arXiv subjects

E. Alex Wollack

Publications and source records attributed to E. Alex Wollack.

14 recordsLinked to original sources

arXiv2025

Surface and Bulk Two-Level System Losses in Lithium Niobate Acoustic Resonators

Lithium niobate (LN) is a promising material for building acoustic resonators used in quantum applications, but its performance is limited by poorly understood material defects called two-level systems (TLS). In this work, we fabricate high-performance acoustic resonators from LN with quality factors up to $6\times10^7$ and use them to separate bulk and surface contributions to TLS loss. By comparing these bulk acoustic wave (BAW) resonators with previous surface acoustic wave and phononic crystal studies, we show that devices with high surface participation ratios are limited by surface TLS, while our BAW devices reveal an intrinsic bulk TLS limit. Through systematic surface treatments and microscopy, we demonstrate that BAW resonator performance remains unchanged despite surface modifications, confirming operation in a bulk-limited regime. Our work establishes quantitative bounds on both surface and bulk TLS losses in LN, within the context of material growth and fabrication approaches we have pursued, and provides guidance for future device engineering and materials development.

cond-mat.mes-hall↗

arXiv2024

Demonstrating a long-coherence dual-rail erasure qubit using tunable transmons

Quantum error correction with erasure qubits promises significant advantages over standard error correction due to favorable thresholds for erasure errors. To realize this advantage in practice requires a qubit for which nearly all errors are such erasure errors, and the ability to check for erasure errors without dephasing the qubit. We demonstrate that a "dual-rail qubit" consisting of a pair of resonantly coupled transmons can form a highly coherent erasure qubit, where transmon $T_1$ errors are converted into erasure errors and residual dephasing is strongly suppressed, leading to millisecond-scale coherence within the qubit subspace. We show that single-qubit gates are limited primarily by erasure errors, with erasure probability $p_\text{erasure} = 2.19(2)\times 10^{-3}$ per gate while the residual errors are $\sim 40$ times lower. We further demonstrate mid-circuit detection of erasure errors while introducing $< 0.1\%$ dephasing error per check. Finally, we show that the suppression of transmon noise allows this dual-rail qubit to preserve high coherence over a broad tunable operating range, offering an improved capacity to avoid frequency collisions. This work establishes transmon-based dual-rail qubits as an attractive building block for hardware-efficient quantum error correction.

quant-ph↗

arXiv2023

Arbitrary electro-optic bandwidth and frequency control in lithium niobate optical resonators

In situ tunable photonic filters and memories are important for emerging quantum and classical optics technologies. However, most photonic devices have fixed resonances and bandwidths determined at the time of fabrication. Here we present an in situ tunable optical resonator on thin-film lithium niobate. By leveraging the linear electro-optic effect, we demonstrate widely tunable control over resonator frequency and bandwidth on two different devices. We observe up to $\sim50\times$ tuning in the bandwidth over $\sim50$ V with linear frequency control of $\sim230$ MHz/V. We also develop a closed-form model predicting the tuning behavior of the device. This paves the way for rapid phase and amplitude control over light transmitted through our device.

physics.optics↗

arXiv2023

Surface Modification and Coherence in Lithium Niobate SAW Resonators

Lithium niobate is a promising material for developing quantum acoustic technologies due to its strong piezoelectric effect and availability in the form of crystalline thin films of high quality. However, at radio frequencies and cryogenic temperatures, these resonators are limited by the presence of decoherence and dephasing due to two-level systems. To mitigate these losses and increase device performance, a more detailed picture of the microscopic nature of these loss channels is needed. In this study, we fabricate several lithium niobate acoustic wave resonators and apply different processing steps that modify their surfaces. These treatments include argon ion sputtering, annealing, and acid cleans. We characterize the effects of these treatments using three surface-sensitive measurements: cryogenic microwave spectroscopy measuring density and coupling of TLS to mechanics, x-ray photoelectron spectroscopy and atomic force microscopy. We learn from these studies that, surprisingly, increases of TLS density may accompany apparent improvements in the surface quality as probed by the latter two approaches. Our work outlines the importance that surfaces and fabrication techniques play in altering acoustic resonator coherence, and suggests gaps in our understanding as well as approaches to address them.

quant-ph↗

arXiv2023

Strong dispersive coupling between a mechanical resonator and a fluxonium superconducting qubit

We demonstrate strong dispersive coupling between a fluxonium superconducting qubit and a 690 megahertz mechanical oscillator, extending the reach of circuit quantum acousto-dynamics (cQAD) experiments into a new range of frequencies. We have engineered a qubit-phonon coupling rate of $g\approx2π\times14~\text{MHz}$, and achieved a dispersive interaction that exceeds the decoherence rates of both systems while the qubit and mechanics are highly nonresonant ($Δ/g\gtrsim10$). Leveraging this strong coupling, we perform phonon number-resolved measurements of the mechanical resonator and investigate its dissipation and dephasing properties. Our results demonstrate the potential for fluxonium-based hybrid quantum systems, and a path for developing new quantum sensing and information processing schemes with phonons at frequencies below 700 MHz to significantly expand the toolbox of cQAD.

quant-ph↗

arXiv2023

Studying phonon coherence with a quantum sensor

In the field of quantum technology, nanomechanical oscillators offer a host of useful properties given their compact size, long lifetimes, and ability to detect force and motion. Their integration with superconducting quantum circuits shows promise for hardware-efficient computation architectures and error-correction protocols based on superpositions of mechanical coherent states. One limitation of this approach is decoherence processes affecting the mechanical oscillator. Of particular interest are two-level system (TLS) defects in the resonator host material, which have been widely studied in the classical domain, primarily via measurements of the material loss tangent. In this manuscript, we use a superconducting qubit as a quantum sensor to perform phonon number-resolved measurements on a phononic crystal cavity. This enables a high-resolution study of mechanical dissipation and dephasing in coherent states of variable size (mean phonon number $\navg\simeq1-10$). We observe nonexponential energy decay and a state size-dependent reduction of the dephasing rate, which we attribute to interactions with TLS. Using a numerical model, we reproduce the energy decay signatures (and to a lesser extent, the dephasing signatures) via mechanical emission into a small ensemble ($N=5$) of saturable and rapidly dephasing TLS. Our findings comprise a detailed examination of TLS-induced phonon decoherence in the quantum regime.

quant-ph↗

arXiv2021

Quantum state preparation, tomography, and entanglement of mechanical oscillators

Precisely engineered mechanical oscillators keep time, filter signals, and sense motion, making them an indispensable part of today's technological landscape. These unique capabilities motivate bringing mechanical devices into the quantum domain by interfacing them with engineered quantum circuits. Proposals to combine microwave-frequency mechanical resonators with superconducting devices suggest the possibility of powerful quantum acoustic processors. Meanwhile, experiments in several mechanical systems have demonstrated quantum state control and readout, phonon number resolution, and phonon-mediated qubit-qubit interactions. Currently, these acoustic platforms lack processors capable of controlling multiple mechanical oscillators' quantum states with a single qubit, and the rapid quantum non-demolition measurements of mechanical states needed for error correction. Here we use a superconducting qubit to control and read out the quantum state of a pair of nanomechanical resonators. Our device is capable of fast qubit-mechanics swap operations, which we use to deterministically manipulate the mechanical states. By placing the qubit into the strong dispersive regime with both mechanical resonators simultaneously, we determine the resonators' phonon number distributions via Ramsey measurements. Finally, we present quantum tomography of the prepared nonclassical and entangled mechanical states. Our result represents a concrete step toward feedback-based operation of a quantum acoustic processor.

quant-ph↗

arXiv2021

Loss channels affecting lithium niobate phononic crystal resonators at cryogenic temperature

We investigate the performance of microwave-frequency phononic crystal resonators fabricated on thin-film lithium niobate for integration with superconducting quantum circuits. For different design geometries at millikelvin temperatures, we achieve mechanical internal quality factors $Q_i$ above $10^5 - 10^6$ at high microwave drive power, corresponding to $5\times10^6$ phonons inside the resonator. By sweeping the defect size of resonators with identical mirror cell designs, we are able to indirectly observe signatures of the complete phononic bandgap via the resonators' internal quality factors. Examination of quality factors' temperature dependence shows how superconducting and two-level system (TLS) loss channels impact device performance. Finally, we observe an anomalous low-temperature frequency shift consistent with resonant TLS decay and find that material choice can help to mitigate these losses.

physics.app-ph↗

arXiv2020

Cryogenic microwave-to-optical conversion using a triply-resonant lithium niobate on sapphire transducer

Quantum networks are likely to have a profound impact on the way we compute and communicate in the future. In order to wire together superconducting quantum processors over kilometer-scale distances, we need transducers that can generate entanglement between the microwave and optical domains with high fidelity. We present an integrated electro-optic transducer that combines low-loss lithium niobate photonics with superconducting microwave resonators on a sapphire substrate. Our triply-resonant device operates in a dilution refrigerator and converts microwave photons to optical photons with an on-chip efficiency of $6.6\times 10^{-6}$ and a conversion bandwidth of 20 MHz. We discuss design trade-offs in this device, including strategies to manage acoustic loss, and outline ways to increase the conversion efficiency in the future.

quant-ph↗

arXiv2019

A silicon-organic hybrid platform for quantum microwave-to-optical transduction

Low-loss fiber optic links have the potential to connect superconducting quantum processors together over long distances to form large scale quantum networks. A key component of these future networks is a quantum transducer that coherently and bidirectionally converts photons from microwave frequencies to optical frequencies. We present a platform for electro-optic photon conversion based on silicon-organic hybrid photonics. Our device combines high quality factor microwave and optical resonators with an electro-optic polymer cladding to perform microwave-to-optical photon conversion from 6.7 GHz to 193 THz (1558 nm). The device achieves an electro-optic coupling rate of 330 Hz in a millikelvin dilution refrigerator environment. We use an optical heterodyne measurement technique to demonstrate the single-sideband nature of the conversion with a selectivity of approximately 10 dB. We analyze the effects of stray light in our device and suggest ways in which this can be mitigated. Finally, we present initial results on high-impedance spiral resonators designed to increase the electro-optic coupling.

quant-ph↗

arXiv2019

Electric fields for light: Propagation of microwave photons along a synthetic dimension

The evenly-spaced modes of an electromagnetic resonator are coupled to each other by appropriate time-modulation, leading to dynamics analogous to those of particles hopping between different sites of a lattice. This substitution of a real spatial dimension of a lattice with a "synthetic'" dimension in frequency space greatly reduces the hardware complexity of an analog quantum simulator. Complex control and read-out of a highly multi-moded structure can thus be accomplished with very few physical control lines. We demonstrate this concept with microwave photons in a superconducting transmission line resonator by modulating the system parameters at frequencies near the resonator's free spectral range and observing propagation of photon wavepackets in time domain. The linear propagation dynamics are equivalent to a tight-binding model, which we probe by measuring scattering parameters between frequency sites. We extract an approximate tight-binding dispersion relation for the synthetic lattice and initialize photon wavepackets with well-defined quasimomenta and group velocities. As an example application of this platform in simulating a physical system, we demonstrate Bloch oscillations associated with a particle in a periodic potential and subject to a constant external field. The simulated field strongly affects the photon dynamics despite photons having zero charge. Our observation of photon dynamics along a synthetic frequency dimension generalizes immediately to topological photonics and single-photon power levels, and expands the range of physical systems addressable by quantum simulation.

quant-ph↗

arXiv2019

Resolving the energy levels of a nanomechanical oscillator

The coherent states that describe the classical motion of a mechanical oscillator do not have well-defined energy, but are rather quantum superpositions of equally-spaced energy eigenstates. Revealing this quantized structure is only possible with an apparatus that measures the mechanical energy with a precision greater than the energy of a single phonon, $\hbarω_\text{m}$. One way to achieve this sensitivity is by engineering a strong but nonresonant interaction between the oscillator and an atom. In a system with sufficient quantum coherence, this interaction allows one to distinguish different phonon number states by resolvable differences in the atom's transition frequency. Such dispersive measurements have been studied in cavity and circuit quantum electrodynamics where experiments using real and artificial atoms have resolved the photon number states of cavities. Here, we report an experiment where an artificial atom senses the motional energy of a driven nanomechanical oscillator with sufficient sensitivity to resolve the quantization of its energy. To realize this, we build a hybrid platform that integrates nanomechanical piezoelectric resonators with a microwave superconducting qubit on the same chip. We excite phonons with resonant pulses of varying amplitude and probe the resulting excitation spectrum of the qubit to observe phonon-number-dependent frequency shifts $\approx 5$ times larger than the qubit linewidth. Our result demonstrates a fully integrated platform for quantum acoustics that combines large couplings, considerable coherence times, and excellent control over the mechanical mode structure. With modest experimental improvements, we expect our approach will make quantum nondemolition measurements of phonons an experimental reality, leading the way to new quantum sensors and information processing approaches that use chip-scale nanomechanical devices.

quant-ph↗

arXiv2019

Quantum dynamics of a few-photon parametric oscillator

Modulating the frequency of a harmonic oscillator at nearly twice its natural frequency leads to amplification and self-oscillation. Above the oscillation threshold, the field settles into a coherent oscillating state with a well-defined phase of either $0$ or $π$. We demonstrate a quantum parametric oscillator operating at microwave frequencies and drive it into oscillating states containing only a few photons. The small number of photons present in the system and the coherent nature of the nonlinearity prevents the environment from learning the randomly chosen phase of the oscillator. This allows the system to oscillate briefly in a quantum superposition of both phases at once - effectively generating a nonclassical Schrödinger's cat state. We characterize the dynamics and states of the system by analyzing the output field emitted by the oscillator and implementing quantum state tomography suited for nonlinear resonators. By demonstrating a quantum parametric oscillator and the requisite techniques for characterizing its quantum state, we set the groundwork for new schemes of quantum and classical information processing and extend the reach of these ubiquitous devices deep into the quantum regime.

quant-ph↗

arXiv2018

Coupling a superconducting quantum circuit to a phononic crystal defect cavity

Connecting nanoscale mechanical resonators to microwave quantum circuits opens new avenues for storing, processing, and transmitting quantum information. In this work, we couple a phononic crystal cavity to a tunable superconducting quantum circuit. By fabricating a one-dimensional periodic pattern in a thin film of lithium niobate and introducing a defect in this artificial lattice, we localize a 6 gigahertz acoustic resonance to a wavelength-scale volume of less than one cubic micron. The strong piezoelectricity of lithium niobate efficiently couples the localized vibrations to the electric field of a widely tunable high-impedance Josephson junction array resonator. We measure a direct phonon-photon coupling rate $g/2π\approx 1.6 \, \mathrm{MHz}$ and a mechanical quality factor $Q_\mathrm{m} \approx 3 \times 10^4$ leading to a cooperativity $C\sim 4$ when the two modes are tuned into resonance. Our work has direct application to engineering hybrid quantum systems for microwave-to-optical conversion as well as emerging architectures for quantum information processing.

quant-ph↗