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E. Clément

Publications and source records attributed to E. Clément.

At least 19 recordsLinked to original sources

Performance of the Particle-Identification Silicon-Telescope Array Coupled with the VAMOS++ Magnetic Spectrometer

The Particle-Identification Silicon-Telescope Array (PISTA) is a new detection system designed for high-resolution studies of the fission process induced by multi-nucleon transfer in inverse kinematics. It is specifically optimized for experiments with the VAMOS++ magnetic spectrometer at GANIL (Grand Accélérateur National d'Ions Lourds). The array comprises eight trapezoidal $Δ$E-E silicon telescopes arranged in a corolla configuration. Each telescope integrates two single-sided stripped silicon detectors, enabling target-like recoil identification, energy loss measurements, and trajectory reconstruction. Positioned in close proximity to the target, PISTA's compact geometry achieves high-efficiency tracking of target-like recoils produced in multi-nucleon transfer reactions at Coulomb barrier energies. The spatial segmentation of the array allows precise determination of the mass and charge of the target-like nucleus, and excitation energy of fissioning systems. This work presents the particle identification and excitation energy reconstruction performances for the interactions of $^{238}$U beam with $^{12}$C target. An excitation energy resolution of 800 keV (FWHM) was determined together with mass resolution of 1.1% (FWHM). The combination of PISTA and VAMOS++ magnetic spectrometer enables unprecedented investigations of the fission process as a function of the excitation energy of the fissioning nucleus, particularly for exotic systems produced in transfer-induced reactions.

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Direct transfer to $^{46,48}$K as a survey of the $π(s_{1/2})$$-ν(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $πs_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$γ$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$γ$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $πs_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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Shape evolution in neutron-rich odd-even $^{105-109}$Nb isotopes

Neutron-rich nuclei around $Z\sim40$ exhibit multiple shape transitions. This region shows one of the sharpest transitions in the nuclear chart, from a spherical vibrator at $N=58$ to a strongly deformed prolate shape at $N=60$, with largest deformations seen for $_{38}$Sr and $_{40}$Zr. Below $Z=36$, a spherical-to-oblate transition is predicted, while above $Z=42$ and $N\ge60$, the shape evolves from axial to triaxial. Even-$Z$ nuclei have been well studied, but odd-$Z$ isotopes such as Nb offer additional insights into these mechanisms. The Nb isotopes lie at the boundary between axially deformed Zr and triaxially deformed Mo nuclei. This work explores the structure of neutron-rich Nb nuclei up to $N=68$, aiming to understand shape evolution with isospin and the onset of triaxiality. Two complementary fission experiments were used: (i) $^{238}$U+$^9$Be at GANIL in inverse kinematics with AGATA, EXOGAM, and VAMOS++, allowing prompt and delayed $γ$-ray spectroscopy with isotopic identification; (ii) spontaneous fission of $^{252}$Cf with the Gammasphere array providing high-fold $γ$-coincidence data. The level scheme of $^{105}$Nb was significantly extended with two new negative-parity bands. A revised scheme is proposed for $^{107}$Nb, differing from previous results, and new structures are reported in $^{109}$Nb. The signature splitting analysis indicates triaxial deformation for positive-parity bands, while negative-parity bands show axial symmetry, similar to Zr. This reveals a shape coexistence in neutron-rich Nb nuclei.

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Unbound neutron $\nu0d_{3/2}$ strength in $^{17}$C and the N=16 shell gap

Significant continuum strength has been observed to be populated in $^{17}$C produced in the d($^{16}$C,p) reaction at a beam energy of 17.2~MeV/nucleon. The strength appears at greater than $\sim$2~MeV above the single-neutron decay threshold and has been identified as arising from transfer into the neutron $0d_{3/2}$ orbital. Guided by shell model predictions the greater majority of the strength is associated with a 3/2$^+$ state at an excitation energy of 4.40$_{-0.14}^{+0.33}$ MeV and a much weaker 3/2$^+$ level at 5.60$_{-0.45}^{+1.35}$ MeV. The corresponding total widths were determined to be 3.45$_{-0.78}^{+1.82}$ and 1.6$_{-1.4}^{+4.6}$ MeV, respectively. From the backward angle proton differential cross sections and the branching ratios for neutron decay to the $^{16}$C(2$_{1}^{+}$) level, the corresponding spectroscopic factors to the ground state were deduced to be 0.47$\pm{10}$ and $<$0.09. Shell-model calculations employing the phenomenological SFO-tls interaction as well as Gamow Shell-Model calculations including continuum effects are in reasonable agreement with experiment, although the predicted strength lies at somewhat lower energy. The size of the N=16 shell gap ($\varepsilon_{ \nu0d_{3/2}}-\varepsilon _{ν1s_{1/2}}$) was estimated to be 5.08$_{-0.33}^{+0.43}$~MeV - some 1.3~MeV larger than found in the SFO-tls shell model calculation.

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Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $γγ$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $γγ$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $γγ$-coincidence and $γ$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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High-resolution spectroscopy of neutron-rich Br isotopes and signatures for a prolate-to-oblate shape transition at N=56

The first systematic experimental study of the neutron-rich Br isotopes with two complementary state-of-the-art techniques is presented. These isotopes have been populated in the fission process at two different facilities, GANIL and ILL. New spectroscopic information has been obtained for odd-even $^{87-93}$Br isotopes and the experimental results have been compared with state-of-the-art Large-Scale Shell-Model and DNO Shell-Model calculations. As a result of such theoretical approaches, a transition from prolate ($^{87,89}$Br) to oblate ($^{91,93}$Br) shapes is obtained from the subtle balance between proton and neutron quadrupole deformations, as a clear signature of pseudo-SU3 quadrupole regime.

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High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $γ$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $γ$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $γ$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

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CATLIFE (Complementary Arm for Target LIke FragmEnts): Spectrometer for Target like fragments at VAMOS++

The multi-nucleon transfer reaction between 136Xe beam and 198Pt target at the beam energy 7 MeV/u was studied using the large acceptance spectrometer VAMOS++ coupled with the newly installed second arm time-of-flight and delayed $γ$-ray spectrometer CATLIFE (Complementary Arm for Target LIke FragmEnts). The CATLIFE detector is composed of a large area multi-wire proportional chamber and the EXOGAM HPGe clover detectors with an ion flight length of 1230 mm. Direct measurement of the target-like fragments (TLF) and the delayed $γ$-rays from the isomeric state helps to improve TLF identification. The use of the velocity of TLFs and the delayed $γ$-ray demonstrate the proof of principle and effectiveness of the new setup.

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Cross-shell states in $^{15}$C: a test for p-sd interactions

The low-lying structure of $^{15}$C has been investigated via the neutron-removal $^{16}$C$(d,t)$ reaction. Along with bound neutron sd-shell hole states, unbound p-shell hole states have been firmly confirmed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the $[(p)^{-1}(sd)^{2}]$ neutron configurations in $^{15}$C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for $^{15}$C. However, a modification of the $p$-$sd$ and $sd$-$sd$ monopole terms was applied in order to reproduce the $N=9$ isotone $^{17}$O. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of $^{15}$C with the $ab~ initio$ self-consistent Green's function method employing the NNLO$_{sat}$ interaction. The results show the sensitivity to the size of the $N=8$ shell gap and highlight the need of going beyond the current truncation scheme in the theory.

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Search for $^{22}$Na in novae supported by a novel method for measuring femtosecond nuclear lifetimes

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,γ$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories.

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$^{178}$Hg and asymmetric fission of neutron-deficient pre-actinides

Fission at low excitation energy is an ideal playground to probe the impact of nuclear structure on nuclear dynamics. While the importance of structural effects in the nascent fragments is well-established in the (trans-)actinide region, the observation of asymmetric fission in several neutron-deficient pre-actinides can be explained by various mechanisms. To deepen our insight into that puzzle, an innovative approach based on inverse kinematics and an enhanced version of the VAMOS++ heavy-ion spectrometer was implemented at the GANIL facility, Caen. Fission of $^{178}$Hg was induced by fusion of $^{124}$Xe and $^{54}$Fe. The two fragments were detected in coincidence using VAMOS++ supplemented with a new SEcond Detection arm. For the first time in the pre-actinide region, access to the pre-neutron mass and total kinetic energy distributions, and the simultaneous isotopic identification of one the fission fragment, was achieved. The present work describes the experimental approach, and discusses the pre-neutron observables in the context of an extended asymmetric-fission island located south-west of $^{208}Pb. A comparison with different models is performed, demonstrating the importance of this "new" asymmetric-fission island for elaborating on driving effects in fission.

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Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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Coulomb and nuclear excitations of $^{70}$Zn and $^{68}$Ni at intermediate energy

The reduced transition probabilities $B(E2; 0^+_{g.s.}\rightarrow2_1^+,2^+_2)$ in $^{70}$Zn and the full $B(E2; 0^+_{g.s.}\rightarrow2^+)$ strength up to S$_n$=7.79 MeV in $^{68}$Ni have been determined at the LISE/GANIL facility using the Coulomb-excitation technique at intermediate beam energy on a $^{208}$Pb target. The $γ$ rays emitted in-flight were detected with an array of 46 BaF$_2$ crystals. The angles of the deflected nuclei were determined in order to disentangle and extract the Coulomb and nuclear contributions to the excitation of the 2$^+$ states. The measured $B(E2; 0^+_{g.s.}\rightarrow2_1^+)$ of 1432(124) e$^2$fm$^4$ for $^{70}$Zn falls in the lower part of the published values which clustered either around 1600 or above 2000 e$^2$fm$^4$, while the $B(E2; 0^+_{g.s.}\rightarrow2^+_2)$ of 53(7) e$^2$fm$^4$ agrees very well with the two published values. The relatively low $B(E2; 0^+_{g.s.}\rightarrow2_1^+)$ of 301(38) e$^2$fm$^4$ for $^{68}$Ni agrees with previous studies and confirms a local magicity at $Z=28, N=40$. Combining the results of the low-energy spectra of $^{68}$Ni and $^{70}$Zn and their shell-model interpretations, it is interesting to notice that four different shapes (spherical, oblate, prolate and triaxial) are present. Finally, a summed $E2$ strength of only about 150 e$^2$fm$^4$ has been found experimentally at high excitation energy, likely due to proton excitations across the $Z=28$ gap. The experimental distribution of this high-energy $E2$ excitation agrees with SM calculations, but its strength is about two times weaker.

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Lifetime Measurements in the Even-Even $^{102-108}$Cd Isotopes

The heaviest N=Z doubly-magic nucleus, $^{100}$Sn, and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction in extreme conditions. In particular, the Cd isotopes are expected to present features similar to those found in the Sn isotopic chain, since they have only two proton holes in the Z=50 shell. In this manuscript, the lifetime measurements of low-lying states in the even-mass $^{102-108}$Cd is presented. Thanks to the powerful detection capabilities of AGATA array and VAMOS++ spectrometer, the unusual employment of multi-nucleon transfer reactions permitted to investigate the first 2$^+$ and 4$^+$ states in all these nuclei, together with various deformed bands in $^{106}$Cd. The results were interpreted in the context of new state-of-the-art beyond-mean-field calculations, using the symmetry-conserving configuration-mixing approach. Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z=48 and Z=50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with $β_2 \approx 0.2$. At this deformation Z=48 becomes a closed-shell configuration, which is favored with respect to the spherical one.

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Evidence for enhanced neutron-proton correlations from the level structure of the $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$

The low-lying excited states in the neutron-deficient $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$ have been studied via the fusion-evaporation reaction $^{54}$Fe($^{36}$Ar, $2n1p$)$^{87}$Tc at the Grand Accélérateur National d'Ions Lourds (GANIL), France. The AGATA spectrometer was used in conjunction with the auxiliary NEDA, Neutron Wall, and DIAMANT detector arrays to measure coincident prompt $γ$-rays, neutrons, and charged particles emitted in the reaction. A level scheme of $^{87}$Tc from the (9/2$^{+}_{g.s.}$) state to the (33/2$^{+}_{1}$) state was established based on 6 mutually coincident $γ$-ray transitions. The constructed level structure exhibits a rotational behavior with a sharp backbending at $\hbarω\approx 0.50$ MeV. A decrease in alignment frequency and increase in alignment sharpness in the odd-mass isotonic chains around $N=44$ is proposed as an effect of the enhanced isoscalar neutron-proton interactions in odd-mass nuclei when approaching the $N=Z$ line.

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HeCTOr: the $^3$He Cryogenic Target of Orsay for direct nuclear reactions with radioactive beams

Direct nuclear reactions with radioactive ion beams represent an extremely powerful tool to extend the study of fundamental nuclear properties far from stability. These measurements require pure and dense targets to cope with the low beam intensities. The $^3$He cryogenic target HeCTOr has been designed to perform direct nuclear reactions in inverse kinematics. The high density of $^3$He scattering centers, of the order of 10$^{20}$ atoms/cm$^2$, makes it particularly suited for experiments where low-intensity radioactive beams are involved. The target was employed in a first in-beam experiment, where it was coupled to state-of-the-art gamma-ray and particle detectors. It showed excellent stability in gas temperature and density over time. Relevant experimental quantities, such as total target thickness, energy resolution and gamma-ray absorption, were determined through dedicated Geant4 simulations and found to be in good agreement with experimental data.

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The MUGAST-AGATA-VAMOS campaign : set-up and performance

The MUGAST-AGATA-VAMOS set-up at GANIL combines the MUGAST highly-segmented silicon array with the state-of-the-art AGATA array and the large acceptance VAMOS spectrometer. The mechanical and electronics integration copes with the constraints of maximum efficiency for each device, in particular γ-ray transparency for the silicon array. This complete set-up offers a unique opportunity to perform exclusive measurements of direct reactions with the radioactive beams from the SPIRAL1 facility. The performance of the set-up is described through its commissioning and two examples of transfer reactions measured during the campaign. High accuracy spectroscopy of the nuclei of interest, including cross-sections and angular distributions, is achieved through the triple-coincidence measurement. In addition, the correction from Doppler effect of the γ-ray energies is improved by the detection of the light particles and the use of two-body kinematics and a full rejection of the background contributions is obtained through the identification of heavy residues. Moreover, the system can handle high intensity beams (up to 108 pps). The particle identification based on the measurement of the time-of-flight between MUGAST and VAMOS and the reconstruction of the trajectories is investigated.

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