enhances the superconducting gap, driving the system toward a strong-coupling regime. This is accompanied by a magnetic-exchange-driven magnetic-field-enhanced superconductivity. We investigate the upper critical magnetic field, Hc2, and superconducting gap of superconducting NENO thin films with x=0.2 to 0.35. Magnetoresistance measurements reveal magnetic-field-enhanced superconductivity in NENO films. We interpret this phenomenon as a result of interaction between magnetic Eu ions and superconducting states in the Ni dx2-y2 orbital. The upper critical magnetic field strongly violates the weak-coupling Pauli limit. Infrared spectroscopy confirms a large gap-to-Tc ratio $2 Δk_B T_c \approx 5 - 6$, indicating a stronger coupling pairing mechanism in NENO relative to the Sr-doped NdNiO2. The substitution of Eu in the rare-earth layer provides a method to modify the superconducting gap in Nd-based nickelates, an essential factor in engineering high-Tc superconductivity in infinite-layer nickelates.

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g-Factor Enhanced Upper Critical Field in Superconducting PdTe2 due to Quantum Confinement

The Pauli limiting field of superconductors determines the maximal possible value of magnetic field at which superconductivity remains possible. For weak-coupling superconductors, it is determined by an established relation that can be found by setting the condensation energy equal to the magnetization free energy. The latter is a function of the carrier g-factor. Here, we demonstrate in a van der Waals superconductor PdTe2, that quantum confinement can tune the effective g-factor causing the Pauli limit to become thickness dependent. We experimentally probe the in-plane upper critical field (Hc2||) of PdTe2 at intermediate thicknesses down to 20mK. Hc2|| is enhanced by more than an order of magnitude as the thickness is varied from 50nm down to 19nm. We model its temperature and thickness dependence, revealing that both orbital and spin Zeeman depairing mechanisms impact its value. While the variation of the orbital interaction is expected, our findings reveal how the Zeeman interaction impacts superconductivity in thin films. They aid in the search for mixed and odd pairing superconductivity where an enhancement of Hc2|| can be occasionally associated with those unconventional pairing symmetries.

cond-mat.supr-con↗

Observation of giant nonlinear Hall conductivity in Bernal bilayer graphene

In a system of two-dimensional electrons, a combination of broken symmetry, interactions, and nontrivial topology can conspire to give rise to a nonlinear transport regime, where electric current density scales as the square of electric field. This regime has become a venue for exciting discoveries such as the nonlinear Hall effect and diode-like nonreciprocal transport. However, interpretation of experimental data is challenging in the nonlinear regime as DC transport is described by a rank-3 conductivity tensor with 6 free parameters. Here, we resolve this challenge by analytically solving for the nonlinear potential distribution across the disk sample for an arbitrary linear and nonlinear conductivity tensors. This allows us to unambiguously extract all components of the nonlinear tensor from experimental measurement. Using this novel tool, we identify giant nonlinear Hall effect in Bernal bilayer graphene. Our methodology provides the first systematic framework for interpreting nonlinear transport and uncovers a new route towards understanding quasi-2D materials.

cond-mat.mes-hall↗

Metamagnetic ripples in the UTe2 high magnetic field phase diagram

The heavy fermion metamagnet uranium ditelluride possesses two distinct magnetic field--induced superconducting states. One of these superconductive phases resides at magnetic fields immediately below a first-order metamagnetic transition to a field--polarized paramagnetic state at a field strength $H_m$, while the other exists predominantly above $H_m$. However, little is known about the microscopic properties of this polarized paramagnetic state. Here we report pulsed magnetic field measurements tracking the evolution of $H_m$ for polar and azimuthal inclinations in the vicinity of the crystallographic $b-a$ plane. We uncover a region of the phase diagram at high fields $>$ 50 T with a ripple-like non-monotonic dependence of $H_m$ on the orientation of field. Within this ripple in the metamagnetic transition surface, $H_m$ exhibits an anomalous temperature dependence. Our results point towards the presence of complex magnetic interactions and possible magnetic sub-phases at high magnetic fields in UTe$_2$, which may have important implications for the manifestation of exotic field-induced superconductivity.

cond-mat.str-el↗

Superconducting Diode Effect in Multiphase Superconductors

We identify a new mechanism for the intrinsic superconducting diode effect (SDE) in multiphase superconductors. Using a Ginzburg-Landau and a microscopic two-band model, we find phase transitions into a mixed phase with finite-momentum Cooper pairs and SDE with high (including maximal) diode efficiencies, despite the individual phases exhibiting no SDE and equal inversion parity. We thus show that parity mixing $-$ invoked in previous proposals $-$ is not a crucial ingredient for SDE. The new mechanism may be relevant in a multitude of known multiphase superconductors like UTe$_2$.

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The Crossover from Ordinary to Higher-Order van Hove Singularity in a Honeycomb System: A Parquet Renormalization Group Analysis

We investigate the crossover from an ordinary van Hove singularity (OVHS) to a higher order van Hove singularity (HOVHS) in a model applicable to Bernal bilayer graphene and rhombohedral trilayer graphene in a displacement field. At small doping, these systems possess three spin-degenerate Fermi pockets near each Dirac point $K$ and $K'$; at larger doping, the three pockets merge into a single one. The transition is of Lifshitz type and includes van Hove singularities. Depending on system parameters, there are either 3 separate OVHS or a single HOVHS. We model this behavior by a one-parameter dispersion relation, which interpolates between OVHS and HOVHS. In each case, the diverging density of states triggers various electronic orders (superconductivity, pair density wave, valley polarization, ferromagnetism, spin and charge density wave). We apply the parquet renormalization group (pRG) technique and analyze how the ordering tendencies evolve between OVHS and HOVHS. We report rich system behavior caused by disappearance/reemergence and pair production/annihilation of the fixed points of the pRG flow.

cond-mat.str-el↗

Angle-resolved transport nonreciprocity and spontaneous symmetry breaking in twisted trilayer graphene

The ability to identify and characterize spontaneous symmetry breaking is central to our understanding of 2D materials with strong correlation, such as the moiré flat bands in magic-angle twisted graphene bilayer and trilayer. In this work, we utilize angle-resolved measurements of transport nonreciprocity to investigate spontaneous symmetry breaking in twisted trilayer graphene. By analyzing the angular dependence of nonreciprocity in both longitudinal and transverse channels, we are able to identify the symmetry axis associated with the underlying electronic order. We report that a hysteretic rotation in the mirror axis can be induced by thermal cycles and a large current bias, which offers unambiguous evidence for the spontaneous breaking of rotational symmetry. Moreover, the onset of nonreciprocity with decreasing temperature coincides with the emergence of orbital ferromagnetism. Combined with the angular dependence of the superconducting diode effect, our findings uncover a direct link between rotational and time-reversal symmetry breaking. These symmetry requirements point towards the exchange-driven instabilities in the momentum space as a possible origin for transport nonreciprocity in tTLG.

cond-mat.mes-hall↗

Cascade of transitions in twisted and non-twisted graphene layers within the van Hove scenario

Motivated by measurements of compressibility and STM spectra in twisted bilayer graphene, we analyze the pattern of symmetry breaking for itinerant fermions near a van Hove singularity. Making use of an approximate SU(4) symmetry of the Landau functional, we show that the structure of the spin/isospin order parameter changes with increasing filling via a cascade of transitions. We compute the feedback from different spin/isospin orders on fermions and argue that each order splits the initially 4-fold degenerate van Hove peak in a particular fashion, consistent with the STM data and compressibility measurements, providing a unified interpretation of the cascade of transitions in twisted bilayer graphene. Our results follow from a generic analysis of an SU(4)-symmetric Landau functional and are valid beyond a specific underlying fermionic model. We argue that an analogous van Hove scenario explains the cascade of phase transitions in non-twisted Bernal bilayer and rhombohedral trilayer graphene.

cond-mat.mes-hall↗

SU(4) symmetry in twisted bilayer graphene - an itinerant perspective

We study symmetry-broken phases in twisted bilayer graphene at small filling above charge neutrality and at Van Hove filling. We argue that the Landau functionals for the particle-hole order parameters at these fillings both have an approximate SU(4) symmetry, but differ in the sign of quartic terms. We determine the order parameter manifold of the ground state and analyze its excitations. For small fillings, we find a strong 1st-order transition to an SU(3)$\otimes$U(1) manifold of orders that break spin-valley symmetry and induce a 3-1 splitting of fermionic excitations. For Van Hove filling, we find a weak 1st-order transition to an SO(4)$\otimes$U(1) manifold of orders that preserves the two-fold band degeneracy. We discuss the effect of particle-hole orders on superconductivity and compare with strong-coupling approaches.

cond-mat.str-el↗

Valley magnetism, nematicity, and density wave orders in twisted bilayer graphene

We analyze density-wave and Pomeranchuk orders in twisted bilayer graphene. This compliments our earlier analysis of the pairing instabilities. We assume that near half-filling of either conduction or valence band, the Fermi level is close to Van Hove points, where the density of states diverges, and study potential instabilities in the particle-hole channel within a patch model with two valley degrees of freedom. The hexagonal symmetry of twisted bilayer graphene allows for either six or twelve Van Hove points. We consider both cases and find the same two leading candidates for particle-hole order. One is an SU(2)-breaking spin state with ferromagnetism within a valley. A subleading inter-valley hopping induces antiferromagnetism between the valleys. The same state has also been obtained in strong coupling approaches, indicating that this order is robust. The other is a mixed state with $120^\circ$ complex spin order and orthogonal complex charge order. In addition, we find a weaker, but still attractive interaction in nematic channels, and discuss the type of a nematic order.

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Nematic superconductivity in twisted bilayer graphene

Twisted bilayer graphene displays insulating and superconducting phases caused by exceptional flattening of its lowest energy bands. Superconductivity with highest $T_c$ appears at hole and electron dopings, near half-filling for valence or conduction bands. In the hole-doped case, the data show that three-fold lattice rotation symmetry is broken in the superconducting phase, i.e., a superconductor is also a nematic. We present the mechanism for nematic superconductivity. We take as an input the fact that at relevant dopings the Fermi energy lies in the vicinity of twist-induced Van Hove singularities in the density of states and argue that the low-energy physics can be properly described by patch models with six Van Hove points for electron doping and twelve Van Hove points for hole doping. We obtain pairing interactions for the patch models in terms of parameters of the microscopic model for the flat bands, which contains both local and twist-induced non-local interactions and show that the latter gives rise to attraction in different superconducting channels. For hole-doping, we find two attractive channels, $g$ and $i$-waves, with almost equal coupling constants. We show that in the co-existence state, where both order parameters are non-zero, the three-fold lattice rotation symmetry is broken, i.e., a superconductor is also a nematic. We find two possible nematic states, one is time-reversal symmetric, the other additionally breaks time-reversal symmetry. Our scenario for nematic superconductivity is based on generic symmetry considerations, and we expect it to be applicable also to other systems with two (or more) attractive channels with similar couplings.

cond-mat.supr-con↗

Specific heat in strongly hole-doped Iron-based superconductors

We compute the specific heat $C(T)$ in an Fe-based superconductor with only hole pockets. We use a three-orbital/three pocket model with two smaller hole pockets made out of $d_{xz}$ and $d_{yz}$ orbitals and a larger pocket made out of $d_{xy}$ orbital. We use as an input the experimental fact that the mass of $d_{xy}$ fermion is much heavier than that of $d_{xz}/d_{yz}$ fermions. We argue that the heavy $d_{xy}$ band contributes most to the specific heat in the normal state, but the superconducting gap on the $d_{xy}$ pocket is parametrically smaller than that on $d_{xz}/d_{yz}$ pockets. We argue that in this situation the jump of $C(T)$ at $T_c$ is determined by $d_{xz}/d_{yz}$ fermions, and the ratio $(C_s-C_n)/C_n$ is a fraction of that in a one-band BCS theory. Below $T_c$, $C(T)$ remains relatively flat down to some $T^*$, below which $C(T)$ rapidly drops. This behavior is consistent with the data for KFe$_2$As$_2$ and related materials. We argue that the data on $C(T)$ can be reproduced without assuming that the quasiparticle residue $Z$ on $d_{xy}$ band is small. We further argue that the very existence of a finite $T^* < T_c$ favors $s^{+-}$ gap structure over $d-$wave, because in the latter case $T^*$ would vanish.

cond-mat.supr-con↗

Winding numbers of nodal points in Fe-based superconductors

We analyze the nodal points in multi-orbital Fe-based superconductors from a topological perspective. We consider the $s^{+-}$ gap structure with accidental nodes, and the $d$-wave gap with nodes along the symmetry directions. In both cases, the nodal points can be moved by varying an external parameter, e.g., a degree of inter-pocket pairing. Eventually, the nodes merge and annihilate via a Lifshitz-type transition. We discuss the Lifshitz transition in Fe-based superconductors from a topological point of view. We show, both analytically and numerically, that the merging nodal points have winding numbers of opposite sign. This is consistent with the general reasoning that the total winding number is a conserved quantity in the Lifshitz transition.

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