arXiv subjects

Dvira Segal

Publications and source records attributed to Dvira Segal.

At least 127 records · Page 7Linked to original sources

arXiv2013

The probe technique far-from-equilibrium: Magnetic field symmetries of nonlinear transport

The probe technique is a simple mean to incorporate elastic and inelastic processes into quantum dynamics. Using numerical simulations, we demonstrate that this tool can be employed beyond the analytically tractable linear response regime, providing a stable solution for the probe parameters: temperature and chemical potential. Adopting four probes: dephasing, voltage, temperature, and voltage-temperature, mimicking different elastic and inelastic effects, we focus on magnetic field and gate voltage symmetries of charge current and heat current in Aharonov-Bohm interferometers, potentially far-from-equilibrium. Considering electron current, we prove analytically that in the linear response regime inelastic scattering processes do not break the Onsager symmetry. Beyond linear response, even (odd) conductance terms obey an odd (even) symmetry with the threading magnetic flux, as long as the system acquires a spatial inversion symmetry. When spatial asymmetry is introduced particle-hole symmetry assures that nonlinear conductance terms maintain certain symmetries with respect to magnetic field and gate voltage. These analytic results are supported by numerical simulations. Analogous results are obtained for the electron heat current. We also demonstrate that a double-dot Aharonov-Bohm interferometer acts as a rectifier when two conditions are met: (i) many-body effects are included, here in the form of inelastic scattering, and (ii) time reversal symmetry is broken.

cond-mat.mes-hall↗

arXiv2013

Magnetic field symmetries of nonlinear transport with elastic and inelastic scattering

We study nonlinear electronic transport symmetries in Aharonov-Bohm interferometers subjected to inelastic scattering effects and show that odd (even) conductance terms are even (odd) in the magnetic field when the junction is (left-right) spatially symmetric. This observation does not hold when an asymmetry is introduced, as we show numerically, but odd conductance terms only manifest a weak breakdown of the magnetic field symmetry. Under elastic dephasing effects, the Onsager-Casimir symmetry is maintained beyond linear response and under spatial asymmetries.

cond-mat.mes-hall↗

arXiv2013

Path-integral simulations with fermionic and bosonic reservoirs: Transport and dissipation in molecular electronic junctions

We expand iterative numerically-exact influence functional path-integral tools and present a method capable of following the nonequilibrium time evolution of subsystems coupled to multiple bosonic and fermionic reservoirs simultaneously. Using this method, we study the real-time dynamics of charge transfer and vibrational mode excitation in an electron conducting molecular junction. We focus on nonequilibrium vibrational effects, particularly, the development of vibrational instability in a current-rectifying junction. Our simulations are performed by assuming large molecular vibrational anharmonicity (or low temperature). This allows us to truncate the molecular vibrational mode to include only a two-state system. Exact numerical results are compared to perturbative Master equation calculations demonstrating an excellent agreement in the weak electron-phonon coupling regime. Significant deviations take place only at strong coupling. Our simulations allow us to quantify the contribution of different transport mechanisms, coherent dynamics and inelastic transport, in the overall charge current. This is done by studying two model variants: The first admits inelastic electron transmission only, while the second one allows for both coherent and incoherent pathways.

cond-mat.mes-hall↗

arXiv2012

Flux-dependent occupations and occupation difference in geometrically symmetric and energy degenerate double-dot Aharonov-Bohm interferometers

We study the steady-state characteristics and the transient behavior of the nonequilibrium double-dot Aharonov-Bohm interferometer using analytical tools and numerical simulations. Our simple setup includes noninteracting degenerate quantum dots that are coupled to two biased metallic leads at the same strength. A magnetic flux $Φ$ is piercing the setup perpendicularly. As we tune the degenerate dots energies away from the symmetric point we observe four nontrivial magnetic flux control effects: (i) flux dependency of the dots occupation, (ii) magnetic flux induced occupation difference between the dots, at degeneracy, (iii) the effect of "phase-localization" of the dots coherence holds only at the symmetric point, while in general both real and imaginary parts of the coherence are nonzero, and (iv) coherent evolution survives even when the dephasing strength, introduced into our model using Büttiker probe, is large and comparable to the dots energies and the bias voltage. Moreover, not only finite dephasing strength does not destroy the coherence features, it can provide new type of coherent oscillations. These four phenomena take place when the dots energies are gated, to be positioned away from the symmetric point, demonstrating that the combination of bias voltage, magnetic flux and gating field, can provide delicate controllability over the occupation of each of the quantum dots, and their coherence.

cond-mat.mes-hall↗

arXiv2012

Ground state cooling is not possible given initial system-thermal bath factorization

In this paper we prove that a fundamental constraint on the cooling dynamic implies that it is impossible to cool, via a unitary system-bath quantum evolution, a system that is embedded in a thermal environment down to its ground state, if the initial state is a factorized product of system and bath states. The latter is a crucial but artificial assumption often included in many descriptions of system-bath dynamics. The analogous conclusion holds for 'cooling' to any pure state of the system.

quant-ph↗

arXiv2012

Full density matrix dynamics for large quantum systems: Interactions, Decoherence and Inelastic effects

We develop analytical tools and numerical methods for time evolving the total density matrix of the finite-size Anderson model. The model is composed of two finite metal grains, each prepared in canonical states of differing chemical potential and connected through a single electronic level (quantum dot or impurity). Coulomb interactions are either excluded all together, or allowed on the dot only. We extend this basic model to emulate decoherring and inelastic scattering processes for the dot electrons with the probe technique. Three methods, originally developed to treat impurity dynamics, are augmented to yield global system dynamics: the quantum Langevin equation method, the well known fermionic trace formula, and an iterative path integral approach. The latter accommodates interactions on the dot in a numerically exact fashion. We apply the developed techniques to two open topics in nonequilibrium many-body physics: (i) We explore the role of many-body electron-electron repulsion effects on the dynamics of the system. Results, obtained using exact path integral simulations, are compared to mean-field quantum Langevin equation predictions. (ii) We analyze aspects of quantum equilibration and thermalization in large quantum systems using the probe technique, mimicking elastic-dephasing effects and inelastic interactions on the dot. Here, unitary simulations based on the fermionic trace formula are accompanied by quantum Langevin equation calculations.

cond-mat.mes-hall↗

arXiv2012

Exact dynamics of interacting qubits in a thermal environment: Results beyond the weak coupling limit

We demonstrate an exact mapping of a class of models of two interacting qubits in thermal reservoirs to two separate spin-bath problems. Based on this mapping, exact numerical simulations of the qubits dynamics can be performed, beyond the weak system-bath coupling limit. Given the time evolution of the system, we study, in a numerically exact way, the dynamics of entanglement between pair of qubits immersed in boson thermal baths, showing a rich phenomenology, including an intermediate oscillatory behavior, the entanglement sudden birth, sudden death, and revival. We find that stationary entanglement develops between the qubits due to their coupling to a thermal environment, unlike the isolated qubits case in which the entanglement oscillates. We also show that the occurrence of entanglement sudden death in this model depends on the portion of the zero and double excitation states in the subsystem initial state. In the long-time limit, analytic expressions are presented at weak system-bath coupling, for a range of relevant qubit parameters.

quant-ph↗

arXiv2012

Analysis technique for exceptional points in open quantum systems and QPT analogy for the appearance of irreversibility

We propose an analysis technique for the exceptional points (EPs) occurring in the discrete spectrum of open quantum systems (OQS), using a semi-infinite chain coupled to an endpoint impurity as a prototype. We outline our method to locate the EPs in OQS, further obtaining an eigenvalue expansion in the vicinity of the EPs that gives rise to characteristic exponents. We also report the precise number of EPs occurring in an OQS with a continuum described by a quadratic dispersion curve. In particular, the number of EPs occurring in a bare discrete Hamiltonian of dimension $n_\textrm{D}$ is given by $n_\textrm{D} (n_\textrm{D} - 1)$; if this discrete Hamiltonian is then coupled to continuum (or continua) to form an OQS, the interaction with the continuum generally produces an enlarged discrete solution space that includes a greater number of EPs, specifically $2^{n_\textrm{C}} (n_\textrm{C} + n_\textrm{D}) [2^{n_\textrm{C}} (n_\textrm{C} + n_\textrm{D}) - 1] $, in which $n_\textrm{C}$ is the number of (non-degenerate) continua to which the discrete sector is attached. Finally, we offer a heuristic quantum phase transition analogy for the emergence of the resonance (giving rise to irreversibility via exponential decay) in which the decay width plays the role of the order parameter; the associated critical exponent is then determined by the above eigenvalue expansion.

quant-ph↗

arXiv2012

Amplification of non-Markovian decay due to bound state absorption into continuum

It is known that quantum systems yield non-exponential (power law) decay on long time scales, associated with continuum threshold effects contributing to the survival probability for a prepared initial state. For an open quantum system consisting of a discrete state coupled to continuum, we study the case in which a discrete bound state of the full Hamiltonian approaches the energy continuum as the system parameters are varied. We find in this case that at least two regions exist yielding qualitatively different power law decay behaviors; we term these the long time `near zone' and long time `far zone.' In the near zone the survival probability falls off according to a $t^{-1}$ power law, and in the far zone it falls off as $t^{-3}$. We show that the timescale $T_Q$ separating these two regions is inversely related to the gap between the discrete bound state energy and the continuum threshold. In the case that the bound state is absorbed into the continuum and vanishes, then the time scale $T_Q$ diverges and the survival probability follows the $t^{-1}$ power law even on asymptotic scales. Conversely, one could study the case of an anti-bound state approaching the threshold before being ejected from the continuum to form a bound state. Again the $t^{-1}$ power law dominates precisely at the point of ejection.

quant-ph↗

arXiv2012

Towards equilibration and thermalization between finite quantum systems: The role of dephasing effects and inelastic interactions

We demonstrate the approach towards a Gibbs-like equilibrium state, with a common temperature and a chemical potential, of two finite metallic grains, prepared with a different number of noninteracting electrons, connected by a weak link that is susceptible to incoherent and inelastic processes. By developing an analytic method and by using an exact numerical approach, the quantum time evolution of the electrons in the metallic grains is followed. In the absence of decoherring and inelastic effects, equilibration is never reached. Introducing dephasing effects on the link only, using a dephasing probe, the two quantum systems equilibrate, but do not evolve towards a Gibbs-like state. In contrast, by mimicking inelastic interactions with a voltage probe, the metal pieces evolve towards a common Gibbs-like equilibrium state, with the probe.

cond-mat.mes-hall↗

arXiv2012

Dynamics of coherences in the interacting double-dot Aharonov-Bohm interferometer: Exact numerical simulations

We study the real time dynamics of electron coherence in a double quantum dot two-terminal Aharonov-Bohm geometry, taking into account repulsion effects between the dots' electrons. The system is simulated by extending a numerically exact path integral method, suitable for treating transport and dissipation in biased impurity models [Phys. Rev. B 82, 205323 (2010)]. Numerical simulations at finite interaction strength are supported by master equation calculations in two other limits: assuming non-interacting electrons, and working in the Coulomb blockade regime. Focusing on the intrinsic coherence dynamics between the double-dot states, we find that its temporal characteristics are preserved under weak-to-intermediate inter-dot Coulomb interaction. In contrast, in the Coulomb blockade limit, a master equation calculation predicts coherence dynamics and a steady-state value which notably deviate from the finite interaction case.

cond-mat.mes-hall↗

arXiv2011

Non-equilibrium spin-boson model: counting statistics and the heat exchange fluctuation theorem

We focus on the non-equilibrium two-bath spin-boson model, a toy model for examining quantum thermal transport in many-body open systems. Describing the dynamics within the NIBA equations, applicable, e.g., in the strong system-bath coupling limit and/or at high temperatures, we derive expressions for the cumulant generating function in both the markovian and non-markovian limits by energy-resolving the quantum master equation of the subsystem. For a markovian bath, we readily demonstrate the validity of a steady-state heat exchange fluctuation theorem. In the non-markovian limit a "weaker" symmetry relation generally holds, a general outcome of microreversibility. We discuss the reduction of this symmetry relation to the universal steady-state fluctuation theorem. Using the cumulant generating function, an analytic expression for the heat current is obtained. Our results establish the validity of the steady-state heat exchange fluctuation theorem in quantum systems with strong system-bath interactions. From the practical point of view, this study provides tools for exploring transport characteristics of the two-bath spin-boson model, a prototype for a nonlinear thermal conductor.

cond-mat.stat-mech↗

arXiv2011

Theory of quantum energy transfer in spin chains: From superexchange to ballistic motion

Quantum energy transfer in a chain of two-level (spin) units, connected at its ends to two thermal reservoirs, is analyzed in two limits: (i) In the off-resonance regime, when the characteristic subsystem excitation energy gaps are larger than the reservoirs frequencies, or the baths temperatures are low. (ii) In the resonance regime, when the chain excitation gaps match populated bath modes. In the latter case the model is studied using a master equation approach, showing that the dynamics is ballistic for the particular chain model explored. In the former case we analytically study the system dynamics utilizing the recently developed Energy-Transfer Born-Oppenheimer formalism [Phys. Rev. E {\bf 83}, 051114 (2011)], demonstrating that energy transfers across the chain in a superexchange (bridge assisted tunneling) mechanism, with the energy current decreasing exponentially with distance. This behavior is insensitive to the chain details. Since at low temperatures the excitation spectrum of molecular systems can be truncated to resemble a spin chain model, we argue that the superexchange behavior obtained here should be observed in widespread systems satisfying the off-resonance condition.

cond-mat.mes-hall↗

arXiv2011

Quantum heat transfer in harmonic chains with self consistent reservoirs: Exact numerical simulations

We describe a numerical scheme for exactly simulating the heat current behavior in a quantum harmonic chain with self-consistent reservoirs. Numerically-exact results are compared to classical simulations and to the quantum behavior under the linear response approximation. In the classical limit or for small temperature biases our results coincide with previous calculations. At large bias and for low temperatures the quantum dynamics of the system fundamentally differs from the close-to-equilibrium behavior, revealing in particular the effect of thermal rectification for asymmetric chains. Since this effect is absent in the classical analog of our model, we conclude that in the quantum model studied here thermal rectification is a purely quantum phenomenon, rooted in the quantum statistics.

cond-mat.mes-hall↗

arXiv2011

Quantum effects in thermal conduction: Nonequilibrium quantum discord and entanglement

We study the process of heat transfer through an entangled pair of two-level system, demonstrating the role of quantum correlations in this nonequilibrium process. While quantum correlations generally degrade with increasing the temperature bias, introducing spatial asymmetry leads to an intricate behavior: Connecting the qubits unequally to the reservoirs one finds that quantum correlations persist and increase with the temperature bias when the system is more weakly linked to the hot reservoir. In the reversed case, linking the system more strongly to the hot bath, the opposite, more natural behavior is observed, with quantum correlations being strongly suppressed upon increasing the temperature bias.

quant-ph↗

arXiv2011

Nonequilibrium transport in quantum impurity models: Exact path integral simulations

We simulate the nonequilibrium dynamics of two generic many-body quantum impurity models by employing the recently developed iterative influence-functional path integral method [Phys. Rev. B {\bf 82}, 205323 (2010)]. This general approach is presented here in the context of quantum transport in molecular electronic junctions. Models of particular interest include the single impurity Anderson model and the related spinless two-state Anderson dot. In both cases we study the time evolution of the dot occupation and the current characteristics at finite temperature. A comparison to mean-field results is presented, when applicable.

cond-mat.mes-hall↗

arXiv2010

DNA breathing dynamics: Analytic results for distribution functions of relevant Brownian functionals

We investigate DNA breathing dynamics by suggesting and examining several different Brownian functionals associated with bubble lifetime and reactivity. Bubble dynamics is described as an overdamped random walk in the number of broken base pairs. The walk takes place on the Poland-Scheraga free energy landscape. We suggest several probability distribution functions that characterize the breathing process, and adopt the recently studied backward Fokker-Planck method and the path decomposition method as elegant and flexible tools for deriving these distributions. In particular, for a bubble of an initial size $x_0$, we derive analytical expressions for (i) the distribution $P(t_f|x_0)$ of the first-passage time $t_f$, characterizing the bubble lifetime, (ii) the distribution $P(A|x_0)$ of the area $A$ till the first-passage time, providing information about the effective reactivity of the bubble to processes within the DNA, (iii) the distribution $P(M)$ of the maximum bubble size $M$ attained before the first-passage time, and (iv) the joint probability distribution $P(M,t_m)$ of the maximum bubble size $M$ and the time $t_m$ of its occurrence before the first-passage time. These distributions are analyzed in the limit of small and large bubble sizes. We supplement our analytical predictions with direct numerical simulations of the related Langevin equation, and obtain a very good agreement in the appropriate limits. The nontrivial scaling behavior of the various quantities analyzed here can, in principle, be explored experimentally.

cond-mat.soft↗

arXiv2010

Quantum heat transfer: A Born Oppenheimer method

We develop a Born-Oppenheimer type formalism for the description of quantum thermal transport along hybrid nanoscale objects. Our formalism is suitable for treating heat transfer in the off-resonant regime, where e.g., the relevant vibrational modes of the interlocated molecule are high relative to typical bath frequencies, and at low temperatures when tunneling effects dominate. A general expression for the thermal energy current is accomplished, in the form of a generalized Landauer formula. In the harmonic limit this expression reduces to the standard Landauer result for heat transfer, while in the presence of nonlinearities multiphonon tunneling effects are realized.

cond-mat.mes-hall↗