arXiv subjects

E. F. van Dishoeck

Publications and source records attributed to E. F. van Dishoeck.

At least 109 records · Page 6Linked to original sources

arXiv2022

Importance of source structure on complex organics emission II. Can disks explain lack of methanol emission from some low-mass protostars?

Some protostellar systems show little or no millimetre line emission of complex organics. This can be interpreted as a low abundance of these molecules, alternatively they could be present in the system but are not seen in the gas. The goal is to investigate the latter hypothesis for methanol. We will attempt to answer the question: Does the presence of a disk and optically thick dust reduce methanol emission even if methanol is abundant in the ices and gas? Using the radiative transfer code RADMC-3D, methanol emission lines from an envelope-only model and an envelope-plus-disk model are calculated and compared with each other and the observations. Methanol emission from the envelope-only model is always stronger than from the envelope-plus-disk model by at least a factor 2 as long as the disk radius is larger than 30 au (for L=8 L$_{\odot}$). In most cases, this is due to lower temperatures and, hence, the smaller amount of warm methanol inside the snow surface of the envelope-plus-disk model. The intensities drop by more than an order of magnitude for models including high mm opacity dust grains and disk radii of at least 50 au (for L=8 L$_{\odot}$) due to continuum over-subtraction. The line intensities from the envelope-only models overproduce the observations of protostars with lower methanol emission even with large dust optical depth effects. The envelope-plus-disk models can explain the bulk of the observations. However, they can only reproduce the observations of sources with high luminosities and low methanol emission when dust optical depth effects especially continuum over-subtraction in the disk becomes effective. Therefore, both the effects of disk and dust optical depth should be considered to explain the observations. In conclusion: Absence of methanol emission does not imply absence of methanol molecules in either gas or ice.

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arXiv2022

Importance of source structure on complex organics emission. I. Observations of CH$_3$OH from low-mass to high-mass protostars

Complex organic molecules (COMs) are often observed toward embedded Class 0 and I protostars. However, not all Class 0 and I protostars exhibit COMs emission. In this work, variations in methanol (CH$_3$OH) emission are studied to test if absence of CH$_3$OH emission can be linked to source properties. Combining both new and archival observations with ALMA and sources from the literature, a sample of 184 low-mass and high-mass protostars is investigated. The warm (T > 100 K) gaseous CH$_3$OH mass, $M_{\rm CH_3OH}$, is determined for each source using primarily optically thin isotopologues. On average, Class I protostellar systems seem to have less warm $M_{\rm CH_3OH}$ ($<10^{-10}$ M$_\odot$) than younger Class 0 sources ($\sim10^{-7}$ M$_\odot$). High-mass sources in our sample show higher warm $M_{\rm CH_3OH}$ up to $10^{-7}-10^{-3}$ M$_\odot$. To take into account the effect of the source's overall mass on $M_{\rm CH_3OH}$, a normalized CH$_3$OH mass is defined as $M_{\rm CH_3OH}/M_{\rm dust,0}$, where $M_{\rm dust,0}$ is the cold + warm dust mass within a fixed radius. Excluding upper limits, a simple power-law fit to the normalized warm CH$_3$OH masses results in $M_{\rm CH_3OH}/M_{\rm dust,0}\propto L_{\rm bol}^{0.70\pm0.05}$. This is in good agreement with a simple hot core toy model which predicts that the normalized $M_{\rm CH_3OH}$ increases with $L_{\rm bol}^{0.75}$ due to the snowline moving outward. Sources for which the size of the disk is equivalent or smaller than the estimated 100 K radius agree well with the best-fit power-law model, whereas sources with significantly larger disks show up to two orders of magnitude lower normalized warm CH$_3$OH masses. Based on the latter results, we suggest that source structure such as a disk can result in colder gas and thus fewer COMs in the gas phase. Additionally, optically thick dust can hide the emission of COMs.

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arXiv2022

Survey of Orion Disks with ALMA (SODA) I: Cloud-level demographics of 873 protoplanetary disks

(Abridged) Surveys of protoplanetary disks in nearby star-forming regions (SFRs) have provided important information on their demographics, but due to their sample sizes, they cannot be used to study how disk properties vary with the environment. We conduct a survey of the unresolved millimeter continuum emission of 873 protoplanetary disks identified by Spitzer in the L1641 and L1647 regions of the Orion A cloud. This is the largest such survey yet, allowing us to identify even weak trends in the median disk mass as a function of position in the cloud and cluster membership. The sample detection rates and median masses are also compared to those of nearby (<300 pc) SFRs. The sample was observed with ALMA at 225 GHz, with a median rms of 0.08 mJy/beam (1.5 M$_{\oplus}$). The data were reduced and imaged using an innovative parallel data processing approach. We detect 58% (502/873) of the observed disks. This includes 20 disks with dust masses >100 M$_{\oplus}$, and two objects associated with extended dust emission. We infer a median disk dust mass in the full sample of $2.2^{+0.2}_{-0.2}$ M$_{\oplus}$. In L1641 and L1647 median dust masses are $2.1^{+0.2}_{-0.2}$ M$_{\oplus}$ and $2.6^{+0.4}_{-0.5}$ M$_{\oplus}$, respectively. The disk mass distribution of the full sample is similar to that of nearby low-mass SFRs at similar ages of 1-3 Myr. We find only weak trends in disk (dust) masses with galactic longitude and between the YSO clusters identified in the sample, with median masses varying by $\lesssim$ 50%. Age differences may explain these median disk mass variations. Apart from this, disk masses are essentially constant at scales of ~100 pc. This also suggests that the majority of disks, even in different SFRs, are formed with similar initial masses and evolve at similar rates, assuming no external irradiation, with disk mass loss rates of $\sim 10^{-8}$ M$_{\odot}$/yr.

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arXiv2022

Tracing pebble drift and trapping using radial carbon depletion profiles in protoplanetary disks

The composition of planets may be largely determined by the chemical processing and accretion of icy pebbles in protoplanetary disks. Recent observations of protoplanetary disks hint at wide-spread depletion of gaseous carbon. The missing volatile carbon is likely frozen in CO and/or CO$_2$ ice on grains and locked into the disk through pebble trapping in pressure bumps or planetesimals. We present the results of the first successful ACA (Atacama Compact Array) [C I] $J$ = 1-0 mini-survey of seven protoplanetary disks. Using tailored azimuthally symmetric DALI (Dust And LInes) thermo-chemical disk models, supported by the [C I] $J$ = 1-0 and resolved CO isotopologue data, we determine the system-averaged elemental volatile carbon abundance in the outer disk of three sources. Six out of seven sources are detected in [C I] $J$ = 1-0 with ACA, four of which show a distinct disk component. Based on the modeling we find severe cold gaseous carbon depletion in the outer disk of DL Tau and moderate depletion in the outer disks of DR Tau and DO Tau. Combining the outer and inner disk carbon abundances, we demonstrate definitive evidence for radial drift in the disk of DL Tau, where the existence of multiple dust rings points to either short lived or leaky dust traps. We find dust locking in the compact and smooth disks of DO Tau and DR Tau, hinting at unresolved dust substructure. Comparing our results with stars of different ages and luminosities, we identify an observational evolutionary trend in gaseous carbon depletion that is consistent with dynamical models of CO depletion processes. Transport efficiency of solids in protoplanetary disks can significantly differ from what we expect based on the current resolved substructure in the continuum observations. This has important implications for our understanding of the impact of radial drift and pebble accretion on planetary compositions.

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arXiv2021

Early planet formation in embedded protostellar disks: Setting the stage for the first generation of planetesimals

(Abridged) Recent surveys of young star formation regions have shown that the average Class II object does not have enough dust mass to make the cores of giant planets. Younger Class 0/I objects have enough dust in their embedded disk, which begs the questions: can the first steps of planet formation occur in these younger systems? The first step is building the first planetesimals, generally believed to be the product of the streaming instability. Hence the question can be restated: are the physical conditions of embedded disks conducive to the growth of the streaming instability? Here we model the collapse of a `dusty' proto-stellar cloud to show that if there is sufficient drift between the falling gas and dust, regions of the embedded disk can become sufficiently enhanced in dust to drive the streaming instability. We include four models, three with different dust grain sizes and one with a different initial cloud angular momentum to test a variety of collapse trajectories. We find a `sweet spot' for planetesimal formation for grain sizes of a few 10s of micron since they fall sufficiently fast relative to the gas to build a high dust-to-gas ratio along the disk midplane, but have slow enough radial drift speeds in the embedded disk to maintain the high dust-to-gas ratio. Unlike the gas, which is held in hydrostatic equilibrium for a time due to gas pressure, the dust can begin collapsing from all radii at a much earlier time. The streaming instability can produce at least between 7-35 M$_\oplus$ of planetesimals in the Class 0/I phase of our smooth embedded disks, depending on the size of the falling dust grains. This first generation of planetesimals could represent the first step in planet formation, and occurs earlier in the lifetime of the young star than is traditionally thought.

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arXiv2021

Probing inner and outer disk misalignments in transition disks

For several transition disks (TDs), dark regions interpreted as shadows have been observed in scattered light imaging and are hypothesized to originate from misalignments between distinct disk regions. We aim to investigate the presence of misalignments in TDs. We study the inner disk geometries of 20 well-known transition disks with VLTI/GRAVITY observations and use complementary $^{12}$CO and $^{13}$CO molecular line data from ALMA to derive the orientation of the outer disk regions. We fit simple models to the GRAVITY data to derive the inner disks inclination and position angles. The outer disk geometries were derived from Keplerian fits to the ALMA velocity maps and compared to the inner disk constraints. We also predicted the locations of shadows for significantly misaligned systems. Our analysis reveals six disks to exhibit significant misalignments between their inner and outer disks. The predicted shadow positions agree well with the scattered light images of HD100453 and HD142527, and we find supporting evidence for a shadow in the disk around CQ Tau. In the other three targets for which we infer significantly misaligned disks, V1247 Ori, V1366 Ori, and RY Lup, we do not see any evident sign of shadows in the scattered light images. The scattered light shadows observed in DoAr44, HD135344B, and HD139614 are consistent with our observations, yet the underlying morphology is likely too complex to be described by our models and the accuracy achieved by our observations. Whereas we can derive precise constraints on the potential shadow positions for well-resolved inner disks around HAeBe stars, the statistical uncertainties for the marginally resolved inner disks around the TTS of our sample make it difficult to extract conclusive constraints for the presence of shadows in these systems.

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arXiv2021

The mass of Beta Pictoris c from Beta Pictoris b orbital motion

We aim to demonstrate that the presence and mass of an exoplanet can now be effectively derived from the astrometry of another exoplanet. We combined previous astrometry of $β$ Pictoris b with a new set of observations from the GRAVITY interferometer. The orbital motion of $β$ Pictoris b is fit using Markov chain Monte Carlo simulations in Jacobi coordinates. The inner planet, $β$ Pictoris c, was also reobserved at a separation of 96\,mas, confirming the previous orbital estimations. From the astrometry of planet b only, we can (i) detect the presence of $β$ Pictoris c and (ii) constrain its mass to $10.04^{+4.53}_{-3.10}\,M_{\rm Jup}$. If one adds the astrometry of $β$ Pictoris c, the mass is narrowed down to $9.15^{+1.08}_{-1.06}\,M_{\rm Jup}$. The inclusion of radial velocity measurements does not affect the orbital parameters significantly, but it does slightly decrease the mass estimate to $8.89^{+0.75}_{-0.75}\,M_{\rm Jup}$. With a semimajor axis of $2.68\pm0.02$\,au, a period of $1221\pm15$ days, and an eccentricity of $0.32\pm0.02$, the orbital parameters of $β$ Pictoris c are now constrained as precisely as those of $β$ Pictoris b. The orbital configuration is compatible with a high-order mean-motion resonance (7:1). The impact of the resonance on the planets' dynamics would then be negligible with respect to the secular perturbations, which might have played an important role in the eccentricity excitation of the outer planet.

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arXiv2021

Modeling accretion shocks at the disk-envelope interface -- Sulfur chemistry

As material from an infalling protostellar envelope hits the forming disk, an accretion shock may develop which could (partially) alter the envelope material entering the disk. Observations with the Atacama Large Millimeter/submillimeter Array (ALMA) indicate that emission originating from warm SO and SO$_2$ might be good tracers of such accretion shocks. The goal of this work is to test under what shock conditions the abundances of gas-phase SO and SO$_2$ increase in an accretion shock at the disk-envelope interface. Detailed shock models including gas dynamics are computed using the Paris-Durham shock code for non-magnetized J-type accretion shocks in typical inner envelope conditions. The effect of pre-shock density, shock velocity, and strength of the ultraviolet (UV) radiation field on the abundance of warm SO and SO$_2$ is explored. Warm gas-phase chemistry is efficient in forming SO under most J-type shock conditions considered. In lower-velocity (~3 km/s) shocks, the abundance of SO is increased through subsequent reactions starting from thermally desorbed CH$_4$ toward H$_2$CO and finally SO. In higher velocity (>4 km/s) shocks, both SO and SO$_2$ are formed through reactions of OH and atomic S. The strength of the UV radiation field is crucial for SO and in particular SO$_2$ formation through the photodissociation of H$_2$O. Thermal desorption of SO and SO$_2$ ice is only relevant in high-velocity (>5 km/s) shocks at high densities ($>10^7$ cm$^{-3}$). Warm emission from SO and SO$_2$ is a possible tracer of accretion shocks at the disk-envelope interface as long as a local UV field is present. Additional observations with ALMA at high-angular resolution could provide further constraints. Moreover, the James Webb Space Telescope will give access to other possible slow, dense shock tracers such as H$_2$, H$_2$O, and [S I] 25$μ$m.

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arXiv2021

ALMA observations of doubly deuterated water: Inheritance of water from the prestellar environment

Establishing the origin of the water D/H ratio in the Solar System is central to our understanding of the chemical trail of water during the star and planet formation process. Recent modeling suggests that comparisons of the D$_2$O/HDO and HDO/H$_2$O ratios are a powerful way to trace the chemical evolution of water and, in particular, determine whether the D/H ratio is inherited from the molecular cloud or established locally. We seek to determine the D$_2$O column density and derive the D$_2$O/HDO ratios in the warm region toward the low-mass Class 0 sources B335 and L483. The results are compared with astrochemical models and previous observations to determine their implications for the chemical evolution of water. We present ALMA observations of the D$_2$O transition at 316.8 GHz toward B335 and L483 at $<$0.5" ($<$ 100 au) resolution, probing the inner warm envelope gas. The column densities of D$_2$O, HDO, and H$_{2}^{18}$O are determined by synthetic spectrum modeling and direct Gaussian fitting, under the assumption of a single excitation temperature and similar spatial extent for the three water isotopologs. D$_2$O is detected toward both sources in the inner warm envelope. The derived D$_2$O/HDO ratios is $(1.0\pm0.2)\times10^{-2}$ for L483 and $(1.4\pm0.1)\times10^{-2}$ for B335. The high D$_2$O/HDO ratios are a strong indication of chemical inheritance of water from the prestellar phase down to the inner warm envelope. This implies that the local cloud conditions in the prestellar phase, such as temperatures and timescales, determine the water chemistry at later stages and could provide a source of chemical differentiation in young systems. In addition, the observed D$_2$O/H$_2$O ratios support an observed dichotomy in the deuterium fractionation of water toward isolated and clustered protostars, namely, a higher D/H ratio toward isolated sources

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arXiv2021

GRAVITY K-band spectroscopy of HD 206893 B: brown dwarf or exoplanet

We aim to reveal the nature of the reddest known substellar companion HD 206893 B by studying its near-infrared colors and spectral morphology and by investigating its orbital motion. We fit atmospheric models for giant planets and brown dwarfs and perform spectral retrievals with petitRADTRANS and ATMO on the observed GRAVITY, SPHERE, and GPI spectra of HD 206893 B. To recover its unusual spectral features, we include additional extinction by high-altitude dust clouds made of enstatite grains in the atmospheric model fits. We also infer the orbital parameters of HD 206893 B by combining the $\sim 100~μ\text{as}$ precision astrometry from GRAVITY with data from the literature and constrain the mass and position of HD 206893 C based on the Gaia proper motion anomaly of the system. The extremely red color and the very shallow $1.4~μ\text{m}$ water absorption feature of HD 206893 B can be fit well with the adapted atmospheric models and spectral retrievals. Altogether, our analysis suggests an age of $\sim 3$-$300~\text{Myr}$ and a mass of $\sim 5$-$30~\text{M}_\text{Jup}$ for HD 206893 B, which is consistent with previous estimates but extends the parameter space to younger and lower-mass objects. The GRAVITY astrometry points to an eccentric orbit ($e = 0.29^{+0.06}_{-0.11}$) with a mutual inclination of $< 34.4~\text{deg}$ with respect to the debris disk of the system. While HD 206893 B could in principle be a planetary-mass companion, this possibility hinges on the unknown influence of the inner companion on the mass estimate of $10^{+5}_{-4}~\text{M}_\text{Jup}$ from radial velocity and Gaia as well as a relatively small but significant Argus moving group membership probability of $\sim 61\%$. However, we find that if the mass of HD 206893 B is $< 30~\text{M}_\text{Jup}$, then the inner companion HD 206893 C should have a mass between $\sim 8$-$15~\text{M}_\text{Jup}$.

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arXiv2021

A major asymmetric ice trap in a planet-forming disk: I. Formaldehyde and methanol

The chemistry of planet-forming disks sets the exoplanet atmosphere composition and the prebiotic molecular content. Dust traps are of particular importance as pebble growth and transport are crucial for setting the chemistry where giant planets are forming. The asymmetric Oph~IRS~48 dust trap located at 60 au radius provides a unique laboratory for studying chemistry in pebble-concentrated environments in warm Herbig disks with low gas-to-dust ratios down to 0.01. We use deep ALMA Band~7 line observations to search the IRS~48 disk for H$_2$CO and CH$_3$OH line emission, the first steps of complex organic chemistry. We report the detection of 7 H$_2$CO and 6 CH$_3$OH lines with energy levels between 17 and 260 K. The line emission shows a crescent morphology, similar to the dust continuum, suggesting that the icy pebbles play an important role in the delivery of these molecules. Rotational diagrams and line ratios indicate that both molecules originate from warm molecular regions in the disk with temperatures $>$100 K and column densities $\sim10^{14}$ cm$^{-2}$ or a fractional abundance of $\sim10^{-8}$ and with H$_2$CO/CH$_3$OH$\sim$0.2, indicative of ice chemistry. Based on arguments from a physical-chemical model with low gas-to-dust ratios, we propose a scenario where the dust trap provides a huge icy grain reservoir in the disk midplane or an `ice trap', which can result in high gas-phase abundances of warm COMs through efficient vertical mixing. This is the first time that complex organic molecules have been clearly linked to the presence of a dust trap. These results demonstrate the importance of including dust evolution and vertical transport in chemical disk models, as icy dust concentrations provide important reservoirs for complex organic chemistry in disks.

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arXiv2021

A major asymmetric ice trap in a planet-forming disk: II. prominent SO and SO2 pointing to C/O < 1

Gas-phase sulphur bearing volatiles appear to be severely depleted in protoplanetary disks. The detection of CS and non-detections of SO and SO2 in many disks have shown that the gas in the warm molecular layer, where giant planets accrete their atmospheres, has a high C/O ratio. In this letter, we report the detection of SO and SO2 in the Oph-IRS 48 disk using ALMA. This is the first case of prominent SO2 emission detected from a protoplanetary disk. The molecular emissions of both molecules is spatially correlated with the asymmetric dust trap. We propose that this is due to the sublimation of ices at the edge of the dust cavity and that the bulk of the ice reservoir is coincident with the millimetre dust grains. Depending on the partition of elemental sulphur between refractory and volatile materials the observed molecules can account for 15-100% of the total sulphur budget in the disk. In strong contrast to previous results, we constrain the C/O ratio from the CS/SO ratio to be < 1 and potentially solar. This has important implications for the elemental composition of planets forming within the cavities of warm transition disks.

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arXiv2021

Complex organic molecules in low-mass protostars on Solar System scales -- II. Nitrogen-bearing species

The chemical inventory of planets is determined by the physical and chemical processes that govern the early phases of star formation. The aim is to investigate N-bearing complex organic molecules towards two Class 0 protostars (B1-c and S68N) at millimetre wavelengths with ALMA. Next, the results of the detected N-bearing species are compared with those of O-bearing species for the same and other sources. ALMA observations in Band 6 ($\sim$ 1 mm) and Band 5 ($\sim$ 2 mm) are studied at $\sim$ 0.5" resolution, complemented by Band 3 ($\sim$ 3 mm) data in a $\sim$ 2.5" beam. NH2CHO, C2H5CN, HNCO, HN13CO, DNCO, CH3CN, CH2DCN, and CHD2CN are identified towards the investigated sources. Their abundances relative to CH3OH and HNCO are similar for the two sources, with column densities that are typically an order of magnitude lower than those of O-bearing species. The largest variations, of an order of magnitude, are seen for NH2CHO abundance ratios with respect to HNCO and CH3OH and do not correlate with the protostellar luminosity. In addition, within uncertainties, the N-bearing species have similar excitation temperatures to those of O-bearing species ($\sim$ 100 $\sim$ 300 K). The similarity of most abundances with respect to HNCO, including those of CH2DCN and CHD2CN, hints at a shared chemical history, especially the high D/H ratio in cold regions prior to star formation. However, some of the variations in abundances may reflect the sensitivity of the chemistry to local conditions such as temperature (e.g. NH2CHO), while others may arise from differences in the emitting areas of the molecules linked to their different binding energies in the ice. The two sources discussed here add to the small number of sources with such a detailed chemical analysis on Solar System scales. Future JWST data will allow a direct comparison between the ice and gas abundances of N-bearing species.

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arXiv2021

Water in star-forming regions (WISH): Physics and chemistry from clouds to disks as probed by Herschel spectroscopy

(abridged) Data and results from the WISH key program are summarized, designed to provide a legacy data set to address its physics and chemistry. WISH targeted ~80 sources along the two axes of luminosity and evolutionary stage: from low- to high-mass protostars and from pre-stellar cores to protoplanetary disks. Lines of H2O, HDO, OH, CO and [O I] were observed with the HIFI and PACS instruments, complemented by molecules that probe UV, X-ray or grain chemistry. Most of the far-infrared water emission from protostars is found to be compact, originating from warm outflowing and shocked gas at high density and temperature in at least two physical components. This gas is not probed by low-J CO lines, only by J>14. Water is a significant, but not dominant, coolant. Its abundance is universally low, of order H2O/H2=2E-6, pointing to shock and outflow cavity models that include UV radiation at 100-1000 times the ISRF. In cold quiescent pre-stellar cores and envelopes, the water abundance structure is accurately probed through velocity-resolved line profiles, confirming basic chemistry networks. The gaseous HDO/H2O ratio of 0.025, much higher than that of bulk ice, is representative of the outer photodesorbed ice layers and cold chemistry. Water abundances in the inner hot cores are high, but with variations from 5E-6 to 2E-4. Combined analyses of water gas and ice show that up to 50% of the oxygen budget may be missing, with possible explanations discussed. Water vapor emission from disks is weak, indicating that water ice is locked up in larger pebbles early on and that these pebbles have settled and drifted inward by the Class II stage. Quantitatively, many oceans of water ice are available. Extragalactic low-J H2O emission is mostly compact and collisionally excited. Prospects for future mid- to far-infrared missions are given.

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arXiv2021

Constraining the Nature of the PDS 70 Protoplanets with VLTI/GRAVITY

We present K-band interferometric observations of the PDS 70 protoplanets along with their host star using VLTI/GRAVITY. We obtained K-band spectra and 100 $μ$as precision astrometry of both PDS 70 b and c in two epochs, as well as spatially resolving the hot inner disk around the star. Rejecting unstable orbits, we found a nonzero eccentricity for PDS 70 b of $0.17 \pm 0.06$, a near-circular orbit for PDS 70 c, and an orbital configuration that is consistent with the planets migrating into a 2:1 mean motion resonance. Enforcing dynamical stability, we obtained a 95% upper limit on the mass of PDS 70 b of 10 $M_\textrm{Jup}$, while the mass of PDS 70 c was unconstrained. The GRAVITY K-band spectra rules out pure blackbody models for the photospheres of both planets. Instead, the models with the most support from the data are planetary atmospheres that are dusty, but the nature of the dust is unclear. Any circumplanetary dust around these planets is not well constrained by the planets' 1-5 $μ$m spectral energy distributions (SEDs) and requires longer wavelength data to probe with SED analysis. However with VLTI/GRAVITY, we made the first observations of a circumplanetary environment with sub-au spatial resolution, placing an upper limit of 0.3~au on the size of a bright disk around PDS 70 b.

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arXiv2021

The ExoGRAVITY project: using single mode interferometry to characterize exoplanets

Combining adaptive optics and interferometric observations results in a considerable contrast gain compared to single-telescope, extreme AO systems. Taking advantage of this, the ExoGRAVITY project is a survey of known young giant exoplanets located in the range of 0.1'' to 2'' from their stars. The observations provide astrometric data of unprecedented accuracy, being crucial for refining the orbital parameters of planets and illuminating their dynamical histories. Furthermore, GRAVITY will measure non-Keplerian perturbations due to planet-planet interactions in multi-planet systems and measure dynamical masses. Over time, repetitive observations of the exoplanets at medium resolution ($R=500$) will provide a catalogue of K-band spectra of unprecedented quality, for a number of exoplanets. The K-band has the unique properties that it contains many molecular signatures (CO, H$_2$O, CH$_4$, CO$_2$). This allows constraining precisely surface gravity, metallicity, and temperature, if used in conjunction with self-consistent models like Exo-REM. Further, we will use the parameter-retrieval algorithm petitRADTRANS to constrain the C/O ratio of the planets. Ultimately, we plan to produce the first C/O survey of exoplanets, kick-starting the difficult process of linking planetary formation with measured atomic abundances.

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arXiv2020

The prebiotic molecular inventory of Serpens SMM1 I. An investigation of the isomers CH$_{3}$NCO and HOCH$_{2}$CN

Methyl isocyanate (CH$_{3}$NCO) and glycolonitrile (HOCH$_{2}$CN) are isomers and prebiotic molecules that are involved in the formation of peptide structures and the nucleobase adenine, respectively. ALMA observations of the intermediate-mass Class 0 protostar Serpens SMM1-a and ALMA-PILS data of the low-mass Class 0 protostar IRAS~16293B are used. Spectra are analysed with the CASSIS line analysis software package in order to identify and characterise molecules. CH$_{3}$NCO, HOCH$_{2}$CN, and various other molecules are detected towards SMM1-a. HOCH$_{2}$CN is identified in the PILS data towards IRAS~16293B in a spectrum extracted at a half-beam offset position from the peak continuum. CH$_{3}$NCO and HOCH$_{2}$CN are equally abundant in SMM1-a at [X]/[CH$_{3}$OH] of 5.3$\times$10$^{-4}$ and 6.2$\times$10$^{-4}$, respectively. A comparison between SMM1-a and IRAS~16293B shows that HOCH$_{2}$CN and HNCO are more abundant in the former source, but CH$_{3}$NCO abundances do not differ significantly. Data from other sources are used to show that the [CH$_{3}$NCO]/[HNCO] ratio is similar in all these sources within $\sim$10\%. The new detections of CH$_{3}$NCO and HOCH$_{2}$CN are additional evidence for a large interstellar reservoir of prebiotic molecules that can contribute to the formation of biomolecules on terrestrial planets. A plausible formation pathway for HOCH$_{2}$CN is the thermal Strecker-like reaction of CN$^{-}$ with H$_{2}$CO. The similar [CH$_{3}$NCO]/[HNCO] ratios indicate that these two species either are chemically related or their formation is affected by physical conditions in the same way. The relatively high abundances of HOCH$_{2}$CN and HNCO in SMM1-a may be explained by a prolonged stage of relatively warm ice mantles, where thermal and energetic processing of HCN in the ice results in the efficient formation of both species.

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arXiv2020

Chemically tracing the water snowline in protoplanetary disks with HCO$^+$

[Abridged] Planet formation is expected to be enhanced around snowlines in protoplanetary disks, in particular around the water snowline. However, the close proximity of the water snowline to the host star and water in the Earth's atmosphere makes a direct detection of the water snowline in protoplanetary disks challenging. Following earlier work on protostellar envelopes, the aim of this research is to investigate the validity of HCO$^+$ and H$^{13}$CO$^+$, as tracers of the water snowline in protoplanetary disks, as HCO$^+$ is destroyed by gas-phase water. Two small chemical networks are used to predict the HCO$^+$ abundance in a typical Herbig Ae disk. Subsequently, the corresponding emission profiles are modelled for H$^{13}$CO$^+$ and HCO$^+$ $J=2-1$, which provides the best balance between brightness and optical depth effects of the continuum emission. The HCO$^+$ abundance jumps by two orders of magnitude just outside the water snowline at 4.5 AU. We find that the emission of H$^{13}$CO$^+$ and HCO$^+$ is ring-shaped due to three effects: destruction of HCO$^+$ by gas-phase water, continuum optical depth, and molecular excitation effects. The presence of gas-phase water causes an additional drop of only $\sim$13% and 24% in the center of the disk, for H$^{13}$CO$^+$ and HCO$^+$, respectively. For the much more luminous outbursting source V883Ori, our models predict that the effect of dust and excitation are not limiting if the snowline is located outside $\sim$40 AU. Our analysis of ALMA observations of HCO$^+$ $J=3-2$ is consistent with the water snowline located around 100 AU. The HCO$^+$ abundance drops steeply around the water snowline, but dust and excitation can conceal the drop in HCO$^+$ emission due to the water snowline. Therefore, locating the water snowline with HCO$^+$ in Herbig disks is very difficult, but it is possible for outbursting sources like V883Ori.

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