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Douglas A. Bonn

Publications and source records attributed to Douglas A. Bonn.

7 recordsLinked to original sources
arXiv2025

Intrinsic defect intolerance in the ultra-pure metal PtSn$_4$

Ultra-pure materials are highly valued as model systems for the study of intrinsic physics. Frequently, however, the crystal growth of such pristine samples requires significant optimization. PtSn$_4$ is a rare example of a material that naturally forms with a very low concentration of crystalline defects. Here, we investigate the origin of its low defect levels using a combination of electrical resistivity measurements, computational modeling, and scanning tunneling microscopy imaging. While typical flux-grown crystals of PtSn$_4$ can have residual resistivity ratios (RRRs) that exceed 1000, we show that even at the most extreme formation speeds, the RRR cannot be suppressed below 100. This aversion to defect formation extends to both the Pt and Sn sublattices, which contribute with equal weight to the conduction properties. Direct local imaging with scanning tunneling microscopy further substantiates the rarity of point defects, while the prohibitive energetic cost of forming a defect is demonstrated through density functional theory calculations. Taken together, our results establish PtSn$_4$ as an intrinsically defect-intolerant material, making it an ideal platform to study other properties of interest, including extreme magnetoresistance and topology.

cond-mat.mtrl-sci↗
arXiv2023

Kinetic theory of the non-local electrodynamic response in anisotropic metals: skin effect in 2D systems

The electrodynamic response of ultra-pure materials at low temperatures becomes spatially non-local. This non-locality gives rise to phenomena such as hydrodynamic flow in transport and the anomalous skin effect in optics. In systems characterized by an anisotropic electronic dispersion, the non-local dynamics becomes dependent on the relative orientation of the sample with respect to the applied field, in ways that go beyond the usual, homogeneous response. Such orientational dependence should manifest itself not only in transport experiments, as recently observed, but also in optical spectroscopy. In this paper we develop a kinetic theory for the distribution function and the transverse conductivity of two- and three-dimensional Fermi systems with anisotropic electronic dispersion. By expanding the collision integral into the eigenbasis of a collision operator, we include momentum-relaxing scattering as well as momentum-conserving collisions. We examine the isotropic 2D case as a reference, as well as anisotropic hexagonal and square Fermi-surface shapes. We apply our theory to the quantitative calculation of the skin depth and the surface impedance, in all regimes of skin effect. We find qualitative differences between the frequency dependence of the impedance in isotropic and anisotropic systems. Such differences are shown to persist even for more complex 2D Fermi surfaces, including the ''supercircle'' geometry and an experimental parametrization for PdCoO$_2$, which deviate from an ideal polygonal shape. We study the orientational dependence of skin effect due to Fermi-surface anisotropy, thus providing guidance for the experimental study of non-local optical effects.

cond-mat.str-el↗
arXiv2021

The Three-Dimensional Electronic Structure of LiFeAs: Strong-coupling Superconductivity and Topology in the Iron Pnictides

Amongst the iron-based superconductors, LiFeAs is unrivalled in the simplicity of its crystal structure and phase diagram. However, our understanding of this canonical compound suffers from conflict between mutually incompatible descriptions of the material's electronic structure, as derived from contradictory interpretations of the photoemission record. Here, we explore the challenge of interpretation in such experiments. By combining comprehensive photon energy- and polarization- dependent angle-resolved photoemission spectroscopy (ARPES) measurements with numerical simulations, we establish the providence of several contradictions in the present understanding of this and related materials. We identify a confluence of surface-related issues which have precluded unambiguous identification of both the number and dimensionality of the Fermi surface sheets. Ultimately, we arrive at a scenario which supports indications of topologically non-trivial states, while also being incompatible with superconductivity as a spin-fluctuation driven Fermi surface instability.

cond-mat.supr-con↗
arXiv2011

Magnetic force microscopy measurement of the penetration depth in superconductors from Meissner repulsion

We report a method to locally measure the penetration depth $λ$ in a superconductor by detecting the diamagnetic response using magnetic force microscopy (MFM). We extract $λ$ by fitting the height dependence of the levitation force in the Meissner state using an analytical model that approximates the MFM tip as a single-domain, truncated conical shell. We demonstrate on two YBa$_2$Cu$_3$O$_{6+x}$ single crystals with two MFM tips that the obtained values agree well with previous results. This approach is not affected by the tip width and can be applied to similar but not identical tips.

cond-mat.supr-con↗
arXiv2008

Magnetic-force-microscope study of interlayer "kinks" in individual vortices in underdoped cuprate YBa$_2$Cu$_3$O$_{6+x}$ superconductor

We use magnetic force microscopy to both image and manipulate individual vortex lines threading single crystalline YBa$_2$Cu$_3$O$_{6.4}$, a layered superconductor. We find that when we pull the top of a pinned vortex, it may not tilt smoothly. Sometimes, we observe a vortex to break into discrete segments that can be described as short stacks of pancake vortices, similar to the "kinked" structure proposed by Benkraouda and Clem. Quantitative analysis gives an estimate of the pinning force and the coupling between the stacks. Our measurements highlight the discrete nature of stacks of pancake vortices in layered superconductors.

cond-mat.supr-con↗
arXiv2008

Mechanics of Individual, Isolated Vortices in a Cuprate Superconductor

Superconductors often contain quantized microscopic whirlpools of electrons, called vortices, that can be modeled as one-dimensional elastic objects. Vortices are a diverse playground for condensed matter because of the interplay between thermal fluctuations, vortex-vortex interactions, and the interaction of the vortex core with the three-dimensional disorder landscape. While vortex matter has been studied extensively, the static and dynamic properties of an individual vortex have not. Here we employ magnetic force microscopy (MFM) to image and manipulate individual vortices in detwinned, single crystal YBa2Cu3O6.991 (YBCO), directly measuring the interaction of a moving vortex with the local disorder potential. We find an unexpected and dramatic enhancement of the response of a vortex to pulling when we wiggle it transversely. In addition, we find enhanced vortex pinning anisotropy that suggests clustering of oxygen vacancies in our sample and demonstrates the power of MFM to probe vortex structure and microscopic defects that cause pinning.

cond-mat.supr-con↗