arXiv subjects

E. M. L. English

Publications and source records attributed to E. M. L. English.

6 recordsLinked to original sources

arXiv2010

Atomic excitation during recollision-free ultrafast multi-electron tunnel ionization

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the states of the remaining electrons are neglected. Such electronic interactions are predicted to be weak, the exception being recollision excitation and ionization caused by linearly-polarized radiation. In contrast, it has recently been suggested that intense field ionization may be accompanied by a two-stage `shake-up' reaction. Here we report a unique combination of experimental techniques that enables us to accurately measure the tunnel ionization probability for argon exposed to 50 femtosecond laser pulses. Most significantly for the current study, this measurement is independent of the optical focal geometry, equivalent to a homogenous electric field. Furthermore, circularly-polarized radiation negates recollision. The present measurements indicate that tunnel ionization results in simultaneous excitation of one or more remaining electrons through shake-up. From an atomic physics standpoint, it may be possible to induce ionization from specific states, and will influence the development of coherent attosecond XUV radiation sources. Such pulses have vital scientific and economic potential in areas such as high-resolution imaging of in-vivo cells and nanoscale XUV lithography.

physics.atom-ph↗

arXiv2009

Ultrastable lasers based on vibration insensitive cavities

We present two ultra-stable lasers based on two vibration insensitive cavity designs, one with vertical optical axis geometry, the other horizontal. Ultra-stable cavities are constructed with fused silica mirror substrates, shown to decrease the thermal noise limit, in order to improve the frequency stability over previous designs. Vibration sensitivity components measured are equal to or better than 1.5e-11 per m.s^-2 for each spatial direction, which shows significant improvement over previous studies. We have tested the very low dependence on the position of the cavity support points, in order to establish that our designs eliminate the need for fine tuning to achieve extremely low vibration sensitivity. Relative frequency measurements show that at least one of the stabilized lasers has a stability better than 5.6e-16 at 1 second, which is the best result obtained for this length of cavity.

physics.optics↗

arXiv2009

Ultra-low noise microwave generation with fiber-based optical frequency comb and application to atomic fountain clock

We demonstrate the use of a fiber-based femtosecond laser locked onto an ultra-stable optical cavity to generate a low-noise microwave reference signal. Comparison with both a liquid Helium cryogenic sapphire oscillator (CSO) and a Ti:Sapphire-based optical frequency comb system exhibit a stability about $3\times10^{-15}$ between 1 s and 10 s. The microwave signal from the fiber system is used to perform Ramsey spectroscopy in a state-of-the-art Cesium fountain clock. The resulting clock system is compared to the CSO and exhibits a stability of $3.5\times10^{-14}τ^{-1/2}$. Our continuously operated fiber-based system therefore demonstrates its potential to replace the CSO for atomic clocks with high stability in both the optical and microwave domain, most particularly for operational primary frequency standards.

physics.atom-ph↗

arXiv2007

Isolated vibrational wavepackets in D2+: Defining superposition conditions and wavepacket distinguishability

Tunnel ionization of room-temperature D$_2$ in an ultrashort (12 femtosecond) near infra-red (800 nm) pump laser pulse excites a vibrational wavepacket in the D2+ ions; a rotational wavepacket is also excited in residual D2 molecules. Both wavepacket types are collapsed a variable time later by an ultrashort probe pulse. We isolate the vibrational wavepacket and quantify its evolution dynamics through theoretical comparison. Requirements for quantum computation (initial coherence and quantum state retrieval) are studied using this well-defined (small number of initial states at room temperature, initial wavepacket spatially localized) single-electron molecular prototype by temporally stretching the pump and probe pulses.

physics.chem-ph↗

arXiv2007

Mapping the Evolution of Optically-Generated Rotational Wavepackets in a Room Temperature Ensemble of D$_2$

A coherent superposition of rotational states in D$_2$ has been excited by nonresonant ultrafast (12 femtosecond) intense (2 $\times$ 10$^{14}$ Wcm$^{-2}$) 800 nm laser pulses leading to impulsive dynamic alignment. Field-free evolution of this rotational wavepacket has been mapped to high temporal resolution by a time-delayed pulse, initiating rapid double ionization, which is highly sensitive to the angle of orientation of the molecular axis with respect to the polarization direction, $θ$. The detailed fractional revivals of the neutral D$_2$ wavepacket as a function of $θ$ and evolution time have been observed and modelled theoretically.

quant-ph↗

arXiv2005

Geometry- and diffraction-independent ionization probabilities in intense laser fields: probing atomic ionization mechanisms with effective intensity matching

We report a novel experimental technique for the comparison of ionization processes in ultrafast laser pulses irrespective of pulse ellipticity. Multiple ionization of xenon by 50 fs 790 nm, linearly and circularly polarized laser pulses is observed over the intensity range 10 TW/cm^2 to 10 PW/cm^2 using Effective Intensity Matching (EIM), which is coupled with Intensity Selective Scanning (ISS) to recover the geometry-independent probability of ionization. Such measurements, made possible by quantifying diffraction effects in the laser focus, are compared directly to theoretical predictions of multiphoton, tunnel and field ionization, and a remarkable agreement demonstrated. EIM-ISS allows the straightforward quantification of the probability of recollision ionization in a linearly polarized laser pulse. Furthermore, probability of ionization is discussed in terms of the Keldysh adiabaticity parameter, gamma, and the influence of the precursor ionic states present in recollision ionization is observed for the first time.

physics.atom-ph↗