arXiv subjects

E. Flurin

Publications and source records attributed to E. Flurin.

12 recordsLinked to original sources

arXiv2026

Precision hyperfine spectroscopy of an individual nuclear-spin-9/2

Single-spin magnetic resonance spectroscopy promises to yield structural and chemical information at the level of individual atoms or molecules, in a non-invasive way. Here, we use an Er3+ paramagnetic center in a CaWO4 crystal, detected by microwave photon counting at 10 mK, as a nanoscale magnetic sensor to measure the NMR spectrum of a proximal individual nuclear-spin-9/2 93Nb impurity with Hertz spectral resolution. From these measurements, we determine the 93Nb insertion site, its position relative to the Er3+ , and its complete quadrupolar tensor. We moreover harness the high spectral resolution of our measurements to establish the presence of two previously unobserved terms in the spin Hamiltonian. The first describes a coupling between the Er3+ spin and the 93Nb nuclear quadrupole; it possibly originates from a spin-dependent electrostatic interaction between the two systems. The second is a nuclear hexadecapolar term, and may be caused by the coupling of the electric field third derivative to the 93Nb nuclear hexadecapolar moment.

quant-ph↗

arXiv2026

FerBo: a noise resilient qubit hybridizing Andreev and fluxonium states

We propose a novel superconducting quantum circuit that should be robust against both relaxation and dephasing over a wide and experimentally accessible parameter range. The circuit consists of a parallel arrangement of a large inductance, a small capacitor, and a well-transmitting Josephson weak link. Protection against relaxation arises from the hybridization between the fermionic degree of freedom associated with Andreev levels in the weak link and the bosonic electromagnetic mode of the LC circuit, hence its name: FerBo. Furthermore, as in the fluxonium qubit, delocalization of the wavefunctions in phase space provides resilience against dephasing.

cond-mat.mes-hall↗

arXiv2025

Addressing spins at the clock transitions with a frequency- and bandwidth-tunable superconducting resonator

Solid-state spin ensembles addressed via superconducting circuits are promising candidates for quantum memory applications, offering multimodal storage capability and second-long coherence times at their clock transition. Implementing practical memory schemes requires dynamic control over both the resonator frequency and bandwidth. In this letter, we report measurements of a superconducting resonator whose frequency can be tuned by passing a DC current through the high-kinetic-inductance thin film, and whose bandwidth can be tuned by parametric coupling to a low-Q buffer resonator. Using this resonator, we address an ensemble of bismuth donors at their clock transition, measuring a Hahn-echo coherence time of 450 ms. We demonstrate RF driving of the bismuth donor hyperfine transitions, as well as dynamic bandwidth control of the resonator.

quant-ph↗

arXiv2024

All-microwave spectroscopy and polarization of individual nuclear spins in a solid

We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum jumps of the nuclear spin state, a proof of their individual nature. By driving the forbidden transitions of the coupled electron-nuclear spin system, we also achieve single-spin solid-effect dynamical nuclear polarization. Relying exclusively on microwave driving and microwave photon counting, the methods reported here are in principle applicable to a large number of electron-nuclear spin systems, in a wide variety of samples.

quant-ph↗

arXiv2024

Two-tone spectroscopy of high-frequency quantum circuits with a Josephson emitter

We perform two-tone spectroscopy on quantum circuits, where high-frequency radiation is generated by a voltage-biased superconductor-normal-superconductor Josephson junction and detection is carried out by an ancillary microwave resonator. We implement this protocol on two different systems, a transmon qubit and a $\lambda/4$ resonator. We demonstrate that this two-tone Josephson spectroscopy operates well into the millimeter-wave band, reaching frequencies larger than 80 GHz, and is well-suited for probing highly coherent quantum systems.

cond-mat.mes-hall↗

arXiv2024

Quantum-enhanced sensing of axion dark matter with a transmon-based single microwave photon counter

We report an axion dark matter search with a haloscope equipped with a microwave photon counter. The haloscope is a tunable high quality factor 3-dimensional microwave cavity placed in a magnetic field. The photon counter, operated cyclically, maps an incoming microwave photon onto the state of a superconducting transmon qubit. The measurement protocol continuously monitors the power emitted by the haloscope cavity as well as the dark count background, and enables tuning of the cavity frequency to probe different axion masses. With this apparatus we enhance by a factor 20 the search speed that can be reached with quantum-limited linear amplifiers, and set a new standard for probing the existence of axions with resonant detectors.

quant-ph↗

arXiv2024

Electron Paramagnetic Resonance spectroscopy of a scheelite crystal using microwave photon counting

Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been introduced as a sensitive new method for electron paramagnetic resonance spectroscopy at millikelvin temperatures. Here, we apply this spin fluorescence method to a scheelite crystal of CaWO4, finding some known ($\mathrm{Er}^{3+}$, $\mathrm{Yb}^{3+}$, $\mathrm{Nd}^{3+}$ and $\mathrm{Fe}^{3+}$) and other unknown paramagnetic impurities. Investigating the zero nuclear spin isotope ($I=0$) transition of $\mathrm{Er}^{3+}:\mathrm{CaWO}_4$ as a model system, we provide a quantitative analysis of the time-dependent photon counting rate following an excitation pulse, as a function of its power. The achieved signal-to-noise ratio is found to be an order of magnitude higher than the one obtained by inductively-detected Hahn echo under identical conditions. Finally, we use spin fluorescence spectroscopy at low excitation power to probe the properties of rare-earth-ions close to a metallic wire deposited on the surface; our data reveal line distortion caused by the mechanical strain imparted by the thermal contractions of the metal relative to the underlying crystal. Coherent oscillations are also observed for the most highly strained ions.

quant-ph↗

arXiv2023

High-sensitivity AC-charge detection with a MHz-frequency fluxonium qubit

Owing to their strong dipole moment and long coherence times, superconducting qubits have demonstrated remarkable success in hybrid quantum circuits. However, most qubit architectures are limited to the GHz frequency range, severely constraining the class of systems they can interact with. The fluxonium qubit, on the other hand, can be biased to very low frequency while being manipulated and read out with standard microwave techniques. Here, we design and operate a heavy fluxonium with an unprecedentedly low transition frequency of $1.8~\mathrm{MHz}$. We demonstrate resolved sideband cooling of the ``hot'' qubit transition with a final ground state population of $97.7~\%$, corresponding to an effective temperature of $23~μ\mathrm{K}$. We further demonstrate coherent manipulation with coherence times $T_1=34~μ\mathrm{s}$, $T_2^*=39~μ\mathrm{s}$, and single-shot readout of the qubit state. Importantly, by directly addressing the qubit transition with a capacitively coupled waveguide, we showcase its high sensitivity to a radio-frequency field. Through cyclic qubit preparation and interrogation, we transform this low-frequency fluxonium qubit into a frequency-resolved charge sensor. This method results in a charge sensitivity of $33~μ\mathrm{e}/\sqrt{\mathrm{Hz}}$, or an energy sensitivity (in joules per hertz) of $2.8~\hbar$. This method rivals state-of-the-art transport-based devices, while maintaining inherent insensitivity to DC charge noise. The high charge sensitivity combined with large capacitive shunt unlocks new avenues for exploring quantum phenomena in the $1-10~\mathrm{MHz}$ range, such as the strong-coupling regime with a resonant macroscopic mechanical resonator.

quant-ph↗

arXiv2021

Spatially-resolved decoherence of donor spins in silicon strained by a metallic electrode

Electron spins are amongst the most coherent solid-state systems known, however, to be used in devices for quantum sensing and information processing applications, they must be typically placed near interfaces. Understanding and mitigating the impacts of such interfaces on the coherence and spectral properties of electron spins is critical to realize such applications, but is also challenging: inferring such data from single-spin studies requires many measurements to obtain meaningful results, while ensemble measurements typically give averaged results that hide critical information. Here, we report a comprehensive study of the coherence of near-surface bismuth donor spins in 28-silicon at millikelvin temperatures. In particular, we use strain-induced frequency shifts caused by a metallic electrode to make spatial maps of spin coherence as a function of depth and position relative to the electrode. By measuring magnetic-field-insensitive clock transitions we separate magnetic noise caused by surface spins from charge noise. Our results include quantitative models of the strain-split spin resonance spectra and extraction of paramagnetic impurity concentrations at the silicon surface. The interplay of these decoherence mechanisms for such near-surface electron spins is critical for their application in quantum technologies, while the combination of the strain splitting and clock transition extends the coherence lifetimes by up to two orders of magnitude, reaching up to 300 ms at a mean depth of only 100nm. The technique we introduce here to spatially map coherence in near-surface ensembles is directly applicable to other spin systems of active interest, such as defects in diamond, silicon carbide, and rare earth ions in optical crystals.

quant-ph↗

arXiv2020

Multimode storage of quantum microwave fields in electron spins over 100 ms

A long-lived multi-mode qubit register is an enabling technology for modular quantum computing architectures. For interfacing with superconducting qubits, such a quantum memory should be able to store incoming quantum microwave fields at the single-photon level for long periods of time, and retrieve them on-demand. Here, we demonstrate the partial absorption of a train of weak microwave fields in an ensemble of bismuth donor spins in silicon, their storage for 100 ms, and their retrieval, using a Hahn-echo-like protocol. The long storage time is obtained by biasing the bismuth donors at a clock transition. Phase coherence and quantum statistics are preserved in the storage.

quant-ph↗

arXiv2015

Stabilizing entanglement via symmetry-selective bath engineering in superconducting qubits

Bath engineering, which utilizes coupling to lossy modes in a quantum system to generate non-trivial steady states, is a tantalizing alternative to gate- and measurement-based quantum science. Here, we demonstrate dissipative stabilization of entanglement between two superconducting transmon qubits in a symmetry-selective manner. We utilize the engineered symmetries of the dissipative environment to stabilize a target Bell state; we further demonstrate suppression of the Bell state of opposite symmetry due to parity selection rules. This implementation is resource-efficient, achieves a steady-state fidelity $\mathcal{F} = 0.70$, and is scalable to multiple qubits.

quant-ph↗

arXiv2015

A compact design for the Josephson mixer: the lumped element circuit

We present a compact and efficient design in terms of gain, bandwidth and dynamical range for the Josephson mixer, the superconducting circuit performing three-wave mixing at microwave frequencies. In an all lumped-element based circuit with galvanically coupled ports, we demonstrate non degenerate amplification for microwave signals over a bandwidth up to 50 MHz for a power gain of 20 dB. The quantum efficiency of the mixer is shown to be about 70$\%$ and its saturation power reaches $-112$ dBm.

cond-mat.supr-con↗