arXiv subjects

E. J. Divall

Publications and source records attributed to E. J. Divall.

3 recordsLinked to original sources

arXiv2010

Observation of a Long-Wavelength Hosing Modulation of a High-Intensity Laser Pulse in Underdense Plasma

We report the first experimental observation of a long-wavelength hosing modulation of a high-intensity laser pulse. Side-view images of the scattered optical radiation at the fundamental wave-length of the laser reveal a transverse oscillation of the laser pulse during its propagation through underdense plasma. The wavelength of the oscillation λ_hosing depends on the background plasma density n_e and scales as λ_hosing~n_e^-3/2. Comparisons with an analytical model and 2-dimensional particle-in-cell simulations reveal that this laser hosing can be induced by a spatio-temporal asymmetry of the intensity distribution in the laser focus which can be caused by a misalignment of the parabolic focussing mirror or of the diffraction gratings in the pulse compressor.

physics.plasm-ph↗

arXiv2010

Atomic excitation during recollision-free ultrafast multi-electron tunnel ionization

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the states of the remaining electrons are neglected. Such electronic interactions are predicted to be weak, the exception being recollision excitation and ionization caused by linearly-polarized radiation. In contrast, it has recently been suggested that intense field ionization may be accompanied by a two-stage `shake-up' reaction. Here we report a unique combination of experimental techniques that enables us to accurately measure the tunnel ionization probability for argon exposed to 50 femtosecond laser pulses. Most significantly for the current study, this measurement is independent of the optical focal geometry, equivalent to a homogenous electric field. Furthermore, circularly-polarized radiation negates recollision. The present measurements indicate that tunnel ionization results in simultaneous excitation of one or more remaining electrons through shake-up. From an atomic physics standpoint, it may be possible to induce ionization from specific states, and will influence the development of coherent attosecond XUV radiation sources. Such pulses have vital scientific and economic potential in areas such as high-resolution imaging of in-vivo cells and nanoscale XUV lithography.

physics.atom-ph↗

arXiv2005

Geometry- and diffraction-independent ionization probabilities in intense laser fields: probing atomic ionization mechanisms with effective intensity matching

We report a novel experimental technique for the comparison of ionization processes in ultrafast laser pulses irrespective of pulse ellipticity. Multiple ionization of xenon by 50 fs 790 nm, linearly and circularly polarized laser pulses is observed over the intensity range 10 TW/cm^2 to 10 PW/cm^2 using Effective Intensity Matching (EIM), which is coupled with Intensity Selective Scanning (ISS) to recover the geometry-independent probability of ionization. Such measurements, made possible by quantifying diffraction effects in the laser focus, are compared directly to theoretical predictions of multiphoton, tunnel and field ionization, and a remarkable agreement demonstrated. EIM-ISS allows the straightforward quantification of the probability of recollision ionization in a linearly polarized laser pulse. Furthermore, probability of ionization is discussed in terms of the Keldysh adiabaticity parameter, gamma, and the influence of the precursor ionic states present in recollision ionization is observed for the first time.

physics.atom-ph↗