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E. Kirilov

Publications and source records attributed to E. Kirilov.

8 recordsLinked to original sources

Optically trapped Feshbach molecules of fermionic 161Dy and 40K

We report on the preparation of a pure ultracold sample of bosonic DyK Feshbach molecules, which are composed of the fermionic isotopes 161Dy and 40K. Employing a magnetic sweep across a resonance located near 7.3 G, we produce up to 5000 molecules at a temperature of about 50 nK. For purification from the remaining atoms, we apply a Stern-Gerlach technique based on magnetic levitation of the molecules in a very weak optical dipole trap. With the trapped molecules we finally reach a high phase-space density of about 0.1. We measure the magnetic field dependence of the molecular binding energy and the magnetic moment, refining our knowledge of the resonance parameters. We also demonstrate a peculiar anisotropic expansion effect observed when the molecules are released from the trap and expand freely in the magnetic levitation field. Moreover, we identify an important lifetime limitation that is imposed by the 1064-nm infrared trap light itself and not by inelastic collisions. The light-induced decay rate is found to be proportional to the trap light intensity and the closed-channel fraction of the Feshbach molecule. These observations suggest a one-photon coupling to electronically excited states to limit the lifetime and point to the prospect of loss suppression by optimizing the wavelength of the trapping light. Our results represent important insights and experimental steps on the way to achieve quantum-degenerate samples of DyK molecules and novel superfluids based on mass-imbalanced fermion mixtures.

cond-mat.quant-gas

Resonantly Interacting Fermi-Fermi Mixture of $^{161}$Dy and $^{40}$K

We report on the realization of a Fermi-Fermi mixture of ultracold atoms that combines mass imbalance, tunability, and collisional stability. In an optically trapped sample of $^{161}$Dy and $^{40}$K, we identify a broad Feshbach resonance centered at a magnetic field of $217\,$G. Hydrodynamic expansion profiles in the resonant interaction regime reveal a bimodal behavior resulting from mass imbalance. Lifetime studies on resonance show a suppression of inelastic few-body processes by orders of magnitude, which we interpret as a consequence of the fermionic nature of our system. The resonant mixture opens up intriguing perspectives for studies on novel states of strongly correlated fermions with mass imbalance.

cond-mat.quant-gas

Accurate Determination of the Dynamical Polarizability of Dysprosium

We report a measurement of the dynamical polarizability of dysprosium atoms in their electronic ground state at the optical wavelength of 1064 nm, which is of particular interest for laser trapping experiments. Our method is based on collective oscillations in an optical dipole trap, and reaches unprecedented accuracy and precision by comparison with an alkali atom (potassium) as a reference species. We obtain values of 184.4(2.4) a.u. and 1.7(6) a.u. for the scalar and tensor polarizability, respectively. Our experiments have reached a level that permits meaningful tests of current theo- retical descriptions and provides valuable information for future experiments utilizing the intriguing properties of heavy lanthanide atoms.

physics.atom-ph

STIRAP preparation of a coherent superposition of ThO $H^3Δ_1$ states for an improved electron EDM measurement

Experimental searches for the electron electric dipole moment (EDM) probe new physics beyond the Standard Model. The current best EDM limit was set by the ACME Collaboration [Science \textbf{343}, 269 (2014)], constraining time reversal symmetry ($T$) violating physics at the TeV energy scale. ACME used optical pumping to prepare a coherent superposition of ThO $H^3Δ_1$ states that have aligned electron spins. Spin precession due to the molecule's internal electric field was measured to extract the EDM. We report here on an improved method for preparing this spin-aligned state of the electron by using STIRAP. We demonstrate a transfer efficiency of $75\pm5\%$, representing a significant gain in signal for a next generation EDM experiment. We discuss the particularities of implementing STIRAP in systems such as ours, where molecular ensembles with large phase-space distributions are transfered via weak molecular transitions with limited laser power and limited optical access.

physics.atom-ph

Zeeman-tuned rotational level-crossing spectroscopy in a diatomic free radical

Rotational levels of molecular free radicals can be tuned to degeneracy using laboratory-scale magnetic fields. Because of their intrinsically narrow width, these level crossings of opposite-parity states have been proposed for use in the study of parity-violating interactions and other applications. We experimentally study a typical manifestation of this system using $^{138}$BaF. Using a Stark-mixing method for detection, we demonstrate level-crossing signals with spectral width as small as 6 kHz. We use our data to verify the predicted lineshapes, transition dipole moments, and Stark shifts, and to precisely determine molecular magnetic g-factors. Our results constitute an initial proof-of-concept for use of this system to study nuclear spin-dependent parity violating effects.

physics.atom-ph

Shot-noise-limited spin measurements in a pulsed molecular beam

Heavy diatomic molecules have been identified as good candidates for use in electron electric dipole moment (eEDM) searches. Suitable molecular species can be produced in pulsed beams, but with a total flux and/or temporal evolution that varies significantly from pulse to pulse. These variations can degrade the experimental sensitivity to changes in spin precession phase of an electri- cally polarized state, which is the observable of interest for an eEDM measurement. We present two methods for measurement of the phase that provide immunity to beam temporal variations, and make it possible to reach shot-noise-limited sensitivity. Each method employs rapid projection of the spin state onto both components of an orthonormal basis. We demonstrate both methods using the eEDM-sensitive H state of thorium monoxide (ThO), and use one of them to measure the magnetic moment of this state with increased accuracy relative to previous determinations.

physics.atom-ph

Search for the electron electric dipole moment using $Ω$-doublet levels in PbO$^*$

We present results of the first experiment to probe for the electric dipole moment (EDM) of the electron using an $Ω$-doublet state in a polar molecule. If the molecule is both massive and has a large molecular-fixed frame dipole moment, then the $Ω$-doublet states have the potential to greatly increase the sensitivity of experiments searching for the EDM while also allowing for new methods of systematic error rejection. Here, we use the metastable $a(1)^3Σ^+$ state of lead monoxide (PbO) to probe for the electron EDM. Our best fit for the electron EDM of $d_e = (-4.4\pm9.5_\text{stat}\pm1.8_\text{syst})\times10^{-27}\ecm$ allows us to place an upper limit on the magnitude of the EDM of $|d_e|<1.7\times10^{-26}\ecm$ (90% confidence). While this is less stringent than limits from other, previous experiments, our work emphasizes the systematic error rejection properties associated with the $Ω$-doublet level structure. The results should inform the work of other, ongoing experiments that use molecules with analogous level structure.

physics.atom-ph

2-photon ionization and necessary laser and vacuum systems for experiments with trapped strontium ions

We describe a efficient way to photoionize strontium atoms in a linear radio-frequency trap. We use a 2-photon second order process to excite the autoionization resonance (4d2 + 5p2) 1D2. A doubled pulsed Ti:Saphire laser system is used at 431nm to provide 100fsec pulses at 82Mhz. The fabrication of the laser systems for addressing the Sr+ transitions necessary for laser cooling and excitation of quantum jumps, vacuum system and ion trap structure are also described in detail. With the current setup a easy and repeatable trapping of linear ion chains is achieved at UHV pressures.

quant-ph