arXiv subjects

Dominique Chauvat

Publications and source records attributed to Dominique Chauvat.

3 recordsLinked to original sources

arXiv2007

Enhancing single-molecule photostability by optical feedback from quantum-jump detection

We report an optical technique that yields an enhancement of single-molecule photostability, by greatly suppressing photobleaching pathways which involve photoexcitation from the triplet state. This is accomplished by dynamically switching off the excitation laser when a quantum-jump of the molecule to the triplet state is optically detected. This procedure leads to a lengthened single-molecule observation time and an increased total number of detected photons. The resulting improvement in photostability unambiguously confirms the importance of photoexcitation from the triplet state in photobleaching dynamics, and may allow the investigation of new phenomena at the single-molecule level.

quant-ph↗

arXiv2006

Balanced homodyne detection in second-harmonic generation microscopy

We demonstrate the association of two-photon nonlinear microscopy with balanced homodyne detection for investigating second harmonic radiation properties at nanoscale dimensions. Variation of the relative phase between second-harmonic and fundamental beams is retrieved, as a function of the absolute orientation of the nonlinear emitters. Sensitivity down to approximately 3.2 photon/s in the spatio-temporal mode of the local oscillator is obtained. This value is high enough to efficiently detect the coherent second-harmonic emission from a single KTiOPO4 crystal of sub-wavelength size.

physics.optics↗

arXiv2005

Demonstration of an optical polarization magnifier with low birefringence

In any polarimetric measurement technique, enhancing the laser polarization change of a laser beam before it reaches the analyzer can help in improving the sensitivity. This can be performed using an optical component having a large linear dichroism, the enhancement factor being equal to the square root of the ratio of the two transmission factors. A pile of parallel plates at Brewster incidence looks appropriate for realizing such a polarization magnifier. In this paper, we address the problem raised by the interference in the plates and between the plates, which affects the measurement by giving rise to birefringence. We demonstrate that wedged plates provide a convenient and efficient way to avoid this interference. We have implemented and characterized devices with 4 and 6 wedged plates at Brewster incidence which have led to a decisive improvement of the signal to noise ratio in our ongoing Parity Violation measurement.

physics.optics↗