arXiv subjects

E. Meehan

Publications and source records attributed to E. Meehan.

4 recordsLinked to original sources

arXiv2025

Improved sensitivity in the search for rare decays of Gd isotopes

Gadolinium is widely used in multiple low-background experiments, making its isotopes accessible for rare decay searches both in-situ and through radiopurity screening data. This study presents an improved search for rare alpha and double-beta decay modes in $^{152}$Gd, $^{154}$Gd, and $^{160}$Gd isotopes using ultra-low background HPGe detectors at the Boulby Underground Screening (BUGS) facility. A total exposure of 6.7 kg$\cdot$yr of natural gadolinium was achieved using gadolinium sulfate octahydrate $(\text{Gd}_2(\text{SO}_4)_3 \cdot 8\text{H}_2\text{O})$ samples, originally screened for radiopurity prior to their deployment in the Super-Kamiokande neutrino experiment. Due to the detection methodology, only decays into excited states accompanied by gamma-ray emission were accessible. A Bayesian analysis incorporating prior experimental results was employed, leading to new lower half-life limits in the range of $10^{19} - 10^{21}$ years - an improvement of approximately two orders of magnitude over previous constraints. No statistically significant decay signals were observed. These results demonstrate the effectiveness of repurposing large-scale radiopurity screening campaigns for fundamental physics research.

nucl-ex↗

arXiv2023

Ultra-Low Background Germanium Assay at the Boulby Underground Laboratory

As we move to an era where next generation low-background particle physics experiments begin to be designed and constructed, the ability to assay materials with high sensitivity and at speed with a variety of techniques will be key. This paper describes the Mirion Technologies (Canberra) specialty ultra-low background detectors installed and commissioned at the Boulby Underground Laboratory between 2017 and 2021. The low background levels of the detectors combine with low background shielding and a radon-reduced dry nitrogen purge system to give sensitivity approaching the best in the world without the need for intricate shielding solutions. For an optimised sample geometry, run for 100 days, it would be possible to reach close to 10 $\mu$Bq/kg ($10^{-12}$ g/g) for background isotopes of interest in neutrinoless double-beta decay.

physics.ins-det↗

arXiv2022

Development of Ultra-pure Gadolinium Sulfate for the Super-Kamiokande Gadolinium Project

This paper reports the development and detailed properties of about 13 tons of gadolinium sulfate octahydrate, $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$, which has been dissolved into Super-Kamiokande (SK) in the summer of 2020. We evaluate the impact of radioactive impurities in $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ on DSNB searches and solar neutrino observation and confirm the need to reduce radioactive and fluorescent impurities by about three orders of magnitude from commercially available high-purity $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$. In order to produce ultra-high-purity $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$, we have developed a method to remove impurities from gadolinium oxide, Gd$_2$O$_3$, consisting of acid dissolution, solvent extraction, and pH control processes, followed by a high-purity sulfation process. All of the produced ultra-high-purity $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ is assayed by ICP-MS and HPGe detectors to evaluate its quality. Because of the long measurement time of HPGe detectors, we have employed several underground laboratories for making parallel measurements including LSC in Spain, Boulby in the UK, and Kamioka in Japan. In the first half of production, the measured batch purities were found to be consistent with the specifications. However,in the latter half, the $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ contained one order of magnitude more $^{228}$Ra than the budgeted mean contamination. This was correlated with the corresponding characteristics of the raw material Gd$_2$O$_3$, in which an intrinsically large contamination was present. Based on their modest impact on SK physics, they were nevertheless introduced into the detector. To reduce $^{228}$Ra for the next stage of Gd loading to SK, a new process has been successfully establised.

physics.ins-det↗

arXiv2017

Low Background Gamma Spectroscopy at the Boulby Underground Laboratory

The Boulby Underground Germanium Suite (BUGS) comprises three low background, high-purity germanium detectors operating in the Boulby Underground Laboratory, located 1.1 km underground in the north-east of England, UK. BUGS utilises three types of detector to facilitate a high-sensitivity, high-throughput radioassay programme to support the development of rare-event search experiments. A Broad Energy Germanium (BEGe) detector delivers sensitivity to low-energy gamma-rays such as those emitted by 210Pb and 234Th. A Small Anode Germanium (SAGe) well-type detector is employed for efficient screening of small samples. Finally, a standard p-type coaxial detector provides fast screening of standard samples. This paper presents the steps used to characterise the performance of these detectors for a variety of sample geometries, including the corrections applied to account for cascade summing effects. For low-density materials, BUGS is able to radio-assay to specific activities down to 3.6 mBq/kg for 234Th and 6.6 mBq/kg for 210Pb both of which have uncovered some significant equilibrium breaks in the 238U chain. In denser materials, where gamma-ray self-absorption increases, sensitivity is demonstrated to specific activities of 0.9 mBq/kg for 226Ra, 1.1 mBq/kg for 228 Ra, 0.3 mBq/kg for 224Ra, and 8.6 mBq/kg for 40K with all upper limits at a 90% confidence level. These meet the requirements of most screening campaigns presently under way for rare-event search experiments, such as the LUX-ZEPLIN (LZ) dark matter experiment. We also highlight the ability of the BEGe detector to probe the X-ray fluorescence region which can be important to identify the presence of radioisotopes associated with neutron production; this is of particular relevance in experiments sensitive to nuclear recoils.

physics.ins-det↗