arXiv subjects

E. M. Forgan

Publications and source records attributed to E. M. Forgan.

At least 37 records · Page 2Linked to original sources

arXiv2014

Vortex lattice structure in BaFe2(As0.67P0.33)2 by the small-angle neutron scattering technique

We have observed a magnetic vortex lattice (VL) in BaFe2(As_{0.67}P_{0.33})2 (BFAP) single crystals by small-angle neutron scattering (SANS). With the field along the c-axis, a nearly isotropic hexagonal VL was formed in the field range from 1 to 16 T, which is a record for this technique in the pnictides, and no symmetry changes in the VL were observed. The temperature-dependence of the VL signal was measured and confirms the presence of (non d-wave) nodes in the superconducting gap structure for measurements at 5 T and below. The nodal effects were suppressed at high fields. At low fields, a VL reorientation transition was observed between 1 T and 3 T, with the VL orientation changing by 45°. Below 1 T, the VL structure was strongly affected by pinning and the diffraction pattern had a fourfold symmetry. We suggest that this (and possibly also the VL reorientation) is due to pinning to defects aligned with the crystal structure, rather than being intrinsic.

cond-mat.str-el↗

arXiv2014

Competing charge, spin, and superconducting orders in underdoped YBa2Cu3Oy

To explore the doping dependence of the recently discovered charge density wave (CDW) order in YBa2Cu3Oy, we present a bulk-sensitive high-energy x-ray study for several oxygen concentrations, including strongly underdoped YBa2Cu3O6.44. Combined with previous data around the so-called 1/8 doping, we show that bulk CDW order exists at least for hole concentrations (p) in the CuO2 planes of 0.078 <~ p <~ 0.132. This implies that CDW order exists in close vicinity to the quantum critical point for spin density wave (SDW) order. In contrast to the pseudogap temperature T*, the onset temperature of CDW order decreases with underdoping to T_CDW ~ 90K in YBa2Cu3O6.44. Together with a weakened order parameter this suggests a competition between CDW and SDW orders. In addition, the CDW order in YBa2Cu3O6.44 shows the same type of competition with superconductivity as a function of temperature and magnetic field as samples closer to p = 1/8. At low p the CDW incommensurability continues the previously reported linear increasing trend with underdoping. In the entire doping range the in-plane correlation length of the CDW order in b-axis direction depends only very weakly on the hole concentration, and appears independent of the type and correlation length of the oxygen-chain order. The onset temperature of the CDW order is remarkably close to a temperature T^\dagger that marks the maximum of 1/(T_1T) in planar 63^Cu NQR/NMR experiments, potentially indicating a response of the spin dynamics to the formation of the CDW. Our discussion of these findings includes a detailed comparison to the charge stripe order in La2-xBaxCuO4.

cond-mat.supr-con↗

arXiv2014

Bulk charge stripe order competing with superconductivity in La2-xSrxCuO4 (x=0.12)

We present a volume-sensitive high-energy x-ray diffraction study of the underdoped cuprate high temperature superconductor La2-xSrxCuO4 (x = 0.12, Tc=27 K) in applied magnetic field. Bulk short-range charge stripe order with propagation vector q_ch = (0.231, 0, 0.5) is demonstrated to exist below T_ch = 85(10) K and shown to compete with superconductivity. We argue that bulk charge ordering arises from fluctuating stripes that become pinned near boundaries between orthorhombic twin domains.

cond-mat.supr-con↗

arXiv2013

An inelastic x-ray study of phonon broadening and charge density wave formation in ortho-II ordered YBa2Cu3O6.54

Inelastic x-ray scattering is used to investigate charge density wave (CDW) formation and the low-energy lattice dynamics of the underdoped high temperature superconductor ortho-II YBa2Cu3O6.54. We find that, for a temperature ~1/3 of the CDW onset temperature (~155 K), the CDW order is static within the resolution of the experiment, that is the inverse lifetime is less than 0.3 meV. In the same temperature region, low-energy phonons near the ordering wavevector of the CDW show large increases in their linewidths. This contrasts with the usual behavior in CDW systems where the phonon anomalies are strongest near the CDW onset temperature

cond-mat.supr-con↗

arXiv2013

X-ray diffraction observation of charge density wave order at zero magnetic field in ortho-II YBa$_2$Cu$_3$O$_{6.54}$

X-ray diffraction measurements show that the high-temperature superconductor YBa$_2$Cu$_3$O$_{6.54}$, with ortho-II oxygen order, has charge density wave order (CDW) in the absence of an applied magnetic field. The dominant wavevector of the CDW is $\mathbf{q}_{\mathrm{CDW}} = (0, 0.328(2), 0.5)$, with the in-plane component parallel to the $\mathbf{b}$-axis (chain direction). It has a similar incommensurability to that observed in ortho-VIII and ortho-III samples, which have different dopings and oxygen orderings. Our results for ortho-II contrast with recent high-field NMR measurements, which suggest a commensurate wavevector along the $\mathbf{a}$-axis. We discuss the relationship between spin and charge correlations in YBa$_2$Cu$_3$O$_{y}$, and recent high-field quantum oscillation, NMR and ultrasound experiments.

cond-mat.supr-con↗

arXiv2012

Polarized Neutron Laue Diffraction on a Crystal Containing Dynamically Polarized Proton Spins

We report on a polarized-neutron Laue diffraction experiment on a single crystal of neodynium doped lanthanum magnesium nitrate hydrate containing polarized proton spins. By using dynamic nuclear polarization to polarize the proton spins, we demonstrate that the intensities of the Bragg peaks can be enhanced or diminished significantly, whilst the incoherent background, due to proton spin disorder, is reduced. It follows that the method offers unique possibilities to tune continuously the contrast of the Bragg reflections and thereby represents a new tool for increasing substantially the signal-to-noise ratio in neutron diffraction patterns of hydrogenous matter.

cond-mat.mtrl-sci↗

arXiv2012

Direct observation of competition between superconductivity and charge density wave order in YBa2Cu3Oy

Superconductivity often emerges in the proximity of, or in competition with, symmetry breaking ground states such as antiferromagnetism or charge density waves (CDW)1-5. A number of materials in the cuprate family, which includes the high-transition-temperature (high-Tc) superconductors, show spin and charge density wave order5-7. Thus a fundamental question is to what extent these ordered states exist for compositions close to optimal for superconductivity. Here we use high-energy x-ray diffraction to show that a CDW develops at zero field in the normal state of superconducting YBa2Cu3O6.67 (Tc = 67 K). Below Tc, the application of a magnetic field suppresses superconductivity and enhances the CDW. Hence, the CDW and superconductivity are competing orders in this typical high-Tc superconductor, and high-Tc superconductivity can form from a pre-existing CDW state. Our results explain observations of small Fermi surface pockets8, negative Hall and Seebeck effect9,10 and the "Tc plateau"11 in this material when underdoped.

cond-mat.supr-con↗

arXiv2012

Spin density wave induced disordering of the vortex lattice in superconducting La$_{2-x}$Sr$_x$CuO$_4$

We use small angle neutron scattering to study the superconducting vortex lattice in La$_{2-x}$Sr$_x$CuO$_4$ as a function of doping and magnetic field. We show that near optimally doping the vortex lattice coordination and the superconducting coherence length $ξ$ are controlled by a van-Hove singularity crossing the Fermi level near the Brillouin zone boundary. The vortex lattice properties change dramatically as a spin-density-wave instability is approached upon underdoping. The Bragg glass paradigm provides a good description of this regime and suggests that SDW order acts as a novel source of disorder on the vortex lattice.

cond-mat.supr-con↗

arXiv2012

Vortex lattice studies in CeCoIn5 with H perpendicular to c

We present small angle neutron scattering studies of the vortex lattice (VL) in CeCoIn5 with magnetic fields applied parallel (H) to the antinodal [100] and nodal [110] directions. For H || [100], a single VL orientation is observed, while a 90 degree reorientation transition is found for H || [110]. For both field orientations and VL configurations we find a distorted hexagonal VL with an anisotropy, Gamma = 2.0 +/- 0.05. The VL form factor shows strong Pauli paramagnetic effects similar to what have previously been reported for H || [001]. At high fields, above which the upper critical field (Hc2) becomes a first-order transition, an increased disordering of the VL is observed.

cond-mat.supr-con↗

arXiv2011

Magnetic-field-induced nonlocal effects on the vortex interactions in twin-free YBa2Cu3O7

The vortex lattice (VL) in the high-kappa superconductor YBa2Cu3O7, at 2 K and with the magnetic field parallel to the crystal c-axis, undergoes a sequence of transitions between different structures as a function of applied magnetic field. However, from structural studies alone, it is not possible to determine precisely the system anisotropy that governs the transitions between different structures. To address this question, here we report new small-angle neutron scattering measurements of both the VL structure at higher temperatures, and the field- and temperature-dependence of the VL form factor. Our measurements demonstrate how the influence of anisotropy on the VL, which in theory can be parameterized as nonlocal corrections, becomes progressively important with increasing magnetic field, and suppressed by increasing the temperature towards Tc. The data indicate that nonlocality due to different anisotropies play important roles in determining the VL properties.

cond-mat.supr-con↗

arXiv2011

Time Resolved Stroboscopic Neutron Scattering of Vortex Lattice Dynamics in Superconducting Niobium

Superconducting vortex lattices, glasses and liquids attract great interest as model systems of crystallization and as a source of microscopic information of the nature of superconductivity. We report for the first time direct microscopic measurements of the vortex lattice tilt modulus c44 in ultra-pure niobium using time-resolved small angle neutron scattering. Besides a general trend to faster vortex lattice dynamics for increasing temperatures we observe a dramatic changeover of the relaxation process associated with the non-trivial vortex lattice morphology in the intermediate mixed state. This changeover is attributed to a Landau-branching of the Shubnikov domains at the surface of the sample. Our study represents a showcase for how to access directly vortex lattice melting and the formation of vortex matter states for other systems.

cond-mat.str-el↗

arXiv2010

The Absence of Vortex Lattice Melting in a Conventional Superconductor

The state of the vortex lattice extremely close to the superconducting to normal transition in an applied magnetic field is investigated in high purity niobium. We observe that thermal fluctuations of the order parameter broaden the superconducting to normal transition into a crossover but no sign of a first order vortex lattice melting transition is detected in measurements of the heat capacity or the small angle neutron scattering (SANS) intensity. Direct observation of the vortices via SANS always finds a well ordered vortex lattice. The fluctuation broadening is considered in terms of the Lowest Landau Level theory of critical fluctuations and scaling is found to occur over a large H_{c2}(T) range.

cond-mat.supr-con↗

arXiv2010

The pairing state in KFe2As2 studied by measurements of the magnetic vortex lattice

Understanding the mechanism and symmetry of electron pairing in iron-based superconductors represents an important challenge in condensed matter physics [1-3]. The observation of magnetic flux lines - "vortices" - in a superconductor can contribute to this issue, because the spatial variation of magnetic field reflects the pairing. Unlike many other iron pnictides, our KFe2As2 crystals have very weak vortex pinning, allowing small-angle-neutron-scattering (SANS) observations of the intrinsic vortex lattice (VL). We observe nearly isotropic hexagonal packing of vortices, without VL-symmetry transitions up to high fields along the fourfold c-axis of the crystals, indicating rather small anisotropy of the superconducting properties around this axis. This rules out gap nodes parallel to the c-axis, and thus d-wave and also anisotropic s-wave pairing [2, 3]. The strong temperature-dependence of the intensity down to T<<Tc indicates either widely different full gaps on different Fermi surface sheets, or nodal lines perpendicular to the axis.

cond-mat.supr-con↗

arXiv2010

Exploring the fragile antiferromagnetic superconducting phase in CeCoIn5

CeCoIn5 is a heavy fermion Type-II superconductor which exhibits clear indications of Pauli-limited superconductivity. A variety of measurements give evidence for a transition at high magnetic fields inside the superconducting state, when the field is applied either parallel to or perpendicular to the c axis. When the field is perpendicular to the c axis, antiferromagnetic order is observed on the high-field side of the transition, with a magnetic wavevector of (q q 0.5), where q = 0.44 reciprocal lattice units. We show that this order remains as the magnetic field is rotated out of the basal plane, but the associated moment eventually disappears above 17 degrees, indicating that the anomalies seen with the field parallel to the c axis are not related to this magnetic order. We discuss the implications of this finding.

cond-mat.str-el↗

arXiv2010

Weak superconducting pairing and a single isotropic energy gap in stoichiometric LiFeAs

We report superconducting (SC) properties of stoichiometric LiFeAs (Tc = 17 K) studied by small-angle neutron scattering (SANS) and angle-resolved photoemission (ARPES). Although the vortex lattice exhibits no long-range order, well-defined SANS rocking curves indicate better ordering than in chemically doped 122-compounds. The London penetration depth of 210 nm, determined from the magnetic field dependence of the form factor, is compared to that calculated from the ARPES band structure with no adjustable parameters. Its temperature dependence is best described by a single isotropic SC gap of 3.0 meV, which agrees with the ARPES value of 3.1 meV and corresponds to the ratio 2Delta/kTc = 4.1, approaching the weak-coupling limit predicted by the BCS theory. This classifies LiFeAs as a weakly coupled single-gap superconductor, similar to conventional metals.

cond-mat.supr-con↗

arXiv2010

Observations of Pauli Paramagnetic Effects on the Flux Line Lattice in CeCoIn5

From small-angle neutron scattering studies of the flux line lattice (FLL) in CeCoIn5, with magnetic field applied parallel to the crystal c-axis, we obtain the field- and temperature-dependence of the FLL form factor, which is a measure of the spatial variation of the field in the mixed state. We extend our earlier work [A.D. Bianchi et al. 2008 Science 319, 177] to temperatures up to 1250 mK. Over the entire temperature range, paramagnetism in the flux line cores results in an increase of the form factor with field. Near H_c2 the form factor decreases again, and our results indicate that this fall-off extends outside the proposed FFLO region. Instead, we attribute the decrease to a paramagnetic suppression of Cooper pairing. At higher temperatures, a gradual crossover towards more conventional mixed state behavior is observed.

cond-mat.supr-con↗

arXiv2009

Symmetry and disorder of the vitreous vortex lattice in an overdoped BaFe_{2-x}Co_xAs_2 superconductor: Indication for strong single-vortex pinning

The disordered flux line lattice in single crystals of the slightly overdoped aFe_{2-x}Co_xAs_2 (x = 0.19, Tc = 23 K) superconductor is studied by magnetization measurements, small-angle neutron scattering (SANS), and magnetic force microscopy (MFM). In the whole range of magnetic fields up to 9 T, vortex pinning precludes the formation of an ordered Abrikosov lattice. Instead, a vitreous vortex phase (vortex glass) with a short-range hexagonal order is observed. Statistical processing of MFM datasets lets us directly measure its radial and angular distribution functions and extract the radial correlation length ζ. In contrast to predictions of the collective pinning model, no increase in the correlated volume with the applied field is observed. Instead, we find that ζdecreases as 1.3*R1 ~ H^(-1/2) over four decades of the applied magnetic field, where R1 is the radius of the first coordination shell of the vortex lattice. Such universal scaling of ζimplies that the vortex pinning in iron arsenides remains strong even in the absence of static magnetism. This result is consistent with all the real- and reciprocal-space vortex-lattice measurements in overdoped as-grown aFe_{2-x}Co_xAs_2 published to date and is thus sample-independent. The failure of the collective pinning model suggests that the vortices remain in the single-vortex pinning limit even in high magnetic fields up to 9 T.

cond-mat.supr-con↗

arXiv2009

Fermi surface and order parameter driven vortex lattice structure transitions in twin-free YBa2Cu3O7

We report on small-angle neutron scattering studies of the intrinsic vortex lattice (VL) structure in detwinned YBa2Cu3O7 at 2 K, and in fields up to 10.8 T. Because of the suppressed pinning to twin-domain boundaries, a new distorted hexagonal VL structure phase is stabilized at intermediate fields. It is separated from a low-field hexagonal phase of different orientation and distortion by a first-order transition at 2.0(2) T that is probably driven by Fermi surface effects. We argue that another first-order transition at 6.7(2) T, into a rhombic structure with a distortion of opposite sign, marks a crossover from a regime where Fermi surface anisotropy is dominant, to one where the VL structure and distortion is controlled by the order-parameter anisotropy.

cond-mat.supr-con↗