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E Wu

Publications and source records attributed to E Wu.

At least 19 recordsLinked to original sources

Memory and thermal amplification in spin--cavity squared commutators

Squared commutators in the Holstein--Primakoff limit of a spin--cavity system provide a compact way to separate propagation from covariance growth in a finite-temperature reservoir with memory. In the finite-temperature NMQSD construction, the linear quadrature commutator is fixed by the retarded spin--cavity propagator, whereas a quadratic commutator carries the same retarded factor together with a covariance factor. For a zero-mean Gaussian state, \(C_{R_i^2,R_j}(t)=4|\kappa_{ij}(t)|^2V_{ii}(t)\); the symmetrized expression gives the spin-side and mixed channels. Since \(\bar n\) enters the covariance sector but not the homogeneous retarded kernel, raising \(\bar n\) from 0 to 1 leaves the linear transfer unchanged while increasing the quadratic signal. Varying the bath-memory rate and the counter-rotating coupling within the stable HP region then shows how stored cavity history changes both the transfer weight and its distribution in time. The calculation separates memory-dependent propagation from thermal covariance growth in collective spin--cavity dynamics.

quant-ph

Chaos Generation and Control with Molecular Optomechanical System

Chaos is central to secure communication and physical random-number generation. Conventional cavity-optomechanical implementations, however, usually rely on weak single-photon optomechanical coupling and low-frequency mechanical modes, so access to deterministic chaotic dynamics often requires large driving power and careful suppression of thermal noise. Here we theoretically study a hybrid molecular optomechanical system formed by coupling a plasmonic nanocavity to a whispering-gallery-mode (WGM) microcavity. The plasmonic nanocavity provides terahertz-scale single-photon optomechanical coupling to a molecular vibration, while the WGM resonator offers a low-loss photonic channel that mitigates the short plasmon lifetime. By integrating the semiclassical equations of motion and evaluating the largest Lyapunov exponent, we map the nonlinear dynamical regimes in the parameter spaces of WGM detuning, plasmon--WGM coupling, and plasmon--vibration optomechanical coupling. We show that increasing the plasmon--vibration coupling drives the system from self-sustained oscillations to chaos through a period-doubling cascade. At moderate coupling strengths, isolated chaos windows can be opened or closed by tuning the WGM detuning and the inter-cavity coupling. These results identify molecular optomechanics as a controllable room-temperature platform for on-chip chaotic light generation and random-signal applications.

physics.optics

Wide-field mid-infrared single-photon upconversion imaging

Frequency upconversion technique, where the infrared signal is nonlinearly translated into the visible band to leverage the silicon sensors, offers a promising alternation for the mid-infrared (MIR) imaging. However, the intrinsic field of view (FOV) is typically limited by the phase-matching condition, thus imposing a remaining challenge to promote subsequent applications. Here, we demonstrate a wide-field upconversion imaging based on the aperiodic quasi-phase-matching configuration. The acceptance angle is significantly expanded to about 30$^\circ$, over tenfold larger than that with the periodical poling crystal. The extended FOV is realized in one shot without the need of parameter scanning or post-processing. Consequently, a fast snapshot allows to facilitate high-speed imaging at a frame rate up to 216 kHz. Alternatively, single-photon imaging at room temperature is permitted due to the substantially suppressed background noise by the spectro-temporal filtering. Furthermore, we have implemented high-resolution time-of-flight 3D imaging based on the picosecond optical gating. These presented MIR imaging features with wide field, fast speed, and high sensitivity might stimulate immediate applications, such as non-destructive defect inspection, in-vivo biomedical examination, and high-speed volumetric tomography.

physics.optics

Highly sensitive detection for infrared photons by non-degenerate two-photon absorption under mid-infrared pumping

We have demonstrated highly-sensitive photon counting in the infrared based on the two-photon absorption (2PA) in a silicon avalanche photodiode, where the required photon energy for inducing effective conductivity was provided by an intense mid-infrared (MIR) field at 3 $\mu$m. The used MIR pumping scheme could not only benefit from the enhanced 2PA coefficient in the non-degenerate regime, but also eliminate the detrimental background noises due to the pump harmonic excitation of the pump. Consequently, the enhancement factor for the signal counting rate unprecedented reached to about $10^{5}$ with input infrared pulses at the femtojoule level. Additionally, the noise equivalent power was substantially improved by two orders of magnitude comparing to conventional schemes with near-infrared pumping. Therefore, the presented configuration might provide an alternative to realize sensitive infrared detection and imaging with desirable features of room-temperature operation, no phase-matching requirement, and broadband responding window, which would find a variety of applications including remote ranging, sensitive sensing, biochemical imaging, and trace spectroscopy.

physics.optics

Mid-Infrared Single-Photon Edge Enhanced Imaging based on Nonlinear Vortex Filtering

Edge enhanced imaging via the spiral phase contrast enables to reveal the phase or amplitude gradients of a target, which has been proved useful in feature recognition, machine vision, and object identification. A long quest is to extend the operation wavelength into the mid-infrared (MIR) region, as highly demanded in various fields including infrared sensing, astronomic observation, and biomedical diagnosis. Here, we demonstrated ultra-sensitive MIR imaging at the single-photon level based on nonlinear frequency upconversion, where the spectrally converted replica of the MIR object image at 3070 nm was captured by a silicon electron multiplying charged coupled device. The imaging sensitivity was significantly improved by the coincidence pulsed pumping with a spectro-temporal optimization. Furthermore, the edge enhancement has been realized by imprinting the spiral phase pattern of the pump onto the upconverted field at the Fourier plane within the nonlinear crystal. Such a nonlinear spatial filter not only provided an effective way to implement the required high-fidelity vortex screening in the edge enhanced detection, but also rendered the MIR illumination into a visible image in an efficient and low-noise fashion. The presented system for MIR edge enhanced imaging might facilitate immediate applications in label-free histopathological diagnosis and non-destructive defect inspection.

physics.optics

Single-Photon Infrared Imaging with a Silicon Camera Based on Long-Wavelength-Pumping Two-Photon Absorption

We experimentally demonstrated an ultra-sensitive imaging system for telecom photons based on the non-degenerate two-photon absorption in a silicon-based electron multiplying charge-coupled device (EMCCD). The proposed long-wavelength-pumping scheme with mid-infrared pulsed excitation could not only effectively increase the two-photon absorption coefficient, but also significantly suppress the background noise caused by the harmonic absorption of the strong pumping field. In comparison to the photoelectric response via the degenerate two-photon absorption, the implemented configuration could offer over 30-folded enhancement of the photon-counting rate in the infrared imaging. The resulting detection sensitivity up to 1 photon/pixel/pulse was unprecedentedly approached, thus facilitating the single-photon operation. The elimination of the stringent phase matching as typically required in the optical parametric conversion has led to a high spatial resolution of 13 $\mu$m. Moreover, the on-chip nonlinearity of the optical imager would enable a broadband spectral window and an enlarged field of view. In combination with the 5-ps temporal resolution due to the coincident optical gating, the presented imaging system would find various promising applications, such as low-light fluorescence lifetime microscopy and photon counting time-of-flight 3D imaging.

physics.optics

High-speed mid-infrared single-photon upconversion spectrometer

Sensitive and fast mid-infrared (MIR) spectroscopy is highly attractive in a variety of applications including astronomical observation, pharmaceutical synthesis, and environmental monitoring. However, the performance of conventional MIR spectrometers has long been hindered by the limited sensitivity of narrow-bandgap detectors and/or the deficient brightness of broadband light sources. Here, we devise and implement an ultra-sensitive and broadband MIR upconversion spectrometer, which integrates a supercontinuum source covering 1.5-4.2 $\mu$m based on a silicon nitride nanophotonic waveguide. High-efficiency and low-noise nonlinear frequency upconversion is realized based on coincidence pulsed pumping with spectro-temporal optimization, which enables to leverage silicon detectors for facilitating MIR single-photon spectroscopy at 0.2 photons/nm/pulse. Furthermore, the upconversion-based array spectrometer is manifested with high-speed spectral acquisition rates beyond 200 kHz, which is about ten-fold faster than the state-of-the-art scan rates for FTIR-based spectrometers at a comparable spectral resolution. The achieved features of broadband spectral coverage, single-photon sensitivity, and sub-MHz refreshing rate might open up new possibilities in infrared transient spectral measurements in combustion analysis, high-throughput sorting and reaction tracking, among others.

physics.optics

Mid-infrared single-photon 3D imaging

Active mid-infrared (MIR) imagers capable of retrieving three-dimensional (3D) structure and reflectivity information are highly attractive in a wide range of biomedical and industrial applications. However, the infrared 3D imaging at low-light levels is still challenging due to the deficiency of sensitive and fast MIR sensors. Here we propose and implement a MIR time-of-flight imaging system that operates at single-photon sensitivity and femtosecond timing resolution. Specifically, back-scattered infrared photons from a scene are optically gated by delay-controlled ultrashort pump pulses through nonlinear frequency upconversion. The upconverted images with time stamps are then recorded by a silicon camera to facilitate the 3D reconstruction with high lateral and depth resolutions. Moreover, an effective numerical denoiser based on spatiotemporal correlation allows us to reveal the object profile and reflectivity under photon-starving conditions with a detected flux below 0.05 photons/pixel/second. The presented MIR 3D imager features with high detection sensitivity, precise timing resolution, and wide-field operation, which may open new possibilities in life and material sciences.

physics.optics

Mid-infrared single-pixel imaging at the single-photon level

Single-pixel cameras have recently emerged as promising alternatives to multi-pixel sensors due to reduced costs and superior durability, which are particularly attractive for mid-infrared (MIR) imaging pertinent to applications including industry inspection and biomedical diagnosis. To date, MIR single-pixel photon-sparse imaging has yet been realized, which urgently calls for high-sensitivity optical detectors and high-fidelity spatial modulators. Here, we demonstrate a MIR single-photon computational imaging with a single-element silicon detector. The underlying methodology relies on nonlinear structured detection, where the encoded time-varying pump patterns are optically imprinted onto the MIR object image through sum-frequency generation. Simultaneously, the MIR radiation is spectrally translated into the visible region, thus permitting infrared single-photon upconversion detection. Then, the use of advanced algorithms of compress sensing and deep learning allows us to reconstruct MIR images under sub-Nyquist sampling and photon-starving illumination. The presented paradigm of single-pixel upconversion imaging is featured with single-pixel simplicity, single-photon sensitivity, and room-temperature operation, which would establish a new path for sensitive imaging at longer infrared wavelengths or terahertz frequencies, where high-sensitivity photon counters and high-fidelity spatial modulators are typically hard to access.

physics.optics

Single-photon time-stretch infrared spectroscopy

Sensitive mid-infrared (MIR) spectroscopy is highly demanded in various fields ranging from industrial inspection, biomedical diagnosis to astronomical observation. However, the detection sensitivity of conventional MIR spectrometers has been severely limited by excessive noises for existing infrared sensors, which hinders widespread use in photon-scarce scenarios. Here, we devise and implement a broadband MIR single-photon time-stretch spectrometer based on high-fidelity spectral upconversion and time-correlated coincidence counting. Specifically, a nanophotonic supercontinuum illumination covering 2.4-4.2 $\mu$m is nonlinearly converted to the near-infrared band, where low-loss single-mode fiber and high-performance silicon detector can be leveraged to facilitate dispersive operation and sensitive detection, respectively. The arrival time for the dispersed upconversion photons is precisely registered with a low-timing-jitter photon counter, which enables us to obtain a high spectral resolution about 0.5 cm$^{-1}$ under a low-light-level illumination down to 0.14 photons/nm/pulse. In comparison to previous MIR upconversion spectrometers, the presented time-stretch architecture favors single-pixel simplicity and high-throughput acquisition for the single-photon spectral measurement. The achieved MIR spectroscopic features of broadband spectral coverage, sub-wavenumber resolution, single-photon sensitivity, and room-temperature operation would stimulate immediate applications in material and life sciences.

physics.optics

Wide-field mid-infrared hyperspectral imaging beyond video rate

Mid-infrared hyperspectral imaging has become an indispensable tool to spatially resolve chemical information in a wide variety of samples. However, acquiring three-dimensional data cubes is typically time-consuming due to the limited speed of raster scanning or wavelength tuning, which impedes real-time visualization with high spatial definition across broad spectral bands. Here, we devise and implement a high-speed, wide-field mid-infrared hyperspectral imaging system relying on broadband parametric upconversion of high-brightness supercontinuum illumination at the Fourier plane. The upconverted replica is spectrally decomposed by a rapid acousto-optic tunable filter, which records high-definition monochromatic images at a frame rate of 10 kHz based on a megapixel silicon camera. Consequently, the hyperspectral imager allows us to acquire 100 spectral bands over 2600-4085 cm$^{-1}$ in 10 ms, corresponding to a refreshing rate of 100 Hz. Moreover, the angular dependence of phase matching in the image upconversion is leveraged to realize snapshot operation with spatial multiplexing for multiple spectral channels, which may further boost the spectral imaging rate. The high acquisition rate, wide-field operation, and broadband spectral coverage could open new possibilities for high-throughput characterization of transient processes in material and life sciences.

physics.optics

High-resolution mid-infrared single-photon upconversion ranging

Single-photon laser ranging has widespread applications in remote sensing and target recognition. However, highly-sensitive light detection and ranging (LiDAR) has long been restricted in visible or near-infrared bands. An appealing quest is to extend the operation wavelength into the mid-infrared (MIR) region, which calls for an infrared photon counting system at high detection sensitivity and precise temporal resolution. Here, we devise and demonstrate a MIR upconversion LiDAR based on nonlinear asynchronous optical sampling. Specifically, the infrared probe is interrogated in a nonlinear crystal by a train of pump pulses at a slightly different repetition rate, which favors for a temporal optical scanning at a picosecond timing resolution and a kilohertz refreshing rate over $\sim$50 ns. Moreover, the cross-correlation upconversion trace is temporally stretched by a factor of 2$\times$10$^4$, which can thus be recorded by a low-bandwidth silicon detector. In combination with time-correlated photon-counting technique, the achieved effective resolution is about two orders of magnitude better than the timing jitter of the detector itself, which facilitates a ranging precision of 4 $\mu$m under a low detected flux of 8$\times$10$^{-5}$ photons per pulse. The presented MIR time-of-flight range finder is featured with single-photon sensitivity and high positioning resolution, which would be particularly useful in infrared sensing and imaging in photon-starved scenarios.

physics.optics

Temporal filtered quantum sensing with the nitrogen-vacancy center in diamond

Nitrogen vacancy centers in diamond are among the leading solid state quantum platforms, offering exceptional spatial resolution and sensitivity for applications such as magnetic field sensing, thermometry, and bioimaging. However, in high background environments,such as those encountered in in vitro diagnostics, the performance of NV based sensors can be compromised by strong background fluorescence, particularly from substrates such as nitrocellulose. In this work, we analytically and experimentally investigate the use of pulsed laser excitation combined with time gating techniques to suppress background fluorescence and enhance the signal to noise ratio in NV based quantum sensing, with an emphasis on spin enhanced biosensing. Through experimental studies using mixed ensembles of silicon vacancy and NV centers in bulk diamond, as well as fluorescent nanodiamonds on NC substrates, we demonstrate significant improvements in NV spin resonance visibility, demonstrated by an increase of the SNR by up to 4x, and a resulting measurement time reduction by 16x. The presented technique and results here can help significantly increase the readout efficiency and speed in future applications of NV centers in high background environments, such as in IVD, where the NV centers are used as a fluorescent label for biomolecules.

quant-ph

Spin noise spectroscopy of optical light shifts

Light induced non-equilibrium spin noise spectroscopy is theoretically and experimentally shown to be an efficient technique to reveal the structure and the coherent effects in the probed transition. Indeed, using metastable helium, the spin noise spectrum is shown to exhibit a dual-peak structure around the Larmor frequency. This previously unobserved feature is due to the light shifts of the involved levels and strongly depends on the probe power, detuning, and polarization orientation. Both numerical and analytical models reproduce very well the details of the split spin noise spectra: this technique thus allows a simple and direct measurement of the light shifts, and its polarization dependence permits to reveal the level structure in a non ambiguous manner.

quant-ph

Nanofiber based displacement sensor

We report on the realization of a displacement sensor based on an optical nanofiber. A single gold nano-sphere is deposited on top of a nanofiber and the system is placed within a standing wave which serves as a position ruler. Scattered light collected within the guided mode of the fiber gives a direct measure of the nanofiber displacement. We calibrated our device and found a sensitivity up to 1.2~nm/$\sqrt{\text{Hz}}$. A mechanical model based on the Mie scattering theory is then used to evaluate the optically induced force on the nanofiber by an external laser. With our sensing system, we demonstrate that an external force of 1~pN applied at the nanofiber waist can be detected.

physics.optics

Compensation of Beer-Lambert attenuation using non-diffracting Bessel beams

We report on a versatile method to compensate the linear attenuation in a medium, independently of its microscopic origin. The method exploits diffraction-limited Bessel beams and tailored on-axis intensity profiles which are generated using a phase-only spatial light modulator. This technique for compensating one of the most fundamental limiting processes in linear optics is shown to be efficient for a wide range of experimental conditions (modifying the refractive index and the attenuation coefficient). Finally, we explain how this method can be advantageously exploited in applications ranging from bio-imaging light sheet microscopy to quantum memories for future quantum communication networks.

physics.optics

Optical nanofiber interferometer and resonator

We report the fabrication and characterization of photonic structures using tapered optical nanofibers. Thanks to the extension of the evanescent electromagnetic field outside of the nanofiber two types of devices can be built: a ring interferometer and a knot resonator. We propose a general approach to predict the properties of these structures using the linear coupling theory. In addition, we describe a new source of birefringence due to the ovalization of a nanofiber under strong bending, known in mechanical engineering as the Brazier effect.

physics.optics

Experimental quantum state engineering with time-separated heraldings from a continuous-wave light source: a temporal-mode analysis

Conditional preparation is a well-established technique for quantum state engineering of light. A general trend is to increase the number of heralding detection events in such realization to reach larger photon-number states or their arbitrary superpositions. In contrast to pulsed implementations, where detections only occur within the pulse window, for continuous-wave light the temporal separation of the conditioning detections is an additional degree of freedom and a critical parameter. Based on the theoretical study by A.E.B. Nielsen and K. Molmer and on a continuous-wave two-mode squeezed vacuum from a nondegenerate optical parametric oscillator, we experimentally investigate the generation of two-photon state with tunable delay between the heralding events. The present work illustrates the temporal multimode features in play for conditional state generation based on continuous-wave light sources.

quant-ph