arXiv subjects

E. Perfetto

Publications and source records attributed to E. Perfetto.

At least 37 records · Page 2Linked to original sources

arXiv2015

Transient dynamics in the Anderson-Holstein model with interfacial screening

We study the combined effects of electron-phonon coupling and dot-lead repulsion in the transport properties of the Anderson-Holstein model. We employ a recently proposed nonperturbative method to calculate the transient response of the system. By varying the initial conditions for the time propagation the current exhibits transient oscillations of different nature. We are able to disentangle two dynamical processes, namely the local charge rearrangement due to the dot-lead contacting and the establishment of the nonequilbrium many-body state due to the application of the external bias. These processes involve either Franck-Condon excitations or transitions between the resonant level and the Fermi energy of the leads.

cond-mat.mes-hall↗

arXiv2014

Time-resolved charge fractionalization in inhomogeneous Luttinger liquids

The recent observation of charge fractionalization in single Tomanga-Luttinger liquids (TLLs) [Kamata et al., Nature Nanotech., 9 177 (2014)] opens new routes for a systematic investigation of this exotic quantum phenomenon. In this Letter we perform measurements on two adjacent TLLs and put forward an accurate theoretical framework to address the experiments. The theory is based on the plasmon scattering approach and can deal with injected charge pulses of arbitrary shape in TLL regions. We accurately reproduce and interpret the time-resolved multiple fractionalization events in both single and double TLLs. The effect of inter-correlations between the two TLLs is also discussed.

cond-mat.mes-hall↗

arXiv2013

Charge dynamics in molecular junctions: Nonequilibrium Green's Function approach made fast

Real-time Green's function simulations of molecular junctions (open quantum systems) are typically performed by solving the Kadanoff-Baym equations (KBE). The KBE, however, impose a serious limitation on the maximum propagation time due to the large memory storage needed. In this work we propose a simplified Green's function approach based on the Generalized Kadanoff-Baym Ansatz (GKBA) to overcome the KBE limitation on time, significantly speed up the calculations, and yet stay close to the KBE results. This is achieved through a twofold advance: first we show how to make the GKBA work in open systems and then construct a suitable quasi-particle propagator that includes correlation effects in a diagrammatic fashion. We also provide evidence that our GKBA scheme, although already in good agreement with the KBE approach, can be further improved without increasing the computational cost.

cond-mat.mes-hall↗

arXiv2013

Screening-induced negative differential conductance in the Franck-Condon blockade regime

Screening effects in nanoscale junctions with strong electron-phonon coupling open new physical scenarios. We propose an accurate many-body approach to deal with the simultaneous occurrence of the Franck-Condon blockade and the screening-induced enhancement of the polaron mobility. We derive a transparent analytic expression for the electrical current: transient and steady-state features are directly interpreted and explained. Moreover, the interplay between phononic and electronic excitations gives rise to a novel mechanism of negative differential conductance. Experimental setup to observe this phenomenon are discussed.

cond-mat.mes-hall↗

arXiv2012

Missing derivative discontinuity of the exchange-correlation energy for attractive interactions: the charge Kondo effect

We show that the energy functional of ensemble Density Functional Theory (DFT) [Perdew et al., Phys. Rev. Lett. 49, 1691 (1982)] in systems with attractive interactions is a convex function of the fractional particle number N and is given by a series of straight lines joining a subset of ground-state energies. As a consequence the exchange-correlation (XC) potential is not discontinuous for all N. We highlight the importance of this exact result in the ensemble-DFT description of the negative-U Anderson model. In the atomic limit the discontinuity of the XC potential is missing for odd N while for finite hybridizations the discontinuity at even N is broadened. We demonstrate that the inclusion of these properties in any approximate XC potential is crucial to reproduce the characteristic signatures of the charge-Kondo effect in the conductance and charge susceptibility.

cond-mat.mes-hall↗

arXiv2012

Dynamical formation and manipulation of Majorana fermions in driven quantum wires

Controlling the dynamics of Majorana fermions (MF) subject to time-varying driving fields is of fundamental importance for the practical realization of topological quantum computing. In this work we study how it is possible to dynamically generate and maintain the topological phase in one-dimensional superconducting nanowires after the temporal variation of the Hamiltonian parameters. Remarkably we show that for a sudden quench the system can never relax towards a state exhibiting fully developed MF, independently of the initial and final Hamiltonians. Only for sufficiently slow protocols the system behaves adiabatically, and the topological phase can be reached. Finally we address the crucial question of how "adiabatic" a protocol must be in order to manipulate the MF inside the topological phase without deteriorating their Majorana character.

cond-mat.str-el↗

arXiv2012

Renormalization of the Coulomb blockade gap due to extended tunneling in nanoscopic junctions

In this work we discuss the combined effects of finite-range electron-electron interaction and finite-range tunneling on the transport properties of ultrasmall tunnel junctions. We show that the Coulomb blockade phenomenon is deeply influenced by the interplay between the geometry and the screening properties of the contacts. In particular if the interaction range is smaller than the size of the tunneling region a "weakly correlated" regime emerges in which the Coulomb blockade gap $\D$ is significantly reduced. In this regime $\D$ is not simply given by the conventional charging energy of the junction, since it is strongly renormalized by the energy that electrons need to tunnel over the extended contact.

cond-mat.mes-hall↗

arXiv2011

Advances in nonequilibrium transport with long-range interactions

The effects of long-range interactions in quantum transport are still largely unexplored, mainly due to the difficulty of devising efficient embedding schemes. In this work we present a substantial progress in the interacting resonant level model by reducing the problem to the solution of Kadanoff-Baym-like equations with a correlated embedding self-energy. The method allows us to deal with short- and long-range interactions and is applicable from the transient to the steady-state regime. Furthermore, memory effects are consistently incorporated and the results are not plagued by negative densities or non-conservation of the electric charge. We employ the method to calculate densities and currents with long-range interactions appropriate to low-dimensional leads, and show the occurrence of a jamming effect which drastically reduces the screening time and suppresses the zero-bias conductance. None of these effects are captured by short-range dot-lead interactions.

cond-mat.mes-hall↗

arXiv2011

On the thermalization of a Luttinger liquid after a sequence of sudden interaction quenches

We present a comprehensive analysis of the relaxation dynamics of a Luttinger liquid subject to a sequence of sudden interaction quenches. We express the critical exponent $β$ governing the decay of the steady-state propagator as an explicit functional of the switching protocol. At long distances $β$ depends only on the initial state while at short distances it is also history dependent. Continuous protocols of arbitrary complexity can be realized with infinitely long sequences. For quenches of finite duration we prove that there exist no protocol to bring the initial non-interacting system in the ground state of the Luttinger liquid. Nevertheless memory effects are washed out at short-distances. The adiabatic theorem is then investigated with ramp-switchings of increasing duration, and several analytic results for both the propagator and the excitation energy are derived.

cond-mat.quant-gas↗

arXiv2010

Correlation induced memory effects in the transport properties of low dimensional systems

We demonstrate the remnant presence of {\em initial} correlations in the {\em steady-state} electrical current flowing between low-dimensional interacting leads. The leads are described as Luttinger liquids and electrons can tunnel via a quantum point-contact. We derive an analytic result for the time-dependent current and show that ground-state correlations have a large impact on the relaxation and long-time behavior. In particular, the I-V characteristic cannot be reproduced by quenching the interaction in time. We further present a universal formula of the steady-state current $j_{S}$ for an arbitrary sequence of interaction quenches. It is established that $j_{S}$ is history dependent provided that the switching process is non-smooth.

cond-mat.mes-hall↗

arXiv2009

Time-dependent transport in graphene nanoribbons

We theoretically investigate the time-dependent ballistic transport in metallic graphene nanoribbons after the sudden switch-on of a bias voltage $V$. The ribbon is divided in three different regions, namely two semi-infinite graphenic leads and a central part of length $L$, across which the bias drops linearly and where the current is calculated. We show that during the early transient time the system behaves like a graphene bulk under the influence of a uniform electric field $E=V/L$. In the undoped system the current does not grow linearly in time but remarkably reaches a temporary plateau with dc conductivity $σ_{1}=πe^{2}/2h$, which coincides with the minimal conductivity of two-dimensional graphene. After a time of order $L/v_{F}$ ($v_{F}$ being the Fermi velocity) the current departs from the first plateau and saturates at its final steady state value with conductivity $σ_{2}=2e^{2}/h$ typical of metallic nanoribbons of finite width.

cond-mat.mes-hall↗

arXiv2008

On the ab initio calculation of CVV Auger spectra in closed-shell systems

We propose an ab initio method to evaluate the core-valence-valence (CVV) Auger spectrum of systems with filled valence bands. The method is based on the Cini-Sawatzky theory, and aims at estimating the parameters by first-principles calculations in the framework of density-functional theory (DFT). Photoemission energies and the interaction energy for the two holes in the final state are evaluated by performing DFT simulations for the system with varied population of electronic levels. Transition matrix elements are taken from atomic results. The approach takes into account the non-sphericity of the density of states of the emitting atom, spin-orbit interaction in core and valence, and non quadratic terms in the total energy expansion with respect to fractional occupation numbers. It is tested on two benchmark systems, Zn and Cu metals, leading in both cases to L23M45M45 Auger peaks within 2 eV from the experimental ones. Detailed analysis is presented on the relative weight of the various contributions considered in our method, providing the basis for future development. Especially problematic is the evaluation of the hole-hole interaction for systems with broad valence bands: our method underestimates its value in Cu, while we obtain excellent results for this quantity in Zn.

cond-mat.str-el↗

arXiv2008

Unconventional quasiparticle lifetime in undoped graphene

We address the question of how small can the quasiparticle decay rate be at low energies in undoped graphene, where kinematical constraints are known to prevent the decay into particle-hole excitations. For this purpose, we study the renormalization of the phonon dispersion by many-body effects, which turns out to be very strong in the case of the out-of-plane phonons at the K point of the spectrum. We show that these evolve into a branch of very soft modes that provide the relevant channel for quasiparticle decay, at energies below the scale of the optical phonon modes. In this regime, we find that the decay rate is proportional to the cube of the quasiparticle energy. This implies that a crossover should be observed in transport properties from the linear dependence characteristic of the high-energy regime to the much slower decay rate due to the soft phonon modes.

cond-mat.mes-hall↗

arXiv2008

Critical currents in graphene Josephson junctions

We study the superconducting correlations induced in graphene when it is placed between two superconductors, focusing in particular on the supercurrents supported by the 2D system. For this purpose we make use of a formalism placing the emphasis on the many-body aspects of the problem, with the aim of investigating the dependence of the critical currents on relevant variables like the distance L between the superconducting contacts, the temperature, and the doping level. Thus we show that, despite the vanishing density of states at the Fermi level in undoped graphene, supercurrents may exist at zero temperature with a natural 1/L^3 dependence at large L. When temperature effects are taken into account, the supercurrents are further suppressed beyond the thermal length L_T (~ v_F / k_B T, in terms of the Fermi velocity v_F of graphene), entering a regime where the decay is given by a 1/L^5 dependence. On the other hand, the supercurrents can be enhanced upon doping, as the Fermi level is shifted by a chemical potential μfrom the charge neutrality point. This introduces a new crossover length L* ~ v_F / μ, at which the effects of the finite charge density start being felt, marking the transition from the short-distance 1/L^3 behavior to a softer 1/L^2 decay of the supercurrents at large L. It turns out that the decay of the critical currents is given in general by a power-law behavior, which can be seen as a consequence of the perfect scaling of the Dirac theory applied to the low-energy description of graphene.

cond-mat.mes-hall↗

arXiv2008

Auger transitions in one-dimensional metals

We present a dynamical theory of the Auger decay in one-dimensional (1D) metals described by the Tomonaga-Luttinger model. An analytic expression of the Auger current is derived in the framework of the 1-step approach, where the finite lifetime of the initial core-hole and the core-valence interaction are taken into account. This allows to capture typical dynamical features like the shake-down effect, in which the Auger spectrum shows a non-vanishing weight above the 2-step high-energy threshold. The obtained results give also a hint to understand the sizable suppression of Auger spectral weight closed to the Fermi energy recently observed in carbon nanotubes with respect to graphite.

cond-mat.str-el↗

arXiv2007

Electronic correlations in graphite and carbon nanotubes from Auger spectroscopy

We have determined the screened on-site Coulomb repulsion in graphite and single wall carbon nanotubes by measuring their Auger spectra and performing a new theoretical analysis based on an extended Cini-Sawatzky approach where only one fit parameter is employed. The experimental lineshape is very well reproduced by the theory and this allows to determine the value of the screened on-site repulsion between $2p$ states, which is found to be 2.1 eV in graphite and 4.6 eV in nanotubes. The latter is robust by varying the nanotube radius from 1 to 2 nm.

cond-mat.str-el↗

arXiv2007

Quantum Hall effect in carbon nanotubes and curved graphene strips

We develop a long wavelength approximation in order to describe the low-energy states of carbon nanotubes in a transverse magnetic field. We show that, in the limit where the square of the magnetic length $l = \sqrt{\hbar c /e B}$ is much larger than the $C$-$C$ distance times the nanotube radius $R$, the low-energy theory is given by the linear coupling of a two-component Dirac spinor to the corresponding vector potential. We investigate in this regime the evolution of the band structure of zig-zag nanotubes for values of $R/l > 1$, showing that for radius $R \approx 20$ nm a clear pattern of Landau levels start to develop for magnetic field strength $B \gtrsim 10$ T. The levels tend to be four-fold degenerate, and we clarify the transition to the typical two-fold degeneracy of graphene as the nanotube is unrolled to form a curved strip. We show that the dynamics of the Dirac fermions leads to states which are localized at the flanks of the nanotube and that carry chiral currents in the longitudinal direction. We discuss the possibility to observe the quantization of the Hall conductivity in thick carbon nanotubes, which should display steps at even multiples of $2 e^2/h$, with values doubled with respect to those in the odd-integer quantization of graphene.

cond-mat.mes-hall↗

arXiv2007

Electronic instabilities of a Hubbard model approached as a large array of coupled chains: competition between d-wave superconductivity and pseudogap phase

We study the electronic instabilities in a 2D Hubbard model where one of the dimensions has a finite width, so that it can be considered as a large array of coupled chains. The finite transverse size of the system gives rise to a discrete string of Fermi points, with respective electron fields that, due to their mutual interaction, acquire anomalous scaling dimensions depending on the point of the string. Using bosonization methods, we show that the anomalous scaling dimensions vanish when the number of coupled chains goes to infinity, implying the Fermi liquid behavior of a 2D system in that limit. However, when the Fermi level is at the Van Hove singularity arising from the saddle points of the 2D dispersion, backscattering and Cooper-pair scattering lead to the breakdown of the metallic behavior at low energies. These interactions are taken into account through their renormalization group scaling, studying in turn their influence on the nonperturbative bosonization of the model. We show that, at a certain low-energy scale, the anomalous electron dimension diverges at the Fermi points closer to the saddle points of the 2D dispersion. The d-wave superconducting correlations become also large at low energies, but their growth is cut off as the suppression of fermion excitations takes place first, extending progressively along the Fermi points towards the diagonals of the 2D Brillouin zone. We stress that this effect arises from the vanishing of the charge stiffness at the Fermi points, characterizing a critical behavior that is well captured within our nonperturbative approach.

cond-mat.str-el↗