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E. Demler

Publications and source records attributed to E. Demler.

At least 19 recordsLinked to original sources

The Ultrafast Superconducting Diode Effect

Nonreciprocal transport is generally observed in superconductors in which time reversal and inversion symmetries are simultaneously broken. This effect, which may become one of the backbones for future superconducting electronics, arises because of asymmetric vortex transport in a magnetic field. However, vortex transport is also intrinsically dissipative and limited in speed. Here, we report on the discovery of ultrafast non-reciprocal transport in centrosymmetric superconductors. For NbN films biased with a quasi-DC supercurrent, picosecond current pulses with the same sign as the bias experience resistive impedance, whereas pulses of opposite polarity encounter an inductive response. Strikingly, the effect is at least three orders of magnitude faster than in conventional superconducting diodes, limited only by ultrafast current-induced depairing. We demonstrate rectification of a 100 GHz signal, with dissipation levels of a few fJ per cycle. We foresee potential for superconducting logic elements, operating at THz bit rates with aJ energy dissipation per operation.

cond-mat.supr-con

Probing picosecond depairing currents in type-II superconductors

Accessing the intrinsic critical current density (Jc*) in type II superconductors has significant fundamental and technological potential, both as a probe of the microscopic superconducting properties and as a means to increase current limits in high magnetic field devices and in electrical power systems. Yet, the experimental critical current density in type II superconductors (Jc), when measured with DC currents, is generally lower than the intrinsic limit, mostly due to vortex motion and self-heating. Here, we show that ultrafast picosecond electrical pulses, which interact with the material on timescales over which vortices are inertially immobile, carry supercurrents up to the intrinsic depairing limit Jc* >> Jc. We probe picosecond critical currents in NbN and YBa2Cu3O7 (YBCO), as representative s-wave and d-wave superconductors, respectively. In NbN, we find a sharp onset of the picosecond depairing at a current density as large as Jc*=2.2 Jc, a limit that is well described by microscopic dynamics based on BCS theory. In contrast, YBCO exhibits a gradual suppression of superconductivity as a function of the picosecond current, reflecting its d-wave symmetry. These results offer a powerful new probe of superconductors beyond the reach of conventional transport measurements. The ability to reach the depairing current may also lead to robust new platforms for superconducting electronics.

cond-mat.supr-con

Photoengineering the Magnon Spectrum in an Insulating Antiferromagnet

Femtosecond optical pulses have opened a new frontier in ultrafast dynamics, enabling direct access to fundamental interactions in quantum materials. In antiferromagnets (AFMs), where the fundamental quantum mechanical exchange interaction governs spin dynamics, this access is especially compelling, enabling the excitation of magnons - collective spin-wave modes - that naturally reach terahertz (THz) frequencies and supersonic velocities. Femtosecond optical pulses provided a route to coherently excite such magnons across the entire Brillouin zone. Controlling their spectral properties - such as the magnon gap and dispersion - represents the next monumental step, enabling dynamic tuning of group velocities, coherence, and interaction pathways. Yet, achieving this remains a challenge, requiring ultrafast and long-lasting manipulation of the underlying exchange interaction. Here, we show that in DyFeO3 - an insulating AFM with strongly coupled electronic and magnetic degrees of freedom - resonant above-bandgap optical excitation leads to a dramatic renormalization of the THz magnon spectrum, including a near-total collapse of the magnon gap. Our analysis reveals this transformation to be consistent with a transient reduction of the exchange interaction by nearly 90% in the near-surface nanoscale region. These findings establish a pathway for light-driven, nanoscale control of AFM spin dynamics, opening opportunities for reconfigurable, high-speed magnonic and spintronic applications.

cond-mat.str-el

Enhanced coherent terahertz emission from critical superconducting fluctuations in YBa$_2$Cu$_3$O$_{6.6}$

Coherent terahertz (THz) emission is emerging as a powerful new tool to probe symmetry breakings in quantum materials. This method relies on second order optical nonlinearities and is complementary to second harmonic generation spectroscopy. Here, we report coherent THz emission from Josephson plasmons in underdoped YBa$_2$Cu$_3$O$_{6+x}$, and find that the amplitude of the emitted field increases dramatically close to the superconducting transition temperature, $T_C$. We show theoretically how emission is enhanced by critical superconducting fluctuations, a nonlinear analogue of critical opalescence. This observation is expected to be of general importance for the study of many thermal and quantum phase transitions.

cond-mat.supr-con

Impurities and polarons in bosonic quantum gases: a review on recent progress

This review describes the field of Bose polarons, arising when mobile impurities are immersed into a bosonic quantum gas. The latter can be realized by a Bose-Einstein condensate (BEC) of ultracold atoms, or of exciton polaritons in a semiconductor, which has led to a series of experimental observations of Bose polarons near inter-species Feshbach resonances that we survey. Following an introduction to the topic, with references to its historic roots and a presentation of the Bose polaron Hamiltonian, we summarize state-of-the-art experiments. Next we provide a detailed discussion of polaron models, starting from the ubiquitous Fr\"ohlich Hamiltonian that applies at weak couplings. We proceed by a survey of concurrent theoretical methods used for solving strongly interacting Bose polaron problems. The subsequent sections are devoted to the large bodies of work investigating strong coupling Bose polarons, including detailed comparisons with radio-frequency (RF) spectra obtained in ultracold atom experiments; to investigations of universal few-body and Efimov states associated with a Feshbach resonance in atomic mixtures; to studies of quantum dynamics and polarons out of equilibrium; Bose polarons in low-dimensional; induced interactions among polarons and bipolaron formation; and to Bose polarons at non-zero temperatures. We end our review by detailed discussions of closely related experimental setups and systems, including ionic impurities, systems with strong light-matter interactions, and variations and extensions of the Bose polaron concepts e.g. to baths with topological order or strong interactions relevant for correlated electrons. Finally, an outlook is presented, highlighting possible future research directions and open questions in the field as a whole.

cond-mat.quant-gas

Squeezed Josephson plasmons in driven YBa$_2$Cu$_3$O$_{6+x}$

The physics of driven collective modes in quantum materials underpin a number of striking non-equilibrium functional responses, which include enhanced magnetism, ferroelectricity and superconductivity. However, the coherent coupling between multiple modes at once are difficult to capture by single-pump probe (one-dimensional) spectroscopy, and often remain poorly understood. One example is phonon-mediated amplification of Josephson plasmons in YBa$_2$Cu$_3$O$_{6+x}$, in which at least three normal modes of the solid are coherently mixed as a source of enhanced superconductivity. Here, we go beyond previous pump-probe experiments in this system and acquire two-dimensional frequency maps using pairs of mutually delayed, carrier envelope phase stable mid-infrared pump pulses, combined with measurements of the time-modulated second-order nonlinear optical susceptibility. We find that the driven zone-center phonons amplify coherent pairs of opposite-momentum Josephson plasma polaritons, generating a squeezed state of interlayer phase fluctuations. The squeezed state is a potentially important ingredient in the microscopic physics of photo-induced superconductivity in this and other materials.

cond-mat.supr-con

Exciton transport in a germanium quantum dot ladder

Quantum systems with engineered Hamiltonians can be used as simulators of many-body physics problems to provide insights beyond the capabilities of classical computers. Semiconductor gate-defined quantum dot arrays have emerged as a versatile platform for quantum simulation of generalized Fermi-Hubbard physics, one of the richest playgrounds in condensed matter physics. In this work, we employ a germanium 4$\times$2 quantum dot array and show that the naturally occurring long-range Coulomb interaction can lead to exciton formation and transport. We tune the quantum dot ladder into two capacitively-coupled channels and exploit Coulomb drag to probe the binding of electrons and holes. Specifically, we shuttle an electron through one leg of the ladder and observe that a hole is dragged along in the second leg under the right conditions. This corresponds to a transition from single-electron transport in one leg to exciton transport along the ladder. Our work paves the way for the study of excitonic states of matter in quantum dot arrays.

cond-mat.mes-hall

Coherent Emission from Surface Josephson Plasmons in Striped Cuprates

The interplay between charge order and superconductivity remains one of the central themes of research in quantum materials. In the case of cuprates, the coupling between striped charge fluctuations and local electromagnetic fields is especially important, as it affects transport properties, coherence and dimensionality of superconducting correlations. Here, we study the emission of coherent terahertz radiation in single-layer cuprates of the La$_{2-x}$Ba$_x$CuO$_4$ family, for which this effect is expected to be forbidden by symmetry. We find that emission vanishes for compounds in which the stripes are quasi-static, but is activated when $c$-axis inversion symmetry is broken by incommensurate or fluctuating charge stripes, such as in La$_{1.905}$Ba$_{0.095}$CuO$_4$ and in La$_{1.845}$Ba$_{0.155}$CuO$_4$. In this case, terahertz radiation is emitted by surface Josephson plasmons, which are generally dark modes, but couple to free space electromagnetic radiation because of the stripe modulation.

cond-mat.supr-con

Rotational Resonances and Regge Trajectories in Lightly Doped Antiferromagnets

Understanding the nature of charge carriers in doped Mott insulators holds the key to unravelling puzzling properties of strongly correlated electron systems, including cuprate superconductors. Several theoretical models suggested that dopants can be understood as bound states of partons, the analogues of quarks in high-energy physics. However, direct signatures of spinon-chargon bound states are lacking, both in experiment and theory. Here we numerically identify long-lived rotational resonances at low doping, which directly reveal the microscopic structure of spinon-chargon bound states. Similar to Regge trajectories reflecting the quark structure of mesons, we establish a linear dependence of the rotational energy on the super-exchange coupling. Rotational excitations are strongly suppressed in standard angle-resolved photo-emission (ARPES) spectra, but we propose a multi-photon rotational extension of ARPES where they have strong spectral weight. Our findings suggest that multi-photon spectroscopy experiments should provide new insights into emergent universal features of strongly correlated electron systems.

cond-mat.str-el

Observation of Wigner crystal of electrons in a monolayer semiconductor

When the Coulomb repulsion between electrons dominates over their kinetic energy, electrons in two dimensional systems were predicted to spontaneously break continuous translation symmetry and form a quantum crystal. Efforts to observe this elusive state of matter, termed a Wigner crystal (WC), in two dimensional extended systems have primarily focused on electrons confined to a single Landau level at high magnetic fields, but have not provided a conclusive experimental signature of the emerging charge order. Here, we use optical spectroscopy to demonstrate that electrons in a pristine monolayer semiconductor with density $ \lesssim 3 \cdot 10^{11}$ cm$^{-2}$ form a WC. The interactions between resonantly injected excitons and electrons arranged in a periodic lattice modify the exciton band structure so that it exhibits a new umklapp resonance, heralding the presence of charge order. Remarkably, the combination of a relatively high electron mass and reduced dielectric screening allows us to observe an electronic WC state even in the absence of magnetic field. The tentative phase diagram obtained from our Hartree-Fock calculations provides an explanation of the striking experimental signatures obtained up to $B = 16$ T. Our findings demonstrate that charge-tunable transition metal dichalcogenide (TMD) monolayers enable the investigation of previously uncharted territory for many-body physics where interaction energy dominates over kinetic energy, even in the absence of a moire potential or external fields.

cond-mat.mes-hall

Dominant fifth-order correlations in doped quantum anti-ferromagnets

Traditionally one and two-point correlation functions are used to characterize many-body systems. In strongly correlated quantum materials, such as the doped 2D Fermi-Hubbard system, these may no longer be sufficient because higher-order correlations are crucial to understanding the character of the many-body system and can be numerically dominant. Experimentally, such higher-order correlations have recently become accessible in ultracold atom systems. Here we reveal strong non-Gaussian correlations in doped quantum anti-ferromagnets and show that higher order correlations dominate over lower-order terms. We study a single mobile hole in the $t-J$ model using DMRG, and reveal genuine fifth-order correlations which are directly related to the mobility of the dopant. We contrast our results to predictions using models based on doped quantum spin liquids which feature significantly reduced higher-order correlations. Our predictions can be tested at the lowest currently accessible temperatures in quantum simulators of the 2D Fermi-Hubbard model. Finally, we propose to experimentally study the same fifth-order spin-charge correlations as a function of doping. This will help to reveal the microscopic nature of charge carriers in the most debated regime of the Hubbard model, relevant for understanding high-$T_c$ superconductivity.

cond-mat.quant-gas

Parametric instabilities in a 2D periodically-driven bosonic system: Beyond the weakly-interacting regime

We experimentally investigate the effects of parametric instabilities on the short-time heating process of periodically-driven bosons in 2D optical lattices with a continuous transverse (tube) degree of freedom. We analyze three types of periodic drives: (i) linear along the x-lattice direction only, (ii) linear along the lattice diagonal, and (iii) circular in the lattice plane. In all cases, we demonstrate that the BEC decay is dominated by the emergence of unstable Bogoliubov modes, rather than scattering in higher Floquet bands, in agreement with recent theoretical predictions. The observed BEC depletion rates are much higher when shaking both along x and y directions, as opposed to only x or only y. This is understood as originating from the interaction-induced non-separability along the two lattice directions. We also report an explosion of the heating rates at large drive amplitudes, and suggest a phenomenological description beyond Bogoliubov theory. In this strongly-coupled regime, circular drives heat faster than diagonal drives, which illustrates the non-trivial dependence of the heating on the choice of drive.

quant-ph

Simulating a quantum commensurate-incommensurate phase transition using two Raman coupled one dimensional condensates

We study a transition between a homogeneous and an inhomogeneous phase in a system of one-dimensional, Raman tunnel-coupled Bose gases. The homogeneous phase shows a flat density and phase profile, whereas the inhomogeneous ground state is characterized by periodic density ripples, and a soliton staircase in the phase difference. We show that under experimentally viable conditions the transition can be tuned by the wavevector difference $Q$ of the Raman beams and can be described by the Pokrovsky-Talapov model for the relative phase between the two condensates. Local imaging available in atom chip experiments allows to observe the soliton lattice directly, while modulation spectroscopy can be used to explore collective modes, such as the phonon mode arising from breaking of translation symmetry by the soliton lattice. In addition, we investigate regimes where the cold atom experiment deviates from the Pokrovsky-Talapov field theory. We predict unusual mesoscopic effects arising from the finite size of the system, such as quantized injection of solitons upon increasing $Q$, or the system size. For moderate values of $Q$ above criticality, we find that the density modulations in the two gases interplay with the relative phase profile and introduce novel features in the spatial structure of the mode wave-functions. Using an inhomogeneous Bogoliubov theory, we show that spatial quantum fluctuations are intertwined with the emerging soliton staircase. Finally, we comment on the prospects of the ultra-cold atom setup as a tunable platform studying quantum aspects of the Pokrovsky-Talapov theory in and out-of-equilibrium.

cond-mat.quant-gas

Parametrically amplified phase-incoherent superconductivity in YBa$_2$Cu$_3$O$_{6+x}$

The possibility of enhancing desirable functional properties of complex materials by optical driving is motivating a series of studies of their nonlinear terahertz response. In high-Tc cuprates, large amplitude excitation of certain infrared-active lattice vibrations has been shown to induce transient features in the reflectivity suggestive of non-equilibrium superconductivity. Yet, a microscopic mechanism for these observations is still lacking. Here, we report measurements of time- and scattering-angle-dependent second-harmonic generation in YBa$_2$Cu$_3$O$_{6+x}$, taken under the same excitation conditions that result in superconductor-like terahertz reflectivity. We discover a three-order-of-magnitude amplification of a 2.5-terahertz electronic mode, which is unique because of its symmetry, momentum, and temperature dependence. A theory for parametric three-wave amplification of Josephson plasmons, which are assumed to be well-formed below T$_c$ but overdamped throughout the pseudogap phase, explains all these observations and provides a mechanism for non-equilibrium superconductivity. More broadly, our work underscores the role of parametric mode mixing to stabilize fluctuating orders in quantum materials.

cond-mat.supr-con

Parametric instabilities of interacting bosons in periodically-driven 1D optical lattices

Periodically-driven quantum systems are currently explored in view of realizing novel many-body phases of matter. This approach is particularly promising in gases of ultracold atoms, where sophisticated shaking protocols can be realized and inter-particle interactions are well controlled. The combination of interactions and time-periodic driving, however, often leads to uncontrollable heating and instabilities, potentially preventing practical applications of Floquet-engineering in large many-body quantum systems. In this work, we experimentally identify the existence of parametric instabilities in weakly-interacting Bose-Einstein condensates in strongly-driven optical lattices through momentum-resolved measurements. Parametric instabilities can trigger the destruction of weakly-interacting Bose-Einstein condensates through the rapid growth of collective excitations, in particular in systems with weak harmonic confinement transverse to the lattice axis.

cond-mat.quant-gas

Non-Abelian symmetries and disorder: a broad non-ergodic regime and anomalous thermalization

Symmetries play a central role in single-particle localization. Recent research focused on many-body localized (MBL) systems, characterized by new kind of integrability, and by the area-law entanglement of eigenstates. We investigate the effect of a non-Abelian $SU(2)$ symmetry on the dynamical properties of a disordered Heisenberg chain. While $SU(2)$ symmetry is inconsistent with the conventional MBL, a new non-ergodic regime is possible. In this regime, the eigenstates exhibit faster than area-law, but still a strongly sub-thermal scaling of entanglement entropy. Using exact diagonalization, we establish that this non-ergodic regime is indeed realized in the strongly disordered Heisenberg chains. We use real-space renormalization group (RSRG) to construct approximate excited eigenstates, and show their accuracy for systems of size up to $L=26$. As disorder strength is decreased, a crossover to the thermalizing phase occurs. To establish the ultimate fate of the non-ergodic regime in the thermodynamic limit, we develop a novel approach for describing many-body processes that are usually neglected by RSRG, accessing systems of size $L>2000$. We characterize the resonances that arise due to such processes, finding that they involve an ever growing number of spins as the system size is increased. The probability of finding resonances grows with the system size. Even at strong disorder, we can identify a large lengthscale beyond which resonances proliferate. Presumably, this eventually would drive the system to a thermalizing phase. However, the extremely long thermalization time scales indicate that a broad non-ergodic regime will be observable experimentally. Our study demonstrates that symmetries control dynamical properties of disordered, many-body systems. The approach introduced here provides a versatile tool for describing a broad range of disordered many-body systems.

cond-mat.str-el

Gaussian states for the variational study of (1+1)-dimensional lattice gauge models

We introduce a variational ansatz based on Gaussian states for (1+1)-dimensional lattice gauge models. To this end we identify a set of unitary transformations which decouple the gauge degrees of freedom from the matter fields. Using our ansatz, we study static aspects as well as real-time dynamics of string breaking in two (1+1)-dimensional theories, namely QED and two-color QCD. We show that our ansatz captures the relevant features and is in excellent agreement with data from numerical calculations with tensor networks.

hep-lat

Variational study of U(1) and SU(2) lattice gauge theories with Gaussian states in 1+1 dimensions

We introduce a method to investigate the static and dynamic properties of both Abelian and non-Abelian lattice gauge models in 1+1 dimensions. Specifically, we identify a set of transformations that disentangle different degrees of freedom, and apply a simple Gaussian variational ansatz to the resulting Hamiltonian. To demonstrate the suitability of the method, we analyze both static and dynamic aspects of string breaking for the U(1) and SU(2) gauge models. We benchmark our results against tensor network simulations and observe excellent agreement, although the number of variational parameters in the Gaussian ansatz is much smaller.

hep-lat