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Domenico de Ceglia

Publications and source records attributed to Domenico de Ceglia.

30 records · Page 2Linked to original sources

Second harmonic double resonance cones in dispersive hyperbolic metamaterials

We study the formation of second harmonic double-resonance cones in hyperbolic metamaterials. An electric dipole on the surface of the structure induces second harmonic light to propagate into two distinct volume plasmon-polariton channels: A signal that propagates within its own peculiar resonance cone; and a phase-locked signal that is trapped under the pump's resonance cone. Metamaterial dispersion and birefringence induce a large angular divergence between the two volume plasmon-polaritons, making these structures ideal for subwavelength second and higher harmonic imaging microscopy.

physics.optics↗

Low-damping epsilon-near-zero slabs: nonlinear and nonlocal optical properties

We investigate second harmonic generation, low-threshold multistability, all-optical switching, and inherently nonlocal effects due to the free-electron gas pressure in an epsilon-near-zero (ENZ) metamaterial slab made of cylindrical, plasmonic nanoshells illuminated by TM-polarized light. Damping compensation in the ENZ frequency region, achieved by using gain medium inside the shells' dielectric cores, enhances the nonlinear properties. Reflection is inhibited and the electric field component normal to the slab interface is enhanced near the effective pseudo-Brewster angle, where the effective ε-near-zero condition triggers a non-resonant, impedance-matching phenomenon. We show that the slab displays a strong effective, spatial nonlocality associated with leaky modes that are mediated by the compensation of damping. The presence of these leaky modes then induces further spectral and angular conditions where the local fields are enhanced, thus opening new windows of opportunity for the enhancement of nonlinear optical processes.

physics.optics↗

Electric Field Enhancement in ε-near-zero Slabs under TM-Polarized Oblique Incidence

We investigate local field enhancement phenomena in subwavelength, ε-near-zero (ENZ) slabs that do not exploit Fabry-Pérot resonances. In particular, we study the linear response of engineered metamaterial slabs of finite thickness based on plasmonic nanoshells that show an ENZ band in the visible range, and naturally occurring materials (e.g., SiO2) that also display ENZ properties, under oblique, TM-polarized plane wave incidence. We then introduce active gain material in engineered metamaterial slabs that adds peculiar spectral and angular features to transmission, reflection, and absorption properties, and leads to a further local field enhancement. These findings are supported by two theoretical studies: First, a simple interface between two semi-infinite media, namely free space and a generic ENZ medium; then, an ENZ slab of finite thickness, with the aim of understanding the system's behavior when varying the ENZ properties as well as the incident angle. For either case we report three distinct physical conditions for which we explain spectral and angular features that might result in strong field enhancement. The gain-assisted metamaterial implementation has the potential of triggering and enhancing low-threshold nonlinear phenomena thanks to the large local fields found at specific frequency and angular bands.

physics.optics↗

Gain assisted harmonic generation in near-zero permittivity metamaterials made of plasmonic nanoshells

We investigate enhanced harmonic generation processes in gain-assisted, near-zero permittivity metamaterials composed of spherical plasmonic nanoshells. We report the presence of narrow-band features in transmission, reflection and absorption induced by the presence of an active material inside the core of the nanoshells. The damping-compensation mechanism used to achieve the near-zero effective permittivity condition also induces a significant increase in field localization and strength and, consequently, enhancement of linear absorption. When only metal nonlinearities are considered, second and third harmonic generation efficiencies obtained by probing the structure in the vicinity of the near-zero permittivity condition approach values as high as for irradiance value as low as . These results clearly demonstrate that a relatively straightforward path now exists to the development of exotic and extreme nonlinear optical phenomena in the KW/cm2 range

physics.optics↗

Experimental demonstration of a novel bio-sensing platform via plasmonic band gap formation in gold nano-patch arrays

We discuss the possibility of implementing a novel bio-sensing platform based on the observation of the shift of the leaky surface plasmon mode that occurs at the edge of the plasmonic band gap of metal gratings when an analyte is deposited on top of the metallic structure. We provide experimental proof of the sensing capabilities of a two-dimensional array of gold nano-patches by observing color variations in the diffracted field when the air overlayer is replaced with a small quantity of Isopropyl Alcohol (IPA). Effects of rounded corners and surface imperfections are also discussed. Finally, we also report proof of changes in color intensities as a function of the air/filling ratio of the structure and discuss their relation with the diffracted spectra.

physics.optics↗

Harmonic generation and energy transport in dielectric and semiconductors at visible and UV wavelengths: the case of GaP

We study inhibition of absorption, transparency, energy and momentum transport of the inhomogeneous component of harmonic pulses in dielectrics and semiconductors, at visible and UV wavelengths, focusing on materials like GaP. In these spectral regions GaP is characterized by large absorption, metallic behavior or a combination of both. We show that phase locking causes the generated inhomogeneous signals to propagate through a bulk metallic medium without being absorbed, that is occurs even in centrosymmetric materials via the magnetic Lorentz force, and that the transport of energy and momentum is quite peculiar and seemingly anomalous. These results make it clear that there are new opportunities in ultrafast nonlinear optics and nano-plasmonics in new wavelength ranges.

physics.optics↗

Energy considerations for a superlens based on metal/dielectric multilayers

We investigate the resolution and absorption losses of a Ag/GaP multilayer superlens. For a fixed source to image distance the resolution is independent of the position of the lens but the losses depend strongly on the lens placement. The absorption losses associated with the evanescent waves can be significantly larger than losses associated with the propagating waves especially when the superlens is close to the source. The interpretation of transmittance values greater than unity for evanescent waves is clarified with respect to the associated absorption losses.

physics.optics↗

Anomalous Momentum States, Non-Specular Reflections, and Negative Refraction of Phase-Locked, Second Harmonic Pulses

We simulate and discuss novel spatio-temporal propagation effects that relate specifically to pulsed, phase-mismatched second harmonic generation in a negative index material having finite length. Using a generic Drude model for the dielectric permittivity and magnetic permeability, the fundamental and second harmonic frequencies are tuned so that the respective indices of refraction are negative for the pump and positive for the second harmonic signal. A phase-locking mechanism causes part of the second harmonic signal generated at the entry surface to become trapped and dragged along by the pump and to refract negatively, even though the index of refraction at the second harmonic frequency is positive. These circumstances culminate in the creation of an anomalous state consisting of a forward-moving second harmonic wave packet that has negative wave vector and momentum density, which in turn leads to non-specular reflections at intervening material interfaces. The forward-generated second harmonic signal trapped under the pump pulse propagates forward, but has all the attributes of a reflected pulse, similar to its twin counterpart generated at the surface and freely propagating backward away from the interface. This describes a new state of negative refraction, associated with nonlinear frequency conversion and parametric processes, whereby a beam generated at the interface can refract negatively even though the index of refraction at that wavelength is positive.

physics.optics↗

Enhancement and Inhibition of Stimulated Processes in a Negative Index Cavity

We study second harmonic generation in a negative index material cavity. The transmission spectrum shows a gap between the electric and magnetic plasma frequencies, so that localized and anti-localized states are allowed at the band edges. The process is made efficient by local phase matching conditions between a forward-propagating pump and a backward-propagating second harmonic signal. By simultaneously exciting the cavity with counter-propagating pulses one is able to enhance or inhibit absorption and stimulated processes. The control parameter is the relative phase difference between the two incident pulses which determines the interference properties of the fields inside the cavity.

physics.optics↗

Analysis of second harmonic generation in photonic-crystal-assisted waveguides

We study second harmonic generation in a planar dielectric waveguide having a low-index, polymer core layer, bounded by two multilayer stacks. This geometry allows exceptionally strong confinement of the light at the fundamental wavelength inside the core region with virtually zero net propagation losses for distances that exceed several centimeters, provided material and scattering losses are neglected. A phase-matched configuration of the waveguide is reported in which the pump signal is the lowest-order mode of the waveguide, and the generated second harmonic signal corresponds to the third propagation mode of the waveguide. Using a polymer waveguide core, having chi(2)=100 pm/V, we predict a conversion efficiency of approximately 90% after a propagation distance of 2 mm, using peak pump intensities inside the core of the waveguide of 1.35 GW/cm^2. If the waveguide core contains polymer layers with different glass transition temperatures, the layers can be poled independently to maximize the overlap integral, and similar pump depletions may be achieved over a distance of approximately 500 microns.

physics.optics↗

Gap solitons in a nonlinear quadratic negative index cavity

By integrating the full Maxwell's equations we predict the existence of gap solitons in a quadratic, Fabry-Perot negative index cavity. An intense, fundamental pump pulse shifts the band structure that forms when magnetic and electric plasma frequencies are different so that a weak, second harmonic pulse initially tuned inside the gap is almost entirely transmitted. The process is due cascading, which occurs far from phase matching conditions, and causes pulse compression. A nonlinear polarization spawns a dark soliton, while a nonlinear magnetization produces a bright soliton.

physics.optics↗

Negative refraction and sub-wavelength imaging using transparent metal-dielectric stacks

Negative refraction is known to occur in materials that simultaneously possess a negative electric permittivity and magnetic permeability; hence they are termed negative index materials. However, there are no known natural materials that exhibit a negative index of refraction. In large part, interest in these materials is due to speculation that they could be used as perfect lenses with superresolution. We propose a new way of achieving negative refraction with currently available technology, based on transparent, metallo-dielectric multilayer structures. The advantage of these structures is that both tunability and transmission (well above 50%) can be achieved in the visible wavelength regime. We demonstrate both negative refraction and superresolution in these structures. Our findings point to a simpler way to fabricate a material that exhibits negative refraction. This opens up an entirely new path not only for negative refraction, but also to expand the exploration of wave propagation effects in metals.

physics.optics↗