arXiv subjects

Dorian A. Gangloff

Publications and source records attributed to Dorian A. Gangloff.

At least 19 recordsLinked to original sources

arXiv2026

Autonomous stabilization of many-body entanglement with Floquet Hamiltonians and weak measurement

Reaching a technological advantage with large quantum systems requires safeguarding their many-body entanglement. Dissipation typically acts to decohere a quantum system via random projective noise but, when judiciously engineered together with coherent interactions, it can funnel the system towards a target entangled state. The native interactions and dissipative channels available to most systems are, however, difficult to combine effectively. Here we propose interleaving Floquet Hamiltonian engineering, which allows the construction of non-native coherent interactions, with weak measurement, which enables a tuneable dissipative channel, to enable programmable and autonomous stabilization of many-body entanglement. We show this analytically and numerically for the central-spin system of a semiconductor quantum dot, for which we construct spin-squeezed and Schrödinger-cat states that are stabilized against realistic levels of dephasing. Our approach is applicable to any system compatible with periodic drives and tuneable measurement strength and could enable novel approaches to practical error correction.

quant-ph↗

arXiv2026

Coherent Control of Quantum-Dot Spins with Cyclic Optical Transitions

Solid-state spins are promising as interfaces from stationary qubits to single photons for quantum communication technologies. Semiconductor quantum dots have excellent optical coherence, exhibit near unity collection efficiencies when coupled to photonic structures, and possess long-lived spins for quantum memory. However, the incompatibility of performing optical spin control and single-shot readout simultaneously has been a challenge faced by almost all solid-state emitters. To overcome this, we leverage light-hole mixing to realize a highly asymmetric lambda system in a negatively charged heavy hole exciton in Faraday configuration. By compensating GHz-scale differential Stark shifts, induced by unequal coupling to Raman control fields, and by performing nuclear-spin cooling, we achieve quantum control of an electron-spin qubit with a $π$-pulse contrast of 97.4% while preserving spin-selective optical transitions with a cyclicity of 471 (50). We demonstrate this scheme for both GaAs and InGaAs quantum dots, and show that it is compatible with the operation of a nuclear quantum memory. Our approach thus enables repeated emission of indistinguishable photons together with qubit control, as required for single-shot readout, photonic cluster-state generation, and quantum repeater technologies.

quant-ph↗

arXiv2026

Crossover from Rabi oscillations to adiabatic population switching in the Faraday optical control of quantum dot spins

Stimulated Raman transitions in Faraday geometry allow for simultaneous single-shot qubit readout and qubit control. It involves driving an unbalanced $Λ$ system via an auxiliary excited state. Due to the simultaneous driving of both transitions with unequal detuning, the resulting time-dependent Stark shift gives rise to additional resonance conditions beyond the conventional picture. We identify a distinct regime in which repeated passages through avoided crossings lead to step-like population inversion arising from Landau-Zener-Stückelberg interference. By changing the detuning beatnote, we demonstrate a controlled continuous crossover from Rabi-like oscillations to adiabatic population switching. These findings establish the oscillating Stark shift as a mechanism for engineering and controlling spin dynamics in Faraday geometry.

cond-mat.mes-hall↗

arXiv2026

Randomised measurements of a disorder-induced entanglement transition in a neutral atom quantum processor

The development and spread of entanglement in complex quantum systems is central to exploring many-body phenomena out of equilibrium. Measuring entanglement dynamics can shed light on information scrambling and thermalisation, namely on transitions from many-body quantum chaos to localisation in disordered, interacting systems. In quantum computing systems, entanglement entropy and other nonlinear functions of the density matrix have been recently measured, in particular by using the randomised measurement toolbox. However, it is difficult to implement the required arbitrary unitary rotations on specific subsystems without universal local control. Here we devise and demonstrate the measurement of entanglement entropy in a programmable analogue quantum simulator using a randomised measurement protocol that leverages local energy tuning together with a global field to bypass the need for local gate control. We implement this on a commercially available neutral-atom quantum simulator, QuEra's Aquila, and use it to show how programmable disorder in the local Hamiltonian parameters leads to a transition from chaotic to localised entanglement dynamics. Given current decoherence times, we clearly resolve disorder-specific, time-dependent entanglement spreading in small systems. Our work extends the utility of programmable analogue quantum simulators, and opens further opportunities for wider randomised measurement toolboxes in a range of other analogue systems.

quant-ph↗

arXiv2026

A fault-tolerant encoding for qubit-controlled collective spins

Quantum error correction (QEC) is indispensable for scalable quantum computing, but implementing it with minimal hardware overhead remains a central challenge. Large spin systems with collective degrees of freedom offer a promising route to reducing the control complexity of qubit architectures while retaining a large Hilbert space for fault-tolerant encoding. However, existing proposals for logical gates and QEC in spin ensembles generally rely on inefficient higher-order interactions. Here we introduce spin-N-Cat codes, which encode logical qubits in superpositions of spin-coherent states and generalize bosonic Cat codes to the modular subspaces of permutationally symmetric spin ensembles. The code corrects collective and individual dephasing, excitation, and decay errors. We also present an efficient physical realization in central-spin systems, such as a quantum dot, where encoding, decoding, and a universal, fault-tolerant, and bias-preserving gate set are implemented using only first-order interactions. Numerical simulations demonstrate high logical fidelity under dephasing and excitation-decay noise, independent of noise bias, and that full QEC cycles are feasible with realistic microscopic parameters. For the large collective spins available in quantum dots, this translates into a substantial extension of coherence time. Our results establish spin-N-Cat codes as a scalable, hardware-efficient approach to QEC in spin-based quantum architectures.

quant-ph↗

arXiv2024

Qudit-based quantum error-correcting codes from irreducible representations of SU(d)

Qudits naturally correspond to multi-level quantum systems, which offer an efficient route towards quantum information processing, but their reliability is contingent upon quantum error correction capabilities. In this paper, we present a general procedure for constructing error-correcting qudit codes through the irreducible representations of $\mathrm{SU}(d)$ for any odd integer $d \geq 3.$ Using the Weyl character formula and inner product of characters, we deduce the relevant branching rules, through which we identify the physical Hilbert spaces that contain valid code spaces. We then discuss how two forms of permutation invariance and the Heisenberg-Weyl symmetry of $\mathfrak{su}(d)$ can be exploited to simplify the construction of error-correcting codes. Finally, we use our procedure to construct an infinite class of error-correcting codes encoding a logical qudit into $(d-1)^2$ physical qudits.

quant-ph↗

arXiv2024

Laser Activation of Single Group-IV Colour Centres in Diamond

Spin-photon interfaces based on group-IV colour centres in diamond offer a promising platform for quantum networks. A key challenge in the field is realizing precise single-defect positioning and activation, which is crucial for scalable device fabrication. Here we address this problem by demonstrating a two-step fabrication method for tin vacancy (SnV-) centres that uses site-controlled ion implantation followed by local femtosecond laser annealing with in-situ spectral monitoring. The ion implantation is performed with sub-50 nm resolution and a dosage that is controlled from hundreds of ions down to single ions per site, limited by Poissonian statistics. Using this approach, we successfully demonstrate site-selective creation and modification of single SnV- centres. The technique opens a window onto materials tuning at the single defect level, and provides new insight into defect structures and dynamics during the annealing process. While demonstrated for SnV- centres, this versatile approach can be readily generalised to other implanted colour centres in diamond and wide-bandgap materials.

quant-ph↗

arXiv2024

Tuning the coherent interaction of an electron qubit and a nuclear magnon

A central spin qubit interacting coherently with an ensemble of proximal spins can be used to engineer entangled collective states or a multi-qubit register. Making full use of this many-body platform requires tuning the interaction between the central spin and its spin register. GaAs quantum dots offer a model realization of the central spin system where an electron qubit interacts with multiple ensembles of $\sim 10^{4}$ nuclear spins. In this work, we demonstrate tuning of the interaction between the electron qubit and the nuclear many-body system in a GaAs quantum dot. The homogeneity of the GaAs system allows us to perform high-precision and isotopically selective nuclear sideband spectroscopy, which reveals the single-nucleus electronic Knight field. Together with time-resolved spectroscopy of the nuclear field, this fully characterizes the electron-nuclear interaction for a priori control. An algorithmic feedback sequence selects the nuclear polarization precisely, which adjusts the electron-nuclear exchange interaction in situ via the electronic g-factor anisotropy. This allows us to tune directly the activation rate of a collective nuclear excitation (magnon) and the coherence time of the electron qubit. Our method is applicable to similar central-spin systems and enables the programmable tuning of coherent interactions in the many-body regime.

quant-ph↗

arXiv2024

Many-body quantum register for a spin qubit

Quantum networks require quantum nodes with coherent optical interfaces and multiple stationary qubits. In terms of optical properties, semiconductor quantum dots are highly compelling, but their adoption as quantum nodes has been impaired by the lack of auxiliary qubits. Here, we demonstrate a functional quantum register in a semiconductor quantum dot leveraging the dense, always-present nuclear spin ensemble. We prepare 13,000 host nuclear spins into a single many-body dark state to operate as the register logic state $|0\rangle$. The logic state $|1\rangle$ is defined as a single nuclear magnon excitation, enabling controlled quantum-state transfer between the electron spin qubit and the nuclear magnonic register. Using 130-ns SWAP gates, we implement a full write-store-retrieve-readout protocol with 68.6(4)% raw overall fidelity and a storage time of 130(16) $μ$s in the absence of dynamical decoupling. Our work establishes how many-body physics can add step-change functionality to quantum devices, in this case transforming quantum dots into multi-qubit quantum nodes with deterministic registers.

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arXiv2023

Time-crystalline behavior in central-spin models with Heisenberg interactions

Time-crystalline behavior has been predicted and observed in quantum central-spin systems with periodic driving and Ising interactions. Here, we theoretically show that it can also arise in central-spin systems with Heisenberg interactions. We present two methods to achieve this: application of a sufficiently large Zeeman splitting on the central spin compared to the satellite spins, or else by applying additional pulses to the central spin every Floquet period. In both cases, we show that the system exhibits a subharmonic response in spin magnetizations in the presence of disorder for both pure Heisenberg and XXZ interactions. Our results pertain to any XXZ central-spin system, including hyperfine-coupled electron-nuclear systems in quantum dots or color centers.

quant-ph↗

arXiv2023

A many-body singlet prepared by a central spin qubit

Controllable quantum many-body systems are platforms for fundamental investigations into the nature of entanglement and promise to deliver computational speed-up for a broad class of algorithms and simulations. In particular, engineering entanglement within a dense spin ensemble can turn it into a robust quantum memory or a computational platform. Recent experimental progress in dense central spin systems motivates the design of algorithms that use a central-spin qubit as a convenient proxy for the ensemble. Here we propose a protocol that uses a central spin to initialize two dense spin ensembles into a pure anti-polarized state and from there creates a many-body entangled state -- a singlet -- from the combined ensemble. We quantify the protocol performance for multiple material platforms and show that it can be implemented even in the presence of realistic levels of decoherence. Our protocol introduces an algorithmic approach to preparation of a known many-body state and to entanglement engineering in a dense spin ensemble, which can be extended towards a broad class of collective quantum states.

quant-ph↗

arXiv2022

Photonic indistinguishability of the tin-vacancy center in nanostructured diamond

Tin-vacancy centers in diamond are promising spin-photon interfaces owing to their high quantum-efficiency, large Debye-Waller factor, and compatibility with photonic nanostructuring. Benchmarking their single-photon indistinguishability is a key challenge for future applications. Here, we report the generation of single photons with $99.7^{+0.3}_{-2.5}\%$ purity and $63(9)\%$ indistinguishability from a resonantly excited tin-vacancy center in a single-mode waveguide. We obtain quantum control of the optical transition with $1.71(1)$-ns-long $π$-pulses of $77.1(8)\%$ fidelity. A modest Purcell enhancement factor of 12 would enhance the indistinguishability to $95$\%. The greater than $100$ ms spectral stability shown would then enable strings of up to $10^6$ identical photons to be generated.

quant-ph↗

arXiv2022

Ideal refocusing of an optically active spin qubit under strong hyperfine interactions

Combining highly coherent spin control with efficient light-matter coupling offers great opportunities for quantum communication and networks, as well as quantum computing. Optically active semiconductor quantum dots have unparalleled photonic properties, but also modest spin coherence limited by their resident nuclei. Here, we demonstrate that eliminating strain inhomogeneity using lattice-matched GaAs-AlGaAs quantum dot devices prolongs the electron spin coherence by nearly two orders of magnitude, beyond 0.113(3) ms. To do this, we leverage the 99.30(5)% fidelity of our optical pi-pulse gates to implement dynamical decoupling. We vary the number of decoupling pulses up to N = 81 and find a coherence time scaling of N^{0.75(2)}. This scaling manifests an ideal refocusing of strong interactions between the electron and the nuclear-spin ensemble, holding the promise of lifetime-limited spin coherence. Our findings demonstrate that the most punishing material science challenge for such quantum-dot devices has a remedy, and constitute the basis for highly coherent spin-photon interfaces.

cond-mat.mes-hall↗

arXiv2021

Witnessing quantum correlations in a nuclear ensemble via an electron spin qubit

A coherent ensemble of spins interfaced with a proxy qubit is an attractive platform to create many-body coherences and probe the regime of collective excitations. An electron spin qubit in a semiconductor quantum dot can act as such an interface to the dense nuclear spin ensemble within the quantum dot consisting of multiple high-spin atomic species. Earlier work has shown that the electron can relay properties of its nuclear environment through the statistics of its mean-field interaction with the total nuclear polarisation, namely its mean and variance. Here, we demonstrate a method to probe the spin state of a nuclear ensemble that exploits its response to collective spin excitations, enabling a species-selective reconstruction beyond the mean field. For the accessible range of optically prepared mean fields, the reconstructed populations indicate that the ensemble is in a non-thermal, correlated nuclear state. The sum over reconstructed species-resolved polarisations exceeds the classical prediction threefold. This stark deviation follows from a spin ensemble that contains inter-particle coherences, and serves as an entanglement witness that confirms the formation of a dark many-body state.

cond-mat.mes-hall↗

arXiv2021

Optimal purification of a spin ensemble by quantum-algorithmic feedback

Purifying a high-temperature ensemble of quantum particles towards a known state is a key requirement to exploit quantum many-body effects. An alternative to passive cooling, which brings a system to its ground state, is based on feedback to stabilise the system actively around a target state. This alternative, if realised, offers additional control capabilities for the design of quantum states. Here we present a quantum feedback algorithm capable of stabilising the collective state of an ensemble from an infinite-temperature state to the limit of single quanta. We implement this on ~50,000 nuclei in a semiconductor quantum dot, and show that the nuclear-spin fluctuations are reduced 83-fold down to 10 spin macrostates. While our algorithm can purify a single macrostate, system-specific inhomogeneities prevent reaching this limit. Our feedback algorithm further engineers classically correlated ensemble states via macrostate tuning, weighted bimodality, and latticed multistability, constituting a pre-cursor towards quantum-correlated macrostates.

quant-ph↗

arXiv2021

Multidimensional cluster states using a single spin-photon interface coupled strongly to an intrinsic nuclear register

Photonic cluster states are a powerful resource for measurement-based quantum computing and loss-tolerant quantum communication. Proposals to generate multi-dimensional lattice cluster states have identified coupled spin-photon interfaces, spin-ancilla systems, and optical feedback mechanisms as potential schemes. Following these, we propose the generation of multi-dimensional lattice cluster states using a single, efficient spin-photon interface coupled strongly to a nuclear register. Our scheme makes use of the contact hyperfine interaction to enable universal quantum gates between the interface spin and a local nuclear register and funnels the resulting entanglement to photons via the spin-photon interface. Among several quantum emitters, we identify the silicon-29 vacancy centre in diamond, coupled to a nanophotonic structure, as possessing the right combination of optical quality and spin coherence for this scheme. We show numerically that using this system a 2x5-sized cluster state with a lower-bound fidelity of 0.5 and repetition rate of 65 kHz is achievable under currently realised experimental performances and with feasible technical overhead. Realistic gate improvements put 100-photon cluster states within experimental reach.

quant-ph↗

arXiv2021

Quantum control of the tin-vacancy spin qubit in diamond

Group-IV color centers in diamond are a promising light-matter interface for quantum networking devices. The negatively charged tin-vacancy center (SnV) is particularly interesting, as its large spin-orbit coupling offers strong protection against phonon dephasing and robust cyclicity of its optical transitions towards spin-photon entanglement schemes. Here, we demonstrate multi-axis coherent control of the SnV spin qubit via an all-optical stimulated Raman drive between the ground and excited states. We use coherent population trapping and optically driven electronic spin resonance to confirm coherent access to the qubit at 1.7 K, and obtain spin Rabi oscillations at a rate of $Ω/2π$=3.6(1) MHz. All-optical Ramsey interferometry reveals a spin dephasing time of $T_2^*$=1.3(3)$μ$s and two-pulse dynamical decoupling already extends the spin coherence time to $T_2$=0.33(14) ms. Combined with transform-limited photons and integration into photonic nanostructures, our results make the SnV a competitive spin-photon building block for quantum networks.

quant-ph↗

arXiv2020

Quantum sensing of a coherent single spin excitation in a nuclear ensemble

The measurement of single quanta in a collection of coherently interacting objects is transformative in the investigations of emergent quantum phenomena. An isolated nuclear-spin ensemble is a remarkable platform owing to its coherence, but detecting its single spin excitations has remained elusive. Here, we use an electron spin qubit in a semiconductor quantum dot to sense a single nuclear-spin excitation (a nuclear magnon) with 1.9-ppm precision via the 200-kHz hyperfine shift on the 28-GHz qubit frequency. We demonstrate this single-magnon precision across multiple modes identified by nuclear species and polarity. Finally, we monitor the coherent dynamics of a nuclear magnon and the emergence of quantum correlations competing against decoherence. A direct extension of this work is to probe engineered quantum states of the ensemble including long-lived memory states.

quant-ph↗