arXiv subjects

E. Charron

Publications and source records attributed to E. Charron.

12 recordsLinked to original sources

arXiv2022

All-Optical Matter-Wave Lens using Time-Averaged Potentials

The stability of matter-wave sensors benefits from interrogating large-particle-number atomic ensembles at high cycle rates. The use of quantum-degenerate gases with their low effective temperatures allows constraining systematic errors towards highest accuracy, but their production by evaporative cooling is costly with regard to both atom number and cycle rate. In this work, we report on the creation of cold matter-waves using a crossed optical dipole trap and shaping it by means of an all-optical matter-wave lens. We demonstrate the trade off between residual kinetic energy and atom number by short-cutting evaporative cooling and estimate the corresponding performance gain in matter-wave sensors. Our method is implemented using time-averaged optical potentials and hence easily applicable in optical dipole trapping setups.

physics.atom-ph↗

arXiv2019

Anisotropy Control in Photoelectron Spectra: A Coherent Two-Pulse Interference Strategy

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single parameter control using two ultra-short light pulses delayed in time. The first pulse prepares a superposition of a few ion rotational states, whereas the second pulse serves as a probe that gives access to a control of the molecular asymmetry parameter $β$ for individual rotational channels. This is achieved by tuning the time delay between the pulses leading to channel interferences that can be turned from constructive to destructive. The illustrative example is the ionization of the $E(1Σ_{g}^{+})$ state of Li$_{2}$. Quantum wave packet evolutions are conducted including both electronic and nuclear degrees of freedom to reach angle-resolved photoelectron spectra. A simple interference model based on coherent phase accumulation during the field-free dynamics between the two pulses is precisely exploited to control the photoelectron angular distributions from almost isotropic, to marked anisotropic.

physics.chem-ph↗

arXiv2019

Concept study and preliminary design of a cold atom interferometer for space gravity gradiometry

We study a space-based gravity gradiometer based on cold atom interferometry and its potential for the Earth's gravitational field mapping. The instrument architecture has been proposed in [Carraz et al., Microgravity Science and Technology 26, 139 (2014)] and enables high-sensitivity measurements of gravity gradients by using atom interferometers in a differential accelerometer configuration. We present the design of the instrument including its subsystems and analyze the mission scenario, for which we derive the expected instrument performances, the requirements on the sensor and its key subsystems, and the expected impact on the recovery of the Earth gravity field.

physics.atom-ph↗

arXiv2019

Optimal control of the transport of Bose-Einstein condensates with atom chips

Using Optimal Control Theory (OCT), we design fast ramps for the controlled transport of Bose-Einstein condensates with atom chips' magnetic traps. These ramps are engineered in the context of precision atom interferometry experiments and support transport over large distances, typically of the order of 1 mm, i.e. about 1,000 times the size of the atomic clouds, yet with durations not exceeding 200 ms. We show that with such transport durations of the order of the trap period, one can recover the ground state of the final trap at the end of the transport. The performance of the OCT procedure is compared to that of a Shortcut-To-Adiabaticity (STA) protocol and the respective advantages / disadvantages of the OCT treatment over the STA one are discussed.

quant-ph↗

arXiv2017

Fast manipulation of Bose-Einstein condensates with an atom chip

We present a detailed theoretical analysis of the implementation of shortcut-to-adiabaticity protocols for the fast transport of neutral atoms with atom chips. The objective is to engineer transport ramps with durations not exceeding a few hundred milliseconds to provide metrologically-relevant input states for an atomic sensor. Aided by numerical simulations of the classical and quantum dynamics, we study the behavior of a Bose-Einstein condensate in an atom chip setup with realistic anharmonic trapping. We detail the implementation of fast and controlled transports over large distances of several millimeters, i.e. distances 1000 times larger than the size of the atomic cloud. A subsequent optimized release and collimation step demonstrates the capability of our transport method to generate ensembles of quantum gases with expansion speeds in the picokelvin regime. The performance of this procedure is analyzed in terms of collective excitations reflected in residual center of mass and size oscillations of the condensate. We further evaluate the robustness of the protocol against experimental imperfections.

quant-ph↗

arXiv2017

Extracting spectroscopic molecular parameters from short pulse photo-electron angular distributions

Using a quantum wave packet simulation including the nuclear and electronic degrees of freedom, we investigate the femtosecond and picosecond energy- and angle-resolved photoelectron spectra of the E($^1Σ_g^+$) electronic state of Li$_2$. We find that the angular distributions of the emitted photoelectrons depend strongly on the pulse duration in the regime of ultrashort laser pulses. This effect is illustrated by the extraction of a time-dependent asymmetry parameter whose variation with pulse duration can be explained by an incoherent average over different ion rotational quantum numbers. We then derive for the variation of the asymmetry parameter a simple analytical formula, which can be used to extract the asymptotic CW asymmetry parameters of individual transitions from measurements performed with ultra-short pulses.

physics.chem-ph↗

arXiv2016

Laser-Induced Electron Diffraction: Inversion of Photoelectron Spectra for Molecular Orbital Imaging

In this paper, we discuss the possibility of imaging molecular orbitals from photoelectron spectra obtained via Laser Induced Electron Diffraction (LIED) in linear molecules. This is an extension of our work published recently in Physical Review A \textbf{94}, 023421 (2016) to the case of the HOMO-1 orbital of the carbon dioxide molecule. We show that such an imaging technique has the potential to image molecular orbitals at different internuclear distances in a sub-femtosecond time scale and with a resolution of a fraction of an Angström.

physics.atom-ph↗

arXiv2016

Laser-Induced Electron Diffraction: Alignment Defects and Symmetry Breaking

The fringe pattern that allows geometrical and orbital structure information to be extracted from LIED spectra of symmetric molecules is shown to reflect a symmetry conservation principle. We show that under a field polarization which preserves certain symmetry elements of the molecule, the symmetry character of the initial wave function is conserved during its time-evolution. We present a symmetry analysis of a deviation from a perfect alignment by decomposing the field into a major, symmetry-determining part, and a minor, symmetry breaking, part. This decomposition leads to a corresponding factorization of the time-evolution operator. The formalism is applied to the analysis of the robustness of LIED readings and inversions with respect to deviations from a perfect perpendicular and parallel alignment of a symmetric ABA triatomic molecule. The results indicate a particularly strong stability of the type of LIED spectra associated with the perpendicular alignment situation.

quant-ph↗

arXiv2016

Inversion of Strong Field Photoelectron Spectra for Molecular Orbital Imaging

Imaging structures at the molecular level is a fast developing interdisciplinary research field that spans across the boundaries of physics and chemistry. High spatial resolution images of molecules can be obtained with photons or ultrafast electrons. In addition, images of valence molecular orbitals can be extracted via tomographic techniques based on the coherent XUV radiation emitted by a molecular gas exposed to an intense ultra-short infrared laser pulse. In this paper, we demonstrate that similar information can be obtained by inverting energy resolved photoelectron spectra using a simplified analytical model.

physics.atom-ph↗

arXiv2010

Effect of picosecond strain pulses on thin layers of the ferromagnetic semiconductor (Ga,Mn)(As,P)

The effect of picosecond acoustic strain pulses (ps-ASP) on a thin layer of (Ga,Mn)As co-doped with phosphorus was probed using magneto-optical Kerr effect (MOKE). A transient MOKE signal followed by low amplitude oscillations was evidenced, with a strong dependence on applied magnetic field, temperature and ps-ASP amplitude. Careful interferometric measurement of the layer's thickness variation induced by the ps-ASP allowed us to model very accurately the resulting signal, and interpret it as the strain modulated reflectivity (differing for $σ_{\pm}$ probe polarizations), independently from dynamic magnetization effects.

cond-mat.mtrl-sci↗

arXiv2008

Molecular orientation entanglement and temporal Bell-type inequalities

We detail and extend the results of [Milman {\it et al.}, Phys. Rev. Lett. {\bf 99}, 130405 (2007)] on Bell-type inequalities based on correlations between measurements of continuous observables performed on trapped molecular systems. We show that for some observables with a continuous spectrum which is bounded, one is able to construct non-locality tests sharing common properties with those for two-level systems. The specific observable studied here is molecular spatial orientation, and it can be experimentally measured for single molecules, as required in our protocol. We also provide some useful general properties of the derived inequalities and study their robustness to noise. Finally, we detail possible experimental scenarii and analyze the role played by different experimental parameters.

quant-ph↗

arXiv2006

Theoretical analysis of the implementation of a quantum phase gate with neutral atoms on atom chips

We present a detailed, realistic analysis of the implementation of a proposal for a quantum phase gate based on atomic vibrational states, specializing it to neutral rubidium atoms on atom chips. We show how to create a double--well potential with static currents on the atom chips, using for all relevant parameters values that are achieved with present technology. The potential barrier between the two wells can be modified by varying the currents in order to realize a quantum phase gate for qubit states encoded in the atomic external degree of freedom. The gate performance is analyzed through numerical simulations; the operation time is ~10 ms with a performance fidelity above 99.9%. For storage of the state between the operations the qubit state can be transferred efficiently via Raman transitions to two hyperfine states, where its decoherence is strongly inhibited. In addition we discuss the limits imposed by the proximity of the surface to the gate fidelity.

quant-ph↗