arXiv subjects

Doan-An Trieu

Publications and source records attributed to Doan-An Trieu.

5 recordsLinked to original sources

arXiv2026

Moderate-terahertz-induced plateau expansion of high-order harmonic generation to soft X-ray region

Extending the high-harmonic cutoff with experimentally accessible fields is essential for advancing tabletop coherent extreme ultraviolet (EUV) and soft X-ray sources. Although terahertz (THz) assistance offers a promising route, cutoff extension at weak, laboratory-accessible THz strengths remain poorly understood. In this report, we comprehensively investigate THz-assisted high-order harmonic generation (HHG) using time-dependent Schr\"odinger equation simulations supported by classical trajectory analysis and Bohmian-based quantum dynamics. By mapping the plateau evolution versus THz strength, we show that even weak THz fields can extend the cutoff, producing a pronounced ``fish-fin'' structure whose prominent rays saturate near $I_p + 8 U_p$. We trace this extension to long electron excursions spanning several optical cycles before recombination, and provide a fully consistent explanation using both classical analysis and Bohmian trajectories flow. Our findings reveal that this cutoff-extension mechanism is remarkably robust, persisting across different atomic species and remaining insensitive to variations in the driving parameters. These results demonstrate that cutoff control is achievable with laboratory-scale THz fields, offering practical guidelines for engineering coherent high-energy HHG, and providing a robust pathway for tracking ultrafast electron motion in real time.

physics.optics↗

arXiv2024

Machine-Learning-Based Construction of Molecular Potential and Its Application in Exploring the Deep-Lying-Orbital Effect in High-Order Harmonic Generation

Creating soft-Coulomb-type (SC) molecular potential within single-active-electron approximation (SAE) is essential since it allows solving time-dependent Schrödinger equations with fewer computational resources compared to other multielectron methods. The current available SC potentials can accurately reproduce the energy of the highest occupied molecular orbital (HOMO), which is sufficient for analyzing nonlinear effects in laser-molecule interactions like high-order harmonic generation (HHG). However, recent discoveries of significant effects of deep-lying molecular orbitals call for more precise potentials to analyze them. In this study, we present a fast and accurate method based on machine learning to construct SC potentials that simultaneously reproduce various molecular features, including energies, symmetries, and dipole moments of HOMO, HOMO-1, and HOMO-2. We use this ML model to create SC SAE potentials of the HCN molecule and then comprehensively analyze the fingerprints of lower-lying orbitals in HHG spectra emitted during the H-CN stretching. Our findings reveal that HOMO-1 plays a role in forming the second HHG plateau. Additionally, as the H-C distance increases, the plateau structure and the smoothness of HHG spectra are altered due to the redistribution of orbital electron density. These results are in line with other experimental and theoretical studies. Lastly, the machine learning approach using deconvolution and convolution neural networks in the present study is so general that it can be applied to construct molecular potential for other molecules and molecular dynamic processes.

physics.chem-ph↗

arXiv2024

Laser-target symmetry-breaking in high harmonic generation: from frequency shift to odd-even intensity modulation

Although the frequency shift and odd-even intensity modulation in high-order harmonic generation (HHG) have both been observed for asymmetric laser-target systems, they are typically studied as two separate phenomena. In this Letter, we provide a comprehensive picture of these two nonlinear optical phenomena, unifying them through a common origin - asymmetry of the laser-target system. By tuning asymmetric laser-target systems, we discover a transition from the harmonic frequency shift to the odd-even intensity modulation upon increasing the duration of the driving laser pulse. Specifically, these phenomena are observed simultaneously for laser pulses with intermediate pulse duration. For numerical evidence, we solve the time-dependent Schr\"{o}dinger equation, while insight into the underlying physics is obtained from a simplified analytically tractable model. Understanding the asymmetric characteristics reflected in the HHG as provided is crucial for retrieving laser-target information, sampling external fields, and probing molecular dynamics.

physics.optics↗

arXiv2024

Analytically controlling laser-induced electron phase in sub-cycle motion

Precise control of the electron phase accumulated during its sub-cycle motion within intense laser fields is essential in strong-field physics, yet remains mostly indirect and complicated so far. In this Letter, we develop a novel approach to control this sub-cycle electron phase by tuning a low-frequency electric field applied on a centrosymmetric gaseous target during its interaction with a few-cycle infrared laser pulse. Our method is based on a universal analytical relation between the low-frequency electric field and its induced harmonic frequency shift, derived by the strong-field approximation. This simple relation and its universality are confirmed numerically by directly solving the time-dependent Schr\"odinger equation. Moreover, we discuss the benefits of the discovered relation in \textit{in situ} applications, including continuously and precisely tuning XUV waves and developing a new method of comprehensively sampling THz pulse.

physics.optics↗

arXiv2023

Universality in odd-even harmonic generation and application in terahertz waveform sampling

Odd-even harmonics emitted from a laser-target system imprint rich, subtle information characterizing the system's dynamical asymmetry, which is desirable to decipher. In this Letter, we discover a simple universal relation between the odd-even harmonics and the asymmetry of the THz-assisted laser-atomic system -- atoms in a fundamental mid-IR laser pulse combined with a THz laser. First, we demonstrate numerically and then analytically formulize the harmonic even-to-odd ratio as a function of the THz electric field, the source of the system's asymmetry. Notably, we suggest a scaling that makes the obtained rule universal, independent of the parameters of both the fundamental pulse and atomic target. This universality facilitates us to propose a general pump-probe scheme for THz waveform sampling from the even-to-odd ratio, measurable within a conventional compact setup.

quant-ph↗