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E. Paspalakis

Publications and source records attributed to E. Paspalakis.

9 recordsLinked to original sources

Quantum surface effects in strong coupling dynamics

Plasmons in nanostructured metals are widely utilized to trigger strong light--matter interactions with quantum light sources. While the nonclassical behavior of such quantum emitters (QEs) is well-understood in this context, the role of quantum and surface effects in the plasmonic resonator is usually neglected. Here, we combine the Green's tensor approach with the Feibelman $d$-parameter formalism to theoretically explore the influence of quantum surface effects in metal-dielectric layered nanostructures on the relaxation dynamics of a proximal two-level QE. Having identified electron spill-out as the dominant source of quantum effects in jellium-like metals, we focus our study on sodium. Our results reveal a clear splitting in the emission spectrum, indicative of having reached the strong-coupling regime, and, more importantly, non-Markovian relaxation dynamics of the emitter. Our findings establish that strong light--matter coupling is not suppressed by the emergence of nonclassical surface effects in the optical response of the metal.

physics.optics

Non-Markovian dynamics in plasmon-induced spontaneous emission interference

We investigate theoretically the non-Markovian dynamics of a degenerate V-type quantum emitter in the vicinity of a metallic nanosphere, a system that exhibits quantum interference in spontaneous emission due to the anisotropic Purcell effect. We calculate numerically the electromagnetic Green's tensor and employ the effective modes differential equation method for calculating the quantum dynamics of the emitter population, with respect to the resonance frequency and the initial state of the emitter, as well as its distance from the nanosphere. We find that the emitter population evolution varies between a gradually total decay and a partial decay combined with oscillatory population dynamics, depending strongly on the specific values of the above three parameters. Under strong coupling conditions, coherent population trapping can be observed in this system. We compare our exact results with results when the flat continuum approximation for the modified by the metallic nanosphere vacuum is applied. We conclude that the flat continuum approximation is an excellent approximation only when the spectral density of the system under study is characterized by non-overlapping plasmonic resonances.

quant-ph

Arbitrary rotation and entanglement of flux SQUID qubits

We propose a new approach for the arbitrary rotation of a three-level SQUID qubit and describe a new strategy for the creation of coherence transfer and entangled states between two three-level SQUID qubits. The former is succeeded by exploring the coupled-uncoupled states of the system when irradiated with two microwave pulses, and the latter is succeeded by placing the SQUID qubits into a microwave cavity and used adiabatic passage methods for their manipulation.

quant-ph

Enhanced Nonlinear Generation in a Three-Level Medium with Spatially Dependent Coherence

We consider a method for efficient parametric generation of a laser pulse. A single laser field is injected to a three-level medium which has two lower states and one excited state. The lower states are prepared initially in a position-dependent coherent superposition state. It is shown that by proper choice of the position dependence of the superposition along the direction of propagation, the incoming field can be converted completely to a new field.

quant-ph

Coherent Phenomena in Photonic Crystals

We study the spontaneous emission, the absorption and dispersion properties of a ${\bf Λ}$-type atom where one transition interacts near resonantly with a double-band photonic crystal. Assuming an isotropic dispersion relation near the band edges, we show that two distinct coherent phenomena can occur. First, the spontaneous emission spectrum of the adjacent free space transition obtains `dark lines' (zeroes in the spectrum). Second, the atom can become transparent to a probe laser field coupling to the adjacent free space transition.

quant-ph

Transient properties of modified reservoir-induced transparency

We investigate the transient response of a $Λ$-type system with one transition decaying to a modified radiation reservoir with an inverse square-root singular density of modes at threshold, under conditions of transparency. We calculate the time evolution of the linear susceptibility for the probe laser field and show that, depending on the strength of the coupling to the modified vacuum and the background decay, the probe transmission can exhibit behaviour ranging from underdamped to overdamped oscillations. Transient gain without population inversion is also possible depending on the system's parameters.

quant-ph

The influence of density of modes on dark lines in spontaneous emission

We study two distinct multi-level atomic models in which one transition is coupled to a Markovian reservoir, while another linked transition is coupled to a non-Markovian reservoir. We show that by choosing appropriately the density of modes of the non-Markovian reservoir the spontaneous emission to the Markovian reservoir is greatly altered. The existence of `dark lines' in the spontaneous emission spectrum in the Markovian reservoir due to the coupling to specific density of modes of the non-Markovian reservoir is also predicted.

quant-ph

Transparency Near a Photonic Band Edge

We study the absorption and dispersion properties of a ${\bf Λ}$-type atom which decays spontaneously near the edge of a photonic band gap (PBG). Using an isotropic PBG model, we show that the atom can become transparent to a probe laser field, even when other dissipative channels are present. This transparency originates from the square root singularity of the density of modes of the PBG material at threshold.

quant-ph

Fluorescence control through multiple interference mechanisms

We discuss the spontaneous emission from a coherently prepared and microwave driven doublet of potentially closely spaced excited states to a common ground level. Multiple interference mechanisms are identified which may lead to fluorescence inhibition in well-separated regions of the spectrum or act jointly in cancelling the spontaneous emission. In addition to phase independent quantum interferences due to combined absorptions and emissions of driving field photons, we distinguish two competing phase dependent interference mechanisms as means of controlling the fluorescence. The indistinguishable quantum paths may involve the spontaneous emission from the same state of the doublet, originating from the two different components of the initial coherent superposition. Alternatively the paths involve a different spontaneous photon from each of two decaying states, necessarily with the same polarization. This makes these photons indistinguishable in principle within the uncertainty of the two decay rates. The phase dependence arises for both mechanisms because the interfering paths differ by an unequal number of stimulated absorptions and emissions of the microwave field photons.

quant-ph