arXiv subjects

E. Mendoza

Publications and source records attributed to E. Mendoza.

At least 37 records · Page 2Linked to original sources

arXiv2022

Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF

This article presents a few selected developments and future ideas related to the measurement of $(n,γ)$ data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with $γ$-ray imaging capability for background suppression, and the development of an array of small-volume organic scintillators aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate $i$ neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area.

nucl-ex↗

arXiv2022

High accuracy, high resolution 235U(n,f) cross section from n_TOF (CERN) in the thermal to 10 keV energy range

The 235U(n,f) cross section was measured in a wide energy range (25 meV - 170 keV) at the n_TOF facility at CERN, relative to 6Li(n,t) and 10B(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between thermal and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the n_TOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement is found in average between the new results and the latest evaluated data files ENDF-B/VIII and JEFF-3.3, as well as with respect to the IAEA reference files. However, some discrepancies are still present in some specific energy regions. The new dataset here presented, characterized by unprecedented resolution and accuracy, can help improving the evaluations in the Resolved Resonance Region and up to 10 keV, and reduce the uncertainties that affect this region.

nucl-ex↗

arXiv2021

SiS formation in the interstellar medium through Si+SH gas phase reactions

Silicon monosulfide is an important silicon bearing molecule detected in circumstellar envelopes and star forming regions. Its formation and destruction routes are not well understood, partially due to the lack of a detailed knowledge on the involved reactions and their rate coefficients. In this work we have calculated and modeled the potential energy surface (PES) of the HSiS system employing highly accurate multireference electronic structure methods. After obtaining an accurate analytic representation of the PES, which includes long-range energy terms in a realistic way via the DMBE method, we have calculated rate coefficients for the Si+SH$\rightarrow$SiS+H reaction over the temperature range of 25-1000K. This reaction is predicted to be fast, with a rate coefficient of $\sim 1\times 10^{-10}\rm cm^3\, s^{-1}$ at 200K, which substantially increases for lower temperatures (the temperature dependence can be described by a modified Arrhenius equation with $α=0.770\times 10^{-10}\rm cm^3\,s^{-1}$, $β=-0.756$ and $γ=9.873\, \rm K$). An astrochemical gas-grain model of a shock region similar to L1157-B1 shows that the inclusion of the Si+SH reaction increases the SiS gas-phase abundance relative to \ce{H2} from $5\times 10^{-10}$ to $1.4\times 10^{-8}$, which perfectly matches the observed abundance of $\sim 2\times 10^{-8}$.

astro-ph.GA↗

arXiv2021

HCN/HNC chemistry in shocks: a study of L1157-B1 with ASAI

HCN and its isomer HNC play an important role in molecular cloud chemistry and the formation of more complex molecules. We investigate here the impact of protostellar shocks on the HCN and HNC abundances from high-sensitivity IRAM 30m observations of the prototypical shock region L1157-B1 and the envelope of the associated Class 0 protostar, as a proxy for the pre-shock gas. The isotopologues H$^{12}$CN, HN$^{12}$C, H$^{13}$CN, HN$^{13}$C, HC$^{15}$N, H$^{15}$NC, DCN and DNC were all detected towards both regions. Abundances and excitation conditions were obtained from radiative transfer analysis of molecular line emission under the assumption of Local Thermodynamical Equilibrium. In the pre-shock gas, the abundances of the HCN and HNC isotopologues are similar to those encountered in dark clouds, with a HCN/HNC abundance ratio $\approx 1$ for all isotopologues. A strong D-enrichment (D/H$\approx 0.06$) is measured in the pre-shock gas. There is no evidence of $^{15}$N fractionation neither in the quiescent nor in the shocked gas. At the passage of the shock, the HCN and HNC abundances increase in the gas phase in different manners so that the HCN/HNC relative abundance ratio increases by a factor 20. The gas-grain chemical and shock model UCLCHEM allows us to reproduce the observed trends for a C-type shock with pre-shock density $n$(H)= $10^5$cm$^{-3}$ and shock velocity $V_s= 40$km/s. We conclude that the HCN/HNC variations across the shock are mainly caused by the sputtering of the grain mantle material in relation with the history of the grain ices.

astro-ph.GA↗

arXiv2021

Interrelations between Astrochemistry and Galactic Dynamics

This paper presents a review of ideas that interconnect Astrochemistry and Galactic Dynamics. Since these two areas are vast and not recent, each one has already been covered separately by several reviews. After a general historical introduction, and a needed quick review of processes like the stellar nucleosynthesis which gives the base to understand the interstellar formation of simple chemical compounds (H2, CO, NH3 and H2O), we focus on a number of topics which are at the crossing of the two areas, Dynamics and Astrochemistry. Astrochemistry is a flourishing field which intends to study the presence and formation of molecules as well as the influence of them into the structure, evolution and dynamics of astronomical objects. The progress in the knowledge on the existence of new complex molecules and of their process of formation originates from the observational, experimental and theoretical areas which compose the field. The interfacing areas include star formation, protoplanetary disks, the role of the spiral arms and the chemical abundance gradients in the galactic disk. It often happens that the physical conditions in some regions of the ISM are only revealed by means of molecular observations. To organise a classification of chemical evolution processes, we discuss about how astrochemistry can act in three different contexts: i. the chemistry of the early universe, including external galaxies, ii. star forming regions, and iii. AGB stars and circumstellar envelopes. We mention that our research is stimulated by plans for instruments and projects, such as the on-going LLAMA, which consists in the construction of a 12m sub-mm radio telescope in the Andes. Thus, modern and new facilities can play a key role in new discoveries not only in astrochemistry but also in radio astronomy and related areas. Furthermore, the research of the origin of life is also a stimulating perspective.

astro-ph.GA↗

arXiv2021

Development of a Reference Database for Beta-Delayed Neutron Emission

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html.

nucl-ex↗

arXiv2020

Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,γ$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,γ$) and $^{56}$Fe($n, γ$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.

physics.ins-det↗

arXiv2020

Physical characterization of S169: A prototypical IR bubble associated with the massive star-forming region IRAS12326-6245

With the aim of studying the properties of Galactic IR bubbles and their impact in massive star formation, we present a study of the IR bubble S169, associated with the massive star forming region IRAS12326-6245. We used CO(2-1),$^{13}$CO(2-1), C$^{18}$O(2-1), HCN(3-2), and HCO+(3-2) line data obtained with the APEX telescope to study the properties of the molecular gas in the nebula and the IRAS source . To analyze the properties and distribution of the dust, we used IRAC-GLIMPSE, Herschel, and ATLASGAL data. The properties of the ionized gas were studied using images obtained from the SUMSS survey and SuperCOSMOS database. In our search for stellar and protostellar objects in the region, we used IR and optical point source calalogs. The new APEX observations allowed us to identify three molecular components associated with the nebula, namely: at $-$39 km/s (component A), $-$25 km/s (component B), and $-$17 km/s (component C). Six molecular condensations (MC1 to MC6) were identified in component A, with MC3 (the densest and more massive one) being the molecular counterpart of IRAS12326-6245. For this source, we estimated an H$_2$ column density up to 8$\times$10$^{23}$ cm$^{-2}$. To explain the morphology and velocity of components A, B, and C, we propose a simple model consisting of a partially complete semisphere-like structure expanding at ~ 12 km/s. The introduction of this model has led to a discussion about the distance to both S169 and IRAS12326-6245, which was estimated to be ~ 2 kpc. Several candidate YSOs were identified, projected mostly onto the molecular condensations MC3, MC4, and MC5, which indicates that the star-formation process is very active at the borders of the nebula. A comparison between observable and modeled parameters was not enough to discern whether the collect-and-collapse mechanism is acting at the edge of S169.

astro-ph.GA↗

arXiv2019

Review and new concepts for neutron-capture measurements of astrophysical interest

The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,γ$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on total energy detectors will be presented to illustrate how, advances in instrumentation have led, over the years, to the assessment and discovery of many new aspects of $s$-process nucleosynthesis and to the progressive refinement of theoretical models of stellar evolution. A summary will be presented on current efforts to develop new detection concepts, such as the Total-Energy Detector with $γ$-ray imaging capability (i-TED). The latter is based on the simultaneous combination of Compton imaging with neutron time-of-flight (TOF) techniques, in order to achieve a superior level of sensitivity and selectivity in the measurement of stellar neutron capture rates.

physics.ins-det↗

arXiv2019

Cyanoacetylene in the outflow/hot molecular core G331.512-0.103

Using APEX-1 and APEX-2 observations, we have detected and studied the rotational lines of the HC$_3$N molecule (cyanoacetylene) in the powerful outflow/hot molecular core G331.512-0.103. We identified thirty-one rotational lines at $J$ levels between 24 and 39; seventeen of them in the ground vibrational state $v$=0 (9 lines corresponding to the main C isotopologue and 8 lines corresponding to the $^{13}$C isotopologues), and fourteen in the lowest vibrationally excited state $v_7$=1. Using LTE-based population diagrams for the beam-diluted $v$=0 transitions, we determined $T_{\rm exc}$=85$\pm$4 K and $N$(HC$_3$N)=(6.9$\pm$0.8)$\times$10$^{14}$ cm$^{-2}$, while for the beam-diluted $v_7$=1 transitions we obtained $T_{\rm exc}$=89$\pm$10 K and $N$(HC$_3$N)=2$\pm$1$\times$10$^{15}$ cm$^{-2}$. Non-LTE calculations using H$_2$ collision rates indicate that the HC$_3$N emission is in good agreement with LTE-based results. From the non-LTE method we estimated $T_{\rm kin}$ $\simeq$90~K, $n$(H$_2$)$\simeq$2$\times$10$^7$~cm$^{-3}$ for a central core of 6 arcsec in size. A vibrational temperature in the range from 130~K to 145~K was also determined, values which are very likely lower limits. Our results suggest that rotational transitions are thermalized, while IR radiative pumping processes are probably more efficient than collisions in exciting the molecule to the vibrationally excited state $v_7$=1. Abundance ratios derived under LTE conditions for the $^{13}$C isotopologues suggest that the main formation pathway of HC$_3$N is ${\rm C}_2{\rm H}_2 + {\rm CN} \rightarrow {\rm HC}_3{\rm N} + {\rm H}$.

astro-ph.GA↗

arXiv2019

Study of multi-neutron emission in the $β$-decay of $^{11}$Li

The kinematics of two-neutron emission following the $β$-decay of $^{11}$Li was investigated for the first time by detecting the two neutrons in coincidence and by measuring their angle and energy. An array of liquid-scintillator neutron detectors was used to reject cosmic-ray and $γ$-ray backgrounds by pulse-shape discrimination. Cross-talk events in which two detectors are fired by a single neutron were rejected using a filter tested on the $β$-1n emitter $^9$Li. A large cross-talk rejection rate is obtained ($> 95 \%$) over most of the energy range of interest. Application to $^{11}$Li data leads to a significant number of events interpreted as $β$-2n decay. A discrete neutron line at $\approx$ 2 MeV indicates sequential two-neutron emission, possibly from the unbound state at 10.6 MeV excitation energy in $^{11}$Be.

nucl-ex↗

arXiv2019

Neutron production induced by $α$-decay with Geant4

Neutron production induced by ($α$,n) reactions is important in various scenarios. One of the most relevant ones is related to underground dark matter experiments, where the neutrons produced by the $α$-decay from radioactive contaminants in the detector materials can generate an irreducible background, limiting the sensitivity of the experiment. A precise estimate of the background due to these neutrons is crucial for the experiments currently taking data and for the design of the next generation detectors. In this work, we prove that Geant4 can be used to calculate neutron yields and energy spectra induced by $α$-decay. These neutrons are produced according to the information compiled in data libraries originally written in the ENDF-6 format. In this article we also review the different databases available, showing the differences and similarities among them. Finally, we compare several Geant4 neutron production yields and spectra with experimental data and other codes.

hep-ph↗

arXiv2019

Measurement of the 235U(n,f) cross section relative to the 6Li(n,t) and 10B(n,alpha) standards from thermal to 170 keV neutron energy range at n_TOF

The 235U(n,f) cross section was measured in a wide energy range at n_TOF relative to 6Li(n,t) and 10B(n,alpha), with high resolution and in a wide energy range, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the reaction yields under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10÷30 keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the evaluated cross section in the 9÷18 keV neutron energy range is indeed overestimated, both in the recent updates of ENDF/B-VIII.0 and of the IAEA reference data. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The new, high accuracy results here reported may lead to a reduction of the uncertainty in the 1÷100 keV neutron energy region. Finally, the present data provide additional confidence on the recently re-evaluated cross section integral between 7.8 and 11 eV.

nucl-ex↗

arXiv2018

First determination of $β$-delayed multiple neutron emission beyond A = 100 through direct neutron measurement: The P$_{2n}$ value of $^{136}$Sb

Background: $β$-delayed multiple neutron emission has been observed for some nuclei with A$\leq$100, with $^{100}$Rb being the heaviest $β$2n emitter measured to date. So far, only 25 P$_{2n}$ values have been determined for the $\sim$300 nuclei that may decay in this way. Accordingly, it is of interest to measure P$_{2n}$ values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such measurement for nuclei with A$>$100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the $r$-process, and safety inputs for nuclear reactors. Purpose: To determine for the first time the two neutron branching ratio, P$_{2n}$ value, for $^{136}$Sb through a direct neutron measurement, and to provide precise P$_{1n}$ values for $^{136}$Sb and $^{136}$Te. Method: Pure beams were provided by the JYFLTRAP at the IGISOL facility of the University of Jyväskylä, Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point, and the BELEN detector, based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the $β$- and neutron- growth-and-decay curves and the $β$-one-neutron and $β$-two-neutron time correlations. Results: The P$_{2n}$ value of $^{136}$Sb was found to be 0.14(3)\% and the measured P$_{1n}$ values for $^{136}$Sb and $^{136}$Te were found to be 32.2(15)\% and 1.47(6)\%, respectively. The measured P$_{2n}$ value is a factor 44 smaller than predicted by the FRDM+QRPA model used for $r$-process calculations.

nucl-ex↗

arXiv2018

Cross section measurements of $^{155,157}$Gd(n,$γ$) induced by thermal and epithermal neutrons

Neutron capture measurements on $^{155}$Gd and $^{157}$Gd were performed using the time-of-flight technique at the n\_TOF facility at CERN. Four samples in form of self-sustaining metallic discs isotopically enriched in $^{155}$Gd and $^{157}$Gd were used. The measurements were carried out at the experimental area (EAR1) at 185 m from the neutron source, with an array of 4 C$_6$D$_6$ liquid scintillation detectors. The capture cross sections of $^{155}$Gd and $^{157}$Gd at neutron kinetic energy of 0.0253 eV have been estimated to be 62.2(2.2) kb and 239.8(9.3) kb, respectively, thus up to 6\% different relative to the ones reported in the nuclear data libraries. A resonance shape analysis has been performed in the resolved resonance region up to 180 eV and 300 eV, respectively, in average resonance parameters have been found in good agreement with evaluations. Above these energies the observed resonance-like structures in the cross section have been tentatively characterised in terms of resonance energy and area up to 1 keV.

nucl-ex↗

arXiv2018

Astrochemical evolution along star formation: Overview of the IRAM Large Program ASAI

Evidence is mounting that the small bodies of our Solar System, such as comets and asteroids, have at least partially inherited their chemical composition from the first phases of the Solar System formation. It then appears that the molecular complexity of these small bodies is most likely related to the earliest stages of star formation. It is therefore important to characterize and to understand how the chemical evolution changes with solar-type protostellar evolution. We present here the Large Program "Astrochemical Surveys At IRAM" (ASAI). Its goal is to carry out unbiased millimeter line surveys between 80 and 272 GHz of a sample of ten template sources, which fully cover the first stages of the formation process of solar-type stars, from prestellar cores to the late protostellar phase. In this article, we present an overview of the surveys and results obtained from the analysis of the 3 mm band observations. The number of detected main isotopic species barely varies with the evolutionary stage and is found to be very similar to that of massive star-forming regions. The molecular content in O- and C- bearing species allows us to define two chemical classes of envelopes, whose composition is dominated by either a) a rich content in O-rich complex organic molecules, associated with hot corino sources, or b) a rich content in hydrocarbons, typical of Warm Carbon Chain Chemistry sources. Overall, a high chemical richness is found to be present already in the initial phases of solar-type star formation.

astro-ph.GA↗

arXiv2018

G331.512-0.103: An Interstellar Laboratory for Molecular Synthesis I. The Ortho-to-para Ratios for CH$_3$OH and CH$_3$CN

Spectral line surveys reveal rich molecular reservoirs in G331.512-0.103, a compact radio source in the center of an energetic molecular outflow. In this first work, we analyse the physical conditions of the source by means of CH$_3$OH and CH$_3$CN. The observations were performed with the APEX telescope. Six different system configurations were defined to cover most of the band within (292-356) GHz; as a consequence we detected a forest of lines towards the central core. A total of 70 lines of $A/E$-CH$_3$OH and $A/E$-CH$_3$CN were analysed, including torsionally excited transitions of CH$_3$OH ($ν_t$=1). In a search for all the isotopologues, we identified transitions of $^{13}$CH$_3$OH. The physical conditions were derived considering collisional and radiative processes. We found common temperatures for each $A$ and $E$ symmetry of CH$_3$OH and CH$_3$CN; the derived column densities indicate an $A/E$ equilibrated ratio for both tracers. The results reveal that CH$_3$CN and CH$_3$OH trace a hot and cold component with $T_k \sim$ 141 K and $T_k \sim$ 74 K, respectively. In agreement with previous ALMA observations, the models show that the emission region is compact ($\lesssim$ 5.5 arcsec) with gas density $n$(H$_2$)=(0.7-1) $\times$ 10$^7$ cm$^{-3}$. The CH$_3$OH/CH$_3$CN abundance ratio and the evidences for pre-biotic and complex organic molecules suggest a rich and active chemistry towards G331.512-0.103.

astro-ph.GA↗

arXiv2018

A search for Cyanopolyynes in L1157-B1

We present here a systematic search for cyanopolyynes in the shock region L1157-B1 and its associated protostar L1157-mm in the framework of the Large Program "Astrochemical Surveys At IRAM" (ASAI), dedicated to chemical surveys of solar-type star forming regions with the IRAM 30m telescope. Observations of the millimeter windows between 72 and 272 GHz permitted the detection of HC$_3$N and its $^{13}$C isotopologues, and HC$_5$N (for the first time in a protostellar shock region). In the shock, analysis of the line profiles shows that the emission arises from the outflow cavities associated with L1157-B1 and L1157-B2. Molecular abundances and excitation conditions were obtained from analysis of the Spectral Line Energy Distributions under the assumption of Local Thermodynamical Equilibrium or using a radiative transfer code in the Large Velocity Gradient approximation. Towards L1157mm, the HC$_3$N emission arises from the cold envelope ($T_{rot}=10$ K) and a higher-excitation region ($T_{rot}$= $31$ K) of smaller extent around the protostar. We did not find any evidence of $^{13}$C or D fractionation enrichment towards L1157-B1. We obtain a relative abundance ratio HC$_3$N/HC$_5$N of 3.3 in the shocked gas. We find an increase by a factor of 30 of the HC$_3$N abundance between the envelope of L1157-mm and the shock region itself. Altogether, these results are consistent with a scenario in which the bulk of HC$_3$N was produced by means of gas phase reactions in the passage of the shock. This scenario is supported by the predictions of a parametric shock code coupled with the chemical model UCL_CHEM.

astro-ph.GA↗