arXiv subjects

E. Dartois

Publications and source records attributed to E. Dartois.

At least 55 records · Page 3Linked to original sources

arXiv2016

Spatial distribution of FIR rotationally excited CH+ and OH emission lines in the Orion Bar PDR

The abundance of CH+ and OH and excitation are predicted to be enhanced by the presence of vibrationally excited H2 or hot gas (~500-1000 K) in PDRs with high incident FUV radiation field. The excitation may also originate in dense gas (>10^5 cm-3) followed by nonreactive collisions. Previous observations suggest that the CH+ and OH correlate with dense and warm gas, and formation pumping contributes to CH+ excitation. We examine the spatial distribution of the CH+ and OH emission in the Orion Bar to establish their physical origin and main formation and excitation mechanisms. We present spatially sampled maps of the CH+ J=3-2 transition at 119.8 μm and the OH Λ-doublet at 84 μm in the Orion Bar over an area of 110"x110" with Herschel (PACS). We compare the spatial distribution of these molecules with those of their chemical precursors, C+, O and H2, and tracers of warm and dense gas. We assess the spatial variation of CH+ J=2-1 velocity-resolved line profile observed with Herschel (HIFI). The OH and CH+ lines correlate well with the high-J CO emission and delineate the warm and dense molecular region. While similar, the differences in the CH+ and OH morphologies indicate that CH+ formation and excitation are related to the observed vibrationally excited H2. This indicates that formation pumping contributes to the excitation of CH+. Interestingly, the peak of the rotationally excited OH 84 μm emission coincides with a bright young object, proplyd 244-440, which shows that OH can be an excellent tracer of UV-irradiated dense gas. The spatial distribution of CH+ and OH revealed in our maps is consistent with previous modeling studies. Both formation pumping and nonreactive collisions in a UV-irradiated dense gas are important CH+ J=3-2 excitation processes. The excitation of the OH Λ-doublet at 84 μm is mainly sensitive to the temperature and density.

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arXiv2016

Early Mars volcanic sulfur storage in the cryosphere and formation of transient SO2-rich atmospheres during the Hesperian

In a previous paper (Chassefière et al., Icarus 223, 878-891, 2013), we have shown that most volcanic sulfur released to early Mars atmosphere could have been trapped in the cryosphere under the form of CO2-SO2 clathrates. Huge amounts of sulfur, up to the equivalent of a ~1 bar atmosphere of SO2, would have been stored in the Noachian cryosphere, then massively released to the atmosphere during Hesperian due to rapidly decreasing CO2 pressure. It would have resulted in the formation of the large sulfate deposits observed mainly in Hesperian terrains, whereas no or little sulfates are found at the Noachian. In the present paper, we first clarify some aspects of our previous work. We discuss the possibility of a smaller cooling effect of sulfur particles, or even of a net warming effect. We point out the fact that CO2-SO2 clathrates formed through a progressive enrichment of a preexisting reservoir of CO2 clathrates and discuss processes potentially involved in the slow formation of a SO2-rich upper cryosphere. We show that episodes of sudden destabilization at the Hesperian may generate 1000 ppmv of SO2 in the atmosphere and contribute to maintaining the surface temperature above the water freezing point.

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arXiv2016

Mantle formation, coagulation and the origin of cloud/core-shine: II. Comparison with observations

Many dense interstellar clouds are observable in emission in the near-IR, commonly referred to as "Cloudshine", and in the mid-IR, the so-called "Coreshine". These C-shine observations have usually been explained with grain growth but no model has yet been able to self-consistently explain the dust spectral energy distribution from the near-IR to the submm. We want to demonstrate the ability of our new core/mantle evolutionary dust model THEMIS (The Heterogeneous dust Evolution Model at the IaS), which has been shown to be valid in the far-IR and submm, to reproduce the C-shine observations. Our starting point is a physically motivated core/mantle dust model. It consists of 3 dust populations: small aromatic-rich carbon grains; bigger core/mantle grains with mantles of aromatic-rich carbon and cores either made of amorphous aliphatic-rich carbon or amorphous silicate. We assume an evolutionary path where these grains, when entering denser regions, may first form a second aliphatic-rich carbon mantle (coagulation of small grains, accretion of carbon from the gas phase), second coagulate together to form large aggregates, and third accrete gas phase molecules coating them with an ice mantle. To compute the corresponding dust emission and scattering, we use a 3D Monte-Carlo radiative transfer code. We show that our global evolutionary dust modelling approach THEMIS allows us to reproduce C-shine observations towards dense starless clouds. Dust scattering and emission is most sensitive to the cloud central density and to the steepness of the cloud density profile. Varying these two parameters leads to changes, which are stronger in the near-IR, in both the C-shine intensity and profile. With a combination of aliphatic-rich mantle formation and low-level coagulation into aggregates, we can self-consistently explain the observed C-shine and far-IR/submm emission towards dense starless clouds.

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arXiv2016

Mantle formation, coagulation and the origin of cloud/core shine: I. Modelling dust scattering and absorption in the infra-red

Context. The observed cloudshine and coreshine (C-shine) have been explained in terms of grain growth leading to enhanced scatter- ing from clouds in the J, H and K photometric bands and the Spitzer IRAC 3.6 and 4.5 μm bands. Aims. Using our global dust modelling approach THEMIS (The Heterogeneous dust Evolution Model at the IaS) we explore the effects of dust evolution in dense clouds, through aliphatic-rich carbonaceous mantle formation and grain-grain coagulation. Methods. We model the effects of wide band gap a-C:H mantle formation and the low-level aggregation of diffuse interstellar medium dust in the moderately-extinguished outer regions of molecular clouds. Results. The formation of wide band gap a-C:H mantles on amorphous silicate and amorphous carbon (a-C) grains leads to a decrease in their absorption cross-sections but no change in their scattering cross-sections at near-IR wavelengths, resulting in higher albedos. Conclusions. The evolution of dust, with increasing density and extinction in the diffuse to dense molecular cloud transition, through mantle formation and grain aggregation, appears to be a likely explanation for the observed C-shine.

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arXiv2016

VUV spectroscopy of carbon dust analogs: contribution to interstellar extinction

A full spectral characterization of carbonaceous dust analogs is necessary to understand their potential as carriers of observed astronomical spectral signatures such as the ubiquitous UV bump at 217.5 nm and the far-ultraviolet (FUV) rise common to interstellar extinction curves. Our goal is to study the spectral properties of carbonaceous dust analogs from the FUV to the mid-infrared (MIR) domain. We seek in particular to understand the spectra of these materials in the FUV range, for which laboratory studies are scarce. We produced analogs to carbonaceous interstellar dust encountered in various phases of the interstellar medium: amorphous hydrogenated carbons (a-C:H), for carbonaceous dust observed in the diffuse interstellar medium, and soot particles, for the polyaromatic component. Analogs to a-C:H dust were produced using a radio-frequency plasma reactor at low pressures, and soot nanoparticles films were produced in an ethylene (C$_2$H$_4$) flame. We measured transmission spectra of these thin films (thickness < 100 nm) in the far-ultraviolet (190 - 250 nm) and in the vacuum-ultraviolet (VUV; 50 - 190 nm) regions using the APEX chamber at the DISCO beam line of the SOLEIL synchrotron radiation facility. These were also characterized through infrared microscopy at the SMIS beam line. We successfully measured the transmission spectra of these analogs from λ = 1 μm to 50 nm. From these, we extracted the laboratory optical constants via Kramers-Kronig inversion. We used these constants for comparison to existing interstellar extinction curves. We extend the spectral measurements of these types of carbonaceous analogs into the VUV and link the spectral features in this range to the 3.4 μm band. We suggest that these two materials might contribute to different classes of interstellar extinction curves.

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arXiv2015

Heavy ion irradiation of crystalline water ice

Under cosmic irradiation, the interstellar water ice mantles evolve towards a compact amorphous state. Crystalline ice amorphisation was previously monitored mainly in the keV to hundreds of keV ion energies. We experimentally investigate heavy ion irradiation amorphisation of crystalline ice, at high energies closer to true cosmic rays, and explore the water-ice sputtering yield. We irradiated thin crystalline ice films with MeV to GeV swift ion beams, produced at the GANIL accelerator. The ice infrared spectral evolution as a function of fluence is monitored with in-situ infrared spectroscopy (induced amorphisation of the initial crystalline state into a compact amorphous phase). The crystalline ice amorphisation cross-section is measured in the high electronic stopping-power range for different temperatures. At large fluence, the ice sputtering is measured on the infrared spectra, and the fitted sputtering-yield dependence, combined with previous measurements, is quadratic over three decades of electronic stopping power. The final state of cosmic ray irradiation for porous amorphous and crystalline ice, as monitored by infrared spectroscopy, is the same, but with a large difference in cross-section, hence in time scale in an astrophysical context. The cosmic ray water-ice sputtering rates compete with the UV photodesorption yields reported in the literature. The prevalence of direct cosmic ray sputtering over cosmic-ray induced photons photodesorption may be particularly true for ices strongly bonded to the ice mantles surfaces, such as hydrogen-bonded ice structures or more generally the so-called polar ices.

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arXiv2014

Interstellar ice analogs: band strengths of H$_2$O, CO$_2$, CH$_3$OH, and NH$_3$ in the far-infrared region

We measure the band strengths in the far-infrared region of interstellar ice analogs of astrophysically relevant species, such as H$_2$O, CO$_2$, CH$_3$OH, and NH$_3$, deposited at low temperature (8-10 $\mathrm{K}$), followed by warm-up, to induce amorphous-crystalline phase transitions when relevant. The spectra of pure H$_2$O, NH$_3$, and CH$_3$OH ices have been measured in the near-, mid- and far-infrared spectroscopic regions using the Interstellar Astrochemistry Chamber (ISAC) ultra-high-vacuum setup. In addition, far-infrared spectra of NH$_3$ and CO$_2$ were measured using a different set-up equipped with a bolometer detector. Band strengths in the far-infrared region were estimated using the corresponding near- and mid-infrared values as a reference. We also performed theoretical calculations of the amorphous and crystalline structures of these molecules using solid state computational programs at density functional theory (DFT) level. Vibrational assignment and mode intensities for these ices were predicted. Infrared band strengths in the 25-500 $μ$m range have been determined for the considered ice samples by direct comparison in the near- and mid-infrared regions. Our values were compared to those we calculated from the literature complex index of refraction. We found differences of a factor of two between the two sets of values. The calculated far-infrared band strengths provide a benchmark for interpreting the observational data from future space telescope missions, allowing the estimation of the ice column densities.

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arXiv2014

Comparison of UV and high-energy ion irradiation of methanol:ammonia ice

The main goal of this work is to compare the effects induced in ices of astrophysical relevance by high-energy ions, simulating cosmic rays, and by vacuum ultraviolet (UV) photons. This comparison relies on in situ infrared spectroscopy of irradiated CH3OH:NH3 ice. Swift heavy ions were provided by the GANIL accelerator. The source of UV was a microwave-stimulated hydrogen flow discharge lamp. The deposited energy doses were similar for ion beams and UV photons to allow a direct comparison. A variety of organic species was detected during irradiation and later during ice warm-up. These products are common to ion and UV irradiation for doses up to a few tens of eV per molecule. Only the relative abundance of the CO product, after ice irradiation, was clearly higher in the ion irradiation experiments. For some ice mixture compositions, the irradiation products formed depend only weakly on the type of irradiation, swift heavy ions, or UV photons. This simplifies the chemical modeling of energetic ice processing in space.

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arXiv2011

Spatial variation of the cooling lines in the Orion Bar from Herschel/PACS

We present spatially resolved Herschel/PACS observations of the Orion Bar. We have characterise the emission of the far-infrared fine-structure lines of [CII] (158um), [OI] (63 and 145um), and [NII] (122um) that trace the gas local conditions. The observed distribution and variation of the lines are discussed in relation to the underlying geometry and linked to the energetics associated with the Trapezium stars. These observations enable us to map the spatial distribution of these fine-structure lines with a spatial resolution between 4" and 11" and covering a total square area of about 120"x105". The spatial profile of the emission lines are modelled using the radiative transfer code Cloudy. We find that the spatial distribution of the [CII] line coincides with that of the [OI] lines. The [NII] line peaks closer to the ionising star than the other three lines, but with a small region of overlap. We can distinguish several knots of enhanced emission within the Bar indicating the presence of an inhomogenous and structured medium. The emission profiles cannot be reproduced by a single photo-dissociation region, clearly indicating that, besides the Bar, there is a significant contribution from additional photo-dissociation region(s) over the area studied. The combination of both the [NII] and [OI] 145um lines can be used to estimate the [CII] emission and distinguish between its ionised or neutral origin. We have calculated how much [CII] emission comes from the neutral and ionised region, and find that at least 82% originates from the photo-dissocciation region. Together, the [CII] 158um and [OI] 63 and 145um lines account for 90% of the power emitted by the main cooling lines in the Bar (including CO, H2, etc...), with [OI] 63um alone accounting for 72% of the total.

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arXiv2010

Nitrogen hydrides in interstellar gas: Herschel/HIFI observations towards G10.6-0.4 (W31C)

The HIFI instrument on board the Herschel Space Observatory has been used to observe interstellar nitrogen hydrides along the sight-line towards G10.6-0.4 in order to improve our understanding of the interstellar chemistry of nitrogen. We report observations of absorption in NH N=1-0, J=2-1 and ortho-NH2 1_1,1-0_0,0. We also observed ortho-NH3 1_0-0_0, and 2_0-1_0, para-NH3 2_1-1_1, and searched unsuccessfully for NH+. All detections show emission and absorption associated directly with the hot-core source itself as well as absorption by foreground material over a wide range of velocities. All spectra show similar, non-saturated, absorption features, which we attribute to diffuse molecular gas. Total column densities over the velocity range 11-54 km/s are estimated. The similar profiles suggest fairly uniform abundances relative to hydrogen, approximately 6*10^-9, 3*10^-9, and 3*10^-9 for NH, NH2, and NH3, respectively. These abundances are discussed with reference to models of gas-phase and surface chemistry.

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arXiv2010

Detection of hydrogen fluoride absorption in diffuse molecular clouds with Herschel/HIFI: a ubiquitous tracer of molecular gas

We discuss the detection of absorption by interstellar hydrogen fluoride (HF) along the sight line to the submillimeter continuum sources W49N and W51. We have used Herschel's HIFI instrument in dual beam switch mode to observe the 1232.4762 GHz J = 1 - 0 HF transition in the upper sideband of the band 5a receiver. We detected foreground absorption by HF toward both sources over a wide range of velocities. Optically thin absorption components were detected on both sight lines, allowing us to measure - as opposed to obtain a lower limit on - the column density of HF for the first time. As in previous observations of HF toward the source G10.6-0.4, the derived HF column density is typically comparable to that of water vapor, even though the elemental abundance of oxygen is greater than that of fluorine by four orders of magnitude. We used the rather uncertain N(CH)-N(H2) relationship derived previously toward diffuse molecular clouds to infer the molecular hydrogen column density in the clouds exhibiting HF absorption. Within the uncertainties, we find that the abundance of HF with respect to H2 is consistent with the theoretical prediction that HF is the main reservoir of gas-phase fluorine for these clouds. Thus, hydrogen fluoride has the potential to become an excellent tracer of molecular hydrogen, and provides a sensitive probe of clouds of small H2 column density. Indeed, the observations of hydrogen fluoride reported here reveal the presence of a low column density diffuse molecular cloud along the W51 sight line, at an LSR velocity of ~ 24kms-1, that had not been identified in molecular absorption line studies prior to the launch of Herschel.

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arXiv2010

Herschel/HIFI measurements of the ortho/para ratio in water towards Sagittarius B2(M) and W31C

We present Herschel/HIFI observations of the fundamental rotational transitions of ortho- and para-H$_2^{16}$O and H$_2^{18}$O in absorption towards Sagittarius~B2(M) and W31C. The ortho/para ratio in water in the foreground clouds on the line of sight towards these bright continuum sources is generally consistent with the statistical high-temperature ratio of 3, within the observational uncertainties. However, somewhat unexpectedly, we derive a low ortho/para ratio of $2.35 \pm 0.35$, corresponding to a spin temperature of $\sim$27~K, towards Sagittarius~B2(M) at velocities of the expanding molecular ring. Water molecules in this region appear to have formed with, or relaxed to, an ortho/para ratio close to the value corresponding to the local temperature of the gas and dust.

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arXiv2010

Herschel/HIFI observations of interstellar OH+ and H2O+ towards W49N: a probe of diffuse clouds with a small molecular fraction

We report the detection of absorption by interstellar hydroxyl cations and water cations, along the sight-line to the bright continuum source W49N. We have used Herschel's HIFI instrument, in dual beam switch mode, to observe the 972 GHz N = 1 - 0 transition of OH+ and the 1115 GHz 1(11) - 0(00) transition of ortho-H2O+. The resultant spectra show absorption by ortho-H2O+, and strong absorption by OH+, in foreground material at velocities in the range 0 to 70 km/s with respect to the local standard of rest. The inferred OH+/H2O+ abundance ratio ranges from ~ 3 to ~ 15, implying that the observed OH+ arises in clouds of small molecular fraction, in the 2 - 8% range. This conclusion is confirmed by the distribution of OH+ and H2O+ in Doppler velocity space, which is similar to that of atomic hydrogen, as observed by means of 21 cm absorption measurements, and dissimilar from that typical of other molecular tracers. The observed OH+/H abundance ratio of a few E-8 suggests a cosmic ray ionization rate for atomic hydrogen of (0.6 - 2.4) E-16 s-1, in good agreement with estimates inferred previously for diffuse clouds in the Galactic disk from observations of interstellar H3+ and other species.

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arXiv2010

Excitation and Abundance of C3 in star forming cores:Herschel/HIFI observations of the sight-lines to W31C and W49N

We present spectrally resolved observations of triatomic carbon (C3) in several ro-vibrational transitions between the vibrational ground state and the low-energy nu2 bending mode at frequencies between 1654-1897 GHz along the sight-lines to the submillimeter continuum sources W31C and W49N, using Herschel's HIFI instrument. We detect C3 in absorption arising from the warm envelope surrounding the hot core, as indicated by the velocity peak position and shape of the line profile. The sensitivity does not allow to detect C3 absorption due to diffuse foreground clouds. From the column densities of the rotational levels in the vibrational ground state probed by the absorption we derive a rotation temperature (T_rot) of ~50--70 K, which is a good measure of the kinetic temperature of the absorbing gas, as radiative transitions within the vibrational ground state are forbidden. It is also in good agreement with the dust temperatures for W31C and W49N. Applying the partition function correction based on the derived T_rot, we get column densities N(C3) ~7-9x10^{14} cm^{-2} and abundance x(C3)~10^{-8} with respect to H2. For W31C, using a radiative transfer model including far-infrared pumping by the dust continuum and a temperature gradient within the source along the line of sight we find that a model with x(C3)=10^{-8}, T_kin=30-50 K, N(C3)=1.5 10^{15} cm^{-2} fits the observations reasonably well and provides parameters in very good agreement with the simple excitation analysis.

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arXiv2010

Herschel-SPIRE observations of the Polaris flare : structure of the diffuse interstellar medium at the sub-parsec scale

We present a power spectrum analysis of the Herschel-SPIRE observations of the Polaris flare, a high Galactic latitude cirrus cloud midway between the diffuse and molecular phases. The SPIRE images of the Polaris flare reveal for the first time the structure of the diffuse interstellar medium down to 0.01 parsec over a 10 square degrees region. These exceptional observations highlight the highly filamentary and clumpy structure of the interstellar medium even in diffuse regions of the map. The power spectrum analysis shows that the structure of the interstellar medium is well described by a single power law with an exponent of -2.7 +- 0.1 at all scales from 30" to 8 degrees. That the power spectrum slope of the dust emission is constant down to the SPIRE angular resolution is an indication that the inertial range of turbulence extends down to the 0.01 pc scale. The power spectrum analysis also allows the identification of a Poissonian component at sub-arcminute scales in agreement with predictions of the cosmic infrared background level at SPIRE wavelengths. Finally, the comparison of the SPIRE and IRAS 100 micron data of the Polaris flare clearly assesses the capability of SPIRE in maping diffuse emission over large areas.

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arXiv2010

Strong absorption by interstellar hydrogen fluoride: Herschel/HIFI observations of the sight-line to G10.6-0.4 (W31C)

We report the detection of strong absorption by interstellar hydrogen fluoride along the sight-line to the submillimeter continuum source G10.6-0.4 (W31C). We have used Herschel's HIFI instrument, in dual beam switch mode, to observe the 1232.4763 GHz J=1-0 HF transition in the upper sideband of the Band 5a receiver. The resultant spectrum shows weak HF emission from G10.6-0.4 at LSR velocities in the range -10 to -3 km/s, accompanied by strong absorption by foreground material at LSR velocities in the range 15 to 50 km/s. The spectrum is similar to that of the 1113.3430 GHz 1(11)-0(00) transition of para-water, although at some frequencies the HF (hydrogen fluoride) optical depth clearly exceeds that of para-H2O. The optically-thick HF absorption that we have observed places a conservative lower limit of 1.6E+14 cm-2 on the HF column density along the sight-line to G10.6-0.4. Our lower limit on the HF abundance, 6E-9 relative to hydrogen nuclei, implies that hydrogen fluoride accounts for between ~ 30 and 100% of the fluorine nuclei in the gas phase along this sight-line. This observation corroborates theoretical predictions that - because the unique thermochemistry of fluorine permits the exothermic reaction of F atoms with molecular hydrogen - HF will be the dominant reservoir of interstellar fluorine under a wide range of conditions.

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arXiv2010

Physical properties of the Sh2-104 HII region as seen by Herschel

Context: Sh2-104 is a Galactic H ii region with a bubble morphology, detected at optical and radio wavelengths. It is considered the first observational confirmation of the collect-and-collapse model of triggered star-formation. Aims: We aim to analyze the dust and gas properties of the Sh2-104 region to better constrain its effect on local future generations of stars. In addition, we investigate the relationship between the dust emissivity index β and the dust temperature, T_dust. Methods: Using Herschel PACS and SPIRE images at 100, 160, 250, 350 and 500 μm we determine T_dust and β throughout Sh2-104, fitting the spectral energy distributions (SEDs) obtained from aperture photometry. With the SPIRE Fourier transform spectrometer (FTS) we obtained spectra at different positions in the Sh2-104 region. We detect J-ladders of CO and 13CO, with which we derive the gas temperature and column density. We also detect proxies of ionizing flux as the [NII] 3P1-3P0 and [CI] 3P2-3P1 transitions. Results: We find an average value of β ~ 1.5 throughout Sh2-104, as well as a T dust difference between the photodissociation region (PDR, ~ 25 K) and the interior (~ 40 K) of the bubble. We recover the anti-correlation between β and dust temperature reported numerous times in the literature. The relative isotopologue abundances of CO appear to be enhanced above the standard ISM values, but the obtained value is very preliminary and is still affected by large uncertainties.

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arXiv2010

Herschel-SPIRE spectroscopy of the DR21 molecular cloud core

We present far-infrared spectra and maps of the DR21 molecular cloud core between 196 and 671 microns, using the Herschel-SPIRE spectrometer. Nineteen molecular lines originating from CO, 13CO, HCO+ and H2O, plus lines of [N II] and [CI] were recorded, including several transitions not previously detected. The CO lines are excited in warm gas with Tkin ~ 125 K and nH2 ~ 7 x 10^4 cm-3, CO column density N(CO) ~ 3.5 x 10^18 cm^-2 and a filling factor of ~ 12%, and appear to trace gas associated with an outflow. The rotational temperature analysis incorporating observations from ground-based telescopes reveals an additional lower excitation CO compoment which has a temperature ~ 78 K and N(CO) ~ 4.5 x 10^21 cm^-2. Astronomy & Astrophysics HERSCHEL special Issue, in press.

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