arXiv subjects

Dung-Hai Lee

Publications and source records attributed to Dung-Hai Lee.

At least 19 recordsLinked to original sources

arXiv2026

Selective coupling of high-order phonons in La2-xSrxCuO4

In crystals and molecules with strong coupling between the charge carriers and atomic vibrations, high order harmonics of the vibrational excitations can be observed with intensity following the Franck-Condon envelope. Here, we uncover a new regime of electron-phonon coupling in La2-xSrxCuO4 using resonant inelastic X-ray scattering. In the undoped compound, we find sharp peaks at approximately 85$\pm$5 meV, 180$\pm$7 meV, and 330$\pm$5 meV with no observable dispersion, and an absence of appreciable intensity from other modes observed in Raman spectroscopy in this energy range. The 180 meV and 330 meV excitations have energies approximately consistent with two-phonon and four-phonon in-plane Cu-O bond stretching mode, suggesting that the resonantly excited valence electrons strongly couple to this mode. These excitations exhibit significant doping dependence, eventually becoming unresolvable at 10% hole doping, where the low energy charge excitations are dominated by dispersive plasmons. The observation of selective coupling to even-ordered phonons and stark contrast with the Raman spectra indicate anomalous electron-phonon coupling beyond the Franck-Condon picture. One intriguing possibility is the existence of locally paired quasiparticles in insulating cuprates.

cond-mat.str-el↗

arXiv2026

Interacting Chern insulator transition on the sphere: revealing the Gross-Neveu-Yukawa criticality

In two spatial dimensions, the transition between topological and trivial Chern insulators exemplifies a class of beyond-Landau critical phenomena. We show that the interaction-driven multicritical point of this transition falls into the Gross-Neveu-Yukawa (GNY) universality class, a topic of considerable interest in both high-energy and condensed matter physics. In this work, we focus on the $N=2$ case of the GNY criticality. We employ exact diagonalization of Dirac fermions on a sphere to circumvent the parity anomaly, capitalize on full $SO(3)$ symmetry to reduce finite-size effects, and directly extract operator scaling dimensions from the excitation spectrum. Despite working with only modest system sizes, our results closely match conformal bootstrap predictions for low-scaling dimension operators and reveal several previously uncharacterized higher primaries. These findings highlight the efficacy of spherical geometry for probing interacting Dirac criticality.

cond-mat.str-el↗

arXiv2026

Terahertz electrodynamics in a zero-field Wigner crystal

In clean two-dimensional (2D) systems, electrons are expected to self-organize into a regular lattice, a Wigner crystal, when their mutual Coulomb repulsion overwhelms kinetic energy. Understanding the Wigner crystal at zero magnetic field is a long-sought goal in physics, thanks to its fundamental simplicity and possible connection to the density-driven metal-insulator transition. To date, evidence for such a crystal has been reported across various platforms. However, the AC conductivity of a zero-field Wigner crystal, a key observable characterizing its electrodynamics, has never been measured. Here, we develop an ultrasensitive on-chip terahertz (THz) spectroscopy technique to probe the AC conductivity in electrostatically gated monolayer MoSe2 encapsulated in hexagonal boron nitride. We observe a sub-THz resonance corresponding to the pinning mode of a zero-field Wigner crystal, whose frequency is orders of magnitude higher than those under high magnetic fields. Using the pinning mode as an indicator, we reveal that moderate disorder notably stabilizes the Wigner crystal. With increasing density towards melting, we find that the pinning mode of the Wigner crystal coexists with a growing Drude component characteristic of an electron liquid, and the competition between these two components in the conductivity spectra leads to the insulator-metal transition of the 2D electron system. Our findings not only elucidate the low-energy electrodynamics of a zero-field Wigner crystal, but also establish on-chip THz spectroscopy as a powerful probe for correlated quantum phases in two-dimensional materials.

cond-mat.mes-hall↗

arXiv2026

Bulk Superconductivity driven by Disorder-Induced Delocalization in 4Hb-Ta(S$_{1-x}$Se$_x$)$_2$

The unconventional superconductor 4Hb-TaS$_2$ is a natural heterostructure that can be broadly understood as interleaving Mott-like and metallic layers. We study the properties of this material as a function of quenched disorder in the form of Se/S substitution and find that while disordered samples show bulk superconductivity, clean samples do not. We show that a disorder-driven delocalization of carriers in the Mott-like ($1T$-) layer forms a new Fermi surface that is absent in the cleanest samples. This suggests that one of the primary drivers for superconductivity is the fragility of the Mott state, whose delocalization brings to life a sea of strongly correlated electrons.

cond-mat.supr-con↗

arXiv2026

Spectroscopic evidence for a molecular orbital Kondo insulator

A Kondo insulator (KI) is a prototypical example of a highly entangled phase of matter, where many-body interactions between local moments and delocalized electrons engender the non-magnetic insulating ground state. Conventionally, the local moments arise from atomic multiplet states with a narrow bandwidth, limiting Kondo coherence to low temperatures. Here, we realize a new paradigm for constructing the KI state with hybridized molecular orbitals in FeSb2. Resonant inelastic X-ray scattering (RIXS) at the Fe L-edge reveals distinct signatures of band-like continuum states and localized states. Comparisons with first-principles calculations establish a mixed-configuration ground state with hybridized Fe d-Sb p molecular orbitals as basis states. By systematically investigating the RIXS momentum, temperature, and doping dependences, we find propagating collective modes commensurate with many-body charge and spin excitations. Our results pave the way for understanding the emerging class of unconventional d electron insulators and engineering high temperature Kondo many-body states.

cond-mat.str-el↗

arXiv2026

Strongly-coupled hybrid lattice-plasmons in layered cuprates

Metallic systems with delocalized valence electrons host collective charge density oscillations known as plasmons. On the other hand, conventional insulators do not have free electrons and the low energy charge degrees of freedom are pinned to the ions. The fate of the collective charge excitations in the intermediate regime is an outstanding question. This problem is especially important for strongly correlated systems such as the layered cuprates, where unconventional superconductivity and other emergent phenomena arise from valence electrons on the border between Mott localization and itinerancy. Using resonant inelastic X-ray scattering, we track this evolution in the prototypical electron-doped cuprate Nd2-xCexCuO4. We find a continuous transformation of the low-energy charge response: from an acoustic plasmon in the metallic regime, to a gapped hybrid mode at intermediate doping, and finally to a nearly dispersionless 139 meV excitation at half filling. Remarkably, the 139 meV excitation has approximately twice the energy of the oxygen breathing phonon responsible for the dispersion kink observed in angle-resolved photoemission spectroscopy, and is consistent with a putative 2-phonon excitation observed in Raman spectroscopy. These results establish a unified picture of collective charge excitations across the phase diagram of electron-doped cuprates, showing that such modes persist across the Mott transition via strong coupling to lattice degrees of freedom and revealing a missing link in the charge dynamics of carrier doped Mott insulators.

cond-mat.str-el↗

arXiv2026

Non-local low energy neutral excitations in a strongly disordered triangular Mott magnet Cr$_3$Se$_2$Br$_5$

Understanding if low-energy excitations can remain itinerant in the presence of strong disorder remains a central challenge in frustrated quantum magnets, where disorder is generally expected to localize excitations through Anderson-like mechanisms. Here we report the emergence of charge-neutral itinerant excitations in a van der Waals compound Cr$_3$Se$_2$Br$_5$, a strongly disordered $S = 3/2$ Mott insulator with a frustrated triangular lattice. Structural analysis reveals substantial intrinsic disorder arising from Cr-site deficiency and Se/Br-site mixing, which appear to be fixed and cannot be readily tuned. No long-range magnetic order or conventional glassy behavior is observed. In addition to its highly insulating nature, the magnetic specific heat C_mag/T and thermal conductivity \k{appa}_xx/T both exhibit linear temperature dependencies with substantial finite intercepts. In particular, a sizeable field-independent residual term $κ/T \approx 0.03~\mathrm{W\,m^{-1}\,K^{-2}}$ is observed, providing compelling evidence of itinerant low-energy excitations that carry entropy without charge. These findings conceptually advance our understanding of quantum matter by demonstrating a rare regime where the interplay of disorder, frustration, and electronic correlations actively reshapes the nature of low-energy excitations, allowing itinerant neutral excitations to coexist with strong intrinsic disorder.

cond-mat.str-el↗

arXiv2026

Discovery of Van Hove Singularities: Electronic Fingerprints of 3Q Magnetic Order in a van der Waals Quantum Magnet

Magnetically intercalated transition metal dichalcogenides are emerging as a rich platform for exploring exotic quantum states in van der Waals magnets. Among them, CoxTaS2 has attracted intense interest following the recent discovery of a distinctive 3Q magnetic ground state and a pronounced topological Hall effect below a critical doping of x=1/3, both intimately tied to cobalt concentration. To date, direct signatures of this enigmatic 3Q magnetic order in the electronic structure remain elusive. Here we report a comprehensive doping dependent angle resolved photoemission spectroscopy study that unveils these long-sought fingerprints. Our data reveal an unexpected "inverse Mexican hat" dispersion along the K-M-K direction, accompanied by two van Hove singularities. These features are consistent with theoretical predictions for a 3Q magnetic order near three-quarters band filling on a cobalt triangular lattice. These results provide evidence of 3Q magnetic order in the electronic structure, establishing TMD van der Waals magnets as tunable materials to explore the interplay between magnetism and topology.

cond-mat.mtrl-sci↗

arXiv2026

Spin-Valley Locking in 2H-TaS2 and Its Co-Intercalated Counterpart: Roles of Surface Domains and Co Intercalation

Tuning and probing spin-valley coupling is key to understanding correlated ground states in 2$\it{H}$-TaS$_2$. Its magnetically intercalated analogue, Co$_{1/3}$TaS$_2$, introduces additional degrees of freedom, including modified interlayer coupling and magnetism, to modulate spin-valley physics. Surface-sensitive probes like ARPES are essential for accessing surface spin texture, yet previous studies on 2$\it{H}$-TMDs have reported conflicting results regarding spin-polarized bands, leaving open whether these discrepancies are intrinsic or extrinsic. Here we performed spatially resolved spin-ARPES measurements on 2$\it{H}$-TaS$_2$ and Co$_{1/3}$TaS$_2$. Our results reveal robust spin-valley locking on both compounds. Importantly, Co intercalation enhances interlayer hybridization and introduces magnetism while preserving the TaS$_2$-derived spin texture. We further observe a spatial reversal of the out-of-plane spin polarization, which we attribute to different surface domains. This effect complicates quantifying spin textures and may underlie prior inconsistent observations. Our findings provide microscopic insight into how interlayer interactions and surface domains together govern spin-valley phenomena in layered TMDs.

cond-mat.mtrl-sci↗

arXiv2025

Hund's coupling assisted orbital-selective superconductivity in Ba1-xKxFe2As2

While the superconducting transition temperature of hole-doped Ba_{1-x}K_{x}Fe_{2}As_{2} decreases past optimal doping, superconductivity does not completely disappear even for the fully doped KFe_{2}As_{2} compound. In fact, superconductivity is robust through a Lifshitz transition where electron bands become hole-like around the zone corner at around x=0.7, thus challenging the conventional understanding of superconductivity in iron-based systems. High-resolution angle-resolved photoemission spectroscopy is used to investigate the superconducting gap structure, as well as the normal state electronic structure, around optimal doping and across the Lifshitz transition. Our findings reveal a largely orbital-dependent superconducting gap structure, where the more strongly correlated d_{xy} band has a vanishing superconducting gap at higher doping, aligning with the Hund's metal behavior observed in the normal state. Notably, the superconducting gap on the d_{xy} band disappears before the Lifshitz transition, suggesting that the Fermi surface topology may play a secondary role. We discuss how these results point to orbital-selective superconducting pairing and how strong correlations via Hund's coupling may shape superconducting gap structures in iron-based and other multiorbital superconductors.

cond-mat.supr-con↗

arXiv2025

Weak phonon coupling to nematic quantum critical mode in $BaFe2(As1-xPx)2$

In this work, we investigate the softening of the in-plane transverse acoustic phonon driven by electronic nematicity in BaFe$_2$(As$_{1-x}$P$_x$)$_2$ using inelastic X-ray scattering, with a focus on the optimally doped sample ($x = 0.31$) sample, a system exhibiting signatures of a putative nematic quantum critical point and minimal disorder among iron pnictides. We observe only a modest softening of the phonon frequency and no evidence of critical damping, suggesting that the nematic quantum critical fluctuations couple only weakly to the lattice from our quantum critical model. Given the close proximity of the structural and magnetic transition temperatures in the underdoped sample, which implies that spin-nematic fluctuations couple strongly to the lattice. We conjecture that the quantum critical nematic fluctuations are predominantly orbital in origin.

cond-mat.str-el↗

arXiv2025

Pair Wavefunction Symmetry in UTe2 from Zero-Energy Surface State Visualization

Although nodal spin-triplet topological superconductivity appears probable in UTe2, its superconductive order-parameter $Δ_k$ remains unestablished. In theory, a distinctive identifier would be the existence of a superconductive topological surface band (TSB), which could facilitate zero-energy Andreev tunneling to an s-wave superconductor, and also distinguish a chiral from non-chiral $Δ_k$ via enhanced s-wave proximity. Here we employ s-wave superconductive scan-tips and detect intense zero-energy Andreev conductance at the UTe2 (0-11) termination surface. Imaging reveals sub-gap quasiparticle scattering interference signatures with a-axis orientation. The observed zero-energy Andreev peak splitting with enhanced s-wave proximity, signifies that $Δ_k$ of UTe2 is a non-chiral state: B1u, B2u or B3u. However, if the quasiparticle scattering along the a-axis is internodal, then a non-chiral B3u state is the most consistent for UTe2.

cond-mat.supr-con↗

arXiv2024

Pair-breaking scattering interference as a mechanism for superconducting gap modulation

We propose the ``pair-breaking scattering interference" as a general source of coherence peak modulations in superconductors. Assuming this mechanism, we present a simple physical picture for the coherence peak modulations in overdoped cuprate Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ (Bi-2223), ferromagnetic iron pnictide EuRbFe$_4$As$_4$ (Eu-1144), and kagome metals $A$V$_3$Sb$_5$ ($A=$ K, Rb, and Cs). Specifically, we explain the wavevectors, the particle-hole symmetry, and the dependence on the internal or external Zeeman-field of the coherence peak modulations. This work is intended as a cautious reminder to the scientific community when asserting the existence of a pair density wave phenomenon in the absence of tunneling conductance modulations in the normal state.

cond-mat.supr-con↗

arXiv2024

Detecting axion dynamics on the surface of magnetic topological insulators

Axions, initially proposed to solve the strong CP problem, have recently gained attention in condensed matter physics, particularly in topological insulators. However, detecting axion dynamics has proven challenging, with no experimental confirmations to date. In this study, we identify the surface of magnetic topological insulators as an ideal platform for observing axion dynamics. The vanishing bulk gap at the surface allows for order $O(1)$ variations in the axion field, making the detection of axion-like phenomena more feasible. In contrast, these phenomena are strongly suppressed in the bulk due to the small magnetic exchange gap. We investigate two-photon decay as a signature of axion dynamics and calculate the branching ratio using a perturbative approach. Our findings reveal that the photon flux emitted from the surface is in-plane and orders of magnitude larger than that from the bulk, making it detectable with modern microwave technology. We also discuss potential material platforms for detecting axion two-photon decay and strategies to enhance the signal-to-noise ratio.

cond-mat.str-el↗

arXiv2024

Contrasting electron-phonon interaction between electron- and hole-doped cuprates

Spin- and charge-lattice interactions are potential key factors in the microscopic mechanism of high-temperature superconductivity in cuprates. Although both interactions can dramatically shape the low-energy electronic structure, their phenomenological roles in superconductivity are usually investigated independently. Employing angle-resolved photoemission spectroscopy, we reveal the spectroscopic fingerprint of short-range antiferromagnetic order in conjunction with enhanced electron-phonon interaction in the electron-doped cuprate superconductor $\mathrm{Nd_{1.85}Ce_{0.15}CuO_4}$. The observed mode coupling exhibits a strong momentum dependence that is in striking contrast to the node-antinode dichotomy previously observed in the hole-doped cuprates. Our results reveal an intimate relationship between electron-phonon coupling and antiferromagnetic fluctuations, which collectively sets the stage for unconventional superconductivity in the electron-doped cuprates.

cond-mat.supr-con↗

arXiv2024

Theory of an infinitely anisotropic phase of a two-dimensional superconductor

We propose a simple model of a two-dimensional ``locally smectic superconductor'' that exhibits power-law non-linear I-V characteristics with different powers for current applied in two orthogonal directions. We discuss the potential relevance of this model to recent experimental findings on interfacial superconductivity in EuO/KTaO$_3$(110) (Nat. Phys. 20, 957 (2024)), where the apparent critical temperature ($T_c$) has been shown experimentally to depend on the current direction.

cond-mat.supr-con↗

arXiv2023

Anomalous normal state gap in an electron-doped cuprate

In the underdoped n-type cuprate Nd2-xCexCuO4, long-ranged antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide range of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After carefully considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to that of the p-type cuprates.

cond-mat.supr-con↗

arXiv2023

Bogoliubov Quasiparticle on the Gossamer Fermi Surface in Electron-Doped Cuprates

In contrast to hole-doped cuprates, electron-doped cuprates consistently exhibit strong antiferromagnetic correlations with a commensurate (π, π) ordering wave vector, leading to the prevalent belief that antiferromagnetic spin fluctuations mediate Cooper pairing in these unconventional superconductors. However, early investigations produced two paradoxical findings: while antiferromagnetic spin fluctuations create the largest pseudogap at "hot spots" in momentum space, Raman scattering and angle-resolved photoemission spectroscopy measurements using the leading-edge method seem to suggest the superconducting gap is also maximized at these locations. This presented a dilemma for spin-fluctuation-mediated pairing: Cooper pairing is strongest at momenta where normal state low energy spectral weight is most suppressed. Here we investigate this dilemma in Nd2-xCexCuO4 using angle-resolved photoemission spectroscopy under significantly improved experimental conditions. The unprecedented signal-to-noise ratio and resolution allow us to directly observe the Bogoliubov quasiparticles, demonstrating the existence and importance of two sectors of states: 1. The reconstructed main band and the states gapped by the antiferromagnetic pseudogap around the hot spots. 2. The gossamer Fermi surface states with distinct dispersion inside the pseudogap, from which Bogoliubov quasiparticle coherence peaks emerge below Tc. Supported by numerical results, we propose that the non-zero modulus of the antiferromagnetic order parameter causes the former, while fluctuations in the antiferromagnetic order parameter orientation are responsible for the latter. Our revelations of the gossamer Fermi surface reconcile the paradoxical observations, deepening our understanding of superconductivity in electron-doped cuprates in particular, and unconventional superconductivity in general.

cond-mat.supr-con↗